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Showing papers on "Ultrashort pulse published in 2021"


Journal ArticleDOI
22 Jan 2021-Science
TL;DR: Ultrafast dark-field electron microscopy is introduced to map the order parameter across a structural phase transition in the layered material 1 T-polytype of tantalum disulfide, and the distinctive benefits of selective contrast enhancement will inspire future beam-shaping technology in ultrafast transmission electron microscope.
Abstract: Understanding microscopic processes in materials and devices that can be switched by light requires experimental access to dynamics on nanometer length and femtosecond time scales. Here, we introduce ultrafast dark-field electron microscopy to map the order parameter across a structural phase transition. We use ultrashort laser pulses to locally excite a 1T-TaS2 (1T-polytype of tantalum disulfide) thin film and image the transient state of the specimen by ultrashort electron pulses. A tailored dark-field aperture array allows us to track the evolution of charge-density wave domains in the material with simultaneous femtosecond temporal and 5-nanometer spatial resolution, elucidating relaxation pathways and domain wall dynamics. The distinctive benefits of selective contrast enhancement will inspire future beam-shaping technology in ultrafast transmission electron microscopy.

80 citations


Journal ArticleDOI
TL;DR: In this article, the authors used WxNb(1−x)Se2 nanosheets as a rising ultrafast photonic device to generate high power mode-locked and Q-switched pulses in a fiber laser.
Abstract: Ternary transition metal chalcogenides (TTMDCs), a novel type of two-dimensional (2D) three-element materials, possess multiple physical and chemical properties and have promising potentials in basic physics and devices. Herein, the usage of WxNb(1−x)Se2 nanosheets as a rising ultrafast photonic device to generate high power mode-locked and Q-switched pulses in a fiber laser is demonstrated. The WxNb(1−x)Se2 nanosheets were successfully prepared by the liquid exfoliation method with thickness less than 3 nm. The nonlinear optical absorption of the WxNb(1−x)Se2-based device was investigated with the saturable intensity of 40.93 MW cm−2 and modulation depth of 5.43%. After integrating the WxNb(1−x)Se2-based device into an Er-doped fiber (EDF) laser cavity, mode-locking and Q-switching laser pulses were formed. In the mode-locked mechanism output, the pulse width is as narrow as 131 fs and the output power is 52.93 mW. In Q-switched operation, the shortest pulse duration is 1.47 μs with the largest pulse energy of 257 nJ. Compared to recent studies, our results showed some improvements. This study suggests that 2D TTMDC-based devices could be developed as efficient ultrafast photonics candidates and widely used in nonlinear optical applications.

78 citations


Journal ArticleDOI
TL;DR: In this article, the authors proposed the soliton distillation by making NFT on a steady pulse generated from a fiber laser, then filtering out the eigenvalues of the resonant continuous wave background in the nonlinear frequency domain, and finally recovering the solitons by inverse NFT (INFT).
Abstract: An elegant method of nonlinear Fourier transform (NFT) has attracted worldwide research interests and such NFT methodology provides a new viewpoint on the physics of laser dynamics. Recently, the use of the NFT has been proposed for the investigation of laser radiation, indicating the capability to characterize the ultrashort pulse in the nonlinear frequency domain. Here, pure solitons are numerically separated from the resonant continuous wave (CW) background in a fiber laser by utilizing NFT. It is identified that the soliton and the resonant CW background have different eigenvalue distributions in the nonlinear frequency domain. Similar to water distillation, we propose the approach of soliton distillation, by making NFT on a steady pulse generated from a fiber laser, then filtering out the eigenvalues of the resonant CW background in the nonlinear frequency domain, and finally recovering the soliton by inverse NFT (INFT). Simulation results verify that the soliton can be distinguished from the resonant CW background in the nonlinear frequency domain and pure solitons can be obtained by INFT.

