Showing papers on "Synchrotron radiation published in 2005"

Hard x-ray nanoprobe based on refractive x-ray lenses

Abstract: Based on nanofocusing refractive x-ray lenses a hard x-ray scanning microscope is currently being developed and is being implemented at beamline ID13 of the European Synchrotron Radiation Facility (Grenoble, France). It can be operated in transmission, fluorescence, and diffraction mode. Tomographic scanning allows one to determine the inner structure of a specimen. In this device, a monochromatic (E=21keV) hard x-ray nanobeam with a lateral extension of 47×55nm2 was generated. Further reduction of the beam size to below 20 nm is targeted.

Review of third and next generation synchrotron light sources

Abstract: Synchrotron radiation (SR) is having a very large impact on interdisciplinary science and has been tremendously successful with the arrival of third generation synchrotron x-ray sources. But the revolution in x-ray science is still gaining momentum. Even though new storage rings are currently under construction, even more advanced rings are under design (PETRA III and the ultra high energy x-ray source) and the uses of linacs (energy recovery linac, x-ray free electron laser) can take us further into the future, to provide the unique synchrotron light that is so highly prized for today's studies in science in such fields as materials science, physics, chemistry and biology, for example. All these machines are highly reliant upon the consequences of Einstein's special theory of relativity. The consequences of relativity account for the small opening angle of synchrotron radiation in the forward direction and the increasing mass an electron gains as it is accelerated to high energy. These are familiar results to every synchrotron scientist. In this paper we outline not only the origins of SR but discuss how Einstein's strong character and his intuition and excellence have not only marked the physics of the 20th century but provide the foundation for continuing accelerator developments into the 21st century.

Klein-Nishina effects in the spectra of non-thermal sources immersed in external radiation fields

Abstract: We provide a systematic numerical and analytical study of Klein-Nishina (KN) effects in the spectrum produced by a steady-state, non-thermal source where rapidly accelerated electrons cool by emitting synchrotron radiation and Compton up-scattering ambient photons produced outside the source. We focus on the case where q, the ratio of the ambient radiation field to source magnetic field energy densities, significantly exceeds unity. We show that the KN reduction in the electron Compton cooling rate causes the steady-state electron spectrum to harden at energies γ? γ KN , where γ KN = 1/4∈ 0 and ∈ 0 = hv 0 /m e c 2 is the characteristic ambient photon energy. This hardening becomes noticeable in the synchrotron radiation from electrons with energies as low as 0.1 γ KN and changes the synchrotron spectral index relative to its Thomson limit value by as much as Aa ∼0.75 for q >> 1. The source synchrotron spectrum thus shows a high-energy 'bump' or excess, even though the electron acceleration spectrum has no such excess. In contrast, the low-energy Compton gamma-ray spectrum shows little distortion because the electron hardening compensates for the KN decline in the scattering rate. For sufficiently high electron energies, however, Compton cooling becomes so inefficient that synchrotron cooling dominates - an effect omitted in most previous studies. The hardening of the electron distribution thus stops, leading to a rapid decline in Compton gamma-ray emission, i.e. a strong spectral break whose location does not depend on the maximum electron energy. This break can limit the importance of Compton gamma-ray pair production on ambient photons and implies that a source's synchrotron luminosity may exceed its Compton luminosity even though q > 1. We discuss the importance of these KN effects in blazars, micro-quasars and pulsar binaries.

The interaction of relativistic particles with strong crystalline fields

Abstract: Crystals present a uniquely simple environment for the investigation of strong electromagnetic fields. When energetic charged particles are incident on crystals close to major crystallographic directions, their electromagnetic interactions depend crucially on the kinematic conditions. The coherence of the crystalline field can produce very strong electric fields in the rest frame of the particle, exceeding the so-called Schwinger field or quantum critical field. In that domain, the radiation emission takes a substantial part of the electron energy and the ``formation zone'' changes character. In this review the theory appropriate to the different kinematics domains is described, concentrating on the effects occurring at extreme fields. Properties discussed include strong field synchrotron radiation, channeling radiation, bremsstrahlung, and photon interactions. Applications are given to radiation sources, bending of particle beams, and sources of polarized GeV photons.

