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Showing papers on "Magnon published in 2020"


Journal ArticleDOI
24 Jan 2020-Science
TL;DR: Using a superconducting qubit as a quantum sensor, a single magnon is detected in a millimeter-sized ferrimagnetic crystal with a quantum efficiency of up to 0.71, establishing the single-photon detector counterpart for magnonics.
Abstract: The recent development of hybrid systems based on superconducting circuits provides the possibility of engineering quantum sensors that exploit different degrees of freedom. Quantum magnonics, which aims to control and read out quanta of collective spin excitations in magnetically ordered systems, provides opportunities for advances in both the study of magnetism and the development of quantum technologies. Using a superconducting qubit as a quantum sensor, we report the detection of a single magnon in a millimeter-sized ferrimagnetic crystal with a quantum efficiency of up to 0.71. The detection is based on the entanglement between a magnetostatic mode and the qubit, followed by a single-shot measurement of the qubit state. This proof-of-principle experiment establishes the single-photon detector counterpart for magnonics.

195 citations


Journal ArticleDOI
27 Jan 2020-Nature
TL;DR: In this article, a sub-terahertz spin pumping was demonstrated for high-frequency spintronic devices in the presence of a heavy metal and an antiferromagnetic insulator.
Abstract: Spin dynamics in antiferromagnets has much shorter timescales than in ferromagnets, offering attractive properties for potential applications in ultrafast devices1–3. However, spin-current generation via antiferromagnetic resonance and simultaneous electrical detection by the inverse spin Hall effect in heavy metals have not yet been explicitly demonstrated4–6. Here we report sub-terahertz spin pumping in heterostructures of a uniaxial antiferromagnetic Cr2O3 crystal and a heavy metal (Pt or Ta in its β phase). At 0.240 terahertz, the antiferromagnetic resonance in Cr2O3 occurs at about 2.7 tesla, which excites only right-handed magnons. In the spin-canting state, another resonance occurs at 10.5 tesla from the precession of induced magnetic moments. Both resonances generate pure spin currents in the heterostructures, which are detected by the heavy metal as peaks or dips in the open-circuit voltage. The pure-spin-current nature of the electrically detected signals is unambiguously confirmed by the reversal of the voltage polarity observed under two conditions: when switching the detector metal from Pt to Ta, reversing the sign of the spin Hall angle7–9, and when flipping the magnetic-field direction, reversing the magnon chirality4,5. The temperature dependence of the electrical signals at both resonances suggests that the spin current contains both coherent and incoherent magnon contributions, which is further confirmed by measurements of the spin Seebeck effect and is well described by a phenomenological theory. These findings reveal the unique characteristics of magnon excitations in antiferromagnets and their distinctive roles in spin–charge conversion in the high-frequency regime. Pure spin currents are simultaneously generated and detected electrically through sub-terahertz magnons in the antiferromagnetic insulator Cr2O3, demonstrating the potential of magnon excitations in antiferromagnets for high-frequency spintronic devices.

172 citations


Journal ArticleDOI
TL;DR: A microscopic theory for collective excitations of quantum anomalous Hall ferromagnets (QAHF) in twisted bilayer graphene is presented, implying that the valley polarized state is more favorable compared to the valley coherent state.
Abstract: We present a microscopic theory for collective excitations of quantum anomalous Hall ferromagnets (QAHF) in twisted bilayer graphene. We calculate the spin magnon and valley magnon spectra by solving Bethe-Salpeter equations and verify the stability of QAHF. We extract the spin stiffness from the gapless spin wave dispersion and estimate the energy cost of a skyrmion-antiskyrmion pair, which is found to be comparable in energy with the Hartree-Fock gap. The valley wave mode is gapped, implying that the valley polarized state is more favorable compared to the valley coherent state. Using a nonlinear sigma model, we estimate the valley ordering temperature, which is considerably reduced from the mean-field transition temperature due to thermal excitations of valley waves.

