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Showing papers on "Brillouin zone published in 2023"


Journal ArticleDOI
TL;DR: In this paper , the experimental observation of antichiral surface states by constructing a 3D modified Haldane model in a magnetic Weyl photonic crystal with two pairs of frequency-shifted Weyl points (WPs) was reported.
Abstract: Chiral edge states that propagate oppositely at two parallel strip edges are a hallmark feature of Chern insulators which were first proposed in the celebrated two-dimensional (2D) Haldane model. Subsequently, counterintuitive antichiral edge states that propagate in the same direction at two parallel strip edges were discovered in a 2D modified Haldane model. Recently, chiral surface states, the 2D extension of one-dimensional (1D) chiral edge states, have also been observed in a photonic analogue of a 3D Haldane model. However, despite many recent advances in antichiral edge states and chiral surface states, antichiral surface states, the 2D extension of 1D antichiral edge states, have never been realized in any physical system. Here, we report the experimental observation of antichiral surface states by constructing a 3D modified Haldane model in a magnetic Weyl photonic crystal with two pairs of frequency-shifted Weyl points (WPs). The 3D magnetic Weyl photonic crystal consists of gyromagnetic cylinders with opposite magnetization in different triangular sublattices of a 3D honeycomb lattice. Using microwave field-mapping measurements, unique properties of antichiral surface states have been observed directly, including the antichiral robust propagation, tilted surface dispersion, a single open Fermi arc connecting two projected WPs and a single Fermi loop winding around the surface Brillouin zone (BZ). These results extend the scope of antichiral topological states and enrich the family of magnetic Weyl semimetals.

3 citations


Journal ArticleDOI
TL;DR: In this article , the spin state of organic linkers and the symmetry/topology of crystal lattices were used to predict a class of multifunctional semiconductors in 2D Cr(II) five-membered heterocyclic metal organic frameworks that simultaneously possess auxetic effect, room-temperature ferrimagnetism, chiral ferroelectricity (FE), electrically reversible spin polarization, and topological nodal lines/points.
Abstract: Two-dimensional (2D) semiconductors (SCs) integrated with two or more functions are the cornerstone for constructing multifunctional nanodevices but remain largely limited. Here, by tuning the spin state of organic linkers and the symmetry/topology of crystal lattices, we predict a class of unprecedented multifunctional SCs in 2D Cr(II) five-membered heterocyclic metal organic frameworks that simultaneously possess auxetic effect, room-temperature ferrimagnetism, chiral ferroelectricity (FE), electrically reversible spin polarization, and topological nodal lines/points. Taking 2D Cr(TDZ)2 (TDZ = 1.2.5-thiadiazole) as an exemplification, the auxetic effect is produced by the antitetra-chiral lattice structure. The high temperature ferrimagnetism originates from the strong d-p direct magnetic exchange interaction between Cr cations and TDZ doublet radical anions. Meanwhile, the clockwise-counterclockwise alignment of TDZ's dipoles results in unique 2D chiral FE with atomic-scale vortex-antivortex states. 2D Cr(TDZ)2 is an intrinsic bipolar magnetic SC where half-metallic conduction with switchable spin-polarization direction can be induced by applying a gate voltage. In addition, the symmetry of the little group C4 of the lattice structure endows 2D Cr(TDZ)2 with topological nodal lines and a quadratic nodal point in the Brillouin zone near the Fermi level.

3 citations


Journal ArticleDOI
TL;DR: In this paper , the electronic band structure of kagome lattice superconductor has been investigated with high-frequency measurements in pulsed fields up to 86 T. The high-field data reveal a sequence of magnetic breakdown orbits that allow the construction of a model for the folded Fermi surface of the superconductivity.
Abstract: The recently discovered layered kagome metals of composition $A{\mathrm{V}}_{3}{\mathrm{Sb}}_{5}$ ($A=\mathrm{K}$, Rb, Cs) exhibit a complex interplay among superconductivity, charge density wave order, topologically nontrivial electronic band structure and geometrical frustration. Here, we probe the electronic band structure underlying these exotic correlated electronic states in ${\mathrm{CsV}}_{3}{\mathrm{Sb}}_{5}$ with quantum oscillation measurements in pulsed fields up to 86 T. The high-field data reveal a sequence of magnetic breakdown orbits that allows the construction of a model for the folded Fermi surface of ${\mathrm{CsV}}_{3}{\mathrm{Sb}}_{5}$. The dominant features are large triangular Fermi surface sheets that cover almost half the folded Brillouin zone. These sheets have not yet been detected in angle resolved photoemission spectroscopy and display pronounced nesting. The Berry phases of the electron orbits have been deduced from Landau level fan diagrams near the quantum limit without the need for extrapolations, thereby unambiguously establishing the nontrivial topological character of several electron bands in this kagome lattice superconductor.