68 citations


Journal ArticleDOI
TL;DR: This work shows how a recurrent neural network with long short-term memory accurately predicts the temporal and spectral evolution of higher-order soliton compression and supercontinuum generation, solely from a given transform-limited input pulse intensity profile.
Abstract: The propagation of ultrashort pulses in optical fibre plays a central role in the development of light sources and photonic technologies, with applications from fundamental studies of light–matter interactions to high-resolution imaging and remote sensing. However, short pulse dynamics are highly nonlinear, and optimizing pulse propagation for application purposes requires extensive and computationally demanding numerical simulations. This creates a severe bottleneck in designing and optimizing experiments in real time. Here, we present a solution to this problem using a recurrent neural network to model and predict complex nonlinear propagation in optical fibre, solely from the input pulse intensity profile. We highlight particular examples in pulse compression and ultra-broadband supercontinuum generation, and compare neural network predictions with experimental data. We also show how the approach can be generalized to model other propagation scenarios for a wider range of input conditions and fibre systems, including multimode propagation. These results open up novel perspectives in the modelling of nonlinear systems, for the development of future photonic technologies and more generally in physics for studies in Bose–Einstein condensates, plasma physics and hydrodynamics. The propagation of ultrashort pulses in optical fibres, of interest in scientific studies of nonlinear systems, depends sensitively on both the input pulse and the fibre characteristics and normally requires extensive numerical simulations. A new approach based on a recurrent neural network can predict complex nonlinear propagation in optical fibre, solely from the input pulse intensity profile, and helps to design experiments in pulse compression and ultra-broadband supercontinuum generation.

63 citations


Journal ArticleDOI
01 Jan 2021
TL;DR: In this paper, post compression of short laser pulses was used to generate high energy few-cycle light pulses for ultrafast science. But this method is not suitable for high-energy few-cycled light pulses.
Abstract: Contemporary ultrafast science requires reliable sources of high-energy few-cycle light pulses. Currently two methods are capable of generating such pulses: post compression of short laser pulses a...

55 citations


Journal ArticleDOI
TL;DR: An ultrafast laser based on coherent beam combination of four ytterbium-doped step-index fiber amplifiers is presented in this article, which delivers an average power of 35 kW and a pulse duration of 430 fs at 80 MHz repetition rate.
Abstract: An ultrafast laser based on coherent beam combination of four ytterbium-doped step-index fiber amplifiers is presented The system delivers an average power of 35 kW and a pulse duration of 430 fs at 80 MHz repetition rate The beam quality is excellent (M2<124x110) and the relative intensity noise is as low as 1% in the frequency span from 1 Hz to 1 MHz The system is turn-key operable as it features an automated spatial and temporal alignment of the interferometric amplification channels

50 citations


Journal ArticleDOI
Bo Guo1, Xinyu Guo1, Lige Tang1, Wenlei Yang1, Qiumei Chen1, Zhongyao Ren1 
TL;DR: In this paper, the authors proposed and demonstrated the cascaded multi-wavelength mode-locked erbium-doped fiber laser (EDFL) based on ULPGs for the first time, to the best of their knowledge.
Abstract: We propose and demonstrate the cascaded multi-wavelength mode-locked erbium-doped fiber laser (EDFL) based on ultra-long-period gratings (ULPGs) for the first time, to the best of our knowledge. Study found that the ULPG can be used as both a mode-locker for pulse shaping and a comb filter for multi-wavelength generation simultaneously. Using the dual-function of ULPG, three-, four-, five-, six-, and seven-wavelength mode-locked pulses are obtained in EDFL, seven of which are the largest number of wavelengths up to now. For the four-wavelength soliton pulses, their pulse width is about 7.8 ps. The maximum average output power and slope efficiency of these pulses are 8.4 mW and 2.03%, respectively. Besides the conventional pulses, hybrid soliton pulses composed of a four-wavelength pulse and single soliton are also observed. Finally, the effect of cavity dispersion on the multi-wavelength mode-locked pulses is also discussed. Our findings indicate that apart from common sensing and filtering, the ULPG may also possess attractive nonlinear pulse-shaping property for ultrafast photonics application.

