Journal ArticleDOI
High-harmonic generation by resonant plasmon field enhancement
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TLDR
This work demonstrates a method of high-harmonic generation that requires no extra cavities by exploiting the local field enhancement induced by resonant plasmons within a metallic nanostructure consisting of bow-tie-shaped gold elements on a sapphire substrate.Abstract:
High-harmonic generation by focusing a femtosecond laser onto a gas is a well-known method of producing coherent extreme-ultraviolet (EUV) light. This nonlinear conversion process requires high pulse intensities, greater than 10(13) W cm(-2), which are not directly attainable using only the output power of a femtosecond oscillator. Chirped-pulse amplification enables the pulse intensity to exceed this threshold by incorporating several regenerative and/or multi-pass amplifier cavities in tandem. Intracavity pulse amplification (designed not to reduce the pulse repetition rate) also requires a long cavity. Here we demonstrate a method of high-harmonic generation that requires no extra cavities. This is achieved by exploiting the local field enhancement induced by resonant plasmons within a metallic nanostructure consisting of bow-tie-shaped gold elements on a sapphire substrate. In our experiment, the output beam emitted from a modest femtosecond oscillator (100-kW peak power, 1.3-nJ pulse energy and 10-fs pulse duration) is directly focused onto the nanostructure with a pulse intensity of only 10(11) W cm(-2). The enhancement factor exceeds 20 dB, which is sufficient to produce EUV wavelengths down to 47 nm by injection with an argon gas jet. The method could form the basis for constructing laptop-sized EUV light sources for advanced lithography and high-resolution imaging applications.read more
Citations
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Plasmonics for extreme light concentration and manipulation.
Jon A. Schuller,Edward S. Barnard,Wenshan Cai,Young Chul Jun,Justin S. White,Mark L. Brongersma +5 more
TL;DR: The basic concepts behind plasmonics-enabled light concentration and manipulation are discussed, an attempt to capture the wide range of activities and excitement in this area is made, and possible future directions are speculated on.
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Antennas for light
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Controlling the synthesis and assembly of silver nanostructures for plasmonic applications
Matthew Rycenga,Claire M. Cobley,Jie Zeng,Weiyang Li,Christine H. Moran,Qiang Zhang,Dong Qin,Younan Xia +7 more
TL;DR: In plasmonics, the metal nanostructures can serve as antennas to convert light into localized electric fields (E-fields) or as waveguides to route light to desired locations with nanometer precision through a strong interaction between incident light and free electrons in the nanostructure.
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Gold nanorods and their plasmonic properties
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Plasmon nano-optical tweezers
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References
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Compression of amplified chirped optical pulses
Donna Strickland,Gerard Mourou +1 more
TL;DR: In this paper, the amplification and subsequent recompression of optical chirped pulses were demonstrated using a system which produces 1.06 μm laser pulses with pulse widths of 2 ps and energies at the millijoule level.
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Theory of high-harmonic generation by low-frequency laser fields.
TL;DR: A simple, analytic, and fully quantum theory of high-harmonic generation by low-frequency laser fields is presented and the exact quantum-mechanical formula for the harmonic cutoff that differs from the phenomenological law Ip+3.17Up is presented.
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TL;DR: N nanometer-scale gold dipole antennas designed to be resonant at optical frequencies are fabricated, in contradiction to classical antenna theory but in qualitative accordance with computer simulations that take into account the finite metallic conductivity at optical frequency.
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