High-resolution three-dimensional imaging of flat objects by synchrotron-radiation computed laminography

Abstract: Computed laminography with synchrotron radiation is developed and carried out for three-dimensional imaging of flat, laterally extended objects with high spatial resolution. Particular experimental conditions of a stationary synchrotron source have been taken into account by a scanning geometry different from that employed with movable conventional laboratory x-ray sources. Depending on the mechanical precision of the sample manipulation system, high spatial resolution down to the scale of 1μm can be attained nondestructively, even for objects of large lateral size. Furthermore, high beam intensity and the parallel-beam geometry enables easy use of monochromatic radiation for optimizing contrast and reducing imaging artifacts. Simulations and experiments on a test object demonstrate the feasibility of the method. Application to the inspection of solder joints in a flip-chip bonded device shows the potential for quality assurance of microsystem devices.

Fast microtomography using high energy synchrotron radiation

Abstract: At the High Energy Beamline ID15A at the European Synchrotron Radiation Facility we have developed a fast three-dimensional x-ray microtomography system, which acquires a complete dataset in typically less than 10s. This unprecedented speed is achieved by combining a high efficiency phosphor screen, a reflecting microscope objective and a fast charge coupled device detector with the very intense high-energy white beam radiation provided by a wiggler source. The achieved spatial resolution is 2μm. The available x-ray energy spectrum spans from 20to250keV and can therefore be used for low and high Z materials. The spectrum can be modified by inserting different filters into the x-ray beam in order to optimize the signal-to-noise ratio and to avoid beam-hardening artifacts. Different phosphors with different energy sensitivity can be used. The very high speed allows in situ studies of systems evolving on the time scale of a few seconds or minutes. Three examples are given on sintering of metallic powders, so...

Particle Acceleration and Magnetic Field Generation in Electron-Positron Relativistic Shocks

Abstract: Shock acceleration is a ubiquitous phenomenon in astrophysical plasmas. Plasma waves and their associated instabilities (e.g., Buneman, Weibel, and other two-stream instabilities) created in collisionless shocks are responsible for particle (electron, positron, and ion) acceleration. Using a three-dimensional relativistic electromagnetic particle (REMP) code, we have investigated particle acceleration associated with a relativistic electron-positron jet front propagating into an ambient electron-positron plasma with and without initial magnetic fields. We find small differences in the results for no ambient and modest ambient magnetic fields. New simulations show that the Weibel instability created in the collisionless shock front accelerates jet and ambient particles both perpendicular and parallel to the jet propagation direction. Furthermore, the nonlinear fluctuation amplitudes of densities, currents, and electric and magnetic fields in the electron-positron shock are larger than those found in the electron-ion shock studied in a previous paper at a comparable simulation time. This comes from the fact that both electrons and positrons contribute to generation of the Weibel instability. In addition, we have performed simulations with different electron skin depths. We find that growth times scale inversely with the plasma frequency, and the sizes of structures created by tine Weibel instability scale proportionally to the electron skin depth. This is the expected result and indicates that the simulations have sufficient grid resolution. While some Fermi acceleration may occur at the jet front, the majority of electron and positron acceleration takes place behind the jet front and cannot be characterized as Fermi acceleration. The simulation results show that the Weibel instability is responsible for generating and amplifying nonuniform, small-scale magnetic fields, which contribute to the electron s (positron s) transverse deflection behind the jet head. This small- scale magnetic field structure is appropriate to the generation of "jitter" radiation from deflected electrons (positrons) as opposed to synchrotron radiation. The jitter radiation has different properties than synchrotron radiation calculated assuming a uniform magnetic field. The jitter radiation resulting from small-scale magnetic field structures may be important for understanding the complex time structure and spectral evolution observed in gamma-ray bursts or other astrophysical sources containing relativistic jets and relativistic collisionless shocks.