45 citations


Journal ArticleDOI
TL;DR: In this article, the authors demonstrate the optical frequency division of an optically carried 3.6 GHz reference down to 300 GHz through a dissipative Kerr soliton, photodetected with an ultrafast uni-travelling-carrier photodiode.
Abstract: Optical frequency division via optical frequency combs has enabled a leap in microwave metrology, leading to noise performance never explored before. Extending this method to the millimetre-wave and terahertz-wave domains is of great interest. Dissipative Kerr solitons in integrated photonic chips offer the unique feature of delivering optical frequency combs with ultrahigh repetition rates from 10 GHz to 1 THz, making them relevant gears for performing optical frequency division in the millimetre-wave and terahertz-wave domains. We experimentally demonstrate the optical frequency division of an optically carried 3.6 THz reference down to 300 GHz through a dissipative Kerr soliton, photodetected with an ultrafast uni-travelling-carrier photodiode. A new measurement system, based on the characterization of a microwave reference phase locked to the 300 GHz signal under test, yields attosecond-level timing-noise sensitivity, overcoming conventional technical limitations. This work places dissipative Kerr solitons as a leading technology in the millimetre-wave and terahertz-wave field, promising breakthroughs in fundamental and civilian applications. A 300 GHz signal is generated by the combination of a low-noise stimulated Brillouin scattering process, dissipative Kerr soliton comb and optical-to-electrical conversion. A phase noise of −100 dBc Hz−1 is achieved at a Fourier frequency of 10 kHz.

44 citations


Journal ArticleDOI
TL;DR: In this paper, an ultrafast fiber chirped-pulse amplifier comprising 8 coherently combined amplifier channels is presented, which delivers 1 kW average power at 1 mJ pulse energy and 260 fs pulse duration.
Abstract: An ultrafast fiber chirped-pulse amplifier comprising 8 coherently combined amplifier channels is presented. The laser delivers 1 kW average power at 1 mJ pulse energy and 260 fs pulse duration. Excellent beam quality and low noise performance are confirmed. The laser has proven suitable for demanding scientific applications. Further power scaling is possible right away using even more amplifier channels

44 citations


Journal ArticleDOI
TL;DR: In this paper, a RexNb(1-x)S2-based saturable absorber (SA) device for ultrafast photonics applications is studied, where the device is assembled by placing Rex NbS2 nanosheets with a thickness of 1-3 nm onto a microfiber to increase their compatibility with an all-fiber laser cavity.
Abstract: Two-dimensional (2D) transition metal chalcogenides (TMCs) become more attractive upon addition of a third element owing to their unique structure and remarkable physical and chemical properties, which endow these materials with considerable potential for applications in nanoscale devices. In this work, a RexNb(1-x)S2-based saturable absorber (SA) device for ultrafast photonics applications is studied. The device is assembled by placing RexNb(1-x)S2 nanosheets with a thickness of 1-3 nm onto a microfiber to increase their compatibility with an all-fiber laser cavity. The prepared RexNb(1-x)S2-based device exhibits a modulation depth of 24.3%, a saturation intensity of 10.1 MW/cm2, and a nonsaturable loss of 28.5%. Furthermore, the RexNb(1-x)S2-based device is used to generate ultrashort pulses in an erbium-doped fiber (EDF) laser cavity. At a pump power of 260 mW, the EDF laser operates in a conventional soliton mode-locked region. The pulse width is 285 fs, and the repetition frequency is 61.993 MHz. In particular, the bound-state soliton mode-locking operation is successfully obtained in a pump power range of 300-900 mW. The bound-state pulses are formed by doubling identical solitons with a temporal interval of 0.8 ps. The output power is as high as 47.9 mW, and the repetition frequency is 123.61 MHz. These results indicate that the proposed RexNb(1-x)S2-based SAs have comparable properties to currently used 2D SAs and provide a basis for their application in the field of ultrafast photonics.

