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Journal ArticleDOI

A light-trapping strategy for nanocrystalline silicon thin-film solar cells using three-dimensionally assembled nanoparticle structures.

TLDR
The multiple plasmon resonances, together with the antireflection functionality arising from the conformally deposited top surface of the 3D solar cell, lead to a 22% and an 11% improvement in power conversion efficiency of the nc-Si:H thin-film solar cells compared to flat cells and cells employing nanoparticle clusters, respectively.
Abstract
We report three-dimensionally assembled nanoparticle structures inducing multiple plasmon resonances for broadband light harvesting in nanocrystalline silicon (nc-Si:H) thin-film solar cells. A three-dimensional multiscale (3DM) assembly of nanoparticles generated using a multi-pin spark discharge method has been accomplished over a large area under atmospheric conditions via ion-assisted aerosol lithography. The multiscale features of the sophisticated 3DM structures exhibit surface plasmon resonances at multiple frequencies, which increase light scattering and absorption efficiency over a wide spectral range from 350–1100 nm. The multiple plasmon resonances, together with the antireflection functionality arising from the conformally deposited top surface of the 3D solar cell, lead to a 22% and an 11% improvement in power conversion efficiency of the nc-Si:H thin-film solar cells compared to flat cells and cells employing nanoparticle clusters, respectively. Finite-difference time-domain simulations were also carried out to confirm that the improved device performance mainly originates from the multiple plasmon resonances generated from three-dimensionally assembled nanoparticle structures.

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Citations
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Design of Nanostructured Solar Cells Using Coupled Optical and Electrical Modeling - eScholarship

TL;DR: It is demonstrated that nanostructures can be tailored to minimize absorption in the doped a-Si:H, improving carrier collection efficiency and suggesting a method for device optimization in which optical design not only maximizes absorption, but also ensures resulting carriers are efficiently collected.
Journal ArticleDOI

Nanomanipulation and controlled self-assembly of metal nanoparticles and nanocrystals for plasmonics

TL;DR: This review discusses how meta-atoms can be assembled into unique plasmonic metastructures using a variety of nanomanipulation methods based on single- or multiple-probes in an atomic force microscope (AFM) or a scanning electron microscope (SEM), optical tweezers, and focused electron-beam nanomonipulation.
Journal ArticleDOI

Moth-Eye TiO2 Layer for Improving Light Harvesting Efficiency in Perovskite Solar Cells.

TL;DR: A moth-eye nanostructured mp-TiO2 film using conventional lithography, nano-imprinting and polydimethyl-siloxane (PDMS) stamping methods is demonstrated for the first time.
Journal ArticleDOI

Multifurcation Assembly of Charged Aerosols and Its Application to 3D Structured Gas Sensors

TL;DR: The gas sensor with the tetrafurcated-NP-assembled structure demonstrates ≈200% enhanced response to 100 ppm CO at 300 °C.
Journal ArticleDOI

Boosting ultrathin aSi-H solar cells absorption through a nanoparticle cross-packed metasurface

TL;DR: In this paper, the insertion of a metasurface based on a cross-patterned ITO contact film, where the crosses are filled with nanospheres was proposed.
References
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Journal ArticleDOI

Plasmonics for improved photovoltaic devices

TL;DR: Recent advances at the intersection of plasmonics and photovoltaics are surveyed and an outlook on the future of solar cells based on these principles is offered.
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Plasmonics: Localization and guiding of electromagnetic energy in metal/dielectric structures

TL;DR: In this article, the basic physics of surface-plasmon excitations occurring at metal/dielectric interfaces with special emphasis on the possibility of using such excitations for the localization of electromagnetic energy in one, two, and three dimensions, in a context of applications in sensing and waveguiding for functional photonic devices.
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Photovoltaic Technology: The Case for Thin-Film Solar Cells

TL;DR: The advantages and limitations of photovoltaic solar modules for energy generation are reviewed with their operation principles and physical efficiency limits, and recent developments suggest that thin-film crystalline silicon (especially microcrystalline silicon) is becoming a prime candidate for future photov electricity generation.
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Anti-reflective coatings: A critical, in-depth review

TL;DR: In this paper, the basic concepts and strategies adopted to minimize reflectance of anti-reflective coatings (ARCs) are described in greater detail and state-of-the-art fabrication techniques have been fully illustrated.
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Thin‐film silicon solar cell technology

TL;DR: In this article, the authors describe the use of hydrogenated amorphous silicon (a-Si:H) and hydrogenated micro-crystalline silicon (μc-Si-H) thin films (layers), both deposited at low temperatures (200°C) by plasma-assisted chemical vapour deposition (PECVD), from a mixture of silane and hydrogen.
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