3 citations


Journal ArticleDOI
TL;DR: In this article , the Brillouin zone folding-induced BICs (BZF-BICs) were proposed to achieve sustainable ultra-high Q factors by engineering BrillouIN zone folding induced BIC, where all the guided modes are folded into the light cone through periodic perturbation.
Abstract: Non-radiative bound states in the continuum (BICs) allow construction of resonant cavities with confined electromagnetic energy and high-quality (Q) factors. However, the sharp decay of the Q factor in the momentum space limits their usefulness for device applications. Here we demonstrate an approach to achieve sustainable ultrahigh Q factors by engineering Brillouin zone folding-induced BICs (BZF-BICs). All the guided modes are folded into the light cone through periodic perturbation that leads to the emergence of BZF-BICs possessing ultrahigh Q factors throughout the large, tunable momentum space. Unlike conventional BICs, BZF-BICs show perturbation-dependent dramatic enhancement of the Q factor in the entire momentum space and are robust against structural disorders. Our work provides a unique design path for BZF-BIC-based silicon metasurface cavities with extreme robustness against disorder while sustaining ultrahigh Q factors, offering potential applications in terahertz devices, nonlinear optics, quantum computing, and photonic integrated circuits.

3 citations


Journal ArticleDOI
TL;DR: In this paper , the authors showed that the pump power density is the limiting factor in narrowing the Stokes linewidth of a short-pulse laser, and they used a wide Brillouin gain to obtain a wider range of linewirths.
Abstract: As an effective means to obtain a narrow-linewidth laser, stimulated Brillouin scattering (SBS) has not only the advantages of pulse compression but also controllable Stokes linewidth output. However, most research thus far has been focused on continuous-wave lasers, with little emphasis on short-pulse lasers. This work demonstrates that the Brillouin gain linewidth and pump power density are the primary factors affecting the linewidth of the Stokes pulse. As the pump power density increases, the Stokes linewidth tends to narrow and approaches the pump linewidth. This is the first study to reveal that the pump linewidth is the limiting factor in narrowing the Stokes linewidth. The Stokes linewidths of different liquid media were compared, and it was found that media with a wide Brillouin gain linewidth can be used to obtain lasers with a wider range of linewidths.

2 citations


Journal ArticleDOI
TL;DR: In this paper , the Brillouin light-scattering spectroscopy under microwave irradiation was used to resolve sets of discrete resonances in the center of nanotubes ranging from 2.5 to 12.5 GHz.
Abstract: We report experimental studies of spin-wave excitations in individual 22-nm-thick ${\mathrm{Ni}}_{80}{\mathrm{Fe}}_{20}$ nanotubes with diameters of about 150 nm. We apply Brillouin light-scattering spectroscopy under microwave irradiation, and we resolve sets of discrete resonances in the center of nanotubes ranging from 2.5 to 12.5 GHz. Comparing to a recent theoretical work and micromagnetic simulations, we identify different characteristic eigenmodes depending on the axial, mixed, or vortex configuration. The mixed and vortex states give rise to modes with helical phase profiles substantiating an unusual nature of confined modes attributed to nonreciprocal spin waves. Our findings provide microscopic insight into realistic tubular spin-wave nanocavities and magnetochiral effects for three-dimensional nanomagnonics.

