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Open AccessJournal ArticleDOI

Toward All Room-Temperature, Solution-Processed, High-Performance Planar Perovskite Solar Cells: A New Scheme of Pyridine-Promoted Perovskite Formation

TLDR
A new, all room-temperature solution process is developed to fabricate efficient, low-cost, and stable perovskite solar cells (PVSCs) that show high efficiency and no hysteresis on rigid and flexible substrates, respectively.
Abstract
A new, all room-temperature solution process is developed to fabricate efficient, low-cost, and stable perovskite solar cells (PVSCs). The PVSCs show high efficiency of 17.10% and 14.19%, with no hysteresis on rigid and flexible substrates, respectively, which are the best efficiencies reported to date for PVSCs fabricated by room-temperature solution-processed techniques. The flexible PVSCs show a remarkable power-per-weight of 23.26 W g-1 .

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Citations
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Journal ArticleDOI

Scalable fabrication of perovskite solar cells

TL;DR: In this paper, the authors review recent progress and challenges in scaling up perovskite solar cells and related efforts to enable the terawatt-scale manufacturing and deployment of this PV technology.
Journal ArticleDOI

Regulating strain in perovskite thin films through charge-transport layers

TL;DR: By using a thermal expandable hole transporting layer to compensate the strain and result in most stable wide-bandgap perovskite solar cells so far, Xue et al. find that compressive strain increases the activation energy for ion migration, improving the stability of perovSKite films.
Journal ArticleDOI

Understanding of perovskite crystal growth and film formation in scalable deposition processes

TL;DR: This review, comprising the mechanistic analysis of perovskite film formation, thin film engineering, scalable deposition technologies and device stability, provides a comprehensive overview of the current challenges and opportunities in the field of PSCs, aiming to promote the future development of cost-effective up-scale fabrication of highly efficient and ultra-stable P SCs for practical applications.
References
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Journal ArticleDOI

Generalized Gradient Approximation Made Simple

TL;DR: A simple derivation of a simple GGA is presented, in which all parameters (other than those in LSD) are fundamental constants, and only general features of the detailed construction underlying the Perdew-Wang 1991 (PW91) GGA are invoked.
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Projector augmented-wave method

TL;DR: An approach for electronic structure calculations is described that generalizes both the pseudopotential method and the linear augmented-plane-wave (LAPW) method in a natural way and can be used to treat first-row and transition-metal elements with affordable effort and provides access to the full wave function.
Journal ArticleDOI

From ultrasoft pseudopotentials to the projector augmented-wave method

TL;DR: In this paper, the formal relationship between US Vanderbilt-type pseudopotentials and Blochl's projector augmented wave (PAW) method is derived and the Hamilton operator, the forces, and the stress tensor are derived for this modified PAW functional.
Journal ArticleDOI

Sequential deposition as a route to high-performance perovskite-sensitized solar cells

TL;DR: A sequential deposition method for the formation of the perovskite pigment within the porous metal oxide film that greatly increases the reproducibility of their performance and allows the fabrication of solid-state mesoscopic solar cells with unprecedented power conversion efficiencies and high stability.
Journal ArticleDOI

Efficient planar heterojunction perovskite solar cells by vapour deposition

TL;DR: It is shown that perovskite absorbers can function at the highest efficiencies in simplified device architectures, without the need for complex nanostructures.
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