Showing papers on "Master equation published in 2015"

Quantum optics of chiral spin networks

Abstract: We study the driven-dissipative dynamics of a network of spin-1/2 systems coupled to one or more chiral 1D bosonic waveguides within the framework of a Markovian master equation. We determine how the interplay between a coherent drive and collective decay processes can lead to the formation of pure multipartite entangled steady states. The key ingredient for the emergence of these many-body dark states is an asymmetric coupling of the spins to left and right propagating guided modes. Such systems are motivated by experimental possibilities with internal states of atoms coupled to optical fibers, or motional states of trapped atoms coupled to a spin-orbit coupled Bose-Einstein condensate. We discuss the characterization of the emerging multipartite entanglement in this system in terms of the Fisher information.

Variational Matrix Product Operators for the Steady State of Dissipative Quantum Systems

Abstract: We present a new variational method based on the matrix product operator (MPO) ansatz, for finding the steady state of dissipative quantum chains governed by master equations of the Lindblad form. Instead of requiring an accurate representation of the system evolution until the stationary state is attained, the algorithm directly targets the final state, thus, allowing for a faster convergence when the steady state is a MPO with small bond dimension. Our numerical simulations for several dissipative spin models over a wide range of parameters illustrate the performance of the method and show that, indeed, the stationary state is often well described by a MPO of very moderate dimensions.

Multiphoton-scattering theory and generalized master equations

Abstract: The analysis of photon scattering is a major challenge in the multiphoton regime. A framework based on a path-integral formalism provides a route to explore such dynamics, helping to investigate the quantum statistics of photons interacting with complex structures.

Relaxation times of dissipative many-body quantum systems.

Abstract: We study relaxation times, also called mixing times, of quantum many-body systems described by a Lindblad master equation. We in particular study the scaling of the spectral gap with the system length, the so-called dynamical exponent, identifying a number of transitions in the scaling. For systems with bulk dissipation we generically observe different scaling for small and for strong dissipation strength, with a critical transition strength going to zero in the thermodynamic limit. We also study a related phase transition in the largest decay mode. For systems with only boundary dissipation we show a generic bound that the gap cannot be larger than ∼1/L. In integrable systems with boundary dissipation one typically observes scaling of ∼1/L(3), while in chaotic ones one can have faster relaxation with the gap scaling as ∼1/L and thus saturating the generic bound. We also observe transition from exponential to algebraic gap in systems with localized modes.

Heavy quark master equations in the Lindblad form at high temperatures

Abstract: We derive the quantum master equations for heavy quark systems in a high-temperature quark-gluon plasma in the Lindblad form. The master equations are derived in the influence functional formalism for open quantum systems in perturbation theory. These master equations have a wide range of applications, such as decoherence of a heavy quarkonium and Langevin dynamics of a heavy quark in the quark-gluon plasma. We also show the equivalence between the quarkonium master equations in the recoilless limit and the Schr\"odinger equations with stochastic potential.

Diffusion with resetting in bounded domains

Abstract: We consider the one-dimensional diffusion in a bounded domain with stochastic resetting. We start our analysis by presenting a method to derive the master equation for different resetting mechanisms. In the next step we compute the non-equilibrium steady state for a special case of this differential equation. Then we consider the existence of an absorbing point in the system and calculate the mean time to absorption of the diffusive particle by the target. Numerical and analytical calculations of the optimal resetting rate reveal a second order phase transition. Finally we discuss different special cases of the presented problem.

Corner-Space Renormalization Method for Driven-Dissipative Two-Dimensional Correlated Systems.

Abstract: We present a theoretical method to study driven-dissipative correlated quantum systems on lattices with two spatial dimensions (2D). The steady-state density matrix of the lattice is obtained by solving the master equation in a corner of the Hilbert space. The states spanning the corner space are determined through an iterative procedure, using eigenvectors of the density matrix of smaller lattice systems, merging in real space two lattices at each iteration and selecting M pairs of states by maximizing their joint probability. The accuracy of the results is then improved by increasing the dimension M of the corner space until convergence is reached. We demonstrate the efficiency of such an approach by applying it to the driven-dissipative 2D Bose-Hubbard model, describing lattices of coupled cavities with quantum optical nonlinearities.

