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Showing papers on "Femtosecond pulse shaping published in 2008"


Journal ArticleDOI
Seungchul Kim1, Jonghan Jin1, Young-Jin Kim1, In-Yong Park1, Yunseok Kim1, Seung-Woo Kim1 
05 Jun 2008-Nature
TL;DR: This work demonstrates a method of high-harmonic generation that requires no extra cavities by exploiting the local field enhancement induced by resonant plasmons within a metallic nanostructure consisting of bow-tie-shaped gold elements on a sapphire substrate.
Abstract: High-harmonic generation by focusing a femtosecond laser onto a gas is a well-known method of producing coherent extreme-ultraviolet (EUV) light. This nonlinear conversion process requires high pulse intensities, greater than 10(13) W cm(-2), which are not directly attainable using only the output power of a femtosecond oscillator. Chirped-pulse amplification enables the pulse intensity to exceed this threshold by incorporating several regenerative and/or multi-pass amplifier cavities in tandem. Intracavity pulse amplification (designed not to reduce the pulse repetition rate) also requires a long cavity. Here we demonstrate a method of high-harmonic generation that requires no extra cavities. This is achieved by exploiting the local field enhancement induced by resonant plasmons within a metallic nanostructure consisting of bow-tie-shaped gold elements on a sapphire substrate. In our experiment, the output beam emitted from a modest femtosecond oscillator (100-kW peak power, 1.3-nJ pulse energy and 10-fs pulse duration) is directly focused onto the nanostructure with a pulse intensity of only 10(11) W cm(-2). The enhancement factor exceeds 20 dB, which is sufficient to produce EUV wavelengths down to 47 nm by injection with an argon gas jet. The method could form the basis for constructing laptop-sized EUV light sources for advanced lithography and high-resolution imaging applications.

1,320 citations


Journal ArticleDOI
TL;DR: In this article, the principles and most recent results of high-power THz generation through optical rectification using a tilted optical pulse front are described and applications in nonlinear THz spectroscopy and THz coherent control are discussed.
Abstract: The principles and most-recent results of high-power THz generation through optical rectification using a tilted optical pulse front are described. Single-cycle THz pulses of multimicrojoule energies are generated at kHz repetition rates, and average THz power levels exceeding 1 mW can be generated at kHz-MHz repetition rates. Applications in nonlinear THz spectroscopy and THz coherent control are discussed.

516 citations


Journal ArticleDOI
TL;DR: In this paper, the nonlinear phase shift accumulated by the pulse, spectral filter bandwidth, and group-velocity dispersion are identified as the key parameters that determine the behavior and properties of all-normal-dispersion mode-locked fiber lasers.
Abstract: We report a systematic study of all-normal-dispersion mode-locked fiber lasers. Spectral filtering of a chirped pulse in the cavity is a major component of the pulse shaping in these lasers. We identify the nonlinear phase shift accumulated by the pulse, spectral filter bandwidth, and group-velocity dispersion as the key parameters that determine the behavior and properties of these lasers. Trends in the performance as these parameters are varied are summarized. A wide range of pulse shapes and evolutions can occur. Experimental results from Yb-doped all-normal-dispersion fiber lasers agree reasonably well with the results of numerical simulations.

374 citations


Journal ArticleDOI
TL;DR: In this paper, the authors discuss the control of high-harmonic spectra by temporal and spatial pulse shaping of the driving laser pulses and its implications on time-resolved XUV spectroscopy and attosecond pulse shaping.
Abstract: High-harmonic generation provides an attractive light source of coherent radiation in the extreme-ultraviolet (XUV) and soft-x-ray regions of the spectrum and allows for the production of single attosecond pulses or pulse trains. This Colloquium covers the control of high-harmonic spectra by temporal and spatial pulse shaping of the driving laser pulses and its implications on time-resolved XUV spectroscopy and attosecond pulse shaping. It summarizes important steps for extending existing pulse shaping techniques and control schemes from the near-infrared or visible part to shorter wavelengths. Using adaptive pulse shaping of the driving laser pulses, several groups have demonstrated control of the high-harmonic spectrum, including the author's work on the complete control over the XUV spectrum of high-order harmonics, generated in a gas-filled hollow fiber. It is possible to achieve both the enhancement and the suppression of single or several selected harmonic orders. These arbitrarily shaped soft-x-ray spectra will allow for important modifications of the resulting harmonic pulses in the temporal domain. This constitutes first steps towards direct attosecond pulse shaping in the soft-x-ray domain. Moreover, high-harmonic generation in a hollow-core fiber can be enhanced by coupling into a single fiber mode using a feedback-controlled adaptive two-dimensional spatial light modulator.

