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Showing papers on "Terahertz radiation published in 2016"


Journal ArticleDOI
TL;DR: In this article, a W/CoFeB/Pt trilayer was used to generate a 1.30 THz range of trilayers from photo-induced spin currents, the inverse spin Hall effect and a broadband Fabry-Perot resonance.
Abstract: Ultrashort pulses covering the 1–30 THz range are generated from a W/CoFeB/Pt trilayer and originate from photoinduced spin currents, the inverse spin Hall effect and a broadband Fabry–Perot resonance. The resultant peak fields are several 100 kV cm–1.

582 citations


Journal ArticleDOI
TL;DR: The ability of the anisotropic coding metasurfaces to generate a beam splitter and realize simultaneous anomalous reflections and polarization conversions, thus providing powerful control of differently polarized electromagnetic waves is demonstrated.
Abstract: Metamaterials based on effective media can be used to produce a number of unusual physical properties (for example, negative refraction and invisibility cloaking) because they can be tailored with effective medium parameters that do not occur in nature. Recently, the use of coding metamaterials has been suggested for the control of electromagnetic waves through the design of coding sequences using digital elements ‘0’ and ‘1,' which possess opposite phase responses. Here we propose the concept of an anisotropic coding metamaterial in which the coding behaviors in different directions are dependent on the polarization status of the electromagnetic waves. We experimentally demonstrate an ultrathin and flexible polarization-controlled anisotropic coding metasurface that functions in the terahertz regime using specially designed coding elements. By encoding the elements with elaborately designed coding sequences (both 1-bit and 2-bit sequences), the x- and y-polarized waves can be anomalously reflected or independently diffused in three dimensions. The simulated far-field scattering patterns and near-field distributions are presented to illustrate the dual-functional performance of the encoded metasurface, and the results are consistent with the measured results. We further demonstrate the ability of the anisotropic coding metasurfaces to generate a beam splitter and realize simultaneous anomalous reflections and polarization conversions, thus providing powerful control of differently polarized electromagnetic waves. The proposed method enables versatile beam behaviors under orthogonal polarizations using a single metasurface and has the potential for use in the development of interesting terahertz devices. An artificial material that controls electromagnetic waves of different polarization independently has been demonstrated by a team in China. Tie Jun Cui from the Southeast University and co-workers have created a metamaterial that can, for example, split incoming unpolarized radiation so that horizontally polarized light goes one way while vertically polarized light goes the other. Metamaterials are structures that can be engineered to have optical properties not found in natural materials, and they consist of a repeated pattern of elements that are smaller than the wavelength of light. The researchers used two types of element, simple squares and dumbbells, which enabled them to independently control beams of long-wavelength radiation known as terahertz waves having differing polarizations. By reducing the size of the metamaterial elements, the same idea could also be applied to visible light.

382 citations


Journal ArticleDOI
10 Nov 2016-Nature
TL;DR: It is anticipated that the combination of lightwave electronics and the atomic resolution of the approach will open the door to visualizing ultrafast photochemistry and the operation of molecular electronics on the single-orbital scale.
Abstract: Watching a single molecule move on its intrinsic timescale has been one of the central goals of modern nanoscience, and calls for measurements that combine ultrafast temporal resolution with atomic spatial resolution. Steady-state experiments access the requisite spatial scales, as illustrated by direct imaging of individual molecular orbitals using scanning tunnelling microscopy or the acquisition of tip-enhanced Raman and luminescence spectra with sub-molecular resolution. But tracking the intrinsic dynamics of a single molecule directly in the time domain faces the challenge that interactions with the molecule must be confined to a femtosecond time window. For individual nanoparticles, such ultrafast temporal confinement has been demonstrated by combining scanning tunnelling microscopy with so-called lightwave electronics, which uses the oscillating carrier wave of tailored light pulses to directly manipulate electronic motion on timescales faster even than a single cycle of light. Here we build on ultrafast terahertz scanning tunnelling microscopy to access a state-selective tunnelling regime, where the peak of a terahertz electric-field waveform transiently opens an otherwise forbidden tunnelling channel through a single molecular state. It thereby removes a single electron from an individual pentacene molecule's highest occupied molecular orbital within a time window shorter than one oscillation cycle of the terahertz wave. We exploit this effect to record approximately 100-femtosecond snapshot images of the orbital structure with sub-angstrom spatial resolution, and to reveal, through pump/probe measurements, coherent molecular vibrations at terahertz frequencies directly in the time domain. We anticipate that the combination of lightwave electronics and the atomic resolution of our approach will open the door to visualizing ultrafast photochemistry and the operation of molecular electronics on the single-orbital scale.

