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Open AccessJournal ArticleDOI

Waveforms for optimal sub-keV high-order harmonics with synthesized two- or three-colour laser fields

TLDR
It is shown that harmonics can be enhanced by one to two orders of magnitude without an increase in the total laser power if the laser's waveform is optimized by synthesizing two- or three-colour fields.
Abstract
High-order harmonics extending to the X-ray region generated in a gas medium by intense lasers offer the potential for providing tabletop broadband light sources but so far are limited by their low conversion efficiency. Here we show that harmonics can be enhanced by one to two orders of magnitude without an increase in the total laser power if the laser's waveform is optimized by synthesizing two- or three-colour fields. The harmonics thus generated are also favourably phase-matched so that radiation is efficiently built up in the gas medium. Our results, combined with the emerging intense high-repetition MHz lasers, promise to increase harmonic yields by several orders to make harmonics feasible in the near future as general bright tabletop light sources, including intense attosecond pulses.

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PatentDOI

Achromatic Metasurface Optical Components by Dispersive Phase Compensation

TL;DR: It is shown that chromatic dispersion, or color dependence, can be compensated for by the judicious design of the surface, and an engineered wavelength-dependent phase shift imparted by a metasurface is demonstrated.
Journal ArticleDOI

Tracing and controlling electronic dynamics in atoms and molecules by attosecond pulses

TL;DR: In this paper, the main theoretical methods and concepts in strong field and attosecond physics were reviewed, and a number of topics including generation of xuv light sources, the probe and steering of the electron motion in the combination of XUV and IR pulses, the photoionization time delay, the electron-electron correlation dynamics in multiple-electRON atoms and molecules, etc.
Journal ArticleDOI

Toward Waveform Nonlinear Optics Using Multimillijoule Sub-Cycle Waveform Synthesizers

TL;DR: In this article, a carrier-envelope-phase (CEP)-stable, multimillijoule three-channel parametric waveform synthesizer was presented for high-energy sub-cycle optical waveform synthesis.
Journal ArticleDOI

Generation of isolated sub-10-attosecond pulses in spatially inhomogenous two-color fields

TL;DR: A theoretical investigation of high-order harmonic generation in spatially inhomogeneous two-color laser fields by solving three dimensional time dependent Schrödinger equation finds that an isolated 8.8 attosecond pulse can be generated directly by the superposition of the supercontinuum harmonics.
Journal ArticleDOI

Attosecond light sources in the water window

TL;DR: In this article, a carrier-envelope phase stable X-ray source was proposed for near-edge absorption spectroscopy with attosecond time resolution and high harmonic generation.
References
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Journal ArticleDOI

Plasma perspective on strong field multiphoton ionization.

TL;DR: During strong-field multiphoton ionization, a wave packet is formed each time the laser field passes its maximum value, and one important parameter which determines the strength of these effects is the rate at which the wave packet spreads in the direction perpendicular to the laser electric field.
Journal ArticleDOI

Theory of high-harmonic generation by low-frequency laser fields.

TL;DR: A simple, analytic, and fully quantum theory of high-harmonic generation by low-frequency laser fields is presented and the exact quantum-mechanical formula for the harmonic cutoff that differs from the phenomenological law Ip+3.17Up is presented.
Journal ArticleDOI

Bright Coherent Ultrahigh Harmonics in the keV X-ray Regime from Mid-Infrared Femtosecond Lasers

TL;DR: By guiding a mid-infrared femtosecond laser in a high-pressure gas, ultrahigh harmonics can be generated that emerge as a bright supercontinuum that spans the entire electromagnetic spectrum from the ultraviolet to more than 1.6 kilo–electron volts, allowing, in principle, the generation of pulses as short as 2.5 attoseconds.
Journal ArticleDOI

Above threshold ionization beyond the high harmonic cutoff.

TL;DR: This work presents high sensitivity electron energy spectra for xenon in a strong 50 ps, 1.053 [mu]m laser field and calculates using the single active electron approximation show excellent agreement with the observed electron distributions.
Journal ArticleDOI

Attosecond Synchronization of High-Harmonic Soft X-rays

TL;DR: It is shown that the synchronization could be improved considerably by controlling the underlying ultrafast electron dynamics, to provide pulses of 130 attoseconds in duration, which would allow us to track fast electron processes in matter.
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