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Journal ArticleDOI

Highly Stretchable and Biocompatible Strain Sensors Based on Mussel-Inspired Super-Adhesive Self-Healing Hydrogels for Human Motion Monitoring.

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TLDR
A novel hydrogel was synthesized by incorporating polydopamine-coated talc (PDA-talc) nanoflakes into a polyacrylamide (PAM)Hydrogel inspired by the natural mussel adhesive mechanism, which displayed strong adhesiveness to various substrates, including human skin, and the adhesion strength surpassed that of commercial double-sided tape and glue sticks.
Abstract
Integrating multifunctionality such as adhesiveness, stretchability, and self-healing ability on a single hydrogel has been a challenge and is a highly desired development for various applications including electronic skin, wound dressings, and wearable devices. In this study, a novel hydrogel was synthesized by incorporating polydopamine-coated talc (PDA–talc) nanoflakes into a polyacrylamide (PAM) hydrogel inspired by the natural mussel adhesive mechanism. Dopamine molecules were intercalated into talc and oxidized, which enhanced the dispersion of talc and preserved catechol groups in the hydrogel. The resulting dopamine–talc–PAM (DTPAM) hydrogel showed a remarkable stretchability, with over 1000% extension and a recovery rate over 99%. It also displayed strong adhesiveness to various substrates, including human skin, and the adhesion strength surpassed that of commercial double-sided tape and glue sticks, even as the hydrogel dehydrated over time. Moreover, the DTPAM hydrogel could rapidly self-heal a...

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Citations
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Journal ArticleDOI

Bio-Integrated Wearable Systems: A Comprehensive Review

TL;DR: This review summarizes the latest advances in this emerging field of "bio-integrated" technologies in a comprehensive manner that connects fundamental developments in chemistry, material science, and engineering with sensing technologies that have the potential for widespread deployment and societal benefit in human health care.
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Advanced Soft Materials, Sensor Integrations, and Applications of Wearable Flexible Hybrid Electronics in Healthcare, Energy, and Environment.

TL;DR: An all-inclusive review of the newly developed WFHE along with a summary of imperative requirements of material properties, sensor capabilities, electronics performance, and skin integrations is provided.
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Muscle‐Inspired Highly Anisotropic, Strong, Ion‐Conductive Hydrogels

TL;DR: The work offers a promising strategy to fabricate a wide variety of strong, anisotropic, flexible, and ionically conductive wood-based hydrogels for potential biomaterials and nanofluidic applications.
Journal ArticleDOI

Stretchable and tough conductive hydrogels for flexible pressure and strain sensors

TL;DR: This review focuses on tough conductive hydrogels for flexible sensors, which have great potential for applications in wearable and implantable devices, soft robotics and artificial skin.
Journal ArticleDOI

Self-Healing Hydrogels: The Next Paradigm Shift in Tissue Engineering?

TL;DR: The recent progress in the development of multifunctional and self‐healable hydrogels for various tissue engineering applications is discussed in detail and their potential applications within the rapidly expanding areas of bioelectronics, cyborganics, and soft robotics are highlighted.
References
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Journal ArticleDOI

Mussel-Inspired Surface Chemistry for Multifunctional Coatings

TL;DR: Inspired by the composition of adhesive proteins in mussels, dopamine self-polymerization is used to form thin, surface-adherent polydopamine films onto a wide range of inorganic and organic materials, including noble metals, oxides, polymers, semiconductors, and ceramics.
Journal ArticleDOI

Skin-like pressure and strain sensors based on transparent elastic films of carbon nanotubes

TL;DR: Transparent, conducting spray-deposited films of single-walled carbon nanotubes are reported that can be rendered stretchable by applying strain along each axis, and then releasing this strain.
Journal ArticleDOI

A stretchable carbon nanotube strain sensor for human-motion detection

TL;DR: A class of wearable and stretchable devices fabricated from thin films of aligned single-walled carbon nanotubes capable of measuring strains up to 280% with high durability, fast response and low creep is reported.
Journal ArticleDOI

Single-molecule mechanics of mussel adhesion

TL;DR: A single-molecule study of the substrate and oxidation-dependent adhesive properties of dopa is reported, in which dopa exploits a remarkable combination of high strength and chemical multifunctionality to accomplish adhesion to substrates of widely varying composition.
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