129 citations


Journal Article
TL;DR: Pure spin currents are simultaneously generated and detected electrically through sub-terahertz magnons in the antiferromagnetic insulator Cr 2 O 3 , demonstrating the potential of magnon excitations in antiferromeagnets for high-frequency spintronic devices.
Abstract: Spin dynamics in antiferromagnets has much shorter timescales than in ferromagnets, offering attractive properties for potential applications in ultrafast devices1–3. However, spin-current generation via antiferromagnetic resonance and simultaneous electrical detection by the inverse spin Hall effect in heavy metals have not yet been explicitly demonstrated4–6. Here we report sub-terahertz spin pumping in heterostructures of a uniaxial antiferromagnetic Cr2O3 crystal and a heavy metal (Pt or Ta in its β phase). At 0.240 terahertz, the antiferromagnetic resonance in Cr2O3 occurs at about 2.7 tesla, which excites only right-handed magnons. In the spin-canting state, another resonance occurs at 10.5 tesla from the precession of induced magnetic moments. Both resonances generate pure spin currents in the heterostructures, which are detected by the heavy metal as peaks or dips in the open-circuit voltage. The pure-spin-current nature of the electrically detected signals is unambiguously confirmed by the reversal of the voltage polarity observed under two conditions: when switching the detector metal from Pt to Ta, reversing the sign of the spin Hall angle7–9, and when flipping the magnetic-field direction, reversing the magnon chirality4,5. The temperature dependence of the electrical signals at both resonances suggests that the spin current contains both coherent and incoherent magnon contributions, which is further confirmed by measurements of the spin Seebeck effect and is well described by a phenomenological theory. These findings reveal the unique characteristics of magnon excitations in antiferromagnets and their distinctive roles in spin–charge conversion in the high-frequency regime. Pure spin currents are simultaneously generated and detected electrically through sub-terahertz magnons in the antiferromagnetic insulator Cr2O3, demonstrating the potential of magnon excitations in antiferromagnets for high-frequency spintronic devices.

125 citations


Journal ArticleDOI
TL;DR: It is shown that parity-time (PT) symmetry can be spontaneously broken in the recently reported energy level attraction of magnons and cavity photons and may open an exciting window to utilize magnon-photon entanglement as a resource for quantum information science.
Abstract: We show that parity-time (PT) symmetry can be spontaneously broken in the recently reported energy level attraction of magnons and cavity photons. In the PT-broken phase, the magnon and photon form a high-fidelity Bell state with maximum entanglement. This entanglement is steady and robust against the perturbation of the environment, which is in contrast to the general wisdom that expects instability of the hybridized state when the symmetry is broken. This anomaly is further understood by the compete of non-Hermitian evolution and particle number conservation of the hybrid system. As a comparison, neither PT-symmetry breaking nor steady magnon-photon entanglement is observed inside the normal level repulsion case. Our results may open an exciting window to utilize magnon-photon entanglement as a resource for quantum information science.

125 citations


Journal ArticleDOI
TL;DR: Key progress concerning the developing research direction utilizing spin current as a probe of quantum materials is reviewed and spin-triplet superconductivity and spin dynamics in the ferromagnet/superconductor heterostructures are focused on.
Abstract: Spin current historically referred to the flow of electrons carrying spin information, in particular since the discovery of giant magnetoresistance in the 1980s. Recently, it has been found that spin current can also be mediated by spin-triplet supercurrent, superconducting quasiparticles, spinons, magnons, spin superfluidity and so on. Here, we review key progress concerning the developing research direction utilizing spin current as a probe of quantum materials. We focus on spin-triplet superconductivity and spin dynamics in the ferromagnet/superconductor heterostructures, quantum spin liquids, magnetic phase transitions, magnon-polarons, magnon-polaritons, magnon Bose–Einstein condensates and spin superfluidity. The unique characteristics of spin current as a probe will be fruitful for future investigation of spin-dependent properties and the identification of new quantum materials. Progress in utilizing spin current as a probe of quantum materials,—including topological insulators, superconductors, spin liquids, magnonic systems and spin superfluidity,—is reviewed.

105 citations


Journal ArticleDOI
TL;DR: Experimental evidence is reported that an easy-plane insulating AFM, an α-Fe 2 O 3 thin film, can efficiently transmit spins over micrometre distances and can realize a bi-stable spin-current switch with a 100% on/off ratio under zero remnant magnetic field.
Abstract: Antiferromagnets (AFMs) possess great potential in spintronics because of their immunity to external magnetic disturbance, the absence of a stray field or the resonance in the terahertz range1,2. The coupling of insulating AFMs to spin–orbit materials3–7 enables spin transport via AFM magnons. In particular, spin transmission over several micrometres occurs in some AFMs with easy-axis anisotropy8,9. Easy-plane AFMs with two orthogonal, linearly polarized magnon eigenmodes own unique advantages for low-energy control of ultrafast magnetic dynamics2. However, it is commonly conceived that these magnon modes are less likely to transmit spins because of their vanishing angular momentum9–11. Here we report experimental evidence that an easy-plane insulating AFM, an α-Fe2O3 thin film, can efficiently transmit spins over micrometre distances. The spin decay length shows an unconventional temperature dependence that cannot be captured considering solely thermal magnon scatterings. We interpret our observations in terms of an interference of two linearly polarized, propagating magnons in analogy to the birefringence effect in optics. Furthermore, our devices can realize a bi-stable spin-current switch with a 100% on/off ratio under zero remnant magnetic field. These findings provide additional tools for non-volatile, low-field control of spin transport in AFM systems. Easy-plane antiferromagnet materials promise low-energy control of ultrafast magnetic dynamics in future spintronics applications, but host magnons with vanishing angular momentum, which makes spin transport via magnons unlikely. Through interference of two linearly polarized propagating magnons, spin transport over micrometre distances is yet possible.