310 citations


Journal ArticleDOI
TL;DR: This paper reports on the results of research into passively modelocked fiber laser with a record-setting optical length of the resonant cavity amounting to 3.8 km, which is the highest pulse energy on record generated directly from a mode-locked laser without Q-switching, cavity dumping techniques, or additional optical amplifiers.
Abstract: This paper reports on the results of research into passively mode-locked fiber laser with a record-setting optical length of the resonant cavity amounting to 3.8 km. Significant elongation of the laser resonator led to more than two orders of magnitude increase in the output pulse energy at the same pump radiation power. At ultra-low (for mode-locked lasers) pulse repetition rate (77 kHz) and pulse duration of 3 ns the energy per pulse reached 3.9 µJ. At this moment this is the highest pulse energy on record generated directly from a mode-locked laser without Q-switching, cavity dumping techniques, or additional optical amplifiers.

217 citations


Journal ArticleDOI
TL;DR: In this article, the theory of the transition-Cherenkov process was studied in detail and compared with recent experimental results for several gases, including CO 2, CO 2 and CO 2.
Abstract: A transition-Cherenkov electromagnetic emission by a femtosecond laser pulse propagating in a self-induced plasma channel in air has been very recently proposed as mechanism for production of terahertz (THz) radiation in the forward direction. In this paper, we study in detail the theory of the transition-Cherenkov process. The theoretical model is developed and compared with recent experimental results for several gases.

181 citations


Journal ArticleDOI
TL;DR: The Yb-doped fiber laser includes a fiber filter, and a saturable absorber based on carbon nanotubes, and generates 1.5-ps, 3-nJ pulses that can be dechirped to 250 fs duration outside the cavity.
Abstract: Spectral filtering of a chirped pulse can be a strong pulse-shaping mechanism in all-normal-dispersion femtosecond fiber lasers. We report an implementation of such a laser that employs only fiber-format components. The Yb-doped fiber laser includes a fiber filter, and a saturable absorber based on carbon nanotubes. The laser generates 1.5-ps, 3-nJ pulses that can be dechirped to 250 fs duration outside the cavity.

167 citations


Journal ArticleDOI
TL;DR: For the first time, femtosecond pulses from a passive single-section InAs/InP quantum-dot (QD) mode-locked laser (MLL) with the active length of 456 microm and ridge width of 2.5 microm are reported.
Abstract: For the first time, we report femtosecond pulses from a passive single-section InAs/InP quantum-dot (QD) mode-locked laser (MLL) with the active length of 456 microm and ridge width of 2.5 microm at the C-band wavelength range. Without any external pulse compression, the transform-limited Gaussian-pulses are generated at the 92 GHz repetition rate with the 312 fs pulse duration, which is the shortest pulse from any directly electric-pumping semiconductor MLLs to our best knowledge. The lasing threshold injection current and external differential quantum efficiency are 17.2 mA and 38%, respectively. We have also investigated the working principles of the proposed QD MLLs.

134 citations


Journal ArticleDOI
TL;DR: The generation of high energy subpicosecond pulses with a pulse energy of up to 25.9 microJ at a pulse duration of 928 fs directly from a thin-disk laser oscillator with active multipass cell is demonstrated.
Abstract: The pulse shaping dynamics of a diode-pumped laser oscillator with active multipass cell was studied experimentally and numerically. We demonstrate the generation of high energy subpicosecond pulses with a pulse energy of up to 25.9µJ at a pulse duration of 928fs directly from a thin-disk laser oscillator. These results are achieved by employing a selfimaging active multipass geometry operated in ambient atmosphere. Stable single pulse operation has been obtained with an average output power in excess of 76W and at a repetition rate of 2.93MHz. Self starting passive mode locking was accomplished using a semiconductor saturable absorber mirror. The experimental results are compared with numerical simulations, showing good agreement including the appearance of Kelly sidebands. Furthermore, a modified soliton-area theorem for approximating the pulse duration is presented.

