Showing papers on "Ultrashort pulse published in 2017"

High-harmonic generation in graphene enhanced by elliptically polarized light excitation

Abstract: The electronic properties of graphene can give rise to a range of nonlinear optical responses. One of the most desirable nonlinear optical processes is high-harmonic generation (HHG) originating from coherent electron motion induced by an intense light field. Here, we report on the observation of up to ninth-order harmonics in graphene excited by mid-infrared laser pulses at room temperature. The HHG in graphene is enhanced by an elliptically polarized laser excitation, and the resultant harmonic radiation has a particular polarization. The observed ellipticity dependence is reproduced by a fully quantum mechanical treatment of HHG in solids. The zero-gap nature causes the unique properties of HHG in graphene, and our findings open up the possibility of investigating strong-field and ultrafast dynamics and nonlinear behavior of massless Dirac fermions.

On-chip photonic synapse

Abstract: The search for new “neuromorphic computing” architectures that mimic the brain’s approach to simultaneous processing and storage of information is intense. Because, in real brains, neuronal synapses outnumber neurons by many orders of magnitude, the realization of hardware devices mimicking the functionality of a synapse is a first and essential step in such a search. We report the development of such a hardware synapse, implemented entirely in the optical domain via a photonic integrated-circuit approach. Using purely optical means brings the benefits of ultrafast operation speed, virtually unlimited bandwidth, and no electrical interconnect power losses. Our synapse uses phase-change materials combined with integrated silicon nitride waveguides. Crucially, we can randomly set the synaptic weight simply by varying the number of optical pulses sent down the waveguide, delivering an incredibly simple yet powerful approach that heralds systems with a continuously variable synaptic plasticity resembling the true analog nature of biological synapses.

Light-field-driven currents in graphene

Abstract: The ability to steer electrons using the strong electromagnetic field of light has opened up the possibility of controlling electron dynamics on the sub-femtosecond (less than 10-15 seconds) timescale. In dielectrics and semiconductors, various light-field-driven effects have been explored, including high-harmonic generation, sub-optical-cycle interband population transfer and the non-perturbative change of the transient polarizability. In contrast, much less is known about light-field-driven electron dynamics in narrow-bandgap systems or in conductors, in which screening due to free carriers or light absorption hinders the application of strong optical fields. Graphene is a promising platform with which to achieve light-field-driven control of electrons in a conducting material, because of its broadband and ultrafast optical response, weak screening and high damage threshold. Here we show that a current induced in monolayer graphene by two-cycle laser pulses is sensitive to the electric-field waveform, that is, to the exact shape of the optical carrier field of the pulse, which is controlled by the carrier-envelope phase, with a precision on the attosecond (10-18 seconds) timescale. Such a current, dependent on the carrier-envelope phase, shows a striking reversal of the direction of the current as a function of the driving field amplitude at about two volts per nanometre. This reversal indicates a transition of light-matter interaction from the weak-field (photon-driven) regime to the strong-field (light-field-driven) regime, where the intraband dynamics influence interband transitions. We show that in this strong-field regime the electron dynamics are governed by sub-optical-cycle Landau-Zener-Stuckelberg interference, composed of coherent repeated Landau-Zener transitions on the femtosecond timescale. Furthermore, the influence of this sub-optical-cycle interference can be controlled with the laser polarization state. These coherent electron dynamics in graphene take place on a hitherto unexplored timescale, faster than electron-electron scattering (tens of femtoseconds) and electron-phonon scattering (hundreds of femtoseconds). We expect these results to have direct ramifications for band-structure tomography and light-field-driven petahertz electronics.

Diffraction and microscopy with attosecond electron pulse trains

Abstract: Attosecond spectroscopy 1–7 can resolve electronic processes directly in time, but a movie-like space–time recording is impeded by the too long wavelength (~100 times larger than atomic distances) or the source–sample entanglement in re-collision techniques 8–11 . Here we advance attosecond metrology to picometre wavelength and sub-atomic resolution by using free-space electrons instead of higher-harmonic photons 1–7 or re-colliding wavepackets 8–11 . A beam of 70-keV electrons at 4.5-pm de Broglie wavelength is modulated by the electric field of laser cycles into a sequence of electron pulses with sub-optical-cycle duration. Time-resolved diffraction from crystalline silicon reveals a < 10-as delay of Bragg emission and demonstrates the possibility of analytic attosecond–angstrom diffraction. Real-space electron microscopy visualizes with sub-light-cycle resolution how an optical wave propagates in space and time. This unification of attosecond science with electron microscopy and diffraction enables space–time imaging of light-driven processes in the entire range of sample morphologies that electron microscopy can access. Attosecond light pulses are used to probe ultrafast processes. The experimental observation of attosecond electron pulses now promises the marriage of these techniques with electron microscopy and diffraction.