2 citations


Journal ArticleDOI
TL;DR: In this paper , a combined Brillouin light scattering (BLS) and micromagnetic simulation investigation of the magnetic-field-dependent spin-wave spectra in a hybrid structure made of permalloy (NiFe) artificial spin-ice (ASI) systems, composed of stadium-shaped nanoislands, deposited on the top of an unpatterned permallioy film with a nonmagnetic spacer layer.
Abstract: We present a combined Brillouin light scattering (BLS) and micromagnetic simulation investigation of the magnetic-field-dependent spin-wave spectra in a hybrid structure made of permalloy (NiFe) artificial spin-ice (ASI) systems, composed of stadium-shaped nanoislands, deposited on the top of an unpatterned permalloy film with a nonmagnetic spacer layer. The thermal spin-wave spectra were recorded by BLS as a function of the magnetic field applied along the symmetry direction of the ASI sample. Magneto-optic Kerr effect magnetometry was used to measure the hysteresis loops in the same orientation as the BLS measurements. The frequency and the intensity of several spin-wave modes detected by BLS were measured as a function of the applied magnetic field. Micromagnetic simulations enabled us to identify the modes in terms of their frequency and spatial symmetry and to extract information about the existence and strength of the dynamic coupling, relevant only to a few modes of a given hybrid system. Using this approach, we suggest a way to understand if the dynamic coupling between ASI and film modes is present or not, with interesting implications for the development of future three-dimensional magnonic applications and devices.

2 citations


Journal ArticleDOI
01 Feb 2023-Sensors
TL;DR: In this paper , an image denoising method using the convolutional neural network (CNN) is applied to the derived Brillouin gain spectrum images to enhance the performance of the frequency shift detection and the strain vibration measurement of the BOTDR system.
Abstract: The Brillouin optical time domain reflectometry (BOTDR) system measures the distributed strain and temperature information along the optic fibre by detecting the Brillouin gain spectra (BGS) and finding the Brillouin frequency shift profiles. By introducing small gain stimulated Brillouin scattering (SBS), dynamic measurement using BOTDR can be realized, but the performance is limited due to the noise of the detected information. An image denoising method using the convolutional neural network (CNN) is applied to the derived Brillouin gain spectrum images to enhance the performance of the Brillouin frequency shift detection and the strain vibration measurement of the BOTDR system. By reducing the noise of the BGS images along the length of the fibre under test with different network depths and epoch numbers, smaller frequency uncertainties are obtained, and the sine-fitting R-squared values of the detected strain vibration profiles are also higher. The Brillouin frequency uncertainty is improved by 24% and the sine-fitting R-squared value of the obtained strain vibration profile is enhanced to 0.739, with eight layers of total depth and 200 epochs.

2 citations


Journal ArticleDOI
Ralf Sorg1
TL;DR: In this paper , the authors explored the first three WC-type topological semimetal compounds in transition metal oxides and studied their structural, thermodynamic, elastic, electronic, and dynamical properties systematically.

2 citations


Journal ArticleDOI
TL;DR: In this paper , the authors anatomize the bulk properties of one-dimensional multiband non-Hermitian systems under open-boundary condition (OBC) and obtain a general expression of Green's functions based on such EBBs and generalized Brillouin zones.
Abstract: Although the non-Bloch band theory is a milestone in elaborating bulk energy bands of non-Hermitian systems under the open-boundary condition (OBC), vital issues related to multivalued functions of non-Hermitian energy bands remain unsolved. In this paper, we anatomize the bulk properties of one-dimensional multiband non-Hermitian systems under OBC. We put forward the energy-band branches (EBBs) to settle the multivalued functions of non-Hermitian energy bands, which become gapped or gapless corresponding to disconnected or connected EBBs in the complex energy plane, where the branch points and branch cuts play a crucial role. We clarify the precise significance of the non-Hermitian skin effect, which illustrates the asymptotic behavior of EBB eigenstates (bulk eigenstates) in the deep bulk and compensates previous non-Bloch band theory. We also obtain a general expression of open-boundary Green's functions based on such EBBs and generalized Brillouin zones, useful for studies on non-Hermitian dynamical evolution.