361 citations


Journal ArticleDOI
TL;DR: Noninvasive, near-field THz imaging with subwavelength resolution and the inherent sensitivity to local conductivity is demonstrated, making it possible to detect fissures in the circuitry wiring of a few micrometers in size.
Abstract: Terahertz (THz) imaging can see through otherwise opaque materials. However, because of the long wavelengths of THz radiation (λ = 400 μm at 0.75 THz), far-field THz imaging techniques suffer from low resolution compared to visible wavelengths. We demonstrate noninvasive, near-field THz imaging with subwavelength resolution. We project a time-varying, intense (>100 μJ/cm2) optical pattern onto a silicon wafer, which spatially modulates the transmission of synchronous pulse of THz radiation. An unknown object is placed on the hidden side of the silicon, and the far-field THz transmission corresponding to each mask is recorded by a single-element detector. Knowledge of the patterns and of the corresponding detector signal are combined to give an image of the object. Using this technique, we image a printed circuit board on the underside of a 115-μm-thick silicon wafer with ~100-μm (λ/4) resolution. With subwavelength resolution and the inherent sensitivity to local conductivity, it is possible to detect fissures in the circuitry wiring of a few micrometers in size. THz imaging systems of this type will have other uses too, where noninvasive measurement or imaging of concealed structures is necessary, such as in semiconductor manufacturing or in ex vivo bioimaging.

342 citations


Journal ArticleDOI
TL;DR: A dual-band perfect absorber, composed of a periodically patterned elliptical nanodisk graphene structure and a metal ground plane spaced by a thin SiO(2) dielectric layer, is proposed and investigated.
Abstract: In this paper, a dual-band perfect absorber, composed of a periodically patterned elliptical nanodisk graphene structure and a metal ground plane spaced by a thin SiO(2) dielectric layer, is proposed and investigated. Numerical results reveal that the absorption spectrum of the graphene-based structure displays two perfect absorption peaks in the terahertz band, corresponding to the absorption value of 99% at 35μm and 97%at 59μm, respectively. And the resonance frequency of the absorber can be tunned by controlling the Fermi level of graphene layer. Further more, it is insensitive to the polarization and remains very high over a wide angular range of incidence around ±60(0). Compared with the previous graphene dual-band perfect absorption, our absorber only has one shape which can greatly simplify the manufacturing process.

298 citations


Journal ArticleDOI
22 Apr 2016-Science
TL;DR: An ultrafast optics approach for generating bunches of electrons and compressing them by more than an order of magnitude to just femtosecond time scales is described, opening up the possibility of imaging ultrafast phenomena with atomic-scale spatial resolution.
Abstract: Short electron pulses are central to time-resolved atomic-scale diffraction and electron microscopy, streak cameras, and free-electron lasers. We demonstrate phase-space control and characterization of 5-picometer electron pulses using few-cycle terahertz radiation, extending concepts of microwave electron pulse compression and streaking to terahertz frequencies. Optical-field control of electron pulses provides synchronism to laser pulses and offers a temporal resolution that is ultimately limited by the rise-time of the optical fields applied. We used few-cycle waveforms carried at 0.3 terahertz to compress electron pulses by a factor of 12 with a timing stability of <4 femtoseconds (root mean square) and measure them by means of field-induced beam deflection (streaking). Scaling the concept toward multiterahertz control fields holds promise for approaching the electronic time scale in time-resolved electron diffraction and microscopy.