Quantitative analysis of magnetic excitations in Landau flux-closure structures using synchrotron-radiation microscopy.

Abstract: We have measured the excitation spectrum of six micron magnetic squares using x-ray magnetic circular dichroism. We observe all three excitations expected in a Landau flux-closure pattern. High temporal and spatial resolution allows quantitative analysis of the excitations. A short magnetic in plane pulse excites the magnetic element and we observe precessional motion of the magnetization within the domains as well as a domain wall mode and vortex motion. The vortex moves perpendicular to the excitation field and relaxes without showing a circulating orbit.

Will reduced radiation damage occur with very small crystals

Abstract: The primary event which occurs when an X-ray photon of energy less than 30 keV is absorbed in a protein crystal (or other organic material) is the production of a photoelectron with a similar energy to that of the absorbed photon. The electron then scatters inelastically off the surrounding material losing energy in the process. This reduction in energy takes place over track lengths of a few µm for 20 keV electrons. The vector distances between the initial and final positions of the photoelectrons are less than the track lengths owing to the non-linear tracks followed by the electrons. For crystals with smaller dimensions than the vector distances, a significant proportion of the energy could leave the crystal with the high-energy electrons. This could provide an advantage in terms of reduced radiation damage. In order to estimate the possible benefits, calculations of the electron tracks are given, initially using the continuous slowing-down approximation. A Monte Carlo approach is then used to provide more accurate values of the vector distance travelled by electrons inside a protein crystal. The calculations indicate that significant reductions in radiation damage could occur for crystals of a few µm in size. The benefits would be greater when operating at higher energies. In addition, a scheme for realising the possible benefits in a practical situation is described. This could then form the basis of trial experiments.

High-Energy Emission from Millisecond Pulsars

Abstract: The X-ray and gamma-ray spectrum of rotation-powered millisecond pulsars is investigated in a model for acceleration and pair cascades on open field lines above the polar caps. Although these pulsars have low surface magnetic fields, their short periods allow them to have large magnetospheric potential drops, but the majority do not produce sufficient pairs to completely screen the accelerating electric field. In these sources, the primary and secondary electrons continue to accelerate to high altitude and their Lorentz factors are limited by curvature and synchrotron radiation reaction. The accelerating particles maintain high Lorentz factors and undergo cyclotron resonant absorption of radio emission, that produces and maintains a large pitch angle, resulting in a strong synchrotron component. The resulting spectra consist of several distinct components: curvature radiation from primary electrons dominating from 1 - 100 GeV, synchrotron radiation from primary and secondary electrons dominating up to about 100 MeV, and much weaker inverse-Compton radiation from primary electrons a t 0.1 - 1 TeV. We find that the relative size of these components depends on pulsar period, period derivative, and neutron star mass and radius with the level of the synchrotron component also depending sensitively on the radio emission properties. This model is successful in describing the observed X-ray and gamma-ray spectrum of PSR J0218+4232 as synchrotron radiation, peaking around 100 MeV and extending up to a turnover around several GeV. The predicted curvature radiation components from a number of millisecond pulsars, as well as the collective emission from the millisecond pulsars in globular clusters, should be detectable with AGILE and GLAST. We also discuss a hidden population of X-ray-quiet and radio-quiet millisecond pulsars which have evolved below the pair death line, some of which may be detectable by telescopes sensitive above 1 GeV. Subject headings: pulsars: general - radiation mechanisms: nonthermal - stars: neutron - gamma rays: theory