43 citations


Journal ArticleDOI
TL;DR: Water-in-salt electrolytes (WiSEs) are a promising candidate for use in energy storage devices because of their wide electrochemical stability window (ESW) that overcomes the thermodynamic limit of as mentioned in this paper.
Abstract: Water-in-salt electrolytes (WiSEs) are a promising candidate for use in energy storage devices because of their wide electrochemical stability window (ESW) that overcomes the thermodynamic limit of

Journal ArticleDOI
TL;DR: In this paper, the authors mainly focus on the control and amplification of double-hump solitons in fiber lasers theoretically, and the bilinear forms and soliton solutions of the coupled Manakov equations are presented.
Abstract: The fiber laser has become an ideal ultrashort pulse source because of its cheap structure, high integration, convenient and controllable output direction, which greatly promotes the development and application of ultrafast optics. This paper mainly focuses on the control and amplification of double-hump solitons in fiber lasers theoretically. The bilinear forms and soliton solutions of the coupled Manakov equations are presented, and the transmission of double-hump solitons is discussed. The factors affecting the stable transmission of double-hump solitons are analyzed. The relevant conclusions have important guiding significance for understanding the generation of stable double-hump solitons in fiber lasers.

Journal ArticleDOI
TL;DR: In this article, the authors demonstrate synchronized multi-wavelength mode-locked soliton fiber lasers generating ultrafast outputs from two to five wavelengths with a high sub-pulse repetition rate.
Abstract: Locking of longitudinal modes in laser cavities is the common path to generate ultrashort pulses. In traditional multi-wavelength mode-locked lasers, the group velocities rely on lasing wavelengths due to the chromatic dispersion, yielding multiple trains of independently evolved pulses. Here, we show that mode-locked solitons at different wavelengths can be synchronized inside the cavity by engineering the intracavity group delay with a programmable pulse shaper. Frequency-resolved measurements fully retrieve the fine temporal structure of pulses, validating the direct generation of synchronized ultrafast lasers from two to five wavelengths with sub-pulse repetition-rate up to ~1.26 THz. Simulation results well reproduce and interpret the key experimental phenomena, and indicate that the saturable absorption effect automatically synchronize multi-wavelength solitons in despite of the small residual group delay difference. These results demonstrate an effective approach to create synchronized complex-structure solitons, and offer an effective platform to study the evolution dynamics of nonlinear wavepackets. The coherence degradation of pulses synchronized to optical cavities is an issue for ultrahigh-repetition-rate lasing. Here the authors demonstrate synchronized multi-wavelength mode-locked soliton fiber lasers generating ultrafast outputs from two to five wavelengths with a high sub-pulse repetition rate.

Journal ArticleDOI
TL;DR: In this article, the authors report an in-depth experimental study of high ultrafast laser ablation efficiency for processing of copper and steel with single-pulses, MHz, GHz, and burst-in-the-burst (biburst) regimes.
Abstract: Here, to the best of our knowledge, for the first time we report an in-depth experimental study of high ultrafast laser ablation efficiency for processing of copper and steel with single-pulses, MHz, GHz, and burst-in-the-burst (biburst) regimes The comparison of burst, biburst, and single-pulse ablation efficiencies was performed for beam-size-optimised regimes, showing the real advantages and disadvantages of milling and drilling processing approaches Highly efficient ultrashort pulse laser processing was achieved for ∼1 µm optical wavelength: 88 µm3/µJ for copper drilling, 56 µm3/µJ for copper milling, and 69 µm3/µJ for steel milling We believe that the huge experimental data collected in this study will serve well for the better understanding of laser burst-matter interaction and theoretical modelling

Journal ArticleDOI
TL;DR: In this article, the authors demonstrate all-optical modulation of second-harmonic generation in MoS2 with a modulation depth of close to 100% and speed limited only by the fundamental pulse duration.
Abstract: Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced functionalities are enabled by modulation of the harmonic generation efficiency, which can be achieved with electrical or all-optical triggers. Electrical control of the harmonic generation efficiency offers large modulation depth at the cost of low switching speed, by contrast to all-optical nonlinear devices, which provide high speed and low modulation depth. Here we demonstrate all-optical modulation of second-harmonic generation in MoS2 with a modulation depth of close to 100% and speed limited only by the fundamental pulse duration. This result arises from a combination of D3h crystal symmetry and the deep subwavelength thickness of the sample, it can therefore be extended to the whole family of transition metal dichalcogenides to provide great flexibility in the design of advanced nonlinear optical devices such as high-speed integrated frequency converters, broadband autocorrelators for ultrashort pulse characterization, and tunable nanoscale holograms.