Few-layer antimonene decorated microfiber: ultra-short pulse generation and all-optical thresholding with enhanced long term stability

Abstract: Antimonene, a new type of mono/few-layer two-dimensional (2D) mono-elemental material purely consisting of antimony similar as graphene and phosphorene, has been theoretically predicted with excellent optical response and enhanced stability. Herein, we experimentally investigated the broadband nonlinear optical response of highly stable few-layer antimonene (FLA) by performing an open-aperture Z-scan laser measurement. Thanks to the direct bandgap and resonant absorption at the telecommunication band, we demonstrated the feasibility of FLA-decorated microfiber not only as an optical saturable absorber for ultrafast photonics operation, but also as a stable all-optical pulse thresholder that can effectively suppress the transmission noise, boost the signal-to-noise ratio (SNR), and reshape the deteriorated input signal. Our findings, as the first prototypic device of absorption of antimonene, might facilitate the development of antimonene-based optical communication technologies towards high stability and practical applications in the future.

Emerging Low-Dimensional Materials for Nonlinear Optics and Ultrafast Photonics.

Abstract: Low-dimensional (LD) materials demonstrate intriguing optical properties, which lead to applications in diverse fields, such as photonics, biomedicine and energy. Due to modulation of electronic structure by the reduced structural dimensionality, LD versions of metal, semiconductor and topological insulators (TIs) at the same time bear distinct nonlinear optical (NLO) properties as compared with their bulk counterparts. Their interaction with short pulse laser excitation exhibits a strong nonlinear character manifested by NLO absorption, giving rise to optical limiting or saturated absorption associated with excited state absorption and Pauli blocking in different materials. In particular, the saturable absorption of these emerging LD materials including two-dimensional semiconductors as well as colloidal TI nanoparticles has recently been utilized for Q-switching and mode-locking ultra-short pulse generation across the visible, near infrared and middle infrared wavelength regions. Beside the large operation bandwidth, these ultrafast photonics applications are especially benefit from the high recovery rate as well as the facile processibility of these LD materials. The prominent NLO response of these LD materials have also provided new avenues for the development of novel NLO and photonics devices for all-optical control as well as optical circuits beyond ultrafast lasers.

Ultrafast nonthermal photo-magnetic recording in a transparent medium

Abstract: Discovering ways to control the magnetic state of media with the lowest possible production of heat and at the fastest possible speeds is important in the study of fundamental magnetism, with clear practical potential. In metals, it is possible to switch the magnetization between two stable states (and thus to record magnetic bits) using femtosecond circularly polarized laser pulses. However, the switching mechanisms in these materials are directly related to laser-induced heating close to the Curie temperature. Although several possible routes for achieving all-optical switching in magnetic dielectrics have been discussed, no recording has hitherto been demonstrated. Here we describe ultrafast all-optical photo-magnetic recording in transparent films of the dielectric cobalt-substituted garnet. A single linearly polarized femtosecond laser pulse resonantly pumps specific d-d transitions in the cobalt ions, breaking the degeneracy between metastable magnetic states. By changing the polarization of the laser pulse, we deterministically steer the net magnetization in the garnet, thus writing '0' and '1' magnetic bits at will. This mechanism outperforms existing alternatives in terms of the speed of the write-read magnetic recording event (less than 20 picoseconds) and the unprecedentedly low heat load (less than 6 joules per cubic centimetre).

