Showing papers by "Yuri S. Kivshar published in 2018"

Asymmetric Metasurfaces with High-Q Resonances Governed by Bound States in the Continuum.

Abstract: We reveal that metasurfaces created by seemingly different lattices of (dielectric or metallic) meta-atoms with broken in-plane symmetry can support sharp high-$Q$ resonances arising from a distortion of symmetry-protected bound states in the continuum. We develop a rigorous theory of such asymmetric periodic structures and demonstrate a link between the bound states in the continuum and Fano resonances. Our results suggest the way for smart engineering of resonances in metasurfaces for many applications in nanophotonics and metaoptics.

Imaging-based molecular barcoding with pixelated dielectric metasurfaces.

Abstract: Metasurfaces provide opportunities for wavefront control, flat optics, and subwavelength light focusing. We developed an imaging-based nanophotonic method for detecting mid-infrared molecular fingerprints and implemented it for the chemical identification and compositional analysis of surface-bound analytes. Our technique features a two-dimensional pixelated dielectric metasurface with a range of ultrasharp resonances, each tuned to a discrete frequency; this enables molecular absorption signatures to be read out at multiple spectral points, and the resulting information is then translated into a barcode-like spatial absorption map for imaging. The signatures of biological, polymer, and pesticide molecules can be detected with high sensitivity, covering applications such as biosensing and environmental monitoring. Our chemically specific technique can resolve absorption fingerprints without the need for spectrometry, frequency scanning, or moving mechanical parts, thereby paving the way toward sensitive and versatile miniaturized mid-infrared spectroscopy devices.

Generalized Kerker effects in nanophotonics and meta-optics [Invited]

Abstract: The original Kerker effect was introduced for a hypothetical magnetic sphere, and initially it did not attract much attention due to a lack of magnetic materials required. Rejuvenated by the recent explosive development of the field of metamaterials and especially its core concept of optically-induced artificial magnetism, the Kerker effect has gained an unprecedented impetus and rapidly pervaded different branches of nanophotonics. At the same time, the concept behind the effect itself has also been significantly expanded and generalized. Here we review the physics and various manifestations of the generalized Kerker effects, including the progress in the emerging field of meta-optics that focuses on interferences of electromagnetic multipoles of different orders and origins. We discuss not only the scattering by individual particles and particle clusters, but also the manipulation of reflection, transmission, diffraction, and absorption for metalattices and metasurfaces, revealing how various optical phenomena observed recently are all ubiquitously related to the Kerker’s concept.

Giant Nonlinear Response at the Nanoscale Driven by Bound States in the Continuum.

Abstract: Being motivated by the recent prediction of high-$Q$ modes in subwavelength dielectric resonators inspired by bound states in the continuum (BIC), we study the second-harmonic generation from isolated subwavelength AlGaAs nanoantennas. We reveal that nonlinear effects at the nanoscale can be enhanced dramatically provided the resonator parameters are tuned to the BIC regime. We predict a record-high conversion efficiency for nanoscale resonators that exceeds by 2 orders of magnitude the conversion efficiency observed at the magnetic dipole Mie resonance, thus opening the way for highly efficient nonlinear metasurfaces and metadevices.

Dynamic Beam Switching by Liquid Crystal Tunable Dielectric Metasurfaces

Abstract: Dynamic steering of laser beams by ultrathin optical metasurfaces is a significant research advance for possible applications in remote ranging and sensing. A unique platform for such important functionalities is offered by dielectric metasurfaces that have the highest transmission efficiency. However, the realization of dynamically tunable metasurfaces still remains a challenge. Here we experimentally demonstrate the dynamic switching of beam deflection by a silicon-nanodisk dielectric metasurface infiltrated with liquid crystals. In particular, we show the switching of a laser beam from 0° to a 12° angle with an efficiency of 50% by heating the metasurface to modify the liquid crystal state from nematic to isotropic. Our results open important opportunities for tunable ultrathin beam steering metadevices.