94 citations


Journal ArticleDOI
TL;DR: In this paper, the authors show that terahertz (1 THz = 10$12}$ Hz) electromagnetic pulses allow coherent navigation of spins over a potential barrier and reveal the corresponding temporal and spectral fingerprints.
Abstract: Future information technology demands ultimately fast, low-loss quantum control. Intense light fields have facilitated important milestones, such as inducing novel states of matter, accelerating electrons ballistically, or coherently flipping the valley pseudospin. These dynamics leave unique signatures, such as characteristic bandgaps or high-order harmonic radiation. The fastest and least dissipative way of switching the technologically most important quantum attribute - the spin - between two states separated by a potential barrier is to trigger an all-coherent precession. Pioneering experiments and theory with picosecond electric and magnetic fields have suggested this possibility, yet observing the actual dynamics has remained out of reach. Here, we show that terahertz (1 THz = 10$^{12}$ Hz) electromagnetic pulses allow coherent navigation of spins over a potential barrier and we reveal the corresponding temporal and spectral fingerprints. This goal is achieved by coupling spins in antiferromagnetic TmFeO$_{3}$ with the locally enhanced THz electric field of custom-tailored antennas. Within their duration of 1 ps, the intense THz pulses abruptly change the magnetic anisotropy and trigger a large-amplitude ballistic spin motion. A characteristic phase flip, an asymmetric splitting of the magnon resonance, and a long-lived offset of the Faraday signal are hallmarks of coherent spin switching into adjacent potential minima, in agreement with a numerical simulation. The switchable spin states can be selected by an external magnetic bias. The low dissipation and the antenna's sub-wavelength spatial definition could facilitate scalable spin devices operating at THz rates.

92 citations


Journal ArticleDOI
TL;DR: In this article, the authors reported the direct observation of 2D magnons through magneto-Raman spectroscopy with optical selection rules that are strictly determined by the honeycomb lattice and magnetic states of atomically thin CrI$_3$.
Abstract: Exfoliated chromium triiodide (CrI$_3$) is a layered van der Waals (vdW) magnetic insulator that consists of ferromagnetic layers coupled through antiferromagnetic interlayer exchange. The resulting permutations of magnetic configurations combined with the underlying crystal symmetry produces tunable magneto-optical phenomena that is unique to the two-dimensional (2D) limit. Here, we report the direct observation of 2D magnons through magneto-Raman spectroscopy with optical selection rules that are strictly determined by the honeycomb lattice and magnetic states of atomically thin CrI$_3$. In monolayers, we observe an acoustic magnon mode of ~0.3 meV with cross-circularly polarized selection rules locked to the magnetization direction. These unique selection rules arise from the discrete conservation of angular momentum of photons and magnons dictated by threefold rotational symmetry in a rotational analogue to Umklapp scattering. In bilayers, by tuning between the layered antiferromagnetic and ferromagnetic-like states, we observe the switching of two magnon modes. The bilayer structure also enables Raman activity from the optical magnon mode at ~17 meV (~4.2 THz) that is otherwise Raman-silent in the monolayer. From these measurements, we quantitatively extract the spin wave gap, magnetic anisotropy, intralayer and interlayer exchange constants, and establish 2D magnets as a new system for exploring magnon physics.

88 citations


Journal ArticleDOI
TL;DR: The present scheme illustrates a new mechanism for creating entangled states of optical fields and enables potential applications in quantum information science and quantum tasks that require entangled microwave fields.
Abstract: We present a scheme to entangle two microwave fields by using the nonlinear magnetostrictive interaction in a ferrimagnet. The magnetostrictive interaction enables the coupling between a magnon mode (spin wave) and a mechanical mode in the ferrimagnet, and the magnon mode simultaneously couples to two microwave cavity fields via the magnetic dipole interaction. The magnon-phonon coupling is enhanced by directly driving the ferrimagnet with a strong red-detuned microwave field, and the driving photons are scattered onto two sidebands induced by the mechanical motion. We show that two cavity fields can be prepared in a stationary entangled state if they are, respectively, resonant with two mechanical sidebands. The present scheme illustrates a new mechanism for creating entangled states of optical fields and enables potential applications in quantum information science and quantum tasks that require entangled microwave fields.