Spatiotemporal mode-locking in multimode fiber lasers

Abstract: A laser is based on the electromagnetic modes of its resonator, which provides the feedback required for oscillation Enormous progress has been made toward controlling the interactions of longitudinal modes in lasers with a single transverse mode For example, the field of ultrafast science has been built on lasers that lock many longitudinal modes together to form ultrashort light pulses However, coherent superposition of longitudinal and transverse modes in a laser has received little attention We show that modal and chromatic dispersions in fiber lasers can be counteracted by strong spatial and spectral filtering This allows locking of multiple transverse and longitudinal modes to create ultrashort pulses with a variety of spatiotemporal profiles Multimode fiber lasers thus open new directions in studies of nonlinear wave propagation and capabilities for applications

Ultrafast synthesis and switching of light polarization in nonlinear anisotropic metamaterials

Abstract: Optical communications, laser science, microscopy and metrology demand control of light polarization, which is also used as a probe of chemical and biological systems. Typically, certain polarization states of light are achieved using macroscopic anisotropic crystals. Metamaterials and metasurfaces have recently been developed to act as efficient passive polarization components of subwavelength dimensions 1–4 . However, active polarization control has so far been mainly limited to microwave and terahertz wavelengths 5–7 . Here, we demonstrate all-optical switching of visible light polarization, achieving up to 60° rotation of the polarization ellipse at picosecond timescales. This is accomplished both under control illumination and in a self-phase modulation regime, where the intensity of light affects its own polarization state, by exploiting the strong anisotropy and nonlinear response of a hyperbolic metamaterial 3,8–10 . The effects are general for any resonant, anisotropic, nonlinear nanoantennas and metasurfaces and are suited to numerous photonic applications and material characterization techniques where ultrafast polarization shaping is required. Picosecond all-optical switching of the polarization of visible light is achieved by using the anisotropy and nonlinearity of a hyperbolic metamaterial.

Tungsten disulfide saturable absorbers for 67 fs mode-locked erbium-doped fiber lasers.

Abstract: In this paper, we demonstrate 67 fs pulse emitting with tungsten disulfide (WS2) in mode-locked erbium-doped fiber (EDF) lasers. Using the pulsed laser deposition method, WS2 is deposited on the surface of the tapered fiber to form the evanescent field. The fiber-taper WS2 saturable absorber (SA) with the large modulation depth is fabricated to support the ultrashort pulse generation. The influences of the WS2 SA are analyzed through contrastive experiments on fiber lasers with or without the WS2 SA. The pulse duration is measured to be 67 fs, which is the shortest pulse duration obtained in the mode-locked fiber lasers with two dimensional (2D) material SAs. Compared to graphene, topological insulator, and other transition metal dichalcogenides (TMDs) SAs, results in this paper indicate that the fiber-taper WS2 SA with large modulation depth is a more promising photonic device in mode-locked fiber lasers with the wide spectrum and ultrashort pulse duration.

Attosecond Electron Pulse Trains and Quantum State Reconstruction in Ultrafast Transmission Electron Microscopy

Abstract: We introduce a framework for the preparation, coherent manipulation and characterization of free-electron quantum states, experimentally demonstrating attosecond pulse trains for electron microscopy. Specifically, we employ phase-locked single-color and two-color optical fields to coherently control the electron wave function along the beam direction. We establish a new variant of quantum state tomography - "SQUIRRELS" - to reconstruct the density matrices of free-electron ensembles and their attosecond temporal structure. The ability to tailor and quantitatively map electron quantum states will promote the nanoscale study of electron-matter entanglement and the development of new forms of ultrafast electron microscopy and spectroscopy down to the attosecond regime.

Tungsten disulphide for ultrashort pulse generation in all-fiber lasers

Abstract: Tungsten disulphide (WS2), which exhibits excellent saturable absorption properties, has attracted much attention in the applications of photonic devices. In this paper, WS2 is applied for the preparation of a saturable absorber (SA). Using the pulsed laser deposition (PLD) method, WS2 is deposited on the side surface of the tapered fiber. In order to obtain larger non-linearity of the SAs with evanescent wave interaction, the tapered fiber had a smaller waist diameter and longer fused zone. Gold film was deposited on the fiber-taper WS2 SAs to improve their reliability and avoid oxidation and corrosion. Employing the balanced twin-detector method, the modulation depth of the fiber-taper WS2 SAs was measured to be 17.2%. With the fiber-taper WS2 SA, a generated pulse with 246 fs duration and a 57 nm bandwidth was obtained at 1561 nm. The electrical signal to noise ratio was better than 92 dB. To our knowledge, the pulse duration was the shortest among the reported all-fiber lasers with transition metal dichalcogenide (TMD) SAs. These results indicate that fiber-taper WS2 SAs with smaller waist diameter and longer fused zone are promising photonic devices for ultrashort pulse generation in all-fiber lasers.