Quantum metasurface for multiphoton interference and state reconstruction

Abstract: Metasurfaces based on resonant nanophotonic structures have enabled innovative types of flat-optics devices that often outperform the capabilities of bulk components, yet these advances remain largely unexplored for quantum applications. We show that nonclassical multiphoton interferences can be achieved at the subwavelength scale in all-dielectric metasurfaces. We simultaneously image multiple projections of quantum states with a single metasurface, enabling a robust reconstruction of amplitude, phase, coherence, and entanglement of multiphoton polarization-encoded states. One- and two-photon states are reconstructed through nonlocal photon correlation measurements with polarization-insensitive click detectors positioned after the metasurface, and the scalability to higher photon numbers is established theoretically. Our work illustrates the feasibility of ultrathin quantum metadevices for the manipulation and measurement of multiphoton quantum states, with applications in free-space quantum imaging and communications.

All-dielectric meta-optics and non-linear nanophotonics

Abstract: Most optical metamaterials fabricated and studied to date employ metallic components resulting in significant losses, heat and overall low efficiencies. A new era of metamaterial physics is associated with all-dielectric meta-optics, which employs electric and magnetic Mie resonances of subwavelength particles with high refractive index for an optically induced magnetic response, thus underpinning a new approach to design and fabricate functional and practical metadevices. Here we review the recent developments in meta-optics and subwavelength dielectric photonics and demonstrate that the Mie resonances can play a crucial role in the realization of the unique functionalities of meta-atoms, also driving novel effects in the fields of metamaterials and nanophotonics. We discuss the recent research frontiers in all-dielectric meta-optics and uncover how Mie resonances can be employed for a flexible control of light with full phase and amplitude engineering, including unidirectional metadevices, highly transparent metasurfaces, non-linear nanophotonics and topological photonics.

Nonlinear Wavefront Control with All-Dielectric Metasurfaces

Abstract: Metasurfaces, two-dimensional lattices of nanoscale resonators, offer unique opportunities for functional flat optics and allow the control of the transmission, reflection, and polarization of a wavefront of light. Recently, all-dielectric metasurfaces reached remarkable efficiencies, often matching or out-performing conventional optical elements. The exploitation of the nonlinear optical response of metasurfaces offers a paradigm shift in nonlinear optics, and dielectric nonlinear metasurfaces are expected to enrich subwavelength photonics by enhancing substantially nonlinear response of natural materials combined with the efficient control of the phase of nonlinear waves. Here, we suggest a novel and rather general approach for engineering the wavefront of parametric waves of arbitrary complexity generated by a nonlinear metasurface. We design all-dielectric nonlinear metasurfaces, achieve a highly efficient wavefront control of a third-harmonic field, and demonstrate the generation of nonlinear beams a...

Noninterleaved Metasurface for (26-1) Spin- and Wavelength-Encoded Holograms.

Abstract: Nanostructured metasurfaces demonstrate extraordinary capabilities to control light at the subwavelength scale, emerging as key optical components to physical realization of multitasked devices. Progress in multitasked metasurfaces has been witnessed in making a single metasurface multitasked by mainly resorting to extra spatial freedom, for example, interleaved subarrays, different angles. However, it imposes a challenge of suppressing the cross-talk among multiwavelength without the help of extra spatial freedom. Here, we introduce an entirely novel strategy of multitasked metasurfaces with noninterleaved single-size Si nanobrick arrays and minimalist spatial freedom demonstrating massive information on 6-bit encoded color holograms. The interference between electric dipole and magnetic dipole in individual Si nanobricks with in-plane orientation enables manipulating six bases of incident photons simultaneously to reconstructed 6-bit wavelength- and spin-dependent multicolor images. Those massively reco...

Light-Emitting Halide Perovskite Nanoantennas.

Abstract: Nanoantennas made of high-index dielectrics with low losses in visible and infrared frequency ranges have emerged as a novel platform for advanced nanophotonic devices. On the other hand, halide perovskites are known to possess high refractive index, and they support excitons at room temperature with high binding energies and quantum yield of luminescence that makes them very attractive for all-dielectric resonant nanophotonics. Here we employ halide perovskites to create light-emitting nanoantennas with enhanced photoluminescence due to the coupling of their excitons to dipolar and multipolar Mie resonances. We demonstrate that the halide perovskite nanoantennas can emit light in the range of 530-770 nm depending on their composition. We employ a simple technique based on laser ablation of thin films prepared by wet-chemistry methods as a novel cost-effective approach for the fabrication of resonant perovskite nanostructures.