84 citations


Journal ArticleDOI
TL;DR: In this article, the entanglement properties among magnons and photons in an antiferromagnet-light system were investigated, and the authors found that the magnon-photon coupling inside a cavity has been experimentally realized and has attracted significant attention for its potential docking with quantum information science.
Abstract: Magnon-photon coupling inside a cavity has been experimentally realized and has attracted significant attention for its potential docking with quantum information science. Whether this coupling implies the steady entanglement of photons and magnons is crucial for its usage in quantum information but is still an open question. Here we study the entanglement properties among magnons and photons in an antiferromagnet-light system and find that the entanglement between a magnon and a photon is nearly zero, while the magnon-magnon entanglement is very strong and can be even further enhanced through the coupling with the cavity photons. The maximum enhancement occurs when the antiferromagnet is resonant with the light. The essential physics can be well understood within the picture of cavity-induced cooling of the magnon-magnon state near its joint vacuum with stronger entanglement. Our findings can be used to cool magnetic magnons toward their ground state and may also be significant to extend the cavity spintronics to quantum manipulation. Furthermore, the hybrid antiferromagnet-light system provides a natural platform to manipulate the deep strong correlations of continuous modes with a generic stable condition and easy tunability.

Journal ArticleDOI
TL;DR: Long-distance spin-transport in the easy-plane canted antiferromagnetic phase of hematite and at room temperature, where the linearly polarized magnons are not intuitively expected to carry spin is reported, highlighting the promising potential of this insulating antiferromaagnet for magnon-based devices.
Abstract: Antiferromagnetic materials can host spin-waves with polarizations ranging from circular to linear depending on their magnetic anisotropies. Until now, only easy-axis anisotropy antiferromagnets with circularly polarized spin-waves were reported to carry spin-information over long distances of micrometers. In this article, we report long-distance spin-transport in the easy-plane canted antiferromagnetic phase of hematite and at room temperature, where the linearly polarized magnons are not intuitively expected to carry spin. We demonstrate that the spin-transport signal decreases continuously through the easy-axis to easy-plane Morin transition, and persists in the easy-plane phase through current induced pairs of linearly polarized magnons with dephasing lengths in the micrometer range. We explain the long transport distance as a result of the low magnetic damping, which we measure to be ≤ 10−5 as in the best ferromagnets. All of this together demonstrates that long-distance transport can be achieved across a range of anisotropies and temperatures, up to room temperature, highlighting the promising potential of this insulating antiferromagnet for magnon-based devices. Hitherto, only circularly polarized antiferromagnetic (AFM) spin-waves (SWs) were expected to convey spin-information. Here, the authors present persistent spin-transport over long distances in the easy-plane AFM phase of hematite, α-Fe2O3, via linearly polarized SW pairs with ultra-low damping.

Journal ArticleDOI
10 Jan 2020
TL;DR: In this article, a modified ab initio model that is consistent with both magnetic specific heat and low-energy features of INS data was proposed to explain all observed phenomena of low energy spin Hamiltonians.
Abstract: What is the correct low-energy spin Hamiltonian description of $$\alpha$$ -RuCl $$_{3}$$ ? The material is a promising Kitaev spin liquid candidate, but is also known to order magnetically, the description of which necessitates additional interaction terms. The nature of these interactions, their magnitudes and even signs, remain an open question. In this work we systematically investigate dynamical and thermodynamic magnetic properties of proposed effective Hamiltonians. We calculate zero-temperature inelastic neutron scattering (INS) intensities using exact diagonalization, and magnetic specific heat using a thermal pure quantum states method. We find that no single current model satisfactorily explains all observed phenomena of $$\alpha$$ -RuCl $$_{3}$$ . In particular, we find that Hamiltonians derived from first principles can capture the experimentally observed high-temperature peak in the magnetic specific heat, while overestimating the magnon energy at the zone center. In contrast, other models reproduce important features of the INS data, but do not adequately describe the magnetic specific heat. To address this discrepancy we propose a modified ab initio model that is consistent with both magnetic specific heat and low-energy features of INS data.

