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Experimental and Numerical Study on Laminar Flame Characteristics of Methane Oxy-fuel Mixtures Highly Diluted with CO2

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TLDR
An experimental and numerical study on laminar flame characteristics of methane oxy-fuel mixtures highly diluted with CO2 was conducted using a constant volume chamber and CHEMKIN package as mentioned in this paper.
Abstract
An experimental and numerical study on laminar flame characteristics of methane oxy-fuel mixtures highly diluted with CO2 was conducted using a constant volume chamber and CHEMKIN package. The effects of high CO2 dilution on combustion chemical reaction, flame instability, and flame radiation of CH4/CO2/O2 mixtures were studied. The laminar burning velocities of CH4/CO2/O2 mixtures decrease with the increase of the CO2 fraction. CO2 directly participates in the chemical reaction through the elementary reaction OH + CO = H + CO2 and inhibits the combustion process by the competition of the H radical between the reverse reaction of OH + CO = H + CO2 and the reaction H + O2 = O + OH. This effect is more obvious for highly diluted CO2 in the case of CH4/CO2/O2 mixtures. CO2 suppresses the flame instability by the combined effect of hydrodynamic and thermal-diffusive instabilities. The radiation of CH4 oxy-fuel combustion is much stronger than that of CH4/air combustion mainly because of the existence of a lar...

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Citations
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Journal ArticleDOI

Comprehensive kinetic study of combustion technologies for low environmental impact: MILD and OXY-fuel combustion of methane

TL;DR: In this article, the CRECK core model is developed upon the Aramco 2.0 mechanism and further extended the validation objectives to MILD and OXY fuel combustion conditions.
Journal ArticleDOI

Comparative study on the effect of CO2 and H2O dilution on laminar burning characteristics of CO/H2/air mixtures

TL;DR: In this paper, the effect of CO2 and H2O dilution on the laminar burning characteristics of CO/H2/air mixtures was conducted at elevated pressures using spherically expanding flames and CHEMKIN package.
Journal ArticleDOI

A Critical Review of CO2 Capture Technologies and Prospects for Clean Power Generation

Najmus S. Sifat, +1 more
- 30 Oct 2019 - 
TL;DR: In this paper, the authors reviewed different methods and updates of the current technologies to capture and separate CO2 generated in a thermal power plant and classified them into two broad categories depending on the requirement of separation of CO2 from the gases.
Journal ArticleDOI

Influence of inert gas addition on propagation indices of methane-air deflagrations

TL;DR: In this article, the authors examined the characteristic indices of laminar deflagrations propagating in methane-air gaseous mixtures diluted by several inert gases: He, Ar, N2 or CO2.
Journal ArticleDOI

Measurements and interpretation of shock tube ignition delay times in highly CO2 diluted mixtures using multiple diagnostics

TL;DR: In this article, the effect of bifurcation has been examined in high-speed camera imagery in comparison with more standard methods (e.g., pressure, emission, and laser absorption spectroscopy) to measure the ignition delay time.
References
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Journal ArticleDOI

Carbon Capture and Storage: How Green Can Black Be?

TL;DR: Urgent action is required if carbon capture and storage is to play a large role in limiting climate change, and many technological, commercial, and political hurdles remain to be overcome.

PREMIX :A F ORTRAN Program for Modeling Steady Laminar One-Dimensional Premixed Flames

TL;DR: In this paper, a Fortran computer program that computes species and temperature profiles in steady-state burner-stabilized and freely propagating laminar flames is described.
Journal ArticleDOI

Oxy-fuel combustion technology for coal-fired power generation

TL;DR: A comprehensive review of CO2 capture in coal-fired combustion plants can be found in this article, where the status of the technology development and assessments providing comparisons with other power generation options, and suggests research needs.
Journal ArticleDOI

Chemical kinetic modeling of hydrocarbon combustion

TL;DR: In this paper, a comprehensive model of high temperature hydrocarbon oxidation in combustion is presented, with emphasis on the hierarchical structure of reaction mechanisms for complex fuels, including both inhibition and promotion of combustion.
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