Quantum metasurface for multi-photon interference and state reconstruction

Abstract: Metasurfaces based on resonant nanophotonic structures have enabled novel types of flat-optics devices often outperforming the capabilities of bulk components, yet these advances remain largely unexplored for quantum applications. We show that non-classical multi-photon interferences can be achieved at the subwavelength scale in all-dielectric metasurfaces. We simultaneously image multiple projections of quantum states with a single metasurface, enabling a robust reconstruction of amplitude, phase, coherence, and entanglement of multi-photon polarization-encoded states. One- and two-photon states are reconstructed through nonlocal photon correlation measurements with polarization-insensitive click-detectors positioned after the metasurface, and the scalability to higher photon numbers is established theoretically. Our work illustrates the feasibility of ultra-thin quantum metadevices for the manipulation and measurement of multi-photon quantum states with applications in free-space quantum imaging and communications.

All-Dielectric Resonant Metasurfaces with a Strong Toroidal Response

Abstract: We demonstrate how to design all-dielectric metasurfaces with a strong axial toroidal response by arranging two types of nanodisks into asymmetric quadrumer clusters. This toroidal response is related to the existence of the trapped (dark) mode that appears due to a symmetry breaking in the cluster. We uncover a correlation between the existence of the toroidal response and asymmetry in the metasurface geometries, which originates from different diameters of nanodisks or notches introduced into nanodisks. Because of the unique field configuration of the toroidal mode, the proposed metasurface could serve as a platform for efficient light–matter interaction for enhanced absorption, nonlinear response, and sensing.

Active Tuning of Spontaneous Emission by Mie-Resonant Dielectric Metasurfaces

Abstract: Mie-resonant dielectric metasurfaces offer comprehensive opportunities for the manipulation of light fields with high efficiency. Additionally, various strategies for the dynamic tuning of the optical response of such metasurfaces were demonstrated, making them important candidates for reconfigurable optical devices. However, dynamic control of the light-emission properties of active Mie-resonant dielectric metasurfaces by an external control parameter has not been demonstrated so far. Here, we experimentally demonstrate the dynamic tuning of spontaneous emission from a Mie-resonant dielectric metasurface that is situated on a fluorescent substrate and embedded into a liquid crystal cell. By switching the liquid crystal from the nematic state to the isotropic state via control of the cell temperature, we induce a shift of the spectral position of the metasurface resonances. This results in a change of the local photonic density of states, which, in turn, governs the enhancement of spontaneous emission fro...

Tunable Hybrid Fano Resonances in Halide Perovskite Nanoparticles

Abstract: © 2018 American Chemical Society. Halide perovskites are known to support excitons at room temperatures with high quantum yield of luminescence that make them attractive for all-dielectric resonant nanophotonics and meta-optics. Here we report the observation of broadly tunable Fano resonances in halide perovskite nanoparticles originating from the coupling of excitons to the Mie resonances excited in the nanoparticles. Signatures of the photon-exciton ("hybrid") Fano resonances are observed in dark-field spectra of isolated nanoparticles, and also in the extinction spectra of aperiodic lattices of such nanoparticles. In the latter case, chemical tunability of the exciton resonance allows reversible tuning of the Fano resonance across the 100 nm bandwidth in the visible frequency range, providing a novel approach to control optical properties of perovskite nanostructures. The proposed method of chemical tuning paves the way to an efficient control of emission properties of on-chip-integrated light-emitting nanoantennas.

