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Journal ArticleDOI

90 GW peak power few-cycle mid-infrared pulses from an optical parametric amplifier

TLDR
A compact 20 Hz repetition-rate mid-IR OPCPA system operating at a central wavelength of 3900 nm with the tail-to-tail spectrum extending over 600 nm and delivering 8 mJ pulses that are compressed to 83 fs opens a range of unprecedented opportunities for tabletop ultrafast science.
Abstract
We demonstrate a compact 20 Hz repetition-rate mid-IR OPCPA system operating at a central wavelength of 3900 nm with the tail-to-tail spectrum extending over 600 nm and delivering 8 mJ pulses that are compressed to 83 fs (<7 optical cycles). Because of the long optical period (∼13 fs) and a high peak power, the system opens a range of unprecedented opportunities for tabletop ultrafast science and is particularly attractive as a driver for a highly efficient generation of ultrafast coherent x-ray continua for biomolecular and element specific imaging.

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Citations
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Dissertation

A novel single-cycle optical source in the mid-infrared

TL;DR: This thesis demonstrates the generation of single-optical-cycle pulses in the midinfrared, which are generated using adiabatic difference frequency in an aperiodically polled lithium niobate crystal, which makes this source immediately suitable for applications requiring shaped pulses.
Journal ArticleDOI

Towards high power broad-band OPCPA at 3000 nm

TL;DR: A four stage optical parametric chirped pulse amplifier (OPCPA) which generates ultrashort pulses at a central wavelength of 3000 nm with 430 μJ energy per pulse at a bandwidth of 490 nm is reported.
Journal ArticleDOI

520-µJ mid-infrared femtosecond laser at 2.8 µm by 1-kHz KTA optical parametric amplifier

TL;DR: In this paper, a 520 µJ, 1-kHz mid-infrared femtosecond optical parametric amplifier system driven by a Ti:sapphire laser system was presented.
Book ChapterDOI

2D Strong-Field Spectroscopy to Elucidate Impulsive and Adiabatic Ultrafast Electronic Control Schemes in Molecules

TL;DR: In this article, a multidimensional spectroscopy approach based on strong-field coherent electronic excitation is presented to elucidate intramolecular dynamics and unveil control mechanisms.
References
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Journal ArticleDOI

The attosecond nonlinear optics of bright coherent X-ray generation

TL;DR: In this paper, the Roentgen X-ray tube was used for high-order harmonic generation with small-scale femtosecond laser technology, which combines the microscopic attosecond science of atoms driven by intense laser fields with the macroscopic extreme nonlinear optics of phase matching.
Journal ArticleDOI

Infrared Two-Color Multicycle Laser Field Synthesis for Generating an Intense Attosecond Pulse

TL;DR: The proposed method enables the requirements for the pump pulse duration to be relaxed but also to reduce ionization of the harmonic medium, which opens the door to create an intense isolated attosecond pulse using a conventional femtosecond laser system.
Journal ArticleDOI

Mid-IR short-pulse OPCPA with micro-Joule energy at 100kHz

TL;DR: A novel mid-IR source based on optical parametric chirped pulse amplification (OPCPA) generating 96 fs pulses (9.0 cycles) at 3.2 mm with an energy of 1.2 microJ, at a repetition rate of 100 kHz is presented.
Journal ArticleDOI

Self-compression of millijoule 1.5 microm pulses.

TL;DR: In this article, the authors demonstrate a four-stage optical parametric chirped-pulse amplification system that delivers carrier-envelope phase-stable approximately 1.5 microm pulses with energies up to 12.5 mJ before recompression.
Journal ArticleDOI

Efficient continuum generation exceeding 200 eV by intense ultrashort two-color driver.

TL;DR: Results indicate the possibility to produce bright attosecond pulses approaching the soft X spectral region and contribute to significantly extending the harmonic emission to higher photon energies, whereas the VIS pulse improves the conversion efficiency of the process.
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