2 citations


Journal ArticleDOI
TL;DR: In this paper , the authors numerically demonstrate that LNOI waveguides may support confined short-wavelength surface acoustic waves that interact strongly with optical fields through backward stimulated Brillouin scattering in both $Z$ and $X$-cut orientation.
Abstract: We numerically demonstrate that Lithium Niobate on Insulator (LNOI) waveguides may support confined short-wavelength surface acoustic waves that interact strongly with optical fields through backward stimulated Brillouin scattering in both $Z$ and $X$-cut orientation. We conduct fully anisotropic simulations that consider not only moving boundary and photoelastic forces, but also roto-optic forces for the Brillouin interaction. Our results indicate that photoelasticity dominates the Brillouin gain and can reach as high as $G_{B}/Q_{m}$ = 0.43 W$^{-1}$m$^{-1}$ in standard ridge waveguides

Journal ArticleDOI
TL;DR: In this article, an exact strain gradient (SG) continuum model was proposed to capture the broadband bandgap characteristics of the prestressed diatomic lattice (PDL) with local/nonlocal interactions.
Abstract: Abstract In this article, an exact strain gradient (SG) continuum model to capture the broadband bandgap characteristics of the prestressed diatomic lattice (PDL) with local/nonlocal interactions has been proposed. By considering the periodicity of wave motion, the wavelength-dependent Taylor expansion is established, leading to a desirable prediction when the wavelength is close to the lattice scale. For PDL, the dispersion curves of the proposed continuum model are always consistent with those of discrete model in the first Brillouin zone. The proposed SG continuum model is used to investigate the effects of structural parameters, orders of SG continua and various nonlocal interactions on bandgap properties of PDL. Highlights Continuum modelling of prestressed acoustic diatomic lattices. Perfect agreements achieved between dispersion diagrams by discrete and proposed continuum models. Effects of prestress, nonlocal interactions, mass and stiffness ratios on band gap structures analyzed. Proper strain gradient (SG) orders determined to guarantee a satisfactory accuracy.

Journal ArticleDOI
TL;DR: In this article , the first principles study of double perovskites Ba2MgPdO6 and Ba2mgPtO6 has been performed utilizing the concepts of Density Functional Theory (DFT).

Journal ArticleDOI
TL;DR: In this paper , an ideal acoustic spin Hall (QSH) with gapless behavior was constructed by constructing a global Tf on both the bulk and the boundary based on bilayer structures, and the ideal QSH phase behaves as a topological phase transition plane that bridges trivial and higher-order phases.
Abstract: Fermionic time-reversal symmetry ([Formula: see text])-protected quantum spin Hall (QSH) materials feature gapless helical edge states when adjacent to arbitrary trivial cladding materials. However, due to symmetry reduction at the boundary, bosonic counterparts usually exhibit gaps and thus require additional cladding crystals to maintain robustness, limiting their applications. In this study, we demonstrate an ideal acoustic QSH with gapless behaviour by constructing a global Tf on both the bulk and the boundary based on bilayer structures. Consequently, a pair of helical edge states robustly winds several times in the first Brillouin zone when coupled to resonators, promising broadband topological slow waves. We further reveal that this ideal QSH phase behaves as a topological phase transition plane that bridges trivial and higher-order phases. Our versatile multi-topology platform sheds light on compact topological slow-wave and lasing devices.

Journal ArticleDOI
TL;DR: In this paper , a spin-orbit coupled Dirac semimetal with the topological Fermi arc crossing the Fermian level on the (010) surface was investigated.
Abstract: The interplay of nontrivial topology and superconductivity in condensed matter physics gives rise to exotic phenomena. However, materials are extremely rare where it is possible to explore the full details of the superconducting pairing. Here, we investigate the momentum dependence of the superconducting gap distribution in a novel Dirac material PdTe. Using high resolution, low temperature photoemission spectroscopy, we establish it as a spin-orbit coupled Dirac semimetal with the topological Fermi arc crossing the Fermi level on the (010) surface. This spin-textured surface state exhibits a fully gapped superconducting Cooper pairing structure below ${T}_{c}\ensuremath{\sim}4.5\text{ }\text{ }\mathrm{K}$. Moreover, we find a node in the bulk near the Brillouin zone boundary, away from the topological Fermi arc. These observations not only demonstrate the band resolved electronic correlation between topological Fermi arc states and the way it induces Cooper pairing in PdTe, but also provide a rare case where surface and bulk states host a coexistence of nodeless and nodal gap structures enforced by spin-orbit coupling.