Directional and Spectral Shaping of Light Emission with Mie-Resonant Silicon Nanoantenna Arrays

Abstract: We study light emission from square arrays of Mie-resonant silicon nanoantennas situated on a fluorescent glass substrate When the spectral positions of the silicon nanoantennas’ resonances overlap with the intrinsic emission from the glass, the emission is selectively enhanced for certain spectral and spatial frequencies detemined by the design of the nanoantenna array We measure the emission spectra of the coupled system for a systematic variation of the nanoantenna geometry, showing that the spectral maximum of the emission coincides with the antenna resonance positions observed in linear-optical transmittance spectra Furthermore, we study the directionality of the emission by back focal plane imaging and numerical calculations based on the Fourier modal method and the reciprocity principle We observe that the nanoantenna array induces a reshaping of the resonantly enhanced emission in the air half-space into a narrow lobe directed out of the substrate plane This reshaping is explained by coherent

Strong Mode Coupling and High-Q Supercavity Modes in Subwavelength Dielectric Resonators

Abstract: We reveal that isolated subwavelength dielectric resonators support states with giant Q-factors similar to bound states in the continuum formed via destructive interference between strongly coupled eigenmodes and characterized by singularities of the Fano parameters.

Selective Third-Harmonic Generation by Structured Light in Mie-Resonant Nanoparticles

Abstract: We study the third-harmonic generation by structured light in subwavelength silicon nanoparticles which support both electric and magnetic multipolar Mie resonances. By tailoring the vectorial structure of the pumping light, we may control both strength and polarization composition of the excited harmonic fields. In this way, we generate nonlinear fields with radial or azimuthal polarizations by addressing selectively a different type of multipolar Mie resonances, also enhancing or suppressing the optically induced nonlinear magnetic response.

Electric-current-induced unidirectional propagation of surface plasmon-polaritons

Abstract: Nonreciprocity and one-way propagation of optical signals are crucial for modern nanophotonic technology, and typically achieved using magneto-optical effects requiring large magnetic biases. Here we suggest a fundamentally novel approach to achieve unidirectional propagation of surface plasmon-polaritons (SPPs) at metal-dielectric interfaces. We employ a direct electric current in metals, which produces a Doppler frequency shift of SPPs due to the uniform drift of electrons. This tilts the SPP dispersion, enabling one-way propagation, as well as zero and negative group velocities. The results are demonstrated for planar interfaces and cylindrical nanowire waveguides.

Meta-optics and bound states in the continuum

Abstract: We discuss the recent advances in meta-optics and nanophotonics associated with the physics of bound states in the continuum (BICs). Such resonant states appear due to a strong coupling between leaky modes in optical guiding structures being supported by subwavelength high-index dielectric Mie-resonant nanoantennas or all-dielectric metasurfaces. First, we review briefly very recent developments in the BIC physics in application to isolated subwavelength particles. We pay a special attention to novel opportunities for nonlinear nanophotonics due to the large field enhancement inside the particle volume creating the resonant states with high-quality (high-$Q$) factors, the so-called quasi-BIC, that can be supported by the subwavelength particles. Second, we discuss novel applications of the BIC physics to all-dielectric optical metasurfaces with broken-symmetry meta-atoms when tuning to the BIC conditions allows to enhance substantially the $Q$ factor of the flat-optics dielectric structures. We also present the original results on nonlinear high-$Q$ metasurfaces and predict that the frequency conversion efficiency can be boosted dramatically by smart engineering of the asymmetry parameter of dielectric metasurfaces in the vicinity of the quasi-BIC regime.

All-dielectric resonant metasurfaces with a strong toroidal response

Abstract: We demonstrate how to create all-dielectric metasurfaces with a strong toroidal response by arranging two types of nanodisks into asymmetric quadrumer clusters. We demonstrate that a strong axial toroidal response of the metasurface is related to conditions of the trapped (dark) mode that is excited due the symmetry breaking in the cluster. We study the correlation between the toroidal response and asymmetry in the metasurface and nanocluster geometries, which appears from the different diameters of nanodisks or notches introduced into the nanodisks.