Multichannel 1 → 2 transition amplitudes in a finite volume

Abstract: We perform a model-independent, non-perturbative investigation of two-point and three-point finite-volume correlation functions in the energy regime where two-particle states can go on-shell. We study three-point functions involving a single incoming particle and an outgoing two-particle state, relevant, for example, for studies of meson decays (e.g., B⁰ → K*l⁺l⁻) or meson photo production (e.g., πγ* → ππ). We observe that, while the spectrum solely depends upon the on-shell scattering amplitude, the correlation functions also depend upon off-shell amplitudes. The main result of this work is a non-perturbative generalization of the Lellouch-Luscher formula relating matrix elements of currents in finite and infinite spatial volumes. We extend that work by considering a theory with multiple, strongly-coupled channels and by accommodating external currents which inject arbitrary four-momentum as well as arbitrary angular-momentum. The result is exact up to exponentially suppressed corrections governed by the pion mass times the box size. We also apply our master equation to various examples, including two processes mentioned above as well as examples where the final state is an admixture of two open channels.

Effective field theory during inflation: Reduced density matrix and its quantum master equation

Abstract: We study the power spectrum of super-Hubble fluctuations of an inflatonlike scalar field, the ``system,'' coupled to another scalar field, the ``environment'' during de Sitter inflation. We obtain the reduced density matrix for the inflaton fluctuations by integrating out the environmental degrees of freedom. These are considered to be massless and conformally coupled to gravity as a proxy to describe degrees of freedom that remain sub-Hubble all throughout inflation. The time evolution of the density matrix is described by a quantum master equation, which describes the decay of the vacuum state, the production of particles and correlated pairs and quantum entanglement between super and sub-Hubble degrees of freedom. The quantum master equation provides a nonperturbative resummation of secular terms from self-energy (loop) corrections to the inflaton fluctuations. In the case studied here these are Sudakov-type double logarithms which result in the decay of the power spectrum of inflaton fluctuations upon horizon crossing with a concomitant violation of scale invariance. The reduced density matrix and its quantum master equation furnish a powerful nonperturbative framework to study the effective field theory of long wavelength fluctuations by tracing short wavelength degrees of freedom.

Dissipative preparation of Chern insulators

Abstract: Engineered dissipation can be employed to prepare interesting quantum many-body states in a nonequilibrium fashion. The basic idea is to obtain the state of interest as the unique steady state of a quantum master equation, irrespective of the initial state. Due to a fundamental competition of topology and locality, the dissipative preparation of gapped topological phases with a nonvanishing Chern number has so far remained elusive. Here, we study the open quantum system dynamics of fermions on a two-dimensional lattice in the framework of a Lindblad master equation. In particular, we discover a mechanism to dissipatively prepare a topological steady state with nonzero Chern number by means of short-range system bath interaction. Quite remarkably, this gives rise to a stable topological phase in a nonequilibrium phase diagram. We demonstrate how our theoretical construction can be implemented in a microscopic model that is experimentally feasible with cold atoms in optical lattices.

Perturbative approach to Markovian open quantum systems

Abstract: The exact treatment of Markovian open quantum systems, when based on numerical diagonalization of the Liouville super-operator or averaging over quantum trajectories, is severely limited by Hilbert space size. Perturbation theory, standard in the investigation of closed quantum systems, has remained much less developed for open quantum systems where a direct application to the Lindblad master equation is desirable. We present such a perturbative treatment which will be useful for an analytical understanding of open quantum systems and for numerical calculation of system observables which would otherwise be impractical.

Gauge-Invariant Perturbations in Hybrid Quantum Cosmology

Abstract: We consider cosmological perturbations around homogeneous and isotropic spacetimes minimally coupled to a scalar field and present a formulation which is designed to preserve covariance. We truncate the action at quadratic perturbative order and particularize our analysis to flat compact spatial sections and a field potential given by a mass term, although the formalism can be extended to other topologies and potentials. The perturbations are described in terms of Mukhanov-Sasaki gauge invariants, linear perturbative constraints, and variables canonically conjugate to them. This set is completed into a canonical one for the entire system, including the homogeneous degrees of freedom. We find the global Hamiltonian constraint of the model, in which the contribution of the homogeneous sector is corrected with a term quadratic in the perturbations, that can be identified as the Mukhanov-Sasaki Hamiltonian in our formulation. We then adopt a hybrid approach to quantize the model, combining a quantum representation of the homogeneous sector with a more standard field quantization of the perturbations. Covariance is guaranteed in this approach inasmuch as no gauge fixing is adopted. Next, we adopt a Born-Oppenheimer ansatz for physical states and show how to obtain a Schrodinger-like equation for the quantum evolution of the perturbations. This evolution is governed by the Mukhanov-Sasaki Hamiltonian, with the dependence on the homogeneous geometry evaluated at quantum expectation values, and with a time parameter defined also in terms of suitable expectation values on that geometry. Finally, we derive effective equations for the dynamics of the Mukhanov-Sasaki gauge invariants, that include quantum contributions, but have the same ultraviolet limit as the classical equations. They provide the master equation to extract predictions about the power spectrum of primordial scalar perturbations.