Journal ArticleDOI
TL;DR: In this article , an ab initio study finds that while oxygen defects are the driving mechanism for the metallicity, tiltings and rotations of the oxygen octahedra significantly impact the electronic structure of the 2DES and its response to externally applied strain deformations.
Abstract: Defect-free $\mathrm{Ca}\mathrm{Ti}{\mathrm{O}}_{3}$ is a band insulator, but angle-resolved photoemission spectroscopy experiments have demonstrated the existence of a nanometer-thin two-dimensional electron system (2DES) at the (001)-oriented surface of this compound. Our ab initio study finds that while oxygen defects are the driving mechanism for the metallicity, tiltings and rotations of the oxygen octahedra significantly impact the electronic structure of the 2DES and its response to externally applied strain deformations. The low-energy conduction subbands have a mixed ${t}_{2g}\text{\ensuremath{-}}{e}_{g}$ orbital character close to the center of the Brillouin zone. Good agreement with the experimental spectra is found for $\mathrm{Ti}{\mathrm{O}}_{2}$ surface divacancy configurations.

Journal ArticleDOI
TL;DR: In this article , the wave dispersion characteristics of two-dimensional architected materials, considering both the linear and nonlinear regimes, were analyzed at high and low frequencies and for two different wave amplitudes.

Journal ArticleDOI
TL;DR: In this article , the authors investigate the generation of phonons and the relaxation of carriers on picosecond timescales across the Brillouin zone of photo-excited Ge by inter-valley electron-phonon scattering.
Abstract: We investigate experimentally and using first-principles theory the generation of phonons and the relaxation of carriers on picosecond timescales across the Brillouin zone of photo-excited Ge by inter-valley electron–phonon scattering. The phonons generated are typical of those generated in semiconductor devices, contributing to the accumulation of heat within the material. We simulate the time-evolution of phonon populations, based on first-principles band structure and electron–phonon and phonon–phonon matrix elements, and compare them to data from time-resolved x-ray diffuse scattering experiments, performed at the Linac Coherent Light Source x-ray free-electron laser facility, following photo-excitation by a 50 fs near-infrared optical pulse. We show that the intensity of the non-thermal x-ray diffuse scattering signal, which is observed to grow substantially near the L-point of the Brillouin zone over 3–5 ps, is due to phonons generated by scattering of carriers between the Δ and L valleys. These phonons have low group velocities, resulting in a heat bottleneck. With the inclusion of phonon decay through 3-phonon processes, the simulations also account for other non-thermal features observed in the x-ray diffuse scattering intensity, which are due to anharmonic phonon–phonon scattering of the phonons initially generated by electron–phonon scattering.

Journal ArticleDOI
TL;DR: In this paper , the relationship between crystal symmetry and geometry of the Rashba-Edelstein effect (REE) that causes spin accumulation in response to an applied electric current was explored.
Abstract: Studies of structure-property relationships in spintronics are essential for the design of materials that can fill specific roles in devices. For example, materials with low symmetry allow unconventional configurations of charge-to-spin conversion, which can be used to generate efficient spin-orbit torques. Here, we explore the relationship between crystal symmetry and geometry of the Rashba-Edelstein effect (REE) that causes spin accumulation in response to an applied electric current. Based on a symmetry analysis performed for 230 crystallographic space groups, we identify classes of materials that can host conventional or collinear REE. Although transverse spin accumulation is commonly associated with the so-called ``Rashba materials'', we show that the presence of specific spin texture does not easily translate to the configuration of REE. More specifically, bulk crystals may simultaneously host different types of spin-orbit fields, depending on the crystallographic point group and the symmetry of the specific $k$ vector, which, averaged over the Brillouin zone, determine the direction and magnitude of the induced spin accumulation. To explore the connection between crystal symmetry, spin texture, and the magnitude of REE, we perform first-principles calculations for representative materials with different symmetries. We believe that our results will be helpful for further computational and experimental studies, as well as the design of spintronics devices.

