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Periodic patterns and energy states of buckled films on compliant substrates

TLDR
In this paper, the authors characterized and ranked the energy of various periodic mode patterns, including checkerboard, hexagonal and herringbone, in terms of the extent to which they reduce the elastic energy of the compliant elastic substrate.
Abstract
Thin stiff films on compliant elastic substrates subject to equi-biaxial compressive stress states are observed to buckle into various periodic mode patterns including checkerboard, hexagonal and herringbone. An experimental setting in which these modes are observed and evolve is described. The modes are characterized and ranked by the extent to which they reduce the elastic energy of the film–substrate system relative to that of the unbuckled state over a wide range of overstress. A new mode is identified and analyzed having nodal lines coincident with an equilateral triangular pattern. Two methods are employed to ascertain the energy in the buckled state: an analytical upper-bound method and a full numerical analysis. The upper-bound is shown to be reasonably accurate to large levels of overstress. For flat films, except at small states of overstress where the checkerboard is preferred, the herringbone mode has the lowest energy, followed by the checkerboard, with the hexagonal, triangular, and one-dimensional modes lowering the energy the least. At low overstress, the hexagonal mode is observed in the experiments not the square mode. It is proposed that a slight initial curvature of the film may play role in selecting the hexagonal pattern accompanied by a detailed analysis. An intriguing finding is that the hexagonal and triangular modes have the same energy in the buckled state and, moreover, a continuous transition between these modes exists involving a linear combination of the two modes with no change in energy. Experimental observations of various periodic modes are discussed with reference to the energy landscape. Discrepancies between observations and theory are identified and open issues are highlighted.

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Citations
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Journal ArticleDOI

Mechanics of morphological instabilities and surface wrinkling in soft materials: a review

TL;DR: Some representative theoretical and numerical approaches aimed at modelling the onset of instabilities as well as the postbuckling evolution involving multiple bifurcations and symmetry breakings are discussed along with the main characteristics and some possible applications of this rich phenomenon.
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Wrinkling Phenomena in Neo-Hookean Film/Substrate Bilayers

TL;DR: In this article, the role of substrate prestretch is considered wherein an unstretched film is bonded to a prestretched substrate with wrinkling arising as the stretch in the substrate is relaxed.
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Curvature-induced symmetry breaking determines elastic surface patterns

TL;DR: A generalized Swift-Hohenberg theory that describes wrinkling morphology and pattern selection in curved elastic bilayer materials is reported that builds on general differential-geometry principles and can be extended to arbitrarily shaped surfaces.
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From Wrinkles to Creases in Elastomers: The Instability and Imperfection-Sensitivity of Wrinkling

TL;DR: The stability of the wrinkling mode experienced by a compressed half-space of neo-Hookean material is investigated using analytical and numerical methods to study the post-bifurcation behavior of periodic solutions as mentioned in this paper.
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Physical biology of human brain development.

TL;DR: This work revisits cortical folding as the instability problem of constrained differential growth in a multi-layered system and illustrates that physical forces can explain cortical malformations as emergent properties of developmental disorders.
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Spontaneous formation of ordered structures in thin films of metals supported on an elastomeric polymer

TL;DR: In this paper, the authors describe the appearance of complex, ordered structures induced by the buckling of thin metal films owing to thermal contraction of an underlying substrate, and account qualitatively for the size and form of the patterned features in terms of the nonuniform stresses developed in the film near steps on the polymer substrate.
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Mechanics of Incremental Deformation

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Journal ArticleDOI

Nonlinear analyses of wrinkles in a film bonded to a compliant substrate

TL;DR: In this article, the amplitude and wavelength of sinusoidal wrinkles were analyzed in a stiff film bonded to a compliant substrate, which in turn is attached to a rigid support, and the simulations showed that the wrinkles can evolve into stripes, labyrinths, or herringbones, depending on the anisotropic of the membrane forces.
Journal ArticleDOI

Surface modification of Sylgard-184 poly(dimethyl siloxane) networks by ultraviolet and ultraviolet/ozone treatment.

TL;DR: The results reveal that when exposed to UV, the PDMS macromolecules in the surface region of Sylgard-184 undergo chain scission, involving both the main chain backbone and the side groups, and form a network whose wetting properties are similar to those of a UV-modified model PDMS.
Journal ArticleDOI

Nested self-similar wrinkling patterns in skins.

TL;DR: In this paper, a hierarchical pattern consisting of self-similar buckles extending over five orders of magnitude in length scale, ranging from a few nanometres to a few millimetres, is presented.
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