Journal ArticleDOI
TL;DR: The experimentally demonstrate quantum sensing of a steady-state magnon population in a magnetostatic mode of a ferrimagnetic crystal using Ramsey interferometry with a sensitivity on the order of 10^{-3} magnons/sqrt[Hz].
Abstract: Hybrid quantum devices expand the tools and techniques available for quantum sensing in various fields. Here, we experimentally demonstrate quantum sensing of a steady-state magnon population in a magnetostatic mode of a ferrimagnetic crystal. Dispersively coupling the magnetostatic mode to a superconducting qubit allows for the detection of magnons using Ramsey interferometry with a sensitivity on the order of 10^{-3} magnons/sqrt[Hz]. The protocol is based on dissipation as dephasing via fluctuations in the magnetostatic mode reduces the qubit coherence proportionally to the number of magnons.

Journal ArticleDOI
TL;DR: In this paper, a ferromagnetic resonance study of an electrically insulating magnetic bi-layer consisting of two yttrium iron garnet (YIG) films epitaxially grown on both sides of a non-magnetic gadolinium gallium garnet slab was performed.
Abstract: We report a ferromagnetic resonance study of an electrically insulating magnetic bi-layer consisting of two yttrium iron garnet (YIG) films epitaxially grown on both sides of a non-magnetic gadolinium gallium garnet (GGG) slab. We show that standing transverse sound waves couple the coherent magnetization dynamics of the two YIG films half millimeter apart through the magnetoelastic interaction, periodically modulating the microwave absorption as a function of frequency. Constructive and destructive interferences between the dynamics of the two YIG layers is observed. This long range coherent coupling by phononic angular momentum currents through non-magnetic dielectric waveguide brings new functionalities to insulator hybrid spin circuits and devices.

Journal ArticleDOI
TL;DR: In this paper, an anti-parity-time (anti-PT) symmetric cavity magnonics system with precise eigenspace controllability was studied, and two different singularities in the same system were observed.
Abstract: By engineering an anti-parity-time (anti-PT) symmetric cavity magnonics system with precise eigenspace controllability, we observe two different singularities in the same system. One type of singularity, the exceptional point (EP), is produced by tuning the magnon damping. Between two EPs, the maximal coherent superposition of photon and magnon states is robustly sustained by the preserved anti-PT symmetry. The other type of singularity, arising from the dissipative coupling of two antiresonances, is an unconventional bound state in the continuum (BIC). At the settings of BICs, the coupled system exhibits infinite discontinuities in the group delay. We find that both singularities coexist at the equator of the Bloch sphere, which reveals a unique hybrid state that simultaneously exhibits the maximal coherent superposition and slow light capability.

Journal ArticleDOI
09 Oct 2020
TL;DR: In this article, the authors demonstrate that biquadratic exchange interactions, which is the simplest and most natural form of non-Heisenberg coupling, assume a key role in the magnetic properties of layered magnets.
Abstract: Magnetism in recently discovered van der Waals materials has opened several avenues in the study of fundamental spin interactions in truly two-dimensions. A paramount question is what effect higher-order interactions beyond bilinear Heisenberg exchange have on the magnetic properties of few-atom thick compounds. Here we demonstrate that biquadratic exchange interactions, which is the simplest and most natural form of non-Heisenberg coupling, assume a key role in the magnetic properties of layered magnets. Using a combination of nonperturbative analytical techniques, non-collinear first-principles methods and classical Monte Carlo calculations that incorporate higher-order exchange, we show that several quantities including magnetic anisotropies, spin-wave gaps and topological spin-excitations are intrinsically renormalized leading to further thermal stability of the layers. We develop a spin Hamiltonian that also contains antisymmetric exchanges (e.g., Dzyaloshinskii–Moriya interactions) to successfully rationalize numerous observations, such as the non-Ising character of several compounds despite a strong magnetic anisotropy, peculiarities of the magnon spectrum of 2D magnets, and the discrepancy between measured and calculated Curie temperatures. Our results provide a theoretical framework for the exploration of different physical phenomena in 2D magnets where biquadratic exchange interactions have an important contribution.