Journal ArticleDOI
TL;DR: In this paper , the spin and electronic structure of bilayer kagome materials was investigated and the spin-Berry curvature of the bilayer bilayer KG was revealed.
Abstract: Kagome materials have emerged as a setting for emergent electronic phenomena that encompass different aspects of symmetry and topology. It is debated whether the XV$_6$Sn$_6$ kagome family (where X is a rare earth element), a recently discovered family of bilayer kagome metals, hosts a topologically non-trivial ground state resulting from the opening of spin-orbit coupling gaps. These states would carry a finite spin-Berry curvature, and topological surface states. Here, we investigate the spin and electronic structure of the XV$_6$Sn$_6$ kagome family. We obtain evidence for a finite spin-Berry curvature contribution at the center of the Brillouin zone, where the nearly flat band detaches from the dispersing Dirac band because of spin-orbit coupling. In addition, the spin-Berry curvature is further investigated in the charge density wave regime of ScV$_6$Sn$_6$, and it is found to be robust against the onset of the temperature-driven ordered phase. Utilizing the sensitivity of angle resolved photoemission spectroscopy to the spin and orbital angular momentum, our work unveils the spin-Berry curvature of topological kagome metals, and helps to define its spectroscopic fingerprint.

Journal ArticleDOI
TL;DR: In this paper , a comprehensive density functional theory based first principles studies on newly dis-covered iron-based RbLn2Fe4As4O2 (Ln = Sm, Tb, Dy, Ho) superconducting compounds is presented.
Abstract: We report a comprehensive density functional theory based first principles studies on newly dis- covered iron-based RbLn2Fe4As4O2 (Ln = Sm, Tb, Dy, Ho) superconducting compounds. A dom- inant Fe-d state, along with small arsenic state contribution is found in the low energy regime of all the four compounds, that constitutes conducting Fe-As layer. Orbital selective evolution of electronic structure is evident in hybrid RbLn2Fe4As4O2 compounds under the effect of chemical pressures induced by various lanthanide substitutions, and moderate on-site electron correlation. The characteristic electronic structure with multi-orbital derived multi-band nature undergoes an orbital-selective evolution. In all the four compounds, an orbital selective Lifshitz transition as well as an orbital-selective bandwidth renormalization is predicted due to on-site electron correlation. The calculated Fermi surfaces show evidence of bilayer splitting due to the interlayer inter-orbital interaction between the two Fe-As layers in a bilayer block. The splitting is found to be minimum along the Brillouin zone centre to the corner and is maximum along the zone centre to (π,0) direc- tion. The largest significant effect due to spin-orbit coupling is the splitting of dxz and dyz derived bands above the Fermi level. The size of spin-orbit coupling is found to be consistent with earlier theoretical calculations on 122 materials. Splitting increases with substitutions of lanthanides in decreasing order of radii. Spin-orbit coupling influences the size of the Fermi radii and thus likely to influence nesting conditions and superconductivity as well. Predictions on possible pairing symme- try based on orbital characters of the Fermi surfaces together with qualitative estimation of nesting conditions for Fermi pockets are provided. The calculated large Fe-As hopping amplitudes based on 32-band Wannier function tight-binding Hamiltonian indicates that electrons mainly hop through As atoms.

Journal ArticleDOI
01 Jan 2023
TL;DR: In this article , a scheme to perform ultra-narrow filter bandwidth and high frequency selectivity microwave photonic filter (MPF) with wide tuning range is proposed and experimentally demonstrated.
Abstract: A scheme to perform ultra-narrow filter bandwidth and high frequency selectivity microwave photonic filter (MPF) with wide tuning range is proposed and experimentally demonstrated. The ultra-narrow bandwidth of the MPF is implemented by a Brillouin laser resonator, which is composed of a cascaded ring Fabry–Pérot (CR-FP) resonator formed by a main cavity with a cavity length of 100 m and a secondary cavity with a cavity length of 10 m. A Brillouin laser resonator is formed by the main cavity to obtain an extremely narrow comb-shaped Brillouin gain spectrum. The Vernier effect of the double ring cavity can effectively suppress the side modes, thereby realizing the narrow linewidth Brillouin laser filtering. Besides, two identical tunable lasers provide the stimulated Brillouin scattering (SBS) pump light and optical carrier signal for this device respectively. After the interaction between the Brillouin gain spectrum and the optical modulation signal, the filter passband can be stably tuned by simply changing the wavelength of SBS pump light. The experimental results show that the microwave photonic filter can be stably tuned in the frequency range of 0–20 GHz, the out-of-band rejection ratio is about 20 dB, and the minimum 3 dB bandwidth is about 114 Hz.