X-ray free-electron lasers

Abstract: In a free-electron laser (FEL) the lasing medium is a high-energy beam of electrons flying with relativistic speed through a periodic magnetic field. The interaction between the synchrotron radiation that is produced and the electrons in the beam induces a periodic bunching of the electrons, greatly increasing the intensity of radiation produced at a particular wavelength. Depending only on a phase match between the electron energy and the magnetic period, the wavelength of the FEL radiation can be continuously tuned within a wide spectral range. The FEL concept can be adapted to produce radiation wavelengths from millimetres to Angstroms, and can in principle produce hard x-ray beams with unprecedented peak brightness, exceeding that of the brightest synchrotron source by ten orders of magnitude or more. This paper focuses on short-wavelength FELs. It reviews the physics and characteristic properties of single-pass FELs, as well as current technical developments aiming for fully coherent x-ray radiation pulses with pulse durations in the 100 fs to 100 as range. First experimental results at wavelengths around 100 nm and examples of scientific applications planned on the new, emerging x-ray FEL facilities are presented.

Spectra of Poynting-flux powered GRB outflows

Abstract: We investigate the production of the gamma-ray spectrum of a Poynting-flux dominated GRB outflow. The very high magnetic field strengths (super-equipartition) in such a flow lead to very efficient synchrotron emission. In contrast with internal shocks, dissipation of magnetic energy by reconnection is gradual and does not produce the spectrum of cooling electrons associated with shock acceleration. We show that a spectrum with a break in the BATSE energy range is produced, instead, if the magnetic dissipation heats a small (∼10 −4 ) population of electrons.

Superradiant and stimulated-superradiant emission in prebunched electron-beam radiators. I. Formulation

Abstract: A formulation for the characterization of superradiant and stimulated-superradiant radiative emission from bunched electron beams is presented. The radiation is characterized in terms of power and spectral power per radiation mode, which provide a measure of the useful spatially coherent radiation power and spectral power emitted by a radiation source. When the bunched electron beam emits superradiantly, these parameters scale like the square of the number of electrons, orders of magnitude more than spontaneous emission. The formulation applies to emission from single bunches, a finite number of bunches in a macropulse, or periodic bunching. It can be employed on any kind of $e$-beam radiation scheme. Specific analytic expressions are derived for coherent synchrotron radiation and prebunched free-electron laser, providing a basis for comparing and understanding their connection.

The Polarization of High-Energy Pulsar Radiation in the Striped Wind Model

Abstract: The Stokes parameters of the pulsed synchrotron radiation produced in the striped pulsar wind model are computed and compared with optical observations of the Crab pulsar. We assume that the main contribution to the wind emissivity comes from a thin transition layer where the dominant toroidal magnetic field reverses its polarity. The radial component of the field is neglected, but a small meridional component is added. The resulting radiation is linearly polarized (Stokes V = 0). In the off-pulse region, the electric vector lies in the direction of the projection on the sky of the rotation axis of the pulsar. This property is unique to the wind model and in good agreement with the data. Other properties such as a reduced degree of polarization and a characteristic sweep of the polarization angle within the pulses are also reproduced. These properties are qualitatively unaffected by variations of the wind Lorentz factor, the electron injection power-law index, and the inclination of the line of sight.

Quantification of Crystallinity in Substantially Amorphous Materials by Synchrotron X-ray Powder Diffractometry

Abstract: The aim of this study was to develop a highly sensitive powder X-ray diffraction (XRD) technique for quantification of crystallinity in substantially amorphous pharmaceuticals, utilizing synchrotron radiation and a 2-D area detector. Diffraction data were acquired at the European Synchrotron Radiation Facility (France) using a 2-D charge-coupled device detector. The crystallization of amorphous sucrose was monitored in situ, isothermally at several temperatures in the range of 90 to 160°C. An algorithm was developed for separation of the crystalline and amorphous intensities from the total diffraction pattern. The synchrotron XRD technique allowed powder diffraction patterns to be recorded with a time resolution of 40 ms. The gradual crystallization of sucrose is analogous to a series of physical mixtures with increasing content of the crystalline component. The in situ crystallization approach circumvented the problem of inhomogeneity in mixing—a potentially serious issue at extreme mixture compositions. The estimated limit of detection of crystalline sucrose in an amorphous matrix was 0.2% w/w, a considerable improvement over the reported value of ∼1% w/w with a conventional XRD. High-intensity XRD can discern subtle changes in the lattice order of materials. The first evidence of crystallization can serve as an indicator of the potential physical instability of the product.