Journal ArticleDOI
TL;DR: Evidence for fractionalized quasiparticles is found by studying magnetic excitations across the field-temperature phase diagram for α-RuCl3, a Kitaev honeycomb material that has properties consistent with predictions of a phase hosting fractionalization Majorana fermions but that could also be explained by conventional magneticexcitations.
Abstract: The pure Kitaev honeycomb model harbors a quantum spin liquid in zero magnetic fields, while applying finite magnetic fields induces a topological spin liquid with non-Abelian anyonic excitations. This latter phase has been much sought after in Kitaev candidate materials, such as α-RuCl3. Currently, two competing scenarios exist for the intermediate field phase of this compound (B = 7 − 10 T), based on experimental as well as theoretical results: (i) conventional multiparticle magnetic excitations of integer quantum number vs. (ii) Majorana fermionic excitations of possibly non-Abelian nature with a fractional quantum number. To discriminate between these scenarios a detailed investigation of excitations over a wide field-temperature phase diagram is essential. Here, we present Raman spectroscopic data revealing low-energy quasiparticles emerging out of a continuum of fractionalized excitations at intermediate fields, which are contrasted by conventional spin-wave excitations. The temperature evolution of these quasiparticles suggests the formation of bound states out of fractionalized excitations. α-RuCl3 has properties consistent with predictions of a phase hosting fractionalized Majorana fermions but that could also be explained by conventional magnetic excitations. Here the authors find evidence for fractionalized quasiparticles by studying magnetic excitations across the field-temperature phase diagram.

Journal ArticleDOI
TL;DR: In this paper, coherent spin pumping in the magnon-magnon hybrid modes of yttrium iron garnet/permalloy (YIG/Py) bilayers was identified.
Abstract: We experimentally identify coherent spin pumping in the magnon-magnon hybrid modes of yttrium iron garnet/permalloy (YIG/Py) bilayers. By reducing the YIG and Py thicknesses, the strong interfacial exchange coupling leads to large avoided crossings between the uniform mode of Py and the spin wave modes of YIG enabling accurate determination of modification of the linewidths due to the dampinglike torque. We identify additional linewidth suppression and enhancement for the in-phase and out-of-phase hybrid modes, respectively, which can be interpreted as concerted dampinglike torque from spin pumping. Furthermore, varying the Py thickness shows that both the fieldlike and dampinglike couplings vary like $1/\sqrt{{t}_{\mathrm{Py}}}$, verifying the prediction by the coupled Landau-Lifshitz equations.

Journal ArticleDOI
18 Dec 2020-Science
TL;DR: The speed of driven magnetic domain walls is fundamentally limited in analogy to special relativity, and record current-driven velocities in excess of 4300 meters per second are achieved—within ~10% of the relativistic limit.
Abstract: A tenet of special relativity is that no particle can exceed the speed of light. In certain magnetic materials, the maximum magnon group velocity serves as an analogous relativistic limit for the speed of magnetic solitons. Here, we drive domain walls to this limit in a low-dissipation magnetic insulator using pure spin currents from the spin Hall effect. We achieve record current-driven velocities in excess of 4300 meters per second-within ~10% of the relativistic limit-and we observe key signatures of relativistic motion associated with Lorentz contraction, which leads to velocity saturation. The experimental results are well explained through analytical and atomistic modeling. These observations provide critical insight into the fundamental limits of the dynamics of magnetic solitons and establish a readily accessible experimental framework to study relativistic solitonic physics.

Journal ArticleDOI
TL;DR: An experimental observation of magnon-magnon coupling in interlayer exchange coupled synthetic antiferromagnets of FeCoB/Ru/FeCoB layers finds that the coupling strength under the specified conditions is larger than the dissipation rates of both the resonance modes, indicating that a strong coupling regime is satisfied.
Abstract: We report an experimental observation of magnon-magnon coupling in interlayer exchange coupled synthetic antiferromagnets of FeCoB/Ru/FeCoB layers. An anticrossing gap of spin-wave resonance between acoustic and optic modes appears when the external magnetic field points to the direction tilted from the spin-wave propagation. The magnitude of the gap (i.e., coupling strength) can be controlled by changing the direction of the in-plane magnetic field and also enhanced by increasing the wave number of excited spin waves. We find that the coupling strength under the specified conditions is larger than the dissipation rates of both the resonance modes, indicating that a strong coupling regime is satisfied. A theoretical analysis based on the Landau-Lifshitz equation shows quantitative agreement with the experiments and indicates that the anticrossing gap appears when the exchange symmetry of two magnetizations is broken by the spin-wave excitation.