131 citations


Journal ArticleDOI
TL;DR: This paper reports two advances in a slow light device consisting of chirped photonic crystal slab coupled waveguide on SOI substrate, indicating the delay-bandwidth product and proposes a technique for externally controlling the chirping to permit variable delay.
Abstract: This paper reports two advances in a slow light device consisting of chirped photonic crystal slab coupled waveguide on SOI substrate. One is concerning the delay-bandwidth product, indicating the buffering capacity of the device. We experimentally evaluated a record high value of 57 (a 40 ps delay and a 1.4 THz bandwidth). We also observed ~1 ps wide optical pulse transmission in the cross-correlation measurement. Regarding the pulse as a signal and considering the broadening of the pulse width due to the imperfect dispersion compensation in the device, storage of more than 12 signal bits was confirmed. The other is a wide-range tuning of the pulse delay. We propose a technique for externally controlling the chirping to permit variable delay. We demonstrate tuning of the pulse delay up to 23 ps, corresponding to a ~7 mm extension of the free space length.

129 citations


01 Jan 2008
TL;DR: In this paper, a novel approach to optically generate chirped millimeter-wave pulses with tunable chirp rate based on spectral shaping and nonlinear frequency-to-time mapping is proposed and experimentally demonstrated.
Abstract: A novel approach to optically generating chirped millimeter-wave pulses with tunable chirp rate based on spectral shaping and nonlinear frequency-to-time mapping is proposed and experimentally demonstrated. In the proposed approach, the optical power spectrum of an ultrashort pulse from a fem- tosecond pulsed laser is shaped by a two-tap Sagnac loop filter that has a sinusoidal frequency response. The spectrum-shaped optical pulse is then sent to a nonlinearly chirped fiber Bragg grating (NL-CFBG) with a tunable nonlinear group delay to serve as a high-order dispersive device to perform the nonlinear frequency-to-time mapping. A chirped electrical pulse with a high central frequency and large chirp rate is then generated at the output of a high-speed photodetector. The NL-CFBG used in the proposed system is produced from a regular linearly chirped fiber Bragg grating based on strain-gradient beam tuning. A detailed theoretical analysis on the chirped pulse generation is developed, which is verified by numerical simulations and experi- ments. Millimeter-wave pulses with a central frequency of around 35 GHz and instantaneous frequency chirp rates of 0.053 and 0.074 GHz/ps are experimentally generated. Index Terms—Chirped pulse generation, chromatic dispersion, frequency-to-time mapping, microwave photonics, nonlinearly chirped fiber Bragg grating (NL-CFBG), pulse compression, radar.

Journal ArticleDOI
TL;DR: In this paper, a low-repetition-rate oscillator that generates pulses with large and linear chirp can replace the standard oscillator, stretcher, pulse-picker, and preamplifier in a chirped-pulse fiber amplifier.
Abstract: A new regime of pulse parameters in a normal-dispersion fiber laser is identified. Dissipative solitons exist with remarkably large pulse duration and chirp, along with large pulse energy. A low-repetition-rate oscillator that generates pulses with large and linear chirp can replace the standard oscillator, stretcher, pulse-picker, and preamplifier in a chirped-pulse fiber amplifier. The theoretical properties of such a giant-chirp oscillator are presented. A fiber laser designed to operate in the new regime generates ~150 ps pulses at a 3 MHz repetition rate. Amplification of these pulses to 1 μJ energy with pulse duration as short as 670 fs demonstrates the promise of this new approach.

Journal ArticleDOI
TL;DR: In this paper, a novel approach to optically generating chirped millimeter-wave pulses with tunable chirp rate based on spectral shaping and nonlinear frequency-to-time mapping is proposed and experimentally demonstrated.
Abstract: A novel approach to optically generating chirped millimeter-wave pulses with tunable chirp rate based on spectral shaping and nonlinear frequency-to-time mapping is proposed and experimentally demonstrated. In the proposed approach, the optical power spectrum of an ultrashort pulse from a femtosecond pulsed laser is shaped by a two-tap Sagnac loop filter that has a sinusoidal frequency response. The spectrum-shaped optical pulse is then sent to a nonlinearly chirped fiber Bragg grating (NL-CFBG) with a tunable nonlinear group delay to serve as a high-order dispersive device to perform the nonlinear frequency-to-time mapping. A chirped electrical pulse with a high central frequency and large chirp rate is then generated at the output of a high-speed photodetector. The NL-CFBG used in the proposed system is produced from a regular linearly chirped fiber Bragg grating based on strain-gradient beam tuning. A detailed theoretical analysis on the chirped pulse generation is developed, which is verified by numerical simulations and experiments. Millimeter-wave pulses with a central frequency of around 35 GHz and instantaneous frequency chirp rates of 0.053 and 0.074 GHz/ps are experimentally generated.

