Electric-Field Controllable Metal-free Materials as Efficient Electrocatalysts for Nitrogen Fixation
Jie Wu,Yang-Xin Yu +1 more
Reads0
Chats0
About:
This article is published in Journal of Physical Chemistry C.The article was published on 2021-11-04 and is currently open access. It has received 21 citations till now. The article focuses on the topics: Electric field.read more
Citations
More filters
Journal ArticleDOI
Methylene blue adsorption derived thermal insulating N, S-co-doped TiC/carbon hybrid aerogel for high-efficient absorption-dominant electromagnetic interference shielding
Zhengzheng Guo,Peng-Gang Ren,Jin Wang,Xin Hou,Jiahui Tang,Zongbin Liu,Zhengyan Chen,Yanling Jin,Fang Ren +8 more
TL;DR: In this article , a facile and environmentally friendly approach was proposed to fabricate N, S-co-doped TiC/carbon hybrid aerogels with hierarchically porous architecture through MXene/cellulose hybrid hydrogels as precursors for adsorbing dyes, followed by freeze drying and carbonization process.
Journal ArticleDOI
Multi-level Descriptor Construction for Screening Eligible Single-Atom-Embedded Ternary B3C2P3 Monolayers as Nitrogen Fixation Catalysts
Journal ArticleDOI
Anchoring boron on a covalent organic framework as an efficient single atom metal-free photo-electrocatalyst for nitrogen fixation: a first-principles analysis.
Supriti Dutta,Swapan K. Pati +1 more
TL;DR: By employing density functional theory, the authors in this paper demonstrated that N2 can be efficiently activated on the B center due to the synergistic effect of B-N. And they found that the NRR happens predominantly by the alternating path with a small limiting potential of 0.13 V.
Journal ArticleDOI
Theoretical prediction on stability, electronic and activity properties of single-atom catalysts anchored graphene and boron phosphide heterostructures
Yanan Tang,Weiguang Chen,Ming Yu Zhao,Jinlei Shi,Yingqi Cui,Zhaohan Li,Zhiwen Wang,Zhenzhe Feng,Xianqi Dai +8 more
TL;DR: In this paper , the effects of added graphene substrate on its electronic property and sensitivity toward the gas reactants are compared with those on BP-TM and BP-SV-TM.
References
More filters
Journal ArticleDOI
High-performance artificial nitrogen fixation at ambient conditions using a metal-free electrocatalyst
Weibin Qiu,Weibin Qiu,Xiao-Ying Xie,Jian-Ding Qiu,Wei-Hai Fang,Ru-Ping Liang,Xiang Ren,Xuqiang Ji,Guanwei Cui,Abdullah M. Asiri,Ganglong Cui,Bo Tang,Xuping Sun +12 more
TL;DR: A metal-free catalyst that selectively reduces nitrogen to ammonia with high efficiency and stability is reported, placing it among the most active aqueous-based nitrogen reduction reaction electrocatalysts.
Journal ArticleDOI
Recent Advances and Challenges of Electrocatalytic N2 Reduction to Ammonia.
Geletu Qing,Reza Ghazfar,Shane T. Jackowski,Faezeh Habibzadeh,Mona Maleka Ashtiani,Chuan Pin Chen,Milton R. Smith,Thomas W. Hamann +7 more
TL;DR: This review provides a comprehensive account of theoretical and experimental studies on electrochemical nitrogen fixation with a focus on the low selectivity for reduction of N2 to ammonia versus protons to H2.
Journal ArticleDOI
Phase coexistence and metal-insulator transition in few-layer phosphorene: a computational study.
Jie Guan,Zhen Zhu,David Tománek +2 more
TL;DR: Based on ab initio density functional calculations, γ-P and δ-P are proposed as two additional stable structural phases of layered phosphorus besides the layered α-P (black) and β- P (blue) phosphorus allotropes.
Journal ArticleDOI
Tackling the Activity and Selectivity Challenges of Electrocatalysts toward the Nitrogen Reduction Reaction via Atomically Dispersed Biatom Catalysts
TL;DR: By means of large-scale density functional theory (DFT) computations, a descriptor-based design principle is reported to explore the large composition space of two-dimensional (2D) bi-atom catalysts (BACs) and identify three homonuclear and 28 heteronuclear BACs which could break the metal-based activity benchmark towards efficient NRR.
Journal ArticleDOI
Single-boron catalysts for nitrogen reduction reaction
Chuangwei Liu,Qinye Li,Chengzhang Wu,Jie Zhang,Yonggang Jin,Douglas R. MacFarlane,Chenghua Sun +6 more
TL;DR: Single boron atoms supported on graphene and substituted into h-MoS2 are identified as the most promising NRR catalysts, offering excellent energy efficiency and selectivity against hydrogen evolution reaction.