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Programmed Multiresponsive Hydrogel Assemblies with Light‐Tunable Mechanical Properties, Actuation, and Fluorescence

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TLDR
The PRLDA method provides new insight into programmed gel property control and has excellent potential for biomaterial and optoelectronic applications.
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This article is published in Advanced Functional Materials.The article was published on 2020-03-01 and is currently open access. It has received 36 citations till now.

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Stimuli-responsive functional materials for soft robotics

TL;DR: This review covers five representative types of soft stimuli-responsive functional materials, namely (i) dielectric elastomers, (ii) hydrogels, (iii) shape memory polymers, (iv) liquid crystal elastomer, and (v) magnetic materials, with focuses on their inherent material properties, working mechanisms, and design strategies for actuation and sensing.
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Reconstructable Gradient Structures and Reprogrammable 3D Deformations of Hydrogels with Coumarin Units as the Photolabile Crosslinks

TL;DR: In this paper, a photo-crosslink-based reprogramming of the gradient structures and 3D deformations of a hydrogel is presented. But existing gradient structures of hydrogels are usually non-reconstructable, once encoded by chemical reactions and covalent bonds.
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Stimuli-responsive hydrogels: Fabrication and biomedical applications

TL;DR: This review presents typical synthetic and natural gelators comprising small molecules and polymers as building blocks of functional architectures and discusses the fabrication strategies of hydrogels varied from supramolecular assembly to dynamic covalent binding.
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Mimicking Color-Changing Organisms to Enable the Multicolors and Multifunctions of Smart Fluorescent Polymeric Hydrogels.

TL;DR: The unique hierarchical multilayer structures of skin chromatophores in structural color-changing reptiles are introduced, followed by an in-depth discussion on how a rational integration of bioinspiration and man-made design makes it possible to largely expand the fluorescence color- changing range of smart FPHs to almost cover the whole visible spectrum.
References
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Synthetic biomaterials as instructive extracellular microenvironments for morphogenesis in tissue engineering

TL;DR: Although modern synthetic biomaterials represent oversimplified mimics of natural ECMs lacking the essential natural temporal and spatial complexity, a growing symbiosis of materials engineering and cell biology may ultimately result in synthetic materials that contain the necessary signals to recapitulate developmental processes in tissue- and organ-specific differentiation and morphogenesis.
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Design, fabrication and control of soft robots

TL;DR: This Review discusses recent developments in the emerging field of soft robotics, and explores the design and control of soft-bodied robots composed of compliant materials.
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Designing materials for biology and medicine

TL;DR: New challenges and directions in biomaterials research are discussed, including synthetic replacements for biological tissues, designing materials for specific medical applications, and materials for new applications such as diagnostics and array technologies.
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Hydrogels in regenerative medicine

TL;DR: The properties of hydrogels that are important for tissue engineering applications and the inherent material design constraints and challenges are discussed.
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