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Status and challenges in enabling the lithium metal electrode for high-energy and low-cost rechargeable batteries

Paul Albertus, +3 more
- 02 Aug 2022 - 
- Vol. 3, Iss: 9, pp 16-21
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This article is published in Nature Energy.The article was published on 2022-08-02 and is currently open access. It has received 693 citations till now. The article focuses on the topics: Lithium (medication) & Electrode.

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Guidelines and trends for next-generation rechargeable lithium and lithium-ion batteries.

TL;DR: This review summarizes the current trends and provides guidelines towards achieving next-generation rechargeable Li and Li-ion batteries with higher energy densities, better safety characteristics, lower cost and longer cycle life by addressing batteries using high-voltage cathodes, metal fluoride electrodes, chalcogen electrodes, Li metal anodes, high-capacity anodes as well as useful electrolyte solutions.
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Recent Advances in Energy Chemistry between Solid-State Electrolyte and Safe Lithium-Metal Anodes

TL;DR: In this article, a review summarizes the issues generated by the marriage of Li-metal anodes and solid-state electrolytes, focusing on the large interfacial resistance, uncontrolled dendrite growth and low operation current or capacity.
Journal ArticleDOI

Benchmarking the performance of all-solid-state lithium batteries

TL;DR: All-solid-state batteries reduced to the bare minimum of compounds, containing only a lithium metal anode, β-Li 3 PS 4 solid electrolyte and Li(Ni 0.6 Co 0.2 Mn 0. 2 )O 2 cathode active material are presented.
References
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Journal ArticleDOI

The Li-ion rechargeable battery: a perspective.

TL;DR: New strategies are needed for batteries that go beyond powering hand-held devices, such as using electrode hosts with two-electron redox centers; replacing the cathode hosts by materials that undergo displacement reactions; and developing a Li(+) solid electrolyte separator membrane that allows an organic and aqueous liquid electrolyte on the anode and cathode sides, respectively.
Journal ArticleDOI

Lithium metal anodes for rechargeable batteries

TL;DR: In this article, various factors that affect the morphology and Coulombic efficiency of Li metal anodes have been analyzed, and the results obtained by modelling of Li dendrite growth have also been reviewed.
Journal ArticleDOI

Promise and reality of post-lithium-ion batteries with high energy densities

TL;DR: A review of post-lithium-ion batteries is presented in this paper with a focus on their operating principles, advantages and the challenges that they face, and the volumetric energy density of each battery is examined using a commercial pouch-cell configuration.
Journal ArticleDOI

High-power all-solid-state batteries using sulfide superionic conductors

TL;DR: Li9.54Si1.74P1.44S11.7Cl0.6P3S12 as discussed by the authors showed that Li 9.54 Si 1.54P 1.74Si 1.44 S11.3 has high specific power that is superior to that of conventional cells with liquid electrolytes.
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