Entanglement dynamics for uniformly accelerated two-level atoms

Abstract: We study, in the paradigm of open quantum systems, the entanglement dynamics of two uniformly accelerated atoms with the same acceleration perpendicular to the separation. The two-atom system is treated as an open system coupled with a bath of fluctuating massless scalar fields in the Minkowski vacuum, and the master equation that governs its evolution is derived. It has been found that, for accelerated atoms with a nonvanishing separation, entanglement sudden death is a general feature when the initial state is entangled, while for those in a separable initial state, entanglement sudden birth only happens for atoms with an appropriate interatomic separation and sufficiently small acceleration. Remarkably, accelerated atoms can get entangled in certain circumstances while the inertial ones in the Minkowski vacuum can not. A comparison between the results of accelerated atoms and those of static ones in a thermal bath shows that, uniformly accelerated atoms exhibit distinct features from those immersed in a thermal bath at the Unruh temperature in terms of entanglement dynamics.

Auxiliary master equation approach within matrix product states: Spectral properties of the nonequilibrium Anderson impurity model

Abstract: The non-equilibrium Anderson impurity model is solved to an unprecedented accuracy to obtain its spectral properties in the steady state using a recently developed approach.

The dissipative Bose-Hubbard model

Abstract: Open many-body quantum systems have attracted renewed interest in the context of quantum information science and quantum transport with biological clusters and ultracold atomic gases. The physical relevance in many-particle bosonic systems lies in the realization of counter-intuitive transport phenomena and the stochastic preparation of highly stable and entangled many-body states due to engineered dissipation. We review a variety of approaches to describe an open system of interacting ultracold bosons which can be modeled by a tight-binding Hubbard approximation. Going along with the presentation of theoretical and numerical techniques, we present a series of results in diverse setups, based on a master equation description of the dissipative dynamics of ultracold bosons in a one-dimensional lattice. Next to by now standard numerical methods such as the exact unravelling of the master equation by quantum jumps for small systems and beyond mean-field expansions for larger ones, we present a coherent-state path integral formalism based on Feynman-Vernon theory applied to a many-body context.

Kinetic Density Functional Theory for Plasmonic Nanostructures: Breaking of the Plasmon Peak in the Quantum Regime and Generation of Hot Electrons

Abstract: We develop a quantum kinetic theory of the dynamic response of typical noble metals. Our approach is based on the density functional theory (DFT) and incorporates new important elements as compared to the conventional time-dependent DFT formalism. The kinetic DFT is derived starting from the master equation of motion for the density matrix, which involves both momentum and energy relaxation processes. Therefore, the quantum system is described by two relaxation parameters, unlike the conventional time-dependent DFT incorporating only one relaxation parameter. This allows us to describe both the absorption of light and the generation of hot plasmonic electrons. Using our kinetic DFT theory, we also observe the transition from the multiple peaks in small size-quantized systems to the intensive plasmonic resonance in large classical systems. Unlike the standard picture of collisional broadening of the plasmon peak in small systems, we observe a very different scenario: the formation of multiple plasmonic-lik...

Effects of system-bath entanglement on the performance of light-harvesting systems: A quantum heat engine perspective

Abstract: We explore energy transfer in a generic three-level system, which is coupled to three non-equilibrium baths. Built on the concept of quantum heat engine, our three-level model describes non-equilibrium quantum processes including light-harvesting energy transfer, nano-scale heat transfer, photo-induced isomerization, and photovoltaics in double quantum-dots. In the context of light-harvesting, the excitation energy is first pumped up by sunlight, then is transferred via two excited states which are coupled to a phonon bath, and finally decays to the ground state. The efficiency of this process is evaluated by steady state analysis via a polaron-transformed master equation; thus a wide range of the system-phonon coupling strength can be covered. We show that the coupling with the phonon bath not only modifies the steady state, resulting in population inversion, but also introduces a finite steady state coherence which optimizes the energy transfer flux and efficiency. In the strong coupling limit, the steady state coherence disappears and the efficiency approaches the heat engine limit given by Scovil and Schultz-Dubois in Phys. Rew. Lett. 2, 262 (1959).

Fewest Switches Surface Hopping in Liouville Space.

