Andrea Christine Wagner

TL;DR: It is shown that organic vapours alone can drive nucleation, and a particle growth model is presented that quantitatively reproduces the measurements and implements a parameterization of the first steps of growth in a global aerosol model that can change substantially in response to concentrations of atmospheric cloud concentration nuclei.

TL;DR: Ion-induced nucleation of pure organic particles constitutes a potentially widespread source of aerosol particles in terrestrial environments with low sulfuric acid pollution.

TL;DR: How NOx suppresses particle formation is shown, while HOMs, sulfuric acid, and NH3 have a synergistic enhancing effect on particle formation, elucidate the complex interactions between biogenic and anthropogenic vapors in the atmospheric aerosol system.

TL;DR: Model simulations show that the pure biogenic particle formation mechanism has a much larger relative effect on CCN concentrations in the preindustrial atmosphere than in the present atmosphere because of the lower aerosol concentrations, and the cooling forcing of anthropogenic aerosols is reduced.

TL;DR: The growth rates are sensitive to particle curvature, explaining widespread atmospheric observations that particle growth rates increase in the single-digit-nanometer size range, and demonstrate that organic vapors can contribute to particle growth over a wide range of tropospheric temperatures from molecular cluster sizes onward.