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The interplay between solid electrolyte interface (SEI) and dendritic lithium growth

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TLDR
In this article, a straightforward approach is proposed to induce the growth of detrimental dendritic Li so the cells are “shorted” frequently and consistently, based on this new protocol, various electrolytes are revisited and the SEI derived are compared and quantified, providing new insights for addressing the challenges in rechargeable Li metal battery technologies.
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This article is published in Nano Energy.The article was published on 2017-10-01. It has received 177 citations till now.

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Recent progress in liquid electrolytes for lithium metal batteries

TL;DR: Li metal batteries are revived as the next generation batteries beyond Li-ion batteries as discussed by the authors, which can reach energy densities of Li/LiMO2 and Li/S,O2 batteries, respectively, which surpass that of the state-of-the-art LIB (280 Whkg−1).
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2 D Materials for Inhibiting the Shuttle Effect in Advanced Lithium–Sulfur Batteries

TL;DR: The controlled spacing of two-dimensional materials, abundant active sites and large transverse size separators and interlayers, and the effects of interlayer and separator based on two- dimensional materials on lithium anode prevent polysulfide dissolution were reviewed.
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Spontaneously formation of SEI layers on lithium metal from LiFSI/DME and LiTFSI/DME electrolytes

TL;DR: In this article, the spontaneous formation of solid electrolyte interphase (s-SEI) on the surface of lithium metal was investigated by AFM and in-depth XPS profile analysis revealed that s-SEIs were similar to the electrochemically reduced SEI layers, mainly composed of inorganic components, such as LiF, Li3N, organic components of alkyl lithium carbonate (ROCO2Li) and lithium alkylsates (ROLi).
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Inducing uniform lithium nucleation by integrated lithium-rich li-in anode with lithiophilic 3D framework

TL;DR: Li-rich Li-In anode with lithiophilic In3Li13 framework was designed and prepared by a facile one-step vacuum evaporation approach as discussed by the authors.
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Effect of polyphenol-polyamine treated polyethylene separator on the ionic conduction and interface properties for lithium-metal anode batteries

TL;DR: In this paper, a detailed study was carried out to clearly explore the influence of separator wettability on ionic conduction and interface properties for lithium-metal anode batteries.
References
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Journal ArticleDOI

Nonaqueous liquid electrolytes for lithium-based rechargeable batteries.

TL;DR: The phytochemical properties of Lithium Hexafluoroarsenate and its Derivatives are as follows: 2.2.1.
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Reviving the lithium metal anode for high-energy batteries

TL;DR: The current understanding on Li anodes is summarized, the recent key progress in materials design and advanced characterization techniques are highlighted, and the opportunities and possible directions for future development ofLi anodes in applications are discussed.
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"Water-in-salt" electrolyte enables high-voltage aqueous lithium-ion chemistries.

TL;DR: A highly concentrated aqueous electrolyte whose window was expanded to ~3.0 volts with the formation of an electrode-electrolyte interphase, which could potentially be replaced with a safer aQueous alternative to lithium-ion batteries.
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Review of selected electrode–solution interactions which determine the performance of Li and Li ion batteries

TL;DR: In this article, the performance of Li, Li-C anodes and Li x MO y cathodes depends on their surface chemistry in solutions, which either contribute to electrode stabilization or to capacity fading due to an increase in the electrodes' impedance.
Journal ArticleDOI

High rate and stable cycling of lithium metal anode

TL;DR: It is reported that the use of highly concentrated electrolytes composed of ether solvents and the lithium bis(fluorosulfonyl)imide salt enables the high-rate cycling of a lithium metal anode at high Coulombic efficiency (up to 99.1%) without dendrite growth.
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