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Metal Acetylacetonate Series in Interface Engineering for Full Low-Temperature-Processed, High-Performance, and Stable Planar Perovskite Solar Cells with Conversion Efficiency over 16% on 1 cm2 Scale

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TLDR
A series of metal acetylacetonates produced by a full low-temperature (below 100 °C) process are successfully employed to obtain both "multistable" and high-performance planar-inverted perovskite solar cells.
Abstract
A series of metal acetylacetonates produced by a full low-temperature (below 100 °C) process are successfully employed to obtain both "multistable" and high-performance planar-inverted perovskite solar cells. All the three kinds of champion cells in small area exhibit over 18% in conversion-efficiency with negligible hysteresis, along with a conversion efficiency above 16% for planar PSCs in an aperture area of over 1 cm2 .

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Citations
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Journal ArticleDOI

Influence of post-deposition annealing on structural, morphological and optical properties of copper (II) acetylacetonate thin films.

TL;DR: The annealing process presented significantly impacted the nonlinear optical properties such as third-order optical susceptibility χ(3) and nonlinear refractive index n2 of cu(acac)2 thin films.
Journal ArticleDOI

Inverted quantum dot light-emitting diodes with conductive interlayers of zirconium acetylacetonate

TL;DR: In this paper, the use of Zirconium acetylacetonate (Zr(acac)4), a low work function and transparent metal chelate, as interlayers simultaneously suppresses interfacial exciton quenching and offers good electron-transporting properties.
Journal ArticleDOI

Material and Interface Engineering for High‐Performance Perovskite Solar Cells: A Personal Journey and Perspective

TL;DR: The historical development and recent progress on the interface engineering of PSCs primarily of the own group are presented, mainly focused on the material and interface design of the conventional n- i-p, inverted p-i-n and carbon electrode-based structure devices from the authors' experience and perspective.
Journal ArticleDOI

Review on engineering two-dimensional nanomaterials for promoting efficiency and stability of perovskite solar cells

TL;DR: In this article , the emerging 2D materials beyond graphene as charge transport layers, buffer layers and additives in perovskite film for enhancing the efficiency and stability of PSCs are summarized.
References
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Journal ArticleDOI

Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells

TL;DR: Two organolead halide perovskite nanocrystals were found to efficiently sensitize TiO(2) for visible-light conversion in photoelectrochemical cells, which exhibit strong band-gap absorptions as semiconductors.
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Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites

TL;DR: A low-cost, solution-processable solar cell, based on a highly crystalline perovskite absorber with intense visible to near-infrared absorptivity, that has a power conversion efficiency of 10.9% in a single-junction device under simulated full sunlight is reported.
Journal ArticleDOI

Electron-hole diffusion lengths exceeding 1 micrometer in an organometal trihalide perovskite absorber.

TL;DR: In this article, transient absorption and photoluminescence-quenching measurements were performed to determine the electron-hole diffusion lengths, diffusion constants, and lifetimes in mixed halide and triiodide perovskite absorbers.
Journal ArticleDOI

Efficient planar heterojunction perovskite solar cells by vapour deposition

TL;DR: It is shown that perovskite absorbers can function at the highest efficiencies in simplified device architectures, without the need for complex nanostructures.
Journal Article

Electron-Hole Diffusion Lengths Exceeding 1 Micrometer in an Organometal Trihalide Perovskite Absorber

TL;DR: In this paper, transient absorption and photoluminescence-quenching measurements were performed to determine the electron-hole diffusion lengths, diffusion constants, and lifetimes in mixed halide and triiodide perovskite absorbers.
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