Journal ArticleDOI
TL;DR: It is demonstrated that by introducing a ferromagnetic layer, conventional coplanar waveguides can be used to efficiently generate exchange magnons, allowing one to harvest the advantages of nanomagnonics by antenna designs exploited in conventional microwave circuits.
Abstract: Exchange magnons are essential for unprecedented miniaturization of GHz electronics and magnon-based logic. However, their efficient excitation via microwave fields is still a challenge. Current methods including nanocontacts and grating couplers require advanced nanofabrication tools which limit the broad usage. Here, we report efficient emission and detection of exchange magnons using micron-sized coplanar waveguides (CPWs) into which we integrated ferromagnetic (m) layers. We excited magnons in a broad frequency band with wavelengths λ down to 100 nm propagating over macroscopic distances in thin yttrium iron garnet. Applying time- and spatially resolved Brillouin light scattering as well as micromagnetic simulations we evidence a significant wavelength conversion process near mCPWs via tunable inhomogeneous fields. We show how optimized mCPWs can form microwave-to-magnon transducers providing phase-coherent exchange magnons with λ of 37 nm. Without any nanofabrication they allow one to harvest the advantages of nanomagnonics by antenna designs exploited in conventional microwave circuits. Magnons - collective excitations of electron spins - promise compact and fast electronics. However, the generation of short wave magnons is still quite challenging. Here, the authors demonstrate that by introducing a ferromagnetic layer, conventional coplanar waveguides can be used to efficiently generate such magnons.

Journal ArticleDOI
TL;DR: In this article, it was shown that magnons in CoTiO have a similar energy-momentum relation to electrons in graphene, setting up CoTiOs as a good system in which to study interactions between so-called Dirac bosons.
Abstract: Experiments show that magnons in CoTiO${}_{3}$ have a similar energy-momentum relation to electrons in graphene, setting up CoTiO${}_{3}$ as a good system in which to study interactions between so-called Dirac bosons.

Journal ArticleDOI
TL;DR: In this paper, the authors theoretically explore nonlinearities of ferromagnets in microwave cavities in the classical and quantum regimes and assess the resources for quantum information, i.e., fluctuation squeezing and bipartite entanglement.
Abstract: We theoretically explore nonlinearities of ferromagnets in microwave cavities in the classical and quantum regimes and assess the resources for quantum information, i.e., fluctuation squeezing and bipartite entanglement. The (semi)classical analysis of the anharmonic oscillator (Duffing) model for the Kittel mode when including all other magnon modes, reveals chaotic and limit-cycle phases that do not survive in quantum calculations. However, magnons with nonzero wave numbers that are driven by the Suhl instability of the Kittel mode, form a genuine limit cycle. We subsequently compute bounds for the distillable entanglement, as well as entanglement of formation for the bipartite configurations of the mixed magnon modes. The former vanishes when obtained from a covariance matrix, but can be recovered by injection locking. The predicted magnon entanglement is experimentally accessible with yttrium iron garnet samples under realistic conditions.

Journal ArticleDOI
TL;DR: Experiments demonstrate coherent control of magnon spin transport and pseudospin dynamics in a thin film of the antiferromagnetic insulator hematite utilizing two Pt strips for all-electrical magnon injection and detection, unlocking the high potential of antiferromeagnetic magnonics toward the realization of rich electronics-inspired phenomena.
Abstract: We report on experiments demonstrating coherent control of magnon spin transport and pseudospin dynamics in a thin film of the antiferromagnetic insulator hematite utilizing two Pt strips for all-electrical magnon injection and detection. The measured magnon spin signal at the detector reveals an oscillation of its polarity as a function of the externally applied magnetic field. We quantitatively explain our experiments in terms of diffusive magnon transport and a coherent precession of the magnon pseudospin caused by the easy-plane anisotropy and the Dzyaloshinskii-Moriya interaction. This experimental observation can be viewed as the magnonic analog of the electronic Hanle effect and the Datta-Das transistor, unlocking the high potential of antiferromagnetic magnonics toward the realization of rich electronics-inspired phenomena.

Journal ArticleDOI
TL;DR: It is identified that spin effects do have clear roles in heat transport, which can be confirmed by phase shifts of voltage output varying with the direction of magnetization, and formulas fit the experimental data very well.
Abstract: The emerging of spin caloritronics leads to a series of new spin-thermal related effects, such as spin Seebeck effect (SSE), spin Nernst effect (SNE) and their corresponding inverse effects. Anomalous Righi–Leduc effect (ARLE) describes that a transverse temperature gradient can be induced by a longitudinal heat flow in ferromagnets. The driving force and the response of the ARLE are all involved with heat. It is curious if spin effects mediate the heat transport and provide extra influence. In this work, we investigate the ARLE and the interplay between the heat current, charge current, and spin current via linear response theory. We identified that spin effects do have clear roles in heat transport, which can be confirmed by phase shifts of voltage output varying with the direction of magnetization. Our formulas fit the experimental data very well. Moreover, we discuss more configuration of magnetization which is expected to be tested in the future. It should be emphasized that the present formalism including spin effects is out of the theory based on magnon transport, which may be conspicuous in the devices within the spin diffusion length.