Journal ArticleDOI
TL;DR: In this paper, a novel approach to generating linearly chirped microwave pulses in the optical domain based on spectral shaping and linear frequency-to-time mapping is proposed and experimentally demonstrated.
Abstract: A novel approach to generating linearly chirped microwave pulses in the optical domain based on spectral shaping and linear frequency-to-time mapping is proposed and experimentally demonstrated. In the proposed system, the spectrum of a femtosecond pulse generated by a mode-locked fiber laser is spectrum-shaped by an optical filter that consists of two superimposed chirped fiber Bragg gratings (SI-CFBGs) with different chirp rates. The SI-CFBGs form a Fabry-Perot cavity with a cavity length linearly dependent on the resonance wavelength, thus a spectral response with an increased or decreased free spectral range is generated. A chirped microwave pulse with the pulse shape identical to the shaped spectrum is obtained at the output of a high-speed photodetector thanks to the frequency-to-time mapping in a dispersive device. The proposed technique is experimentally demonstrated, a linearly chirped microwave pulse with a central frequency of 15 GHz and a chirp rate of 0.0217 GHz/ps is experimentally generated.

Journal ArticleDOI
TL;DR: Using an intensity grating to enhance the pondermotive force is able to fully characterize electron pulses and to confirm many body simulations with laser pulse energies on the microjoule level, solving one of the last barriers to the highest possible time resolution for electron probes.
Abstract: Real time views of atomic motion can be achieved using electron pulses as structural probes. The requisite time resolution requires knowledge of both the electron pulse duration and the exact timing of the excitation pulse and the electron probe to within 10 - 100 fs accuracy. By using an intensity grating to enhance the pondermotive force, we are now able to fully characterize electron pulses and to confirm many body simulations with laser pulse energies on the microjoule level. This development solves one of the last barriers to the highest possible time resolution for electron probes.

Journal ArticleDOI
TL;DR: A femtosecond fiber laser based on thulium-doped double-clad silica fiber with an internal dispersion compensation is presented that generates pulses at a center wavelength of 1976 nm with an energy of 4.3 nJ and a duration of 1.2 ps.
Abstract: A femtosecond fiber laser based on thulium-doped double-clad silica fiber with an internal dispersion compensation is presented that generates pulses at a center wavelength of 1976 nm with an energy of 4.3 nJ and a duration of 1.2 ps. The dechirped pulse duration is 294 fs. The pulse energy is more than 2 orders of magnitude above the pulse energy demonstrated previously. Mode locking is achieved using additive pulse mode locking, and dispersion compensation is facilitated by a grating stretcher arrangement.

Journal ArticleDOI
TL;DR: In this paper, an optimized imaging setup is proposed for the creation of the tilted pulse front inside the LiNbO3 crystal, where there is no principal limitation on the pump spot size and hence on the terahertz energy.
Abstract: Recently, the generation of near-single-cycle terahertz pulses with 10μJ energy was demonstrated by optical rectification of ultrashort laser pulses with tilted pulse front in LiNbO3. Here, an optimized imaging setup is proposed for the creation of the tilted pulse front inside the LiNbO3 crystal. Furthermore, a compact setup is proposed which creates the tilted pulse front without imaging, where there is no principal limitation on the pump spot size and, hence, on the terahertz energy. According to model calculations, application of these setups can increase the efficiency by one order of magnitude for 5mm spot size.

