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Few-Layer Graphdiyne Nanosheets Applied for Multiplexed Real-Time DNA Detection

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TLDR
This study develops few-layer graphdiyne (GD) nanosheets that are used as novel sensing platforms for a variety of fluorophores real-time detection of DNA with low background and high signal-to-noise ratio, which show a distinguished fluorescence quenching ability and different affinities toward single-Stranded DNA and double-stranded DNA.
Abstract
Despite recent progress in 2D nanomaterials-based biosensing, it remains challenging to achieve sensitive and high selective detection. This study develops few-layer graphdiyne (GD) nanosheets (NSs) that are used as novel sensing platforms for a variety of fluorophores real-time detection of DNA with low background and high signal-to-noise ratio, which show a distinguished fluorescence quenching ability and different affinities toward single-stranded DNA and double-stranded DNA. Importantly, for the first time, a few-layer GD NSs-based multiplexed DNA sensor is developed.

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Chemical Vapor Deposition Growth and Applications of Two-Dimensional Materials and Their Heterostructures

TL;DR: This review of the challenges in the CVD growth of 2D materials highlights recent advances in the controlled growth of single crystal 2Dmaterials, with an emphasis on semiconducting transition metal dichalcogenides.
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Progress in Research into 2D Graphdiyne-Based Materials

TL;DR: GDY has recently revealed the practicality of GDY as catalyst; in rechargeable batteries, solar cells, electronic devices, magnetism, detector, biomedicine, and therapy; and for gas separation as well as water purification.
Journal ArticleDOI

Few-layer graphdiyne doped with sp-hybridized nitrogen atoms at acetylenic sites for oxygen reduction electrocatalysis.

TL;DR: Chemically defined sp-hybridized nitrogen atoms have been selectively introduced to the acetylene groups in ultrathin graphdiynes, resulting in good catalytic activity for the oxygen reduction reaction in both alkaline and acidic media.
Journal ArticleDOI

Graphdiyne: synthesis, properties, and applications

TL;DR: This review aims at providing a comprehensive update on the synthesis of GDY and GDY-based materials, as well as their properties, including structural, electronic, mechanical, and spectral properties, and their applications in nanotechnology.
Journal ArticleDOI

Graphdiyne and its Assembly Architectures: Synthesis, Functionalization, and Applications

TL;DR: Recent advances in the fabrication of GDY-based nanostructures and their applications, and corresponding mechanisms, are covered, and future critical perspectives are also discussed.
References
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Journal ArticleDOI

Architecture of graphdiyne nanoscale films

TL;DR: A methodology to generate large area graphdiyne films with 3.61 cm(2) on the surface of copper via a cross-coupling reaction using hexaethynylbenzene is demonstrated and shows conductivity of 2.516 x 10(-4) S m(-1) indicating a semiconductor property.
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Single‐Layer Semiconducting Nanosheets: High‐Yield Preparation and Device Fabrication

TL;DR: The common feature of these materials is that the bulk material forms are layeredstructures with strong covalent bonding in each layer and weak van der Waals forces between the layers.
Journal ArticleDOI

Graphene and graphene oxide: biofunctionalization and applications in biotechnology

TL;DR: This review selectively analyzes current advances in the field of graphene bioapplications, and focuses on the biofunctionalization of graphene for biological applications, fluorescence-resonance-energy-transfer-based biosensor development by using graphene or graphene-based nanomaterials, and the investigation of grapheneor graphene- based nanommaterials for living cell studies.
Journal ArticleDOI

A Graphene Nanoprobe for Rapid, Sensitive, and Multicolor Fluorescent DNA Analysis

TL;DR: A graphene oxide (GO)‐based multicolor fluorescent DNA nanoprobe that allows rapid, sensitive, and selective detection of DNA targets in homogeneous solution by exploiting interactions between GO and DNA molecules is reported.
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