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Near-infrared to ultra-violet frequency conversion in chalcogenide metasurfaces.

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TLDR
In this article, a phase locking mechanism between the pump and the inhomogeneous portion of the third harmonic signal is proposed to enable near-infrared to ultraviolet frequency conversion in an As2S3-based metasurface.
Abstract
Chalcogenide photonics offers unique solutions for a broad range of applications from mid-infrared sensing to integrated, ultrafast, ultrahigh-bandwidth signal processing. However, to date its usage has been limited to the infrared part of the electromagnetic spectrum, thus avoiding ultraviolet and visible ranges due to absorption of chalcogenide glasses. Here, we experimentally demonstrate and report near-infrared to ultraviolet frequency conversion in an As2S3-based metasurface, enabled by a phase locking mechanism between the pump and the inhomogeneous portion of the third harmonic signal. Due to the phase locking, the inhomogeneous component co-propagates with the pump pulse and encounters the same effective dispersion as the infrared pump, and thus experiences little or no absorption, consequently opening previously unexploited spectral range for chalcogenide glass science and applications, despite the presence of strong material absorption in this range. The use of chalcogenide glass in optical science and applications at the UV frequencies has been so far hindered by its absorption in this spectral region. Here the authors demonstrate that a nanostructured chalcogenide glass can efficiently generate third harmonic radiation, leading to a strong UV light source at the nanoscale.

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Journal ArticleDOI

Recent Advances in Tunable Metasurfaces: Materials, Design, and Applications.

TL;DR: In this paper , a review of recent advances in tunable metasurfaces in terms of the active materials and tuning mechanisms, design methodologies, and practical applications is presented.
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Soliton Microcombs in Integrated Chalcogenide Microresonators

TL;DR: In this paper , a home-developed chalcogenide glasses-Ge25Sb10S65 (GeSbS) for nonlinear photonic integration and for dissipative soliton microcomb generation is presented.
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Integrated Chalcogenide Photonics for Microresonator Soliton Combs

TL;DR: In this article , a chalcogenide glass, Ge25Sb10S65 (GeSbS), is presented for nonlinear photonic integration and for dissipative soliton microcomb generation.
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The past, present and future of photonic glasses: A review in homage to the United Nations International Year of Glass 2022

TL;DR: A review of the past, present, and future of photonic glasses can be found in this article , where the authors pay homage to the United Nations International Year of Glass 2022.
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All-optical tunable wavelength conversion in opaque nonlinear nanostructures

TL;DR: In this paper , a femtosecond-scale wavelength tunable, subwavelength-thick nanostructure that performs efficient wavelength conversion from the infrared to the ultraviolet was demonstrated.
References
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Journal ArticleDOI

Optical properties and applications of chalcogenide glasses: a review

TL;DR: In this paper, a review of chalcogenide glasses and the current status of their applications is given, and the possibilities of fabricating active devices, such as fiber amplifiers and lasers, are presented.
Journal ArticleDOI

Light waves at the boundary of nonlinear media

TL;DR: In this paper, a nonlinear plane parallel slab is presented which describes the harmonic generation in experimental situations, and an integral equation formulation for wave propagation in nonlinear media is sketched.
Journal ArticleDOI

Ultraviolet Communications: Potential and State-Of-The-Art

TL;DR: This article presents the state-of-the-art of associated systems and their components and discusses related issues including communication link characterization, channel modeling, and link capacity study, as well as transceiver design, link duplexing, multiple access, and networking.
Journal ArticleDOI

Active and passive chalcogenide glass optical fibers for IR applications: a review

TL;DR: In this article, the authors asserted that the research and development of chalcogenide glasses will grow in the foreseeable future, especially with respect to improvements in the optical quality of the fibers and the performance of the fiber in existing and future applications.
Journal ArticleDOI

Second- and third-harmonic generation in metal-based structures

TL;DR: In this article, a theoretical approach to the study of second and third harmonic generation from metallic structures and nanocavities filled with a nonlinear material in the ultrashort pulse regime is presented.
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