291 citations


Journal ArticleDOI
TL;DR: In this paper, the authors present a review of the development and application of intense terahertz (THz) sources, including photoconductive antennas (PCAs), optical rectification sources (ORS), DAST sources and relativistic laser-plasma sources.
Abstract: In this paper, we will review both past and recent progresses in the generation, detection and application of intense terahertz (THz) radiation. We will restrict the review to laser based intense few-cycle THz sources, and thus will not include sources such as synchrotron-based or narrowband sources. We will first review the various methods used for generating intense THz radiation, including photoconductive antennas (PCAs), optical rectification sources (especially the tilted-pulse-front lithium niobate source and the DAST source, but also those using other crystals), air plasma THz sources and relativistic laser–plasma sources. Next, we will give a brief introduction on the common methods for coherent THz detection techniques (namely the PCA technique and the electro-optic sampling), and point out the limitations of these techniques for measuring intense THz radiation. We will then review three techniques that are highly suited for detecting intense THz radiation, namely the air breakdown coherent detection technique, various single-shot THz detection techniques, and the spectral-domain interferometry technique. Finally, we will give an overview of the various applications that have been made possible with such intense THz sources, including nonlinear THz spectroscopy of condensed matter (optical-pump/THz-probe, THz-pump/THz-probe, THz-pump/optical-probe), nonlinear THz optics, resonant and non-resonant control of material (such as switching of superconductivity, magnetic and polarization switching) and controlling the nonlinear response of metamaterials. We will also provide a short perspective on the future of intense THz sources and their applications.

281 citations


Journal ArticleDOI
20 Oct 2016-Nature
TL;DR: Direct probing, confinement and control of the waveform of intraband currents inside solids on attosecond timescales establish a method of realizing multi-petahertz coherent electronics and is expected to enable new ways of exploring the interplay between electron dynamics and the structure of condensed matter on the atomic scale.
Abstract: Investigations using single-cycle intense optical fields to drive electron motion in bulk silicon dioxide show that the light-induced electric currents extend in frequency up to about 8 petahertz. The speed of electronics, and hence of computing, is limited by the frequencies of the electric currents that are used. Light fields can induce and manipulate electric currents at vastly higher frequencies than are achievable in conventional devices, and Eleftherios Goulielmakis and colleagues now extend this approach to reach an even faster regime. They use single-cycle intense optical fields to drive electron motion in the bulk of silicon dioxide and show that the light-induced intraband electric currents extend in frequency up to about eight petahertz. This demonstration of real-time access to the dynamic nonlinear conductivity of silicon dioxide, with the ability to directly probe and control the intraband currents on attosecond timescales, establishes intense light fields as a platform for multi-petahertz coherent electronics and points to new opportunities for fundamental studies of electron dynamics in condensed matter. The frequency of electric currents associated with charge carriers moving in the electronic bands of solids determines the speed limit of electronics and thereby that of information and signal processing1. The use of light fields to drive electrons promises access to vastly higher frequencies than conventionally used, as electric currents can be induced and manipulated on timescales faster than that of the quantum dephasing of charge carriers in solids2. This forms the basis of terahertz (1012 hertz) electronics in artificial superlattices2, and has enabled light-based switches3,4,5 and sampling of currents extending in frequency up to a few hundred terahertz. Here we demonstrate the extension of electronic metrology to the multi-petahertz (1015 hertz) frequency range. We use single-cycle intense optical fields (about one volt per angstrom) to drive electron motion in the bulk of silicon dioxide, and then probe its dynamics by using attosecond (10−18 seconds) streaking6,7 to map the time structure of emerging isolated attosecond extreme ultraviolet transients and their optical driver. The data establish a firm link between the emission of the extreme ultraviolet radiation and the light-induced intraband, phase-coherent electric currents that extend in frequency up to about eight petahertz, and enable access to the dynamic nonlinear conductivity of silicon dioxide. Direct probing, confinement and control of the waveform of intraband currents inside solids on attosecond timescales establish a method of realizing multi-petahertz coherent electronics. We expect this technique to enable new ways of exploring the interplay between electron dynamics and the structure of condensed matter on the atomic scale.

267 citations



Journal ArticleDOI
TL;DR: In this article, a large increase in oscillation frequency was achieved in resonant-tunneling-diode (RTD) terahertz oscillators by reducing the conduction loss.
Abstract: A large increase in oscillation frequency was achieved in resonant-tunneling-diode (RTD) terahertz oscillators by reducing the conduction loss. An n+-InGaAs layer under the air-bridge electrode connected to the RTD was observed to cause a large conduction loss for high-frequency current due to the skin effect. By introducing a new fabrication process removing the InGaAs layer, we obtained 1.92-THz oscillation, which extended the highest frequency of room-temperature electronic single oscillators. Theoretical calculations reasonably agreed with the experiment, and an oscillation above 2 THz is further expected with an improved structure of the slot antenna used as a resonator and radiator.