Attosecond electron pulse trains and quantum state reconstruction in ultrafast transmission electron microscopy

Abstract: Ultrafast electron and X-ray imaging and spectroscopy are the basis for an ongoing revolution in the understanding of dynamical atomic-scale processes in matter. The underlying technology relies heavily on laser science for the generation and characterization of ever shorter pulses. Recent findings suggest that ultrafast electron microscopy with attosecond-structured wavefunctions may be feasible. However, such future technologies call for means to both prepare and fully analyse the corresponding free-electron quantum states. Here, we introduce a framework for the preparation, coherent manipulation and characterization of free-electron quantum states, experimentally demonstrating attosecond electron pulse trains. Phase-locked optical fields coherently control the electron wavefunction along the beam direction. We establish a new variant of quantum state tomography—‘SQUIRRELS’—for free-electron ensembles. The ability to tailor and quantitatively map electron quantum states will promote the nanoscale study of electron–matter entanglement and new forms of ultrafast electron microscopy down to the attosecond regime. Attosecond electron pulse trains in electron microscopy are demonstrated through the coupling of phase-locked multicolour optical fields with electron pulses. A new variant of quantum state tomography for free-electron ensembles is established.

Tailored semiconductors for high-harmonic optoelectronics

Abstract: The advent of high-harmonic generation in gases 30 years ago set the foundation for attosecond science and facilitated ultrafast spectroscopy in atoms, molecules, and solids. We explore high-harmonic generation in the solid state by means of nanostructured and ion-implanted semiconductors. We use wavelength-selective microscopic imaging to map enhanced harmonic emission and show that the generation medium and the driving field can be locally tailored in solids by modifying the chemical composition and morphology. This enables the control of high-harmonic technology within precisely engineered solid targets. We demonstrate customized high-harmonic wave fields with wavelengths down to 225 nanometers (ninth-harmonic order of 2-micrometer laser pulses) and present an integrated Fresnel zone plate target in silicon, which leads to diffraction-limited self-focusing of the generated harmonics down to 1-micrometer spot sizes.

Photoionization in the time and frequency domain

Abstract: Ultrafast processes in matter, such as the electron emission after light absorption, can now be studied using ultrashort light pulses of attosecond duration (10 −18 seconds) in the extreme ultraviolet spectral range. The lack of spectral resolution due to the use of short light pulses has raised issues in the interpretation of the experimental results and the comparison with theoretical calculations. We determine photoionization time delays in neon atoms over a 40–electron volt energy range with an interferometric technique combining high temporal and spectral resolution. We spectrally disentangle direct ionization from ionization with shake-up, in which a second electron is left in an excited state, and obtain excellent agreement with theoretical calculations, thereby solving a puzzle raised by 7-year-old measurements.

Direct measurement of sub-10 fs relativistic electron beams with ultralow emittance

Abstract: Ultralow emittance (≤20 nm, normalized) electron beams with 10^{5} electrons per bunch are obtained by tightly focusing an ultrafast (∼100 fs) laser pulse on the cathode of a 1.6 cell radio frequency photoinjector. Taking advantage of the small initial longitudinal emittance, a downstream velocity bunching cavity is used to compress the beam to <10 fs rms bunch length. The measurement is performed using a thick high-voltage deflecting cavity which is shown to be well suited to measure ultrashort durations of bunching beams, provided that the beam reaches a ballistic longitudinal focus at the cavity center.

High average power and single-cycle pulses from a mid-IR optical parametric chirped pulse amplifier

Abstract: In attosecond and strong-field physics, the acquisition of data in an acceptable time demands the combination of high peak power with high average power. We report a 21 W mid-IR optical parametric chirped pulse amplifier (OPCPA) that generates 131 μJ and 97 fs (sub-9-cycle) pulses at a 160 kHz repetition rate and at a center wavelength of 3.25 μm. Pulse-to-pulse stability of the carrier envelope phase (CEP)-stable output is excellent with a 0.33% rms over 288 million pulses (30 min) and compression close to a single optical cycle was achieved through soliton self-compression inside a gas-filled mid-IR antiresonant-guiding photonic crystal fiber. Without any additional compression device, stable generation of 14.5 fs (1.35-optical-cycle) pulses was achieved at an average power of 9.6 W. The resulting peak power of 3.9 GW in combination with the near-single-cycle duration and intrinsic CEP stability makes our OPCPA a key-enabling technology for the next generation of extreme photonics, strong-field attosecond research, and coherent x-ray science.

