Journal ArticleDOI
Carbon quantum dots/TiO2 composites for efficient photocatalytic hydrogen evolution
Huijun Yu,Yufei Zhao,Chao Zhou,Lu Shang,Yong Peng,Yinhu Cao,Li-Zhu Wu,Chen-Ho Tung,Tierui Zhang +8 more
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TLDR
In this article, carbon quantum dots modified P25 TiO2 composites (CQDs/P25) with a "dyade"-like structure were prepared via a facile one-step hydrothermal reaction.Abstract:
Carbon quantum dots modified P25 TiO2 composites (CQDs/P25) with a “dyade”-like structure were prepared via a facile one-step hydrothermal reaction. CQDs/P25 exhibited improved photocatalytic H2 evolution under UV-Vis and visible light (λ > 450 nm) irradiation without loading any noble metal cocatalyst, compared to pure P25. A possible mechanism of the photocatalytic H2 production activity over CQDs/P25 was proposed based on detailed measurements of the transient photocurrent response, surface photovoltage and hydroxyl radicals. CQDs play dual roles on the improved photocatalytic activity of CQDs/P25. Under UV-Vis light irradiation CQDs act as an electron reservoir to improve the efficient separation of the photoinduced electron–hole pairs of P25. However, under visible light irradiation CQDs act as a photosensitizer to sensitize P25 into a visible light response “dyade” structure for H2 evolution.read more
Citations
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Carbon quantum dots: synthesis, properties and applications
Youfu Wang,Aiguo Hu +1 more
TL;DR: Carbon quantum dots (CQDs, C-dots or CDs) have found wide use in more and more fields during the last few years as discussed by the authors, focusing on their synthetic methods, size control, modification strategies, photoelectric properties, luminescent mechanism, and applications in biomedicine, optronics, catalysis and sensor issues.
Journal ArticleDOI
Particulate Photocatalysts for Light-Driven Water Splitting: Mechanisms, Challenges, and Design Strategies
TL;DR: This review illustrates that it is possible to employ the fundamental principles underlying photosynthesis and the tools of chemical and materials science to design and prepare photocatalysts for overall water splitting.
Journal ArticleDOI
Carbon and Graphene Quantum Dots for Optoelectronic and Energy Devices: A Review
TL;DR: In this article, recent exciting progresses on CD and GQD-based optoelectronic and energy devices, such as light emitting diodes (LEDs), solar cells (SCs), photodetctors (PDs), photocatalysis, batteries, and supercapacitors are highlighted.
Journal ArticleDOI
Recent progress in carbon quantum dots: synthesis, properties and applications in photocatalysis
TL;DR: In this paper, the authors discuss the challenges and future direction of CQD-based materials in this booming research field, with a perspective toward the ultimate achievement of highly efficient and long-term stable carbon quantum dot-based photocatalysts.
Journal ArticleDOI
Dual Cocatalysts in TiO 2 Photocatalysis.
TL;DR: Concluding perspectives on the challenges and opportunities for the further exploration of dual cocatalyst-modified TiO2 photocatalysts are presented.
References
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Journal ArticleDOI
Visible-Light Photocatalysis in Nitrogen-Doped Titanium Oxides
TL;DR: Film and powders of TiO2-x Nx have revealed an improvement over titanium dioxide (TiO2) under visible light in optical absorption and photocatalytic activity such as photodegradations of methylene blue and gaseous acetaldehyde and hydrophilicity of the film surface.
Journal ArticleDOI
Highly Photoluminescent Carbon Dots for Multicolor Patterning, Sensors, and Bioimaging
Shoujun Zhu,Qingnan Meng,Lei Wang,Junhu Zhang,Yubin Song,Han Jin,Kai Zhang,Hongchen Sun,Hai-Yu Wang,Bai Yang +9 more
TL;DR: A facile and highoutput strategy for the fabrication of CDs, which is suitable for industrial-scale production and is almost equal to fluorescent dyes, is discussed.
Journal ArticleDOI
P25-Graphene Composite as a High Performance Photocatalyst
TL;DR: A chemically bonded TiO(2) (P25)-graphene nanocomposite photocatalyst with graphene oxide and P25, using a facile one-step hydrothermal method could provide new insights into the fabrication of a TiO (2)-carbon composite as high performance photocatalysts and facilitate their application in the environmental protection issues.
Journal ArticleDOI
Graphene-Like Carbon Nitride Nanosheets for Improved Photocatalytic Activities
TL;DR: In this article, a top-down thermal oxidation etching of bulk g-C3N4 in air has been shown to improve the photocatalytic activities of the material in terms of OH radical generation and hydrogen evolution.
Journal ArticleDOI
Water‐Soluble Fluorescent Carbon Quantum Dots and Photocatalyst Design
Haitao Li,Xiaodie He,Zhenhui Kang,Zhenhui Kang,Hui Huang,Yang Liu,Yang Liu,Jinglin Liu,Suoyuan Lian,Chi Him A. Tsang,Xiao-Bao Yang,Shuit-Tong Lee +11 more
TL;DR: The facile one-step alkali-assisted electrochemical fabrication of CQDs with sizes of 1.2– 3.8 nm which possess size-dependent photoluminescence (PL) and excellent upconversion luminescence properties are reported and the design of photocatalysts is demonstrated to harness the use of the full spectrum of sunlight.
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