Journal ArticleDOI
TL;DR: This paper deals with the pulse-shaping properties of birefringent filters that feature an optical layout similar to a Solc fan filter and finds that this filter is particularly well suited for generation of flattop pulses featuring a 20-ps-long plateau and rising and falling edges shorter than 2 ps.
Abstract: This paper deals with the pulse-shaping properties of birefringent filters that feature an optical layout similar to a Solc fan filter. A simple computational model is given that explains the pulse-shaping process in the fan filter in two steps: First, the input pulse is split into several mutually delayed replicas due to the birefringence of the crystals. Second, these replicas interfere at the output polarizer of the filter and form the shaped output pulse. Fine-tuning of the phases of the replicas of the input pulse is permitted by tuning the temperature of the crystals. A birefringent pulse shaper containing ten birefringent crystals was investigated experimentally. The shape of the output pulses was measured by means of a special cross-correlation technique. Although a variety of pulse shapes can be generated with the described filter, it is particularly well suited for generation of flattop pulses featuring a 20-ps-long plateau and rising and falling edges shorter than 2 ps.

Journal ArticleDOI
TL;DR: This work introduces an inherently phase-stable setup for coherent two-dimensional femtosecond spectroscopy in noncollinear box geometry using only conventional beam splitters, mirrors, and delay stages.
Abstract: We introduce an inherently phase-stable setup for coherent two-dimensional femtosecond spectroscopy in noncollinear box geometry using only conventional beam splitters, mirrors, and delay stages. Avoiding diffractive optics, pulse shapers, and active phase-locking loops, our spectroscopy setup is simple, robust, and works for ultrabroad bandwidths in all spectral regimes (infrared, visible, and ultraviolet).

Journal ArticleDOI
TL;DR: An optical parametric chirpedpulse amplifier at a 1-kHz repetition rate with a 5.5-fs pulse duration, a 2.7-mJ pulse energy and carrier-envelope phase-control is reported on.
Abstract: We report on the development of an optical parametric chirped-pulse amplifier at a 1-kHz repetition rate with a 5.5-fs pulse duration, a 2.7-mJ pulse energy and carrier-envelope phase-control. The amplifier is pumped by a 450-nm pulse from a frequency-doubled Ti:sapphire laser.

Journal ArticleDOI
TL;DR: In this article, the authors demonstrate that a pulse shaper is able to simultaneously act as an optical waveform generator and a short pulse characterization device when combined with an appropriate nonlinear element and show that control over the carrier envelope phase allows continuous tuning between an intensity-like and an interferometric autocorrelation.
Abstract: We demonstrate that a pulse shaper is able to simultaneously act as an optical waveform generator and a short pulse characterization device when combined with an appropriate nonlinear element. We present autocorrelation measurements and their frequency resolved counterparts. We show that control over the carrier envelope phase allows continuous tuning between an intensity-like and an interferometric autocorrelation. By changing the transfer function other measurement techniques, for example STRUT, are easily realized without any modification of the optical setup.

Journal ArticleDOI
TL;DR: In this paper, a soliton light pulse with wavelength of 1550 nm is entered into the multistage microring resonators, where the ring radii of the recent integrated device product are within the range from 5 to 10 microns.
Abstract: We propose a new system of an attosecond pulse generation by using the integrated nonlinear microring devices. A soliton light pulse with wavelength of 1550 nm is entered into the multistage microring resonators, where the ring radii of the recent integrated device product are within the range from 5 to 10 microns. Results obtained have shown that the ultrashort pulse width in the attoscale regime and beyond can be easily generated. When the input peak power of 12 W is applied into the system, the generated pulse with pulse width of 50 is achieved. © 2008 Wiley Periodicals, Inc. Microwave Opt Technol Lett 50: 3108–3111, 2008; Published online in Wiley InterScience (www.interscience.wiley.com). DOI 10.1002/mop.23888

Journal ArticleDOI
TL;DR: In this paper, a novel approach to characterize the parabolically-shaped pulses that can be generated from more conventional pulses via nonlinear propagation in cascaded sections of commercially available normally dispersive (ND) fibers was proposed.
Abstract: We propose a novel approach to characterize the parabolically-shaped pulses that can be generated from more conventional pulses via nonlinear propagation in cascaded sections of commercially available normally dispersive (ND) fibers. The impact of the initial pulse chirp on the passive pulse reshaping is examined. We furthermore demonstrate that the combination of pulse pre-chirping and propagation in a single ND fiber yields a simple, passive method for generating various temporal waveforms of practical interest.