252 citations


Journal ArticleDOI
TL;DR: The combined effect of spin pumping and current-induced torques introduces a dynamic feedback that sustains steady-state oscillations with amplitudes controllable via the applied current in insulating antiferromagnets.
Abstract: We consider the current-induced dynamics of insulating antiferromagnets in a spin Hall geometry. Sufficiently large in-plane currents perpendicular to the N\'eel order trigger spontaneous oscillations at frequencies between the acoustic and the optical eigenmodes. The direction of the driving current determines the chirality of the excitation. When the current exceeds a threshold, the combined effect of spin pumping and current-induced torques introduces a dynamic feedback that sustains steady-state oscillations with amplitudes controllable via the applied current. The ac voltage output is calculated numerically as a function of the dc current input for different feedback strengths. Our findings open a route towards terahertz antiferromagnetic spin-torque oscillators.

Journal ArticleDOI
TL;DR: In this article, a review of light sources from relativistic electrons produced by laser-wakefield accelerators is presented, and their potential applications are identified in a broad range of fields: medical and biological applications, military, defense and industrial applications.
Abstract: Laser-wakefield accelerators (LWFAs) were proposed more than three decades ago, and while they promise to deliver compact, high energy particle accelerators, they will also provide the scientific community with novel light sources. In a LWFA, where an intense laser pulse focused onto a plasma forms an electromagnetic wave in its wake, electrons can be trapped and are now routinely accelerated to GeV energies. From terahertz radiation to gamma-rays, this article reviews light sources from relativistic electrons produced by LWFAs, and discusses their potential applications. Betatron motion, Compton scattering and undulators respectively produce x-rays or gamma-rays by oscillating relativistic electrons in the wakefield behind the laser pulse, a counter-propagating laser field, or a magnetic undulator. Other LWFA-based light sources include bremsstrahlung and terahertz radiation. We first evaluate the performance of each of these light sources, and compare them with more conventional approaches, including radio frequency accelerators or other laser-driven sources. We have then identified applications, which we discuss in details, in a broad range of fields: medical and biological applications, military, defense and industrial applications, and condensed matter and high energy density science.

Journal ArticleDOI
TL;DR: Using terahertz (10(12) Hz) emission spectroscopy and exploiting the spin-orbit interaction, this work demonstrates the optical generation of electric photocurrents in metallic ferromagnetic heterostructures at the femtosecond timescale.
Abstract: The spin–orbit interaction can be used to optically generate and control terahertz electric photocurrents in metallic ferromagnetic heterostructures.

Journal ArticleDOI
02 Jun 2016-Nature
TL;DR: It is demonstrated that attosecond metrology extends the resolution to petahertz frequencies of visible light and Quantitative determination of dissipation within a signal manipulation cycle of only a few femtoseconds duration reveals the feasibility of dielectric optical switching at clock rates above 100 teraherz.
Abstract: Petahertz-bandwidth metrology is demonstrated in the measurement of nonlinear polarization in silica. Recent years have seen an increased interest in light–matter interactions in solid-state systems at ultrafast timescales. Ferenc Krausz and colleagues study the nonlinear polarization of silica in response to intense infrared light fields with a spectroscopy method in the attosecond time range. The method makes it possible to unravel details of the reversible and irreversible energy exchange between infrared light and electrons and points to the feasibility of using light-based switching techniques for signal processing in solid-state devices above 100 terahertz. Electric-field-induced charge separation (polarization) is the most fundamental manifestation of the interaction of light with matter and a phenomenon of great technological relevance. Nonlinear optical polarization1,2 produces coherent radiation in spectral ranges inaccessible by lasers and constitutes the key to ultimate-speed signal manipulation. Terahertz techniques3,4,5,6,7,8 have provided experimental access to this important observable up to frequencies of several terahertz9,10,11,12,13. Here we demonstrate that attosecond metrology14 extends the resolution to petahertz frequencies of visible light. Attosecond polarization spectroscopy allows measurement of the response of the electronic system of silica to strong (more than one volt per angstrom) few-cycle optical (about 750 nanometres) fields. Our proof-of-concept study provides time-resolved insight into the attosecond nonlinear polarization and the light–matter energy transfer dynamics behind the optical Kerr effect and multi-photon absorption. Timing the nonlinear polarization relative to the driving laser electric field with sub-30-attosecond accuracy yields direct quantitative access to both the reversible and irreversible energy exchange between visible–infrared light and electrons. Quantitative determination of dissipation within a signal manipulation cycle of only a few femtoseconds duration (by measurement and ab initio calculation) reveals the feasibility of dielectric optical switching at clock rates above 100 terahertz. The observed sub-femtosecond rise of energy transfer from the field to the material (for a peak electric field strength exceeding 2.5 volts per angstrom) in turn indicates the viability of petahertz-bandwidth metrology with a solid-state device.