Journal ArticleDOI
TL;DR: To the best of the knowledge, this is the first time that optical microfiber coupler based saturable absorber (OMC-SA) for mode-locked fiber laser is demonstrated.
Abstract: We demonstrated a mode-locked fiber laser based on a novel photonic device that combined optical microfiber coupler (OMC) and saturable absorption materials. The stable ultrafast laser was formed based on the interaction between the deposited Indium Antimonide (InSb) and the evanescent field on OMC. Different from optical microfiber (OM), OMC can directly output the mode-locked laser without additional beam splitting devices, which further improves the integrated characteristics of the fiber laser. The pulse duration of the output pulse is 405 fs at the central wavelength of 1560 nm. To the best of our knowledge, this is the first time that optical microfiber coupler based saturable absorber (OMC-SA) for mode-locked fiber laser is demonstrated.

Journal ArticleDOI
TL;DR: Through rigorous semiclassical theory involving a quantum description of the electrons, it is shown that monochromatic optical fields focused in vacuum can be used to correct electron beam aberrations and produce selected focal shapes.
Abstract: We exploit free-space interactions between electron beams and tailored light fields to imprint on-demand phase profiles on the electron wave functions. Through rigorous semiclassical theory involving a quantum description of the electrons, we show that monochromatic optical fields focused in vacuum can be used to correct electron beam aberrations and produce selected focal shapes. Stimulated elastic Compton scattering is exploited to imprint the required electron phase, which is proportional to the integral of the optical field intensity along the electron path and depends on the transverse beam position. The required light intensities are attainable in currently available ultrafast electron microscope setups, thus opening the field of free-space optical manipulation of electron beams.

Journal ArticleDOI
TL;DR: In this paper, a perspective review over the recent development of short-pulsed Raman fiber laser (RFLs), which can provide laser emissions with flexible wavelengths for a variety of applications as well as an excellent platform to investigate various nonlinear pulse dynamics behaviors that cannot be captured in conventional rare-earth (RE) doped counterparts, is provided.
Abstract: We provide a perspective review over the recent development of short-pulsed Raman fiber lasers (RFLs), which can provide laser emissions with flexible wavelengths for a variety of applications as well as an excellent platform to investigate various nonlinear pulse dynamics behaviors that cannot be captured in conventional rare-earth (RE) doped counterparts Various pulse generation techniques have been explored in RFLs However, the output pulse performance in terms of the pulse energy, duration and stability from short-pulsed RFLs is still inferior to their RE-doped counterparts despite significant advances made over the past few decades Therefore, more efforts are required to improve these targets In this review, we present a detailed overview of the short-pulsed RFLs based on different mechanisms from the principle to the experiment, including the Q-switching, gain-switching, mode-locking, synchronous pumping and other innovative techniques In addition, Raman-induced pulse dynamics in ultrafast RFLs and RE-doped mode-locked fiber lasers (MLFLs) are briefly reviewed Finally, a perspective outlook for the future ultrafast RFLs is provided based on their potential applications in industrial and scientific research areas

Journal ArticleDOI
14 Oct 2021
TL;DR: In this article, the authors use laser light and a transmission electron microscope to modulate a free-electron beam into high-contrast electron pulses and freeelectron qubits by using temporal Talbot revivals.
Abstract: We use laser light and a transmission electron microscope to modulate a free-electron beam into high-contrast electron pulses and free-electron qubits by using temporal Talbot revivals. At large enough propagation distances, the discrete energy sidebands from a laser modulation acquire special phases and group delays that optimize or cancel their time-domain interference, producing a revival or alternatively a pulse train at close to 100% modulation depth. A sequence of two laser interactions at an optimized propagation distance allows us to coherently control adjacent energy sidebands in amplitude and phase in the way of a qubit. The use of continuous-wave laser light provides these modulations at almost the full brightness of the beam source. Free electrons under large-distance laser control are therefore a promising tool for ultrafast material characterizations or investigations of free-electron quantum mechanics.