Bound states in the continuum and Fano resonances in the strong mode coupling regime

Abstract: The study of resonant dielectric nanostructures with high refractive index is a new research direction in nanoscale optics and metamaterial-inspired nanophotonics. Because of the unique optically-induced electric and magnetic Mie resonances, high-index nanoscale structures are expected to complement or even replace different plasmonic components in a range of potential applications. Here we study strong coupling between modes of a single subwavelength high-index dielectric resonator and analyse the mode transformation and Fano resonances when resonator's aspect ratio varies. We demonstrate that strong mode coupling results in resonances with high quality factors, which are related to the physics of bound states in the continuum when the radiative losses are almost suppressed due to the Friedrich-Wintgen scenario of destructive interference. We explain the physics of these states in terms of multipole decomposition and show that their appearance is accompanied by drastic change of the far-field radiation pattern. We reveal a fundamental link between the formation of the high-quality resonances and peculiarities of the Fano parameter in the scattering cross-section spectra. Our theoretical findings are confirmed by microwave experiments for the scattering of a high-index cylindrical resonators with a tunable aspect ratio. The proposed mechanism of the strong mode coupling in single subwavelength high-index resonators accompanied by resonances with high quality factor helps to extend substantially functionalities of all-dielectric nanophotonics that opens new horizons for active and passive nanoscale metadevices.

Nanoscale Generation of White Light for Ultrabroadband Nanospectroscopy

Abstract: Achieving efficient localization of white light at the nanoscale is a major challenge due to the diffraction limit, and nanoscale emitters generating light with a broadband spectrum require complicated engineering. Here we suggest a simple, yet highly efficient, nanoscale white-light source based on a hybrid Si/Au nanoparticle with ultrabroadband (1.3–3.4 eV) spectral characteristics. We incorporate this novel source into a scanning-probe microscope and observe broadband spectrum of photoluminescence that allows fast mapping of local optical response of advanced nanophotonic structures with submicron resolution, thus realizing ultrabroadband near-field nanospectroscopy.

Multipolar second-harmonic generation by Mie-resonant dielectric nanoparticles

Abstract: By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation by individual high-index dielectric nanoparticles made of centrosymmetric materials Considering both bulk and surface nonlinearities, we describe second-harmonic nonlinear scattering from a silicon nanoparticle optically excited in the vicinity of the magnetic and electric dipolar resonances We discuss the contributions of different nonlinear sources and the effect of the low-order optical Mie modes on the characteristics of the generated far field We demonstrate that the multipolar expansion of the radiated field is dominated by dipolar and quadrupolar modes (two axially symmetric electric quadrupoles, an electric dipole, and a magnetic quadrupole) and the interference of these modes can ensure directivity of the nonlinear scattering The developed multipolar analysis can be instructive for interpreting the far-field measurements of the nonlinear scattering and it provides prospective insights into a design of complementary metal-oxide-semiconductor compatible nonlinear nanoantennas fully integrated with silicon-based photonic circuits, as well as methods of nonlinear diagnostics

Near-Field Coupling Effects in Mie-Resonant Photonic Structures and All-Dielectric Metasurfaces

Abstract: We reveal that strong near-field coupling effects can be observed for dissimilar Mie-resonant dielectric meta-atoms and demonstrate that both properties and functionalities of high-index all-dielectric photonic structures can be controlled by engineering their geometry and changing the distance between meta-atoms thus enhancing the effective magnetic response. We describe dielectric dimers, quadrumers, and metasurfaces with a staggered structure of optically induced magnetic moments (the so-called ”optical antiferromagnetism”) and also demonstrate that a strong toroidal response can be introduced in metasurfaces by engineering asymmetric nanoparticle quadrumers as building blocks for novel designs in all-dielectric resonant meta-optics.

A comparative analysis of surface and bulk contributions to second-harmonic generation in centrosymmetric nanoparticles

Abstract: Second-harmonic generation (SHG) from nanoparticles made of centrosymmetric materials provides an effective tool to characterize many important properties of photonic structures at the subwavelength scale. Here we study the relative contribution of surface and bulk effects to SHG for plasmonic and dielectric nanostructures made of centrosymmetric materials in both dispersive and non-dispersive regimes. Our calculations of the far-fields generated by the nonlinear surface and bulk currents reveal that the size of the nanoparticle strongly influences the amount and relative contributions of the surface and bulk SHG effects. Importantly, our study reveals that, whereas for plasmonic nanoparticles the surface contribution is always dominant, the bulk and surface SHG effects can become comparable for dielectric nanoparticles, and thus they both should be taken into account when analyzing nonlinear optical properties of all-dielectric nanostructures.