Journal ArticleDOI
TL;DR: The successful operation of an analogue computer designed to factor numbers is reported on, which relies solely on the interference of classical light and brings together the field of ultrashort laser pulses with number theory.
Abstract: We report on the successful operation of an analogue computer designed to factor numbers. Our device relies solely on the interference of classical light and brings together the field of ultrashort laser pulses with number theory. Indeed, the frequency component of the electric field corresponding to a sequence of appropriately shaped femtosecond pulses is determined by a Gauss sum which allows us to find the factors of a number.

Journal ArticleDOI
TL;DR: In this article, a study of collinear geometry double-pulse femtosecond LIBS analysis of solids in ambient environment is presented, where the influence of the delay between pulses in the LIBS signal intensity was investigated and two intervals of interaction were established.

Journal ArticleDOI
TL;DR: In this paper, it is shown that during the propagation of intense femtosecond laser pulses in a transparent medium, pulse shortening can occur without external guiding, and a description of its physical origin is given.
Abstract: During the propagation of intense femtosecond laser pulses in a transparent medium, pulse shortening can occur without external guiding Experimental evidence for this effect and a description of its physical origin are presented Nearly single cycle pulses at 800 nm with an energy of 0120 mJ can be obtained with excellent beam quality Carrier envelope offset phase (CEP) stability is conserved or even improved after the nonlinear propagation stage Prospects for further improvement are discussed

Journal ArticleDOI
TL;DR: An octave-spanning Ti:sapphire oscillator supporting Fourier-limited pulses as short as 3.7 fs is presented, allowing for full control of the electric pulse field on a sub-femtosecond time-scale.
Abstract: We present an octave-spanning Ti:sapphire oscillator supporting Fourier-limited pulses as short as 3.7 fs. This laser system can be directly CEO-phase stabilized delivering an average output power of about 90 mW with a pulse duration of 4.4 fs. The phase-stabilization is realized without additional spectral broadening using an f-2f interferometer approach allowing for full control of the electric pulse field on a sub-femtosecond time-scale.

Journal ArticleDOI
TL;DR: In this article, two models are studied to describe the laser pulse interaction with nanoparticles in the femtosecond, picosecond and nanosecond regimes, and a comparison of the two modeling strategies shows that the two-temperature model gives a good approximation for the fem-time mode, but fails to accurately describe the longer pulses.
Abstract: The interaction between nanoparticles and ultrashort laser pulses holds great interest in laser nanomedicine, introducing such possibilities as selective cell targeting to create highly localized cell damage. Two models are studied to describe the laser pulse interaction with nanoparticles in the femtosecond, picosecond, and nanosecond regimes. The first is a two-temperature model using two coupled diffusion equations: one describing the heat conduction of electrons, and the other that of the lattice. The second model is a one-temperature model utilizing a heat diffusion equation for the phonon subsystem and applying a uniform heating approximation throughout the particle volume. A comparison of the two modeling strategies shows that the two-temperature model gives a good approximation for the femtosecond mode, but fails to accurately describe the laser heating for longer pulses. On the contrary, the simpler one-temperature model provides an adequate description of the laser heating of nanoparticles in the femtosecond, picosecond, and nanosecond modes.

Journal ArticleDOI
TL;DR: The description of ultrashort laser pulse filamentation in condensed media as a spontaneous formation of X waves is shown to apply also to filaments generated in air.
Abstract: The description of ultrashort laser pulse filamentation in condensed media as a spontaneous formation of X waves is shown to apply also to filaments generated in air. Within this framework, a simple explanation is brought for several features of the filament such as the subdiffractive propagation and the energy flux from the weakly localized tails of the X-waves to the intense core.

Journal Article
TL;DR: In this paper, a numerical approach that allows for the solution of the time-dependent Schr\\\"odinger equation (TDSE) describing molecules exposed to intense short laser pulses was developed.
Abstract: A numerical approach that allows for the solution of the time-dependent Schr\\\"odinger equation (TDSE) describing molecules exposed to intense short laser pulses was developed. The molecular response to the strong field is described within the single-active electron approximation (SAE). The method is applied in the fixed-nuclei approximation to molecular hydrogen with parallel orientation of the internuclear axis to the laser field. The validity of the SAE is investigated by comparing the ionization and electronic excitation yields to full two-electron solutions of the TDSE. The present results are also used to investigate the validity of approximate SAE methods like the molecular Ammosov-Delone-Krainov and the strong-field approximation.