Journal ArticleDOI
TL;DR: In this article, the authors review the efficient generation of customized focus distributions from the near-infrared down to the deep ultraviolet, e.g., based on nondiffracting beams and three-dimensional-beam splitters, and demonstrate their impact for micro-and nanomachining of a wide range of materials.
Abstract: The industrial maturity of ultrashort pulsed lasers has triggered the development of a plethora of material processing strategies. Recently, the combination of these remarkable temporal pulse properties with advanced structured light concepts has led to breakthroughs in the development of laser application methods, which will now gradually reach industrial environments. We review the efficient generation of customized focus distributions from the near-infrared down to the deep ultraviolet, e.g., based on nondiffracting beams and three-dimensional-beam splitters, and demonstrate their impact for micro- and nanomachining of a wide range of materials. In the beam shaping concepts presented, special attention was paid to suitability for both high energies and high powers.

Journal ArticleDOI
07 Jul 2021
TL;DR: In this paper, a molecular attosecond interferometry that enables the in situ manipulation of holes in carbon dioxide molecules via the interference of phase-locked electrons (propagating in opposite directions) of a laser-triggered rotational wave packet is presented.
Abstract: Understanding the evolution of molecular electronic structures is the key to explore and control photochemical reactions and photobiological processes. Subjected to strong laser fields, electronic holes are formed upon ionization and evolve in the attosecond timescale. It is crucial to probe the electronic dynamics in real time with attosecond-temporal and atomic-spatial precision. Here, we present molecular attosecond interferometry that enables the in situ manipulation of holes in carbon dioxide molecules via the interferometry of the phase-locked electrons (propagating in opposite directions) of a laser-triggered rotational wave packet. The joint measurement on high-harmonic and terahertz spectroscopy (HATS) provides a unique tool for understanding electron dynamics from picoseconds to attoseconds. The optimum phases of two-color pulses for controlling the electron wave packet are precisely determined owing to the robust reference provided with the terahertz pulse generation. It is noteworthy that the contribution of HOMO-1 and HOMO-2 increases reflecting the deformation of the hole as the harmonic order increases. Our method can be applied to study hole dynamics of complex molecules and electron correlations during the strong-field process. The threefold control through molecular alignment, laser polarization, and the two-color pulse phase delay allows the precise manipulation of the transient hole paving the way for new advances in attochemistry.

Journal ArticleDOI
TL;DR: In this article, the authors studied the lifetime of polycyclic aromatic hydrocarbons following ionization by an ultrashort X-ray/XUV pulse and showed the universal role of correlation bands created by electron correlation.
Abstract: Modern ultrashort X-ray/XUV (extreme ultraviolet) sources provide unique opportunities to investigate the primary reactions of matter upon energetic excitation. Understanding these processes in molecules on ultrafast timescales is required to improve bespoke high-energy radiation detectors, nanomedicine schemes or to study the molecular composition of interstellar media. However, current experiments struggle to provide a general framework because of the uniqueness and complexity of each system. Here we show the universal role of correlation bands—features created by electron correlation. This is done by studying ultrafast energy relaxation of size-scalable two-dimensional molecules following ionization by an ultrashort XUV pulse. We observed long lifetimes that nonlinearly increase with the number of valence electrons. A general law based on solid-like electron–phonon scattering is proposed, which explains both our results and previously reported measurements. This offers new opportunities in attosecond science and high-energy photophysics. The size-dependent lifetimes observed in the ultrafast molecular relaxation dynamics of an entire class of polycyclic aromatic hydrocarbons can be explained by correlation bands and electron–phonon scattering, reminiscent of solid-state systems.

Journal ArticleDOI
TL;DR: In this article, the influence of USP polishing on surface properties of 1.2738 tool steel including surface roughness, surface topography and microstructure of the remelted surface layer was investigated.