Relativistic electron beams driven by kHz single-cycle light pulses

Abstract: Laser-plasma acceleration(1,2) is an emerging technique for accelerating electrons to high energies over very short distances. The accelerated electron bunches have femtosecond duration(3,4), making them particularly relevant for applications such as ultrafast imaging(5) or femtosecond X-ray generation(6,7). Current laser-plasma accelerators deliver 100 MeV (refs 8-10) to GeV (refs 11, 12) electrons using Joule-class laser systems that are relatively large in scale and have low repetition rates, with a few shots per second at best. Nevertheless, extending laser-plasma acceleration to higher repetition rates would be extremely useful for applications requiring lower electron energy. Here, we use single-cycle laser pulses to drive high-quality MeV relativistic electron beams, thereby enabling kHz operation and dramatic downsizing of the laser system. Numerical simulations indicate that the electron bunches are only similar to 1 fs long. We anticipate that the advent of these kHz femtosecond relativistic electron sources will pave the way to applications with wide impact, such as ultrafast electron diffraction in materials(13,14) with an unprecedented sub-10 fs resolution(15).

Phosphorene quantum dot saturable absorbers for ultrafast fiber lasers.

Abstract: We fabricate ultrasmall phosphorene quantum dots (PQDs) with an average size of 2.6 ± 0.9 nm using a liquid exfoliation method involving ultrasound probe sonication followed by bath sonication. By coupling the as-prepared PQDs with microfiber evanescent light field, the PQD-based saturable absorber (SA) device exhibits ultrafast nonlinear saturable absorption property, with an optical modulation depth of 8.1% at the telecommunication band. With the integration of the all-fiber PQD-based SA, a continuous-wave passively mode-locked erbium-doped (Er-doped) laser cavity delivers stable, self-starting pulses with a pulse duration of 0.88 ps and at the cavity repetition rate of 5.47 MHz. Our results contribute to the growing body of work studying the nonlinear optical properties of ultrasmall PQDs that present new opportunities of this two-dimensional (2D) nanomaterial for future ultrafast photonic technologies.

Size-dependent nonlinear optical properties of black phosphorus nanosheets and their applications in ultrafast photonics

Abstract: Multi-layer black phosphorus nanosheets (BPs) with different sizes are synthesized by using a basic solvent exfoliation method in association with controlled gradient centrifugation. Size-dependent nonlinear saturable absorption and Kerr nonlinearity as well as ultrafast carrier dynamics of BPs is systematically studied by using a Z-scan and pump–probe technique. Furthermore, an ultrashort pulse with a pulse duration of about 635 fs centered at a wavelength of 1562 nm is generated by using smaller sized BPs as a saturable absorber. These results directly reveal the physical processes of size-dependent nonlinear optical (NLO) properties of BPs and provide researchers with a viable approach in tailoring the NLO response of BPs through controlling the sizes, paving the way towards BP based electronics and optoelectronics applications such as ultrafast optical switches, modulators, fiber lasers, etc.

MoS2 for Ultrafast All-Optical Switching and Modulation of THz Fano Metaphotonic Devices

Abstract: In recent years, the stunning performance of transition metal dichalcogenides (TMDCs) has been utilized in the area of field effect transistors, integrated circuits, photodetectors, light generation and harvesting, valleytronics, and van der Waals (vdW) heterostructures. However, the optoelectronic application of TMDCs in realizing efficient, ultrafast metaphotonic devices in the terahertz part of the electromagnetic spectrum has remained unexplored. The most studied member of the TMDC family, i.e., MoS2, shows an ultrafast carrier relaxation after photoexcitation with near-infrared femtosecond pulse of energy above the bandgap. Here, this study investigates the photoactive properties of MoS2 to demonstrate an ultrasensitive active switching and modulation of the sharp Fano resonances in MoS2-coated metamaterials consisting of asymmetric split ring resonator arrays. The results show that all-optical switching and modulation of micrometer scale subwavelength Fano resonators can be achieved on a timescale of hundred picoseconds at moderate excitation pump fluences. The precise and active control of the MoS2-based hybrid metaphotonic devices open up opportunities for the real-world technologies and realization of ultrafast switchable sensors, modulators, filters, and nonlinear devices.