Journal ArticleDOI
TL;DR: In this paper, a novel metamaterial absorber integrated microfluidic (MAIM) sensor is proposed and demonstrated in terahertz (THz) range, where the dielectric layer of the MDM structure is hollow and acts as the microfluideic channel, and greatly confined electromagnetic fields can be obtained in the channel resulting in significantly enhanced interaction between the analytes and the THz wave.
Abstract: Spatial overlap between the electromagnetic fields and the analytes is a key factor for strong light-matter interaction leading to high sensitivity for label-free refractive index sensing Usually, the overlap and therefore the sensitivity are limited by either the localized near field of plasmonic antennas or the decayed resonant mode outside the cavity applied to monitor the refractive index variation In this paper, by constructing a metal microstructure array-dielectric-metal (MDM) structure, a novel metamaterial absorber integrated microfluidic (MAIM) sensor is proposed and demonstrated in terahertz (THz) range, where the dielectric layer of the MDM structure is hollow and acts as the microfluidic channel Tuning the electromagnetic parameters of metamaterial absorber, greatly confined electromagnetic fields can be obtained in the channel resulting in significantly enhanced interaction between the analytes and the THz wave A high sensitivity of 35 THz/RIU is predicted The experimental results of devices working around 1 THz agree with the simulation ones well The proposed idea to integrate metamaterial and microfluid with a large light-matter interaction can be extended to other frequency regions and has promising applications in matter detection and biosensing

Journal ArticleDOI
TL;DR: In this article, a novel electric dipole-mediated mechanism of nonlinear terahertz-spin coupling that is much stronger than linear Zeeman coupling to the teraherstz magnetic field was explored.
Abstract: Future information technologies, such as ultrafast data recording, quantum computation or spintronics, call for ever faster spin control by light1, 2, 3, 4, 5, 6, 7, 8, 9, 10, 11, 12, 13, 14, 15, 16. Intense terahertz pulses can couple to spins on the intrinsic energy scale of magnetic excitations5, 11. Here, we explore a novel electric dipole-mediated mechanism of nonlinear terahertz-spin coupling that is much stronger than linear Zeeman coupling to the terahertz magnetic field5, 10. Using the prototypical antiferromagnet thulium orthoferrite (TmFeO3), we demonstrate that resonant terahertz pumping of electronic orbital transitions modifies the magnetic anisotropy for ordered Fe3+ spins and triggers large-amplitude coherent spin oscillations. This mechanism is inherently nonlinear, it can be tailored by spectral shaping of the terahertz waveforms and its efficiency outperforms the Zeeman torque by an order of magnitude. Because orbital states govern the magnetic anisotropy in all transition-metal oxides, the demonstrated control scheme is expected to be applicable to many magnetic materials.

Journal ArticleDOI
TL;DR: Experimental measurements of the frequency-angular spectrum generated by 130-fs laser pulses agree with numerical simulations based on a unidirectional pulse propagation model and show ring-shaped spatial distributions of the THz radiation are shown to be of universal nature.
Abstract: We have solved the long-standing problem of the mechanism of terahertz (THz) generation by a two-color filament in air and found that both neutrals and plasma contribute to the radiation. We reveal that the contribution from neutrals by four-wave mixing is much weaker and higher in frequency than the distinctive plasma lower-frequency contribution. The former is in the forward direction while the latter is in a cone and reveals an abrupt down-shift to the plasma frequency. Ring-shaped spatial distributions of the THz radiation are shown to be of universal nature and they occur in both collimated and focusing propagation geometries. Experimental measurements of the frequency-angular spectrum generated by 130-fs laser pulses agree with numerical simulations based on a unidirectional pulse propagation model.