Journal ArticleDOI
TL;DR: In this paper , temperature-dependent structural distortion is the main source of various temperature-induced magnetic states in CsPbBr3 perovskite quantum dots (PQDs) attributed to Br defects.
Abstract: Herein, we report temperature- and field-induced magnetic states in CsPbBr3 perovskite quantum dots (PQDs) attributed to Br defects. We find that temperature-dependent structural distortion is the main source of various temperature-induced magnetic states in Br-defect host CsPbBr3 PQDs. Comprehensively examined magnetization data through Arrott plots, Langevin and Brillouin function fitting, and structural analysis reveal the presence of various oxidation states (i.e., Pb0, Pb+, Pb2+, and Pb3+) yielding different magnetic states, such as diamagnetic states above 90 K, paramagnetic states below ≈90 K, and perhaps locally ordered states between 58 and 90 K. It is realized from theoretical fits that paramagnetic ions exist (i.e., superparamagnetic behavior) due to Br defects causing Pb+ (and/or Pb3+ ions) in the diamagnetic region. We anticipate that our findings will spur future research of the development of spin-optoelectronics, such as spin light-emitting diodes, and spintronics devices based on CsPbBr3 PQDs.

Journal ArticleDOI
TL;DR: In this paper , the authors used triple-axis neutron scattering to measure the magnon spectrum throughout the Brillouin zone in the antiferromagnetically ordered phase, and determined the dominant exchange interactions from linear spin-wave theory.
Abstract: We report neutron scattering measurements on ${\mathrm{YbMnSb}}_{2}$ which shed light on the nature of the magnetic moments and their interaction with Dirac fermions. Using half-polarized neutron diffraction we measured the field-induced magnetization distribution in the paramagnetic phase and found that the magnetic moments are well localized on the Mn atoms. Using triple-axis neutron scattering we measured the magnon spectrum throughout the Brillouin zone in the antiferromagnetically ordered phase, and we determined the dominant exchange interactions from linear spin-wave theory. The analysis shows that the interlayer exchange is five times larger than in several related compounds containing Bi instead of Sb. We argue that the coupling between the Mn local magnetic moments and the topological band states is more important in ${\mathrm{YbMnSb}}_{2}$ than in the Bi compounds.

Journal ArticleDOI
TL;DR: In this article , the authors show that the non-Hermitian skin effect (NHSE) can be engineered in mesoscopic heterojunctions (system plus reservoir) in which electrons in two channels of the system moving towards each other have asymmetric coupling to those of the reservoir.
Abstract: The pursuit of the non-Hermitian skin effect (NHSE) in various physical systems is of great research interest. Compared with recent progress in non-electronic systems, the implementation of the NHSE in condensed matter physics remains elusive. Here, we show that the NHSE can be engineered in the mesoscopic heterojunctions (system plus reservoir) in which electrons in two channels of the system moving towards each other have asymmetric coupling to those of the reservoir. This makes electrons in the system moving forward and in the opposite direction have unequal lifetimes, and so gives rise to a point-gap spectral topology. Accordingly, the electron eigenstates exhibit NHSE under the open boundary condition, consistent with the description of the generalized Brillouin zone. Such a reservoir-engineered NHSE visibly manifests itself as the nonreciprocal charge current that can be probed by the standard transport measurements. Further, we generalize the scenario to the spin-resolved NHSE, which can be probed by the nonreciprocal spin transport. Our work opens a new research avenue for implementing and detecting the NHSE in electronic mesoscopic systems, which will lead to interesting device applications.


Journal ArticleDOI
TL;DR: In this article , the temperature dependence of the energy band gap in zirconium pentatelluride (ZrTe$_5$) was determined using Landau level spectroscopy.
Abstract: Using Landau level spectroscopy, we determine the temperature dependence of the energy band gap in zirconium pentatelluride (ZrTe$_5$). We find that the band gap reaches $E_g=(5 \pm 1)$ meV at low temperatures and increases monotonously when the temperature is raised. This implies that ZrTe$_5$ is a weak topological insulator, with non-inverted ordering of electronic bands in the center of the Brillouin zone. Our magneto-transport experiments performed in parallel show that the resistivity anomaly in ZrTe$_5$ is not connected with the temperature dependence of the band gap.