Abstract: The novel approach to nonadiabatic quantum dynamics greatly increases the accuracy of the most popular semiclassical technique while maintaining its simplicity and efficiency. Unlike the standard Tully surface hopping in Hilbert space, which deals with population flow, the new strategy in Liouville space puts population and coherence on equal footing. Dual avoided crossing and energy transfer models show that the accuracy is improved in both diabatic and adiabatic representations and that Liouville space simulation converges faster with the number of trajectories than Hilbert space simulation. The constructed master equation accurately captures superexchange, tunneling, and quantum interference. These effects are essential for charge, phonon and energy transport and scattering, exciton fission and fusion, quantum optics and computing, and many other areas of physics and chemistry.

Transport through an Anderson impurity: Current ringing, nonlinear magnetization, and a direct comparison of continuous-time quantum Monte Carlo and hierarchical quantum master equations

Abstract: We give a detailed comparison of the hierarchical quantum master equation (HQME) method to a continuous-time quantum Monte Carlo (CT-QMC) approach, assessing the usability of these numerically exact schemes as impurity solvers in practical nonequilibrium calculations. We review the main characteristics of the methods and discuss the scaling of the associated numerical effort. We substantiate our discussion with explicit numerical results for the nonequilibrium transport properties of a single-site Anderson impurity. The numerical effort of the HQME scheme scales linearly with the simulation time but increases (at worst exponentially) with decreasing temperature. In contrast, CT-QMC is less restricted by temperature at short times, but in general the cost of going to longer times is also exponential. After establishing the numerical exactness of the HQME scheme, we use it to elucidate the influence of different ways to induce transport through the impurity on the initial dynamics, discuss the phenomenon of coherent current oscillations, known as current ringing, and explain the nonmonotonic temperature dependence of the steady-state magnetization as a result of competing broadening effects. We also elucidate the pronounced nonlinear magnetization dynamics, which appears on intermediate time scales in the presence of an asymmetric coupling to the electrodes.

Three-terminal quantum-dot refrigerators.

Abstract: Based on two capacitively coupled quantum dots in the Coulomb-blockade regime, a model of three-terminal quantum-dot refrigerators is proposed. With the help of the master equation, the transport properties of steady-state charge current and energy flow between two quantum dots and thermal reservoirs are revealed. It is expounded that such a structure can be used to construct a refrigerator by controlling the voltage bias and temperature ratio. The thermodynamic performance characteristics of the refrigerator are analyzed, including the cooling power, coefficient of performance (COP), maximum cooling power, and maximum COP. Moreover, the optimal regions of main performance parameters are determined. The influence of dissipative tunnel processes on the optimal performance is discussed in detail. Finally, the performance characteristics of the refrigerators operated in two different cases are compared.

Self-gravitating spherically symmetric solutions in scalar-torsion theories

Abstract: We studied spherically symmetric solutions in scalar-torsion gravity theories in which a scalar field is coupled to torsion with a derivative coupling. We obtained the general field equations from which we extracted a decoupled master equation, the solution of which leads to the specification of all other unknown functions. We first obtained an exact solution which represents a new wormhole-like solution dressed with a regular scalar field. Then, we found large distance linearized spherically symmetric solutions in which the space asymptotically is AdS.

Modelling exciton-phonon interactions in optically driven quantum dots

Abstract: We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing, the rates of which depend on the excitation conditions, intrinsic properties of the QD sample, and its temperature. We describe several techniques, which include weak-coupling master equations that are perturbative in the exciton-phonon coupling, as well as those based on the polaron transformation that can remain valid for strong phonon interactions. We additionally consider the role of phonons in altering the optical emission characteristics of quantum dot devices, outlining how we must modify standard quantum optics treatments to account for the presence of the solid-state environment.

Energy transfer in structured and unstructured environments: master equations beyond the Born-Markov approximations

Abstract: We explore excitonic energy transfer dynamics in a molecular dimer system coupled to both structured and unstructured oscillator environments. By extending the reaction coordinate master equation technique developed in [J. Iles-Smith, N. Lambert, and A. Nazir, Phys. Rev. A 90, 032114 (2014)], we go beyond the commonly used Born-Markov approximations to incorporate system-environment correlations and the resultant non-Markovian dynamical effects. We obtain energy transfer dynamics for both underdamped and overdamped oscillator environments that are in perfect agreement with the numerical hierarchical equations of motion over a wide range of parameters. Furthermore, we show that the Zusman equations, which may be obtained in a semiclassical limit of the reaction coordinate model, are often incapable of describing the correct dynamical behaviour. This demonstrates the necessity of properly accounting for quantum correlations generated between the system and its environment when the Born-Markov approximations no longer hold. Finally, we apply the reaction coordinate formalism to the case of a structured environment comprising of both underdamped (i.e. sharply peaked) and overdamped (broad) components simultaneously. We find that though an enhancement of the dimer energy transfer rate can be obtained when compared to an unstructured environment, its magnitude is rather sensitive to both the dimer-peak resonance conditions and the relative strengths of the underdamped and overdamped contributions.

