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Interlayer Material Selection for Lithium-Sulfur Batteries

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TLDR
In this article, a review of the advanced interlayer systems is presented, and the operating mechanisms and widespread availability of interlayers in lithium-sulfur batteries are concluded.
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This article is published in Joule.The article was published on 2019-02-20 and is currently open access. It has received 340 citations till now.

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Guidelines and trends for next-generation rechargeable lithium and lithium-ion batteries.

TL;DR: This review summarizes the current trends and provides guidelines towards achieving next-generation rechargeable Li and Li-ion batteries with higher energy densities, better safety characteristics, lower cost and longer cycle life by addressing batteries using high-voltage cathodes, metal fluoride electrodes, chalcogen electrodes, Li metal anodes, high-capacity anodes as well as useful electrolyte solutions.
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Single Atom Array Mimic on Ultrathin MOF Nanosheets Boosts the Safety and Life of Lithium-Sulfur Batteries.

TL;DR: A "single atom array mimic" on ultrathin metal organic framework (MOF) nanosheet-based bifunctional separator for achieving the highly safe and long life Li-S batteries.
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Rational Design of a Ni3N0.85 Electrocatalyst to Accelerate Polysulfide Conversion in Lithium-Sulfur Batteries.

TL;DR: The high efficiency of rationally-designed Ni3N0.85 demonstrates the effectiveness of the d-band tuning strategy to de-velop low-activation-energy catalysts and to promote the atomic understanding of polysulfides conversion in Li-S batteries.
References
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Journal ArticleDOI

A highly efficient polysulfide mediator for lithium-sulfur batteries.

TL;DR: A strategy to entrap polysulfides in the cathode that relies on a chemical process, whereby a host--manganese dioxide nanosheets serve as the prototype--reacts with initially formed lithium polysolfides to form surface-bound intermediates, which are among the best reported to date.
PatentDOI

Graphene oxide as a sulfur immobilizer in high performance lithium/sulfur cells

TL;DR: In this article, a chemical approach to immobilize sulfur and lithium polysulfides via the reactive functional groups on graphene oxide was proposed, which obtains a uniform and thin (˜tens of nanometers) sulfur coating.
Journal ArticleDOI

Liquid electrolyte lithium/sulfur battery: Fundamental chemistry, problems, and solutions

TL;DR: Li et al. as discussed by the authors discussed the problems and solutions of liquid electrolyte Li/S battery and showed that the dissolution of lithium polysulfide (PS) is essential for the performance of a Li-S cell.
Journal ArticleDOI

Lithium–sulphur batteries with a microporous carbon paper as a bifunctional interlayer

TL;DR: A simple adjustment to the traditional lithium-sulphur battery configuration is reported to achieve high capacity with a long cycle life and rapid charge rate and with a significant improvement not only in the active material utilization but also in capacity retention without involving complex synthesis or surface modification.
Journal ArticleDOI

The synergetic effect of lithium polysulfide and lithium nitrate to prevent lithium dendrite growth

TL;DR: It is demonstrated that a stable and uniform solid electrolyte interphase layer is formed due to a synergetic effect of both lithium polysulfide and lithium nitrate as additives in ether-based electrolyte, preventing dendrite growth and minimizing electrolyte decomposition.
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