Journal ArticleDOI
TL;DR: In this article , the authors provided an exhaustive list of valley LWP phonons at high-symmetry points (HSPs) in 2D by searching the entire 80 layer groups (LGs).
Abstract: The discovery of topological quantum states in two-dimensional (2D) systems is one of the most promising advancements in condensed matter physics. Linear Weyl point (LWP) phonons have been theoretically investigated in some 2D materials. Especially, Jin, Wang, and Xu [Nano Lett. 18, 7755 (2018)] proposed in 2018 that the candidates with threefold rotational symmetry at the corners of the hexagonal Brillouin zone can host LWP phonons with a quantized valley Berry phase. Note that all the candidates with hexagonal lattices may not host LWP phonons at $K$ (${K}^{\ensuremath{'}}$) high-symmetry points (HSPs). Hence a strategy for narrowing the search range for LWP phonons in 2D is highly required. This work provides an exhaustive list of valley LWP phonons at HSPs in 2D by searching the entire 80 layer groups (LGs). We found that the valley LWP phonons can be obtained at HSPs in 11 of the 80 LGs. Guided by the symmetry analysis, we also contributed to realizing the ideal 2D material with valley LWP phonons. We identified the existence of the valley LWP phonons in 11 2D material candidates with 11 LGs. This work offers a method to search for valley LWPs in 2D phononic systems and proposes 2D material candidates to obtain the valley LWP phonons.

Journal ArticleDOI
TL;DR: In this paper , the authors demonstrate the possibility of moving the Dirac bands along the Γ-M symmetry line in reciprocal space by varying the concentration of K atoms adsorbed onto the surface of cleaved BaNiS2 single crystals.
Abstract: In the Dirac semimetal BaNiS2, the Dirac nodes are located along the Γ-M symmetry line of the Brillouin zone, instead of being pinned at fixed high-symmetry points. We take advantage of this peculiar feature to demonstrate the possibility of moving the Dirac bands along the Γ-M symmetry line in reciprocal space by varying the concentration of K atoms adsorbed onto the surface of cleaved BaNiS2 single crystals. By means of first-principles calculations, we give a full account of this observation by considering the effect of the electrons donated by the K atom on the charge transfer gap, which establishes a promising tool for engineering Dirac states at surfaces, interfaces, and heterostructures.

Journal ArticleDOI
TL;DR: In this article , the adaptive genetic algorithm was used to predict the structures of the Li-B-C system at 100 GPa, and consecutive calculations using the full Brillouin zone confirm the existence of the strong electron-phonon coupling (EPC) in this system.
Abstract: Layer Li-B-C compounds have been shown to have feasible superconductivity. Using the adaptive genetic algorithm, we predict the structures of the Li-B-C system at 100 GPa. We identify several low-enthalpy metallic phases with stoichiometries of $\mathrm{Li}{\mathrm{B}}_{2}\mathrm{C}$, $\mathrm{Li}{\mathrm{B}}_{3}\mathrm{C}$, ${\mathrm{Li}}_{2}\mathrm{B}{\mathrm{C}}_{2}$, ${\mathrm{Li}}_{3}{\mathrm{B}}_{2}{\mathrm{C}}_{3}$, ${\mathrm{Li}}_{3}\mathrm{BC}$, and ${\mathrm{Li}}_{5}\mathrm{BC}$. Using a fast screening method of electron-phonon interaction, we find that $\mathrm{Li}{\mathrm{B}}_{3}\mathrm{C}$ is a promising candidate for superconductivity. The consecutive calculations using the full Brillouin zone confirm the existence of the strong electron-phonon coupling (EPC) in this system. The anharmonic B-C phonon modes near the zone center provide the major contribution to the EPC. The EPC constant is 1.40, and the estimated critical temperature is 22 K. In this paper, we indicate that superconductivity can also happen without a layered structural motif in the Li-B-C system. We also demonstrate an effective strategy for crystal structure prediction of superconducting materials.