Journal ArticleDOI
TL;DR: In this article, a review provides an overview and illustrative examples of how intense terahertz transients can be used to resonantly control matter, with particular focus on strongly correlated electron systems and high temperature superconductors.
Abstract: Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as powerful tools to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The recent developments in high-power sources in the 0.1–30 THz frequency range, both from table-top laser systems and from free-electron lasers, have provided access to excitations of molecules and solids, which can be stimulated at their resonance frequencies. Amongst these, we discuss free electrons in metals, superconducting gaps and Josephson plasmons in layered superconductors, and vibrational modes of the crystal lattice (phonons), as well as magnetic excitations. This review provides an overview and illustrative examples of how intense terahertz transients can be used to resonantly control matter, with particular focus on strongly correlated electron systems and high-temperature superconductors.

Journal ArticleDOI
TL;DR: A new scheme for realizing thermal-controlled chirality using a hybrid terahertz metamaterial with embedded vanadium dioxide (VO2) films with high-efficiency thermal modulation of linear polarization conversion is theoretically demonstrated.
Abstract: Polarization manipulations of electromagnetic waves can be obtained by chiral and anisotropic metamaterials routinely, but the dynamic and high-efficiency modulations of chiral properties still remain challenging at the terahertz range. Here, we theoretically demonstrate a new scheme for realizing thermal-controlled chirality using a hybrid terahertz metamaterial with embedded vanadium dioxide (VO2) films. The phase transition of VO2 films in 90° twisted E-shaped resonators enables high-efficiency thermal modulation of linear polarization conversion. The asymmetric transmission of linearly polarized wave and circular dichroism simultaneously exhibit a pronounced switching effect dictated by temperature-controlled conductivity of VO2 inclusions. The proposed hybrid metamaterial design opens exciting possibilities to achieve dynamic modulation of terahertz waves and further develop tunable terahertz polarization devices.

Journal ArticleDOI
TL;DR: In this article, an all-dielectric metasurface operating in the terahertz band was demonstrated, which is capable of engineering a reflected beam's spatial properties with high efficiency.
Abstract: We demonstrate an all-dielectric metasurface operating in the terahertz band that is capable of engineering a reflected beam’s spatial properties with high efficiency. The metasurface is formed from an array of silicon cube resonators which simultaneously support electric and magnetic dipolar Mie resonances. By controlling the interference between these modes, the amplitude and phase of a reflected wave can be arbitrarily controlled over a subwavelength area. We demonstrate the flexibility and utility of this metasurface by optimizing the surface to produce several reflected beam types including vortex and Bessel beams; the latter being useful for diffraction-free point-to-point terahertz communications. Additionally, we show theoretically and experimentally how the metasurface can produce an all-dielectric magnetic mirror in the terahertz band.

Journal ArticleDOI
TL;DR: Condensed-matter physics meets quantum optics in a study of light-matter interaction in the strong-coupling regime using a two-dimensional electron gas in a high-quality-factor terahertz cavity as mentioned in this paper.
Abstract: Condensed-matter physics meets quantum optics in a study of light–matter interaction in the strong-coupling regime using a two-dimensional electron gas in a high-quality-factor terahertz cavity.

Journal ArticleDOI
TL;DR: In this article, the authors proposed terahertz metasurfaces based on aligned rectangular graphene patches placed on top of a dielectric layer to convert the transmitted linearly polarized waves to circular or elliptical polarized radiation.
Abstract: We present terahertz metasurfaces based on aligned rectangular graphene patches placed on top of a dielectric layer to convert the transmitted linearly polarized waves to circular or elliptical polarized radiation. Our results lead to the design of an ultrathin broadband terahertz quarter-wave plate. In addition, ultrathin metasurfaces based on the arrays of L-shaped graphene periodic patches are demonstrated to achieve broadband cross-polarization transformation in reflection and transmission. The proposed metasurface designs have tunable responses and are envisioned to become the building blocks of several integrated terahertz systems.