Ultrafast magnetization reversal by picosecond electrical pulses

Abstract: The field of spintronics involves the study of both spin and charge transport in solid-state devices. Ultrafast magnetism involves the use of femtosecond laser pulses to manipulate magnetic order on subpicosecond time scales. We unite these phenomena by using picosecond charge current pulses to rapidly excite conduction electrons in magnetic metals. We observe deterministic, repeatable ultrafast reversal of the magnetization of a GdFeCo thin film with a single sub–10-ps electrical pulse. The magnetization reverses in ~10 ps, which is more than one order of magnitude faster than any other electrically controlled magnetic switching, and demonstrates a fundamentally new electrical switching mechanism that does not require spin-polarized currents or spin-transfer/orbit torques. The energy density required for switching is low, projecting to only 4 fJ needed to switch a (20 nm) 3 cell. This discovery introduces a new field of research into ultrafast charge current–driven spintronic phenomena and devices.

Photoionization in the time and frequency domain

Abstract: Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral resolution due to the use of short light pulses may raise serious issues in the interpretation of the experimental results and the comparison with detailed theoretical calculations. Here, we determine photoionization time delays in neon atoms over a 40 eV energy range with an interferometric technique combining high temporal and spectral resolution. We spectrally disentangle direct ionization from ionization with shake up, where a second electron is left in an excited state, thus obtaining excellent agreement with theoretical calculations and thereby solving a puzzle raised by seven-year-old measurements. Our experimental approach does not have conceptual limits, allowing us to foresee, with the help of upcoming laser technology, ultra-high resolution time-frequency studies from the visible to the x-ray range.

Ultrafast laser-scanning time-stretch imaging at visible wavelengths.

Abstract: Optical time-stretch imaging enables the continuous capture of non-repetitive events in real time at a line-scan rate of tens of MHz—a distinct advantage for the ultrafast dynamics monitoring and high-throughput screening that are widely needed in biological microscopy. However, its potential is limited by the technical challenge of achieving significant pulse stretching (that is, high temporal dispersion) and low optical loss, which are the critical factors influencing imaging quality, in the visible spectrum demanded in many of these applications. We present a new pulse-stretching technique, termed free-space angular-chirp-enhanced delay (FACED), with three distinguishing features absent in the prevailing dispersive-fiber-based implementations: (1) it generates substantial, reconfigurable temporal dispersion in free space (>1 ns nm−1) with low intrinsic loss (<6 dB) at visible wavelengths; (2) its wavelength-invariant pulse-stretching operation introduces a new paradigm in time-stretch imaging, which can now be implemented both with and without spectral encoding; and (3) pulse stretching in FACED inherently provides an ultrafast all-optical laser-beam scanning mechanism at a line-scan rate of tens of MHz. Using FACED, we demonstrate not only ultrafast laser-scanning time-stretch imaging with superior bright-field image quality compared with previous work but also, for the first time, MHz fluorescence and colorized time-stretch microscopy. Our results show that this technique could enable a wider scope of applications in high-speed and high-throughput biological microscopy that were once out of reach. A new pulse-stretching technique has enabled ultrafast laser-scanning time-stretch imaging to be achieved in the important visible region. Optical time-stretching is used to realize real-time continuous imaging at ultrahigh frame rates, but current technologies based on dispersive fibers are generally restricted to near-infrared wavelengths. Now, a team at the University of Hong Kong led by Kevin Tsia has overcome this limitation by developing a pulse-stretching technique that they dub free-space angular-chirp-enhanced delay. It has the advantages of generating a large dispersion in free space with low loss and of enabling wavelength-invariant stretching. The researchers demonstrated its potential by realizing ultrafast laser-scanning time-stretch imaging with excellent bright-field image quality. They also used it to achieve megahertz fluorescence and color time-stretch microscopy at the optical wavelength of 700 nm.

Stabilization of Black Phosphorous Quantum Dots in PMMA Nanofiber Film and Broadband Nonlinear Optics and Ultrafast Photonics Application

Abstract: The stabilization of black phosphorous quantum dots (BPQDs) for optical application under ambient conditions is highly challenging. Here, a facile approach is presented to substantially stabilize BPQDs by making a uniform BPQDs/polymethyl methacrylate (PMMA) composite nanofiber film via an electrospinning technique. As verified by femtosecond laser Z-scan measurement, the BPQDs/PMMA composite nanofiber film that has been stored for three months exhibits almost the same nonlinear optical properties as the fresh BPQDs. Additionally, the BPQDs/PMMA composite nanofiber film demonstrates broadband nonlinear optical response ranging from the visible bandwidth (400 nm) to the mid-IR bandwidth (at least 1930 nm). By employing the BPQDs/PMMA composite nanofiber film as an optical saturable absorber, an ultrashort pulse with the pulse duration of ≈1.07 ps centered at the wavelength of 1567.6 nm is generated in a mode-locked fiber laser. These results suggest that the BPQDs/PMMA composite nanofiber film can combine the advantage of convenient integration and mitigation of the drawback of the easy oxidation of black phosphorous and pave the way for BP-based practical optoelectronic devices.