Locally Enhanced Image Quality with Tunable Hybrid Metasurfaces

Abstract: Metasurfaces represent a new paradigm in artificial subwavelength structures due to their potential to overcome many challenges typically associated with bulk metamaterials. The ability to make very thin structures and change their properties dynamically makes metasurfaces an exceptional meta-optics platform for engineering advanced electromagnetic and photonic metadevices. Here, we suggest and demonstrate experimentally a tunable metasurface capable of enhancing significantly the local image quality in magnetic resonance imaging. We present a design of the hybrid metasurface based on electromagnetically coupled dielectric and metallic elements. We demonstrate how to tailor the spectral characteristics of the metasurface eigenmodes by changing dynamically the effective permittivity of the structure. By maximizing a coupling between metasurface eigenmodes and transmitted and received fields in the magnetic resonance imaging (MRI) system, we enhance the device sensitivity that results in a substantial improvement of the image quality.

Transparent Dielectric Metasurfaces for Spatial Mode Multiplexing

Abstract: Expanding the use of physical degrees of freedom to employ spatial multiplexing of data in optical communication is considered to be the most disruptive and effective solution for meeting the capacity demand of the growing information traffic. Development of space division–multiplexing methods stimulated research on spatial encoding, detection, and processing of data, attracting interest from various fields of science. Here a passive all-dielectric metasurface with near-unity transmission is demonstrated that engineers spatial mode profiles, potentially of an arbitrary complexity. The broadband response of the metasurface covers all S, C, and L bands of fiber communications. Unlike conventional phase plates, the metasurface allows for both phase and polarization conversion, providing full flexibility for the mode engineering. The dielectric metasurface is employed for mode multiplexing in a free-space optical communication system with an extinction ratio in excess of 20 dB over the whole C-band with negligible penalty even for 100 Gb s−1 data transmission. These results merge two seemingly different fields, optical communication and metamaterials, and they suggest a novel approach for an ultimate miniaturization of mode multiplexers and advanced LiFi technologies.

Coexistence of collapse and stable spatiotemporal solitons in multimode fibers

Abstract: We analyze spatiotemporal solitons in multimode optical fibers and demonstrate the existence of stable solitons, in a sharp contrast to earlier predictions of collapse of multidimensional solitons in three-dimensional media. We discuss the coexistence of blow-up solutions and collapse stabilization by a low-dimensional external potential in graded-index media, and also predict the existence of stable higher-order nonlinear waves such as dipole-mode spatiotemporal solitons. To support the main conclusions of our numerical studies we employ a variational approach and derive analytically the stability criterion for input powers for the collapse stabilization.

Topological Floquet edge states in periodically curved waveguides

Abstract: We study the Floquet edge states in arrays of periodically curved optical waveguides described by the modulated Su-Schrieffer-Heeger model. Beyond the bulk-edge correspondence, our study explores the interplay between band topology and periodic modulations. By analyzing the quasienergy spectra and Zak phase, we reveal that, although topological and nontopological edge states can exist for the same parameters, they cannot appear in the same spectral gap. In the high-frequency limit, we find analytically all boundaries between the different phases and study the coexistence of topological and nontopological edge states. In contrast to unmodulated systems, the edge states appear due to either band topology or modulation-induced defects. This means that periodic modulations may not only tune the parametric regions with nontrivial topology, but may also support novel edge states.

Toward Silicon-Based Metamaterials

Abstract: We study periodic lattices of silicon nanorods and introduce the concept of a phase diagram that characterizes a transition between the regimes of photonic crystals and the dielectric metamaterials when the lattice spacing and operational wavelength vary. We find the conditions when a hexagonal periodic lattice of silicon nanorods can operate as a metamaterial described by averaged parameters. In general, we reveal that the metamaterial regime can be achieved for dielectric permittivity exceeding the value e = 14, being commonly available for semiconductors in both visible and near-infrared frequency ranges. Thus, advanced semiconductor technologies can offer a versatile platform for novel designs of all-dielectric Mie-resonant metadevices.