Journal ArticleDOI
TL;DR: In this article, the authors present a theory of competing ferromagnetic and superconducting orders in a twisted double bilayer graphene system and show that the single-particle moir\'e bands can be drastically modified by a perpendicular electric displacement field.
Abstract: Twisted double bilayer graphene is a highly tunable moir\'e system to study strongly interacting physics. Here, the authors present a theory of competing ferromagnetic and superconducting orders in this system. They show that the single-particle moir\'e bands can be drastically modified by a perpendicular electric displacement field. As a result, the ferromagnetic insulating gap driven by Coulomb interaction has a dome shape dependence on the layer potential difference, as observed in several experiments. The stability of the ferromagnetic insulator against collective excitations, including spin and valley magnons, is theoretically verified. Furthermore, the authors investigate the possibility of phonon-mediated intervalley equal-spin pairing, using the property that the acoustic phonon mediated attraction respects an enlarged SU(2)\ifmmode\times\else\texttimes\fi{}SU(2) symmetry.

Journal ArticleDOI
TL;DR: This work derives general formulae for single magnon excitation rates from dark matter scattering, and demonstrates as a proof of principle the projected reach of a yttrium iron garnet target for several dark matter models with spin-dependent interactions.
Abstract: Scattering of light dark matter with sub-eV energy deposition can be detected with collective excitations in condensed matter systems. When dark matter has spin-independent couplings to atoms or ions, it has been shown to efficiently excite phonons. Here we show that, if dark matter couples to the electron spin, magnon excitations in materials with magnetic dipole order offer a promising detection path. We derive general formulae for single magnon excitation rates from dark matter scattering, and demonstrate as a proof of principle the projected reach of a yttrium iron garnet target for several dark matter models with spin-dependent interactions. This highlights the complementarity of various collective excitations in probing different dark matter interactions.

Journal ArticleDOI
TL;DR: In this article, the authors proposed two different mechanisms for observing the magnon blockade effect in the ferromagnetic sphere and showed that the much stronger magnon antibunching with significantly increased steady-state mean magnon numbers can be realized by the destructive interference for the two-magnon excitation.
Abstract: We study the generation of a magnon blockade in a single-crystalline yttrium-iron-garnet (YIG) sphere coupled to a three-dimensional superconducting microwave resonator that interacts with a superconducting qubit. Based on the indirect coupling between the Kittel mode of YIG and the superconducting qubit mediated by the virtual photon excitation in the microwave cavity, we propose two different mechanisms for observing the magnon blockade effect in the ferromagnetic sphere. The first one is to use the strong anharmonicity of the dressed states of the coupled qubit-magnon system. However, the strong magnon antibunching can only be achieved under the strong-coupling regime. To relax this constraint, we propose another quantum interference method to produce and enhance the magnon blockade effect with the moderate-coupling strength. By optimizing the relative phase and the strength ratio of the external driving fields applied to the YIG and qubit, we show that the much stronger magnon antibunching with significantly increased steady-state mean magnon numbers can be realized by the destructive interference for the two-magnon excitation.

Journal ArticleDOI
TL;DR: In this paper, the authors demonstrate that biquadratic exchange interactions, which is the simplest and most natural form of non-Heisenberg coupling, assume a key role in the magnetic properties of layered magnets.
Abstract: Magnetism in recently discovered van der Waals materials has opened new avenues in the study of fundamental spin interactions in truly two-dimensions. A paramount question is what effect higher-order interactions beyond bilinear Heisenberg exchange have on the magnetic properties of few-atom thick compounds. Here we demonstrate that biquadratic exchange interactions, which is the simplest and most natural form of non-Heisenberg coupling, assume a key role in the magnetic properties of layered magnets. Using a combination of nonperturbative analytical techniques, non-collinear first-principles methods and classical Monte Carlo calculations that incorporate higher-order exchange, we show that several quantities including magnetic anisotropies, spin-wave gaps and topological spin-excitations are intrinsically renormalized leading to further thermal stability of the layers. We develop a spin Hamiltonian that also contains antisymmetric exchanges (e.g. Dzyaloshinskii-Moriya interactions) to successfully rationalize numerous observations currently under debate, such as the non-Ising character of several compounds despite a strong magnetic anisotropy, peculiarities of the magnon spectrum of 2D magnets, and the discrepancy between measured and calculated Curie temperatures. Our results lay the foundation of a universal higher-order exchange theory for novel 2D magnetic design strategies.