Journal ArticleDOI
07 Jul 2021-ACS Nano
TL;DR: In this article, the authors proposed and experimentally demonstrated ultrafast all-optical modulation of the second harmonic (SH) from a single nanoantenna based on a subwavelength AlGaAs nanopillar driven by a control femtosecond light pulse in the visible range.
Abstract: The enhancement of nonlinear optical effects via nanoscale engineering is a hot topic of research. Optical nanoantennas increase light-matter interaction and provide, simultaneously, a high throughput of the generated harmonics in the scattered light. However, nanoscale nonlinear optics has dealt so far with static or quasi-static configurations, whereas advanced applications would strongly benefit from high-speed reconfigurable nonlinear nanophotonic devices. Here we propose and experimentally demonstrate ultrafast all-optical modulation of the second harmonic (SH) from a single nanoantenna. Our design is based on a subwavelength AlGaAs nanopillar driven by a control femtosecond light pulse in the visible range. The control pulse photoinjects free carriers in the nanostructure, which in turn induce dramatic permittivity changes at the band edge of the semiconductor. This results in an efficient modulation of the SH signal generated at 775 nm by a second femtosecond pulse at the 1.55 μm telecommunications (telecom) wavelength. Our results can lead to the development of ultrafast, all optically reconfigurable, nonlinear nanophotonic devices for a broad class of telecom and sensing applications.

Journal ArticleDOI
20 Nov 2021
TL;DR: In this article, an isotropic nanovoid is generated with pulse energy above the microexplosion threshold and then elongated to an anisotropic nanolamella-like structure via the near-field enhancement effect by lower energy pulses, minimizing the unwanted thermal effects from megahertz-rate fs pulses.
Abstract: It is challenging to store the exponentially increasing amount of data in the information age. The multiplexed optical data storage with merits of high data density (hundreds of terabytes/disk), low energy consumption, and long lifetime could open a new era in data storage technology. The recent progress in five-dimensional (5D) optical data storage based on anisotropic nanostructures written by femtosecond (fs) laser pulses in transparent materials reveals its potential for real-world applications, but high writing speed and density remain a major challenge. Here, we propose a method for rapid and energy-efficient writing of highly localized anisotropic nanostructures in silica glass by energy modulated megahertz-rate fs pulses. An isotropic nanovoid is initially generated with pulse energy above the microexplosion threshold and then elongated to an anisotropic nanolamella-like structure via the near-field enhancement effect by lower energy pulses, minimizing the unwanted thermal effects from megahertz-rate fs pulses. The anisotropic nanostructures are exploited for 5D data storage with a rate of 106voxels/s, corresponding to a demonstrated fast information recording of ∼225kB/s and a potentially high-density data storage of ∼500TB/disk.

Journal ArticleDOI
TL;DR: In this paper, several layers of germanene were prepared with Dirac electronic characteristics and its morphology, band structure, carrier dynamics, and nonlinear optical properties were systematically investigated, and it was surprisingly found that Germanene has a fast carrier-relaxation time comparable to that of graphene and a relatively large nonlinear absorption coefficient, which is an order of magnitude higher than that of GAs in the near-infrared wavelength range.
Abstract: Bulk germanium as a group-IV photonic material has been widely studied due to its relatively large refractive index and broadband and low propagation loss from near-infrared to mid-infrared. Inspired by the research of graphene, the 2D counterpart of bulk germanium, germanene, has been discovered and the characteristics of Dirac electrons have been observed. However, the optical properties of germanene still remain elusive. In this work, several layers of germanene are prepared with Dirac electronic characteristics and its morphology, band structure, carrier dynamics, and nonlinear optical properties are systematically investigated. It is surprisingly found that germanene has a fast carrier-relaxation time comparable to that of graphene and a relatively large nonlinear absorption coefficient, which is an order of magnitude higher than that of graphene in the near-infrared wavelength range. Based on these findings, germanene is applied as a new saturable absorber to construct an ultrafast mode-locked laser, and sub-picosecond pulse generation in the telecommunication band is realized. The results suggest that germanene can be used as a new type of group-IV material for various nonlinear optics and photonic applications.