Optically Clear and Resilient Free-Form µ-Optics 3D-Printed via Ultrafast Laser Lithography

Abstract: We introduce optically clear and resilient free-form micro-optical components of pure (non-photosensitized) organic-inorganic SZ2080 material made by femtosecond 3D laser lithography (3DLL). This is advantageous for rapid printing of 3D micro-/nano-optics, including their integration directly onto optical fibers. A systematic study of the fabrication peculiarities and quality of resultant structures is performed. Comparison of microlens resiliency to continuous wave (CW) and femtosecond pulsed exposure is determined. Experimental results prove that pure SZ2080 is ∼20 fold more resistant to high irradiance as compared with standard lithographic material (SU8) and can sustain up to 1.91 GW/cm2 intensity. 3DLL is a promising manufacturing approach for high-intensity micro-optics for emerging fields in astro-photonics and atto-second pulse generation. Additionally, pyrolysis is employed to homogeneously shrink structures up to 40% by removing organic SZ2080 constituents. This opens a promising route towards downscaling photonic lattices and the creation of mechanically robust glass-ceramic microstructures.

From attosecond to zeptosecond coherent control of free-electron wave functions using semi-infinite light fields

Abstract: Light-electron interaction in empty space is the seminal ingredient for free-electron lasers and also for controlling electron beams to dynamically investigate materials and molecules. Pushing the coherent control of free electrons by light to unexplored timescales, below the attosecond, would enable unprecedented applications in light-assisted electron quantum circuits and diagnostics at extremely small timescales, such as those governing intramolecular electronic motion and nuclear phenomena. We experimentally demonstrate attosecond coherent manipulation of the electron wave function in a transmission electron microscope, and show that it can be pushed down to the zeptosecond regime with existing technology. We make a relativistic pulsed electron beam interact in free space with an appropriately synthesized semi-infinite light field generated by two femtosecond laser pulses reflected at the surface of a mirror and delayed by fractions of the optical cycle. The amplitude and phase of the resulting coherent oscillations of the electron states in energymomentum space are mapped via momentum-resolved ultrafast electron energy-loss spectroscopy. The experimental results are in full agreement with our theoretical framework for light-electron interaction, which predicts access to the zeptosecond timescale by combining semi-infinite X-ray fields with free electrons.

Nanoscale interface confinement of ultrafast spin transfer torque driving non-uniform spin dynamics

Abstract: Spintronics had a widespread impact over the past decades due to transferring information by spin rather than electric currents. Its further development requires miniaturization and reduction of characteristic timescales of spin dynamics combining the sub-nanometre spatial and femtosecond temporal ranges. These demands shift the focus of interest towards the fundamental open question of the interaction of femtosecond spin current (SC) pulses with a ferromagnet (FM). The spatio-temporal properties of the impulsive spin transfer torque exerted by ultrashort SC pulses on the FM open the time domain for probing non-uniform magnetization dynamics. Here we employ laser-generated ultrashort SC pulses for driving ultrafast spin dynamics in FM and analysing its transient local source. Transverse spins injected into FM excite inhomogeneous high-frequency spin dynamics up to 0.6 THz, indicating that the perturbation of the FM magnetization is confined to 2 nm.

Plasmon-assisted high-harmonic generation in graphene.

Abstract: High-harmonic generation in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. While graphene is anticipated to efficiently generate high-order harmonics due to its anharmonic charge-carrier dispersion, experiments performed on extended samples using THz illumination have revealed only a weak effect. The situation is further complicated by the enormous electromagnetic field intensities required by this highly nonperturbative nonlinear optical phenomenon. Here we argue that the large light intensity required for high-harmonic generation to occur can be reached by exploiting localized plasmons in doped graphene nanostructures. We demonstrate through rigorous time-domain simulations that the synergistic combination of strong plasmonic near-field enhancement and a pronounced intrinsic nonlinearity result in efficient broadband high-harmonic generation within a single material. Our results support the strong potential of nanostructured graphene as a robust, electrically tunable platform for high-harmonic generation.