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Colloquium : Optimal control of high-harmonic generation

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TLDR
In this paper, the authors discuss the control of high-harmonic spectra by temporal and spatial pulse shaping of the driving laser pulses and its implications on time-resolved XUV spectroscopy and attosecond pulse shaping.
Abstract
High-harmonic generation provides an attractive light source of coherent radiation in the extreme-ultraviolet (XUV) and soft-x-ray regions of the spectrum and allows for the production of single attosecond pulses or pulse trains. This Colloquium covers the control of high-harmonic spectra by temporal and spatial pulse shaping of the driving laser pulses and its implications on time-resolved XUV spectroscopy and attosecond pulse shaping. It summarizes important steps for extending existing pulse shaping techniques and control schemes from the near-infrared or visible part to shorter wavelengths. Using adaptive pulse shaping of the driving laser pulses, several groups have demonstrated control of the high-harmonic spectrum, including the author's work on the complete control over the XUV spectrum of high-order harmonics, generated in a gas-filled hollow fiber. It is possible to achieve both the enhancement and the suppression of single or several selected harmonic orders. These arbitrarily shaped soft-x-ray spectra will allow for important modifications of the resulting harmonic pulses in the temporal domain. This constitutes first steps towards direct attosecond pulse shaping in the soft-x-ray domain. Moreover, high-harmonic generation in a hollow-core fiber can be enhanced by coupling into a single fiber mode using a feedback-controlled adaptive two-dimensional spatial light modulator.

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Citations
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Extremely high-intensity laser interactions with fundamental quantum systems

TL;DR: In this article, a review of recent investigations on high-energy processes within the realm of relativistic quantum dynamics, quantum electrodynamics, and nuclear and particle physics, occurring in extremely intense laser fields is presented.
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Control of quantum phenomena: past, present and future

TL;DR: Adaptive feedback control (AFC) as mentioned in this paper is a state-of-the-art technique for quantum control. But it is not suitable for the case of femtosecond laser sources.
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Macroscopic aspects of attosecond pulse generation

TL;DR: In this article, a complete understanding of the way in which attosecond pulses arrive at a target where they can be characterized and used in an experiment is discussed, and a number of results from calculations of the attoscond pulse generation obtained by simultaneous solution of the time-dependent Schrodinger equation and the Maxwell wave equation are discussed.
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Electron and X‐Ray Methods of Ultrafast Structural Dynamics: Advances and Applications

TL;DR: The state of the art in the determination of structures with ultrafast electrons and X-rays is highlighted, and a comprehensive referencing to current research is provided.
Journal ArticleDOI

A newcomer's guide to ultrashort pulse shaping and characterization

TL;DR: An overview of the most widespread techniques of both ultrashort pulse shaping and pulse characterization can be found in this paper, where the authors also present a detailed survey of the techniques used for both tasks.
References
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Journal ArticleDOI

X-Ray Interactions: Photoabsorption, Scattering, Transmission, and Reflection at E = 50-30,000 eV, Z = 1-92

TL;DR: In this article, the atomic scattering factors for all angles of coherent scattering and at the higher photon energies are obtained from these tabulated forward-scattering values by adding a simple angle-dependent form-factor correction.
Journal ArticleDOI

Plasma perspective on strong field multiphoton ionization.

TL;DR: During strong-field multiphoton ionization, a wave packet is formed each time the laser field passes its maximum value, and one important parameter which determines the strength of these effects is the rate at which the wave packet spreads in the direction perpendicular to the laser electric field.
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Stimulated Optical Radiation in Ruby

TL;DR: Schawlow and Townes as discussed by the authors proposed a technique for the generation of very monochromatic radiation in the infra-red optical region of the spectrum using an alkali vapour as the active medium.
Journal Article

Stimulated optical radiation in ruby

T. H. Maiman
TL;DR: Schawlow and Townes as discussed by the authors proposed a technique for the generation of very monochromatic radiation in the infra-red optical region of the spectrum using an alkali vapour as the active medium.
Journal ArticleDOI

Interactions between light waves in a nonlinear dielectric

TL;DR: In this paper, the induced nonlinear electric dipole and higher moments in an atomic system, irradiated simultaneously by two or three light waves, are calculated by quantum-mechanical perturbation theory.
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