Journal ArticleDOI
TL;DR: Three-dimensional topological insulators are fascinating materials with insulating bulk yet metallic surfaces that host highly mobile charge carriers with locked spin and momentum, and photon-helicity-dependent photocurrents are found to be orders of magnitude smaller than expected from generation scenarios based on asymmetric depopulation of the Dirac cone.
Abstract: Three-dimensional topological insulators are fascinating materials with insulating bulk yet metallic surfaces that host highly mobile charge carriers with locked spin and momentum. Remarkably, surface currents with tunable direction and magnitude can be launched with tailored light beams. To better understand the underlying mechanisms, the current dynamics need to be resolved on the timescale of elementary scattering events (∼10 fs). Here, we excite and measure photocurrents in the model topological insulator Bi2Se3 with a time resolution of 20 fs by sampling the concomitantly emitted broadband terahertz (THz) electromagnetic field from 0.3 to 40 THz. Strikingly, the surface current response is dominated by an ultrafast charge transfer along the Se-Bi bonds. In contrast, photon-helicity-dependent photocurrents are found to be orders of magnitude smaller than expected from generation scenarios based on asymmetric depopulation of the Dirac cone. Our findings are of direct relevance for broadband optoelectronic devices based on topological-insulator surface currents.

Journal ArticleDOI
TL;DR: The potential of electromagnetic hybrids--materials incorporating mixtures of SPPs and SPhPs--for overcoming the limitations of the individual polaritons are discussed, and a new type of atomic-scale hybrid--the crystalline hybrid--is proposed that could enable the creation of novel actively tunable, yet low-loss optics at the nanoscale.
Abstract: The field of nanophotonics focuses on the ability to confine light to nanoscale dimensions, typically much smaller than the wavelength of light. The goal is to develop light-based technologies that are impossible with traditional optics. Subdiffractional confinement can be achieved using either surface plasmon polaritons (SPPs) or surface phonon polaritons (SPhPs). SPPs can provide a gate-tunable, broad-bandwidth response, but suffer from high optical losses; whereas SPhPs offer a relatively low-loss, crystal-dependent optical response, but only over a narrow spectral range, with limited opportunities for active tunability. Here, motivated by the recent results from monolayer graphene and multilayer hexagonal boron nitride heterostructures, we discuss the potential of electromagnetic hybrids--materials incorporating mixtures of SPPs and SPhPs--for overcoming the limitations of the individual polaritons. Furthermore, we also propose a new type of atomic-scale hybrid--the crystalline hybrid--where mixtures of two or more atomic-scale (∼3 nm or less) polar dielectric materials lead to the creation of a new material resulting from hybridized optic phonon behaviour of the constituents, potentially allowing direct control over the dielectric function. These atomic-scale hybrids expand the toolkit of materials for mid-infrared to terahertz nanophotonics and could enable the creation of novel actively tunable, yet low-loss optics at the nanoscale.

Journal ArticleDOI
TL;DR: In this paper, a transmission-type coding metasurface is proposed to bend normally incident terahertz beams in anomalous directions and generate nondiffractive Bessel beams in normal and oblique directions.
Abstract: Coding metasurfaces, composed of an array of coding particles with discrete phase responses, are encoded with predesigned coding sequences to manipulate wavefronts of electromagnetic (EM) waves and realize novel functionalities such as anomalous beam deflection, broadband diffusion, and polarization conversion. Such a new concept can be viewed as a bridge linking metamaterial and digital codes, yielding the investigation of metamaterials from a digital perspective and eventually the realization of real-time control of EM waves. Here, we propose and experimentally demonstrate a transmission-type coding metasurface to bend normally incident terahertz beams in anomalous directions and generate nondiffractive Bessel beams in normal and oblique directions. To overcome the larger reflection and strong Fabry–Perot resonance that usually originate from a thick silicon substrate, a free-standing design is presented for the coding particle, which is formed by stacking three metallic layers with four polyimide space...

