Journal ArticleDOI
Early-stage evaluation of emerging CO2 utilization technologies at low technology readiness levels
Kosan Roh,André Bardow,Dominik Bongartz,Jannik Burre,Won-Suk Chung,Sarah Deutz,Dongho Han,Matthias Heßelmann,Yannik Kohlhaas,Andrea König,Jeehwan S. Lee,Raoul Meys,Simon Völker,Matthias Wessling,Matthias Wessling,Jay H. Lee,Alexander Mitsos,Alexander Mitsos +17 more
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TLDR
Most CO2 utilization technologies are at low technology readiness levels (TRLs), and screening to identify the most promising technologies should be conducted before allocating large RD co-electrolysis of CO2 and water for ethylene production as discussed by the authors.About:
This article is published in Green Chemistry.The article was published on 2020-06-22. It has received 59 citations till now.read more
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Techno-economic assessment of low-temperature carbon dioxide electrolysis
TL;DR: In this article, the authors provide a comprehensive techno-economic assessment of four major products and prioritizes the technological development with systematic guidelines to facilitate the market deployment of low-temperature CO2 electrolysis.
Journal ArticleDOI
Electrochemical Routes for the Valorization of Biomass-Derived Feedstocks: From Chemistry to Application
Francisco Willian de Souza Lucas,R. Gary Grim,Sean A. Tacey,Courtney A. Downes,Joseph C. Hasse,Alex M. Román,Carrie A. Farberow,Joshua A. Schaidle,Adam Holewinski +8 more
TL;DR: The drive to reduce consumption of fossil resources, coupled with expanding capacity for renewable electricity, invites the exploration of new routes to utilize this energy for the sustainable prod... as mentioned in this paper, where the authors propose a new route for renewable energy for transportation.
Journal ArticleDOI
Integration of techno-economic analysis and life cycle assessment for sustainable process design – A review
TL;DR: The current state-of-the-art in TEA and LCA is reviewed to identify the methodological challenges of TEA-LCA integration approaches and Lack of consistent methodological guidelines and compatible software tools, inconsistent system boundary and functional unit selection, limited data availability and uncertainty are key methodological challenges for integration of LCA and TEA.
Journal ArticleDOI
Limits to Paris compatibility of CO2 capture and utilization
Kiane de Kleijne,Steef V. Hanssen,Lester van Dinteren,Mark A. J. Huijbregts,Rosalie van Zelm,Heleen de Coninck +5 more
TL;DR: In this paper , the authors investigated which CO2 capture and utilization (CCU) technologies are Paris compatible, based on life cycle emissions and technological maturity criteria and found that CCU with technology readiness levels (TRLs) of 6 or higher can be Paris compatible in 2030 for construction materials, enhanced oil recovery, horticulture industry, and some chemicals.
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Comparative life cycle assessment of electrochemical upgrading of CO2 to fuels and feedstocks
TL;DR: In this article, the authors present a comparative cradle-to-gate life cycle assessment (LCA) of one and two-step electrochemical conversion of CO2 to eight major value-added products; wherein they consider CO2 capture, conversion and product separation in their process model.
References
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Journal ArticleDOI
CO2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Cao-Thang Dinh,Thomas Burdyny,Golam Kibria,Ali Seifitokaldani,Christine M. Gabardo,F. Pelayo García de Arquer,Amirreza Kiani,Jonathan P. Edwards,Phil De Luna,Oleksandr S. Bushuyev,Chengqin Zou,Chengqin Zou,Rafael Quintero-Bermudez,Yuanjie Pang,David Sinton,Edward H. Sargent +15 more
TL;DR: A copper electrocatalyst at an abrupt reaction interface in an alkaline electrolyte reduces CO2 to ethylene with 70% faradaic efficiency at a potential of −0.55 volts versus a reversible hydrogen electrode (RHE).
Journal ArticleDOI
Sustainable Conversion of Carbon Dioxide: An Integrated Review of Catalysis and Life Cycle Assessment
Jens Artz,Thomas Müller,Katharina Thenert,Johanna Kleinekorte,Raoul Meys,André Dirk Sternberg,André Bardow,Walter Leitner,Walter Leitner +8 more
TL;DR: The motivation to develop CO2-based chemistry does not depend primarily on the absolute amount of CO2 emissions that can be remediated by a single technology and is stimulated by the significance of the relative improvement in carbon balance and other critical factors defining the environmental impact of chemical production in all relevant sectors in accord with the principles of green chemistry.
Journal ArticleDOI
Review on methanation – From fundamentals to current projects
Stefan Rönsch,Jens Schneider,Steffi Matthischke,Michael Schlüter,M. Götz,J. Lefebvre,Praseeth Prabhakaran,Siegfried Bajohr +7 more
TL;DR: A comprehensive overview of methanation research conducted during the last century is presented in this paper, where application-oriented research focusing on reactor developments, reactor modeling, and pilot plant investigation is reviewed.
Journal ArticleDOI
The cost of CO2 capture and storage
TL;DR: In this paper, the authors assess the current costs of CO2 capture and storage for new fossil fuel power plants and compare those results to the costs reported a decade ago in the IPCC Special Report on Carbon Dioxide Capture and Storage (SRCCS).