Journal ArticleDOI
Benhai Wang1, Haobin Han1, Lijun Yu1, Yueyue Wang1, Chaoqing Dai1 
TL;DR: In this article, an ultrashort pulse fiber laser based on VSe2/GO nanocomposite was reported and verified the formation process of soliton and soliton molecules by the numerical simulation.
Abstract: Recently, in addition to exploring the application of new saturable absorber devices in fiber lasers, soliton dynamics has also become a focus of current research. In this article, we report an ultrashort pulse fiber laser based on VSe2/GO nanocomposite and verify the formation process of soliton and soliton molecules by the numerical simulation. The prepared VSe2/GO-based device shows excellent saturable absorption characteristics with a modulation depth of 14.3% and a saturation absorption intensity of 0.93MW/cm2. The conventional soliton is obtained with pulse width of 573fs, which is currently the narrowest pulse width based on VSe2-related material, and has a signal-to-noise ratio of 60.4 dB. In addition, the soliton molecules are realized based on the VSe2/GO for the first time and have a pulse interval of ~2.2ps. We study the soliton dynamics through numerical simulation and reveal that before the formation of the soliton, it undergoes multiple nonlinear stages, such as soliton mode-locking, soliton splitting, and soliton oscillation. Furthermore, the results of numerical simulation are agreed well with the experimental data. These results indicate that the VSe2/GO might be another promising saturable absorber material for ultrafast photonics, and deepen the understanding of soliton dynamics in ultrafast fiber lasers.

Journal ArticleDOI
TL;DR: In this paper, a four-dimensional spatio-temporal approach is presented that extends and unifies both concepts of conical waves and helicon beams, mainly studied in bulk media, by taking advantage of tight correlations between the spatial modes, the topological charges, and the frequencies embedded in an optical field.
Abstract: Propagation-invariant or non-diffracting optical beams have received considerable attention during the last two decades. However, the pulsed nature of light waves and the structured property of optical media like waveguides are often overlooked. We here present a four-dimensional spatiotemporal approach that extends and unifies both concepts of conical waves and helicon beams, mainly studied in bulk media. By taking advantage of tight correlations between the spatial modes, the topological charges, and the frequencies embedded in an optical field, we reveal propagation-invariant (dispersion- and diffraction-free) space-time wavepackets carrying orbital angular momentum (OAM) that evolve on spiraling trajectories in both time and space in bulk media or multimode fibers. Besides their intrinsic linear nature, we show that such wave structures can spontaneously emerge when a rather intense ultrashort pulse propagates nonlinearly in OAM modes. With emerging technologies of pulse/beam shaping, multimode fibers and modal multiplexing, our proposed scheme to create OAM-carrying helicon wavepackets could find a plethora of applications.

Journal ArticleDOI
TL;DR: In this paper, the first mode-locked fiber laser was reported to operate in the femtosecond regime well beyond 3.5 µm with a minimum duration of 580 fs at a repetition rate of 68 MHz.
Abstract: We report the first mode-locked fiber laser to operate in the femtosecond regime well beyond 3 {\mu}m. The laser uses dual-wavelength pumping and non-linear polarisation rotation to produce 3.5 {\mu}m wavelength pulses with minimum duration of 580 fs at a repetition rate of 68 MHz. The pulse energy is 3.2 nJ, corresponding to a peak power of 5.5 kW.

Journal ArticleDOI
TL;DR: In this article, a fully polarization maintaining (PM) integrated laser features a chirped fiber Bragg grating (CFBG) for dispersion compensation and a fiber integrated compact non-reciprocal phase bias device, which is alignment free.
Abstract: We report a simple and compact design of a dispersion compensated mode-locked Yb:fiber oscillator based on a nonlinear amplifying loop mirror (NALM). The fully polarization maintaining (PM) fiber integrated laser features a chirped fiber Bragg grating (CFBG) for dispersion compensation and a fiber integrated compact non-reciprocal phase bias device, which is alignment-free. The main design parameters were determined by numerically simulating the pulse evolution in the oscillator and by analyzing their impact on the laser performance. Experimentally, we achieved an 88 fs compressed pulse duration with sub-fs timing jitter at 54 MHz repetition rate and 51 mW of output power with 5.5 * 10-5 [20 Hz, 1 MHz] integrated relative intensity noise (RIN). Furthermore, we demonstrate tight phase-locking of the laser's carrier-envelope offset frequency (fceo) to a stable radio frequency (RF) reference and of one frequency comb tooth to a stable optical reference at 291 THz.