Journal ArticleDOI
TL;DR: A flexible and wearable terahertz scanner based on carbon nanotubes is demonstrated at room temperature over a broad frequency band ranging from 0.14 THz to 39 THz as mentioned in this paper.
Abstract: Imaging technologies based on terahertz (THz) waves have great potential for use in powerful non-invasive inspection methods. However, most real objects have various three-dimensional curvatures and existing THz technologies often encounter difficulties in imaging such configurations, which limits the useful range of THz imaging applications. Here, we report the development of a flexible and wearable THz scanner based on carbon nanotubes. We achieved room-temperature THz detection over a broad frequency band ranging from 0.14 to 39 THz and developed a portable THz scanner. Using this scanner, we performed THz imaging of samples concealed behind opaque objects, breakages and metal impurities of a bent film and multi-view scans of a syringe. We demonstrated a passive biometric THz scan of a human hand. Our results are expected to have considerable implications for non-destructive and non-contact inspections, such as medical examinations for the continuous monitoring of health conditions. A flexible and wearable terahertz scanner based on carbon nanotubes is demonstrated at room temperature over a frequency range 0.14 THz to 39 THz. The terahertz photothermoelectricity is enhanced by using different electrode materials.

Journal ArticleDOI
TL;DR: This article presents an indoor multiuser terahertz system with array-of-subarrays architecture to accommodate hardware constraints as well as channel characteristics in the terAhertz band to alleviate spectrum limitation of current wireless systems.
Abstract: Enabling terahertz communications will alleviate the spectrum limitation of current wireless systems. This article presents an indoor multiuser terahertz system with array-of-subarrays architecture to accommodate hardware constraints as well as channel characteristics in the terahertz band. Specifically, the difference between terahertz and millimeter-wave communications is first clarified. Then the advantage of the array-of-subarrays structure is explained through comparison with the fully connected structure in both spectral and energy efficiency. Furthermore, a distance-aware multi-carrier scheme with the array-of-subarrays structure is introduced for wideband terahertz communications. Finally, the associated open issues and future research directions are discussed.

Journal ArticleDOI
TL;DR: In this paper, a novel and simple design of a triple-band terahertz absorber formed by only an asymmetric cross is presented, and the theoretical results show that the proposed structure has three distinct absorption bands whose peaks are all over 99%.
Abstract: For a general metamaterial absorber, single patterned structure has only one resonance absorption peak. Therefore, a multi-band perfect absorber can be obtained by employing multiple different-sized metallic patterns. However, this kind of design strategy removes the novelty of their resonance mechanism and is also quite troublesome in regard to fabrication. Here, a novel and simple design of a triple-band terahertz absorber formed by only an asymmetric cross is presented. Theoretical results show that the proposed structure has three distinct absorption bands whose peaks are all over 99%. The first two absorption peaks are due to the magnetic resonances of the different sections of the asymmetric cross, and the third peak is based on the surface response of the structure. Moreover, sensing performance of the absorber is investigated in terms of the surrounding index. It is found that the figure of merit and quality factor of the third peak is much larger than those of the first two peaks, which reveals the proposed absorber's, in particular the third resonance mode of the metamaterial, potential applications in sensing and detection.

Journal ArticleDOI
TL;DR: In this article, the authors used terahertz time-gated spectral imaging to extract occluded text from paper pages with subwavelength spacing, which may be used to non-destructively detect and study defects and structures within materials.
Abstract: Terahertz radiation may be used to nondestructively detect and study defects and structures within materials. Here the authors use terahertz time-gated spectral imaging to extract occluded text from paper pages with subwavelength spacing.

Journal ArticleDOI
TL;DR: In this paper, periodic arrays of graphene rings are proposed to introduce tunable light trapping with good angle polarization tolerance and enhance the absorption in the light-absorbing materials nearby to more than one order.
Abstract: Surface plasmon resonance (SPR) has been intensively studied and widely employed for light trapping and absorption enhancement. In the mid-infrared and terahertz (THz) regime, graphene supports the tunable SPR via manipulating its Fermi energy and enhances light-matter interaction at the selective wavelength. In this work, periodic arrays of graphene rings are proposed to introduce tunable light trapping with good angle polarization tolerance and enhance the absorption in the light-absorbing materials nearby to more than one order. Moreover, the design principle here could be set as a template to achieve multi-band plasmonic absorption enhancement by introducing more graphene concentric rings into each unit cell. This work not only opens up new ways of employing graphene SPR, but also leads to practical applications in high-performance simultaneous multi-color photodetection with high efficiency and tunable spectral selectivity.