Connecting the irreversible capacity loss in Li-ion batteries with the electronic insulating properties of solid electrolyte interphase (SEI) components
Reads0
Chats0
TLDR
In this paper, the authors proposed an analytical model based on the tunneling results to connect the irreversible capacity loss, due to the Li ions consumed in forming these solid electrolyte interphase (SEI) component layers on the surface of negative electrodes.About:
This article is published in Journal of Power Sources.The article was published on 2016-03-31 and is currently open access. It has received 171 citations till now. The article focuses on the topics: Band gap & Work function.read more
Citations
More filters
Journal ArticleDOI
Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review.
TL;DR: This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth, summarizing the theoretical and experimental achievements and endeavors to realize the practical applications of lithium metal batteries.
Journal ArticleDOI
Review on modeling of the anode solid electrolyte interphase (SEI) for lithium-ion batteries
TL;DR: In this article, a review of state-of-the-art modeling progress in the investigation of solid electrolyte interphase (SEI) films on the anodes, ranging from electronic structure calculations to mesoscale modeling, covering the thermodynamics and kinetics of electrolyte reduction reactions, SEI formation, modification through electrolyte design, correlation of SEI properties with battery performance, and the artificial SEI design.
Journal ArticleDOI
Current Li-Ion Battery Technologies in Electric Vehicles and Opportunities for Advancements
TL;DR: In this paper, the authors present and compare key components of Li-ion batteries and describe associated battery management systems, as well as approaches to improve the overall battery efficiency, capacity, and lifespan.
Journal ArticleDOI
How Solid-Electrolyte Interphase Forms in Aqueous Electrolytes
Liumin Suo,Dahyun Oh,Dahyun Oh,Yuxiao Lin,Zengqing Zhuo,Oleg Borodin,Tao Gao,Fei Wang,Fei Wang,Akihiro Kushima,Ziqiang Wang,Ho-Cheol Kim,Yue Qi,Wanli Yang,Feng Pan,Ju Li,Kang Xu,Chunsheng Wang +17 more
TL;DR: By establishing basic laws governing the successful formation of an aqueous SEI, the in-depth understanding presented in this work will assist the efforts in tailor-designing better interphases that enable more energetic chemistries operating farther away from equilibria in aqueously media.
Journal ArticleDOI
High-voltage liquid electrolytes for Li batteries: progress and perspectives
Xiulin Fan,Chunsheng Wang +1 more
TL;DR: In this article, the authors present a comprehensive and in-depth overview on the recent advances, fundamental mechanisms, scientific challenges, and design strategies for the novel high-voltage electrolyte systems, especially focused on stability issues of the electrolytes, the compatibility and interactions between electrolytes and the electrodes, and reaction mechanisms.
References
More filters
Journal ArticleDOI
Generalized Gradient Approximation Made Simple
TL;DR: A simple derivation of a simple GGA is presented, in which all parameters (other than those in LSD) are fundamental constants, and only general features of the detailed construction underlying the Perdew-Wang 1991 (PW91) GGA are invoked.
Journal ArticleDOI
Lithium Batteries and Cathode Materials
TL;DR: This paper will describe lithium batteries in more detail, building an overall foundation for the papers that follow which describe specific components in some depth and usually with an emphasis on the materials behavior.
Journal ArticleDOI
Accurate band gaps of semiconductors and insulators with a semilocal exchange-correlation potential.
Fabien Tran,Peter Blaha +1 more
TL;DR: This semilocal exchange potential, which recovers the local-density approximation for a constant electron density, mimics very well the behavior of orbital-dependent potentials and leads to calculations which are barely more expensive than LDA calculations, which can be applied to very large systems in an efficient way.
Journal ArticleDOI
Generalized Formula for the Electric Tunnel Effect between Similar Electrodes Separated by a Thin Insulating Film
TL;DR: In this article, a formula for the electric tunnel effect through a potential barrier of arbitrary shape existing in a thin insulating film was derived for a rectangular barrier with and without image forces, where the true image potential was considered and compared to the approximate parabolic solution derived by Holm and Kirschstein.
Journal ArticleDOI
Insertion Electrode Materials for Rechargeable Lithium Batteries
TL;DR: In this article, the performance and safety of rechargeable batteries depend strongly on the materials used and future trends, such as alternative materials for achieving higher specific charges are discussed, and a review of the insertion materials suitable for negative and positive insertion electrodes is presented.