Coherent quantum transport in disordered systems: A unified polaron treatment of hopping and band-like transport

Abstract: Quantum transport in disordered systems is studied using a polaron-based master equation. The polaron approach is capable of bridging the results from the coherent band-like transport regime governed by the Redfield equation to incoherent hopping transport in the classical regime. A non-monotonic dependence of the diffusion coefficient is observed both as a function of temperature and system-phonon coupling strength. In the band-like transport regime, the diffusion coefficient is shown to be linearly proportional to the system-phonon coupling strength and vanishes at zero coupling due to Anderson localization. In the opposite classical hopping regime, we correctly recover the dynamics described by the Fermi’s Golden Rule and establish that the scaling of the diffusion coefficient depends on the phonon bath relaxation time. In both the hopping and band-like transport regimes, it is demonstrated that at low temperature, the zero-point fluctuations of the bath lead to non-zero transport rates and hence a finite diffusion constant. Application to rubrene and other organic semiconductor materials shows a good agreement with experimental mobility data.

Accurate nonadiabatic quantum dynamics on the cheap: Making the most of mean field theory with master equations

Abstract: In this article, we show how Ehrenfest mean field theory can be made both a more accurate and efficient method to treat nonadiabatic quantum dynamics by combining it with the generalized quantum master equation framework. The resulting mean field generalized quantum master equation (MF-GQME) approach is a non-perturbative and non-Markovian theory to treat open quantum systems without any restrictions on the form of the Hamiltonian that it can be applied to. By studying relaxation dynamics in a wide range of dynamical regimes, typical of charge and energy transfer, we show that MF-GQME provides a much higher accuracy than a direct application of mean field theory. In addition, these increases in accuracy are accompanied by computational speed-ups of between one and two orders of magnitude that become larger as the system becomes more nonadiabatic. This combination of quantum-classical theory and master equation techniques thus makes it possible to obtain the accuracy of much more computationally expensive approaches at a cost lower than even mean field dynamics, providing the ability to treat the quantum dynamics of atomistic condensed phase systems for long times.

Quantum coherence in ultrastrong optomechanics

Abstract: Ultrastrong light-matter interaction in an optomechanical system can result in nonlinear optical effects such as photon blockade. The system-bath couplings in such systems play an essential role in observing these effects. Here we study the quantum coherence of an optomechanical system with a dressed-state master equation approach. Our master equation includes photon-number-dependent terms that induce dephasing in this system. Cavity dephasing, second-order photon correlation, and two-cavity entanglement are studied with the dressed-state master equation.

Fluctuating hydrodynamics of multi-species reactive mixtures

Abstract: We formulate and study computationally the fluctuating compressible Navier-Stokes equations for reactive multi-species fluid mixtures. We contrast two different expressions for the covariance of the stochastic chemical production rate in the Langevin formulation of stochastic chemistry, and compare both of them to predictions of the chemical master equation for homogeneous well-mixed systems close to and far from thermodynamic equilibrium. We develop a numerical scheme for inhomogeneous reactive flows, based on our previous methods for non-reactive mixtures [Balakrishnan , Phys. Rev. E 89, 013017 (2014)]. We study the suppression of non-equilibrium long-ranged correlations of concentration fluctuations by chemical reactions, as well as the enhancement of pattern formation by spontaneous fluctuations. Good agreement with available theory demonstrates that the formulation is robust and a useful tool in the study of fluctuations in reactive multi-species fluids. At the same time, several problems with Langevin formulations of stochastic chemistry are identified, suggesting that future work should examine combining Langevin and master equation descriptions of hydrodynamic and chemical fluctuations.

Ancillary qubit spectroscopy of vacua in cavity and circuit quantum electrodynamics.

Abstract: We investigate theoretically how the spectroscopy of an ancillary qubit can probe cavity (circuit) QED ground states containing photons. We consider three classes of systems (Dicke, Tavis-Cummings, and Hopfield-like models), where nontrivial vacua are the result of ultrastrong coupling between $N$ two-level systems and a single-mode bosonic field. An ancillary qubit detuned with respect to the boson frequency is shown to reveal distinct spectral signatures depending on the type of vacua. In particular, the Lamb shift of the ancilla is sensitive to both ground state photon population and correlations. Backaction of the ancilla on the cavity ground state is investigated, taking into account the dissipation via a consistent master equation for the ultrastrong coupling regime. The conditions for high-fidelity measurements are determined.