Quantitative Rietveld texture analysis of zirconium from single synchrotron diffraction images

Abstract: Preferred orientation is immediately visible on synchrotron diffraction images as intensity variations along Debye rings. In this report, the Rietveld method is applied to obtain quantitative information about the orientation distribution from the analysis of a single synchrotron diffraction image. The method is illustrated for hexagonal cold-rolled zirconium, investigated in situ in a vacuum furnace with high-energy X-rays, both before and after the onset of recrystallization.

Studies of electronic excitations in MgMoO4, CaMoO4 and CdMoO4 crystals using VUV synchrotron radiation

Abstract: Reflection, emission and luminescence spectra of Czochralski grown molybdate crystals, i.e. MgMoO4, CaMoO4 and CdMoO4 have been investigated over a 8–295 K temperature range using VUV synchrotron radiation. Preliminary interpretation of the spectroscopic properties has been carried out on the basis of present knowledge of the electronic structure and emission properties of these materials. The results of this study support the conclusion that molybdate crystals have good prospect for application in the search for rare events as cryogenic phonon-scintillation detectors. (© 2005 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim)

Pointlike gamma ray sources as signatures of distant accelerators of ultrahigh energy cosmic rays.

Abstract: We discuss the possibility of observing distant accelerators of ultrahigh energy cosmic rays in synchrotron gamma rays. Protons propagating away from their acceleration sites produce extremely energetic electrons during photopion interactions with cosmic microwave background photons. If the accelerator is embedded in a magnetized region, these electrons will emit high energy synchrotron radiation. The resulting synchrotron source is expected to be pointlike, steady, and detectable in the GeV-TeV energy range if the magnetic field is at the nanoGauss level.

Polarization of high-energy pulsar radiation in the striped wind model

Abstract: The Stokes parameters of the pulsed synchrotron radiation produced in the striped pulsar wind model are computed and compared with optical observations of the Crab pulsar. We assume the main contribution to the wind emissivity comes from a thin transition layer where the dominant toroidal magnetic field reverses its polarity. The radial component of the field is neglected, but a small meridional component is added. The resulting radiation is linearly polarized (Stokes V=0). In the off-pulse region, the electric vector lies in the direction of the projection on the sky of the rotation axis of the pulsar. This property is unique to the wind model and in good agreement with the data. Other properties such as a reduced degree of polarization and a characteristic sweep of the polarization angle within the pulses are also reproduced. These properties are qualitatively unaffected by variations of the wind Lorentz factor, the electron injection power law index and the inclination of the line of sight.

Double-sided laser heating system for in situ high pressure–high temperature monochromatic x-ray diffraction at the esrf

Abstract: A new double-sided laser heating system optimized for monochromatic X-ray diffraction at high pressure and high temperature has been developed at beamline ID27 of the European Synchrotron Radiation Facility (ESRF). The main components of this system including optimized focusing optics to produce a large and homogenous heated area, optimized mirror optics for temperature measurements and a state-of-the-art diffraction setup are described in details. Preliminary data collected at high pressure and high temperature on tungsten and iron are presented.

Laser based synchrotron radiation

Abstract: Beams of x rays in the kiloelectronvolt energy range have been produced from laser-matter interaction. Here, energetic electrons are accelerated by a laser wakefield, and experience betatron oscillations in an ion channel formed in the wake of the intense femtosecond laser pulse. Experiments using a 50 TW laser (30 fs duration) are described, as well as comparisons with numerical simulations. These results pave the way of a new generation of radiation in the x-ray spectral range, with a high collimation and an ultrafast pulse duration, produced by the use of compact laser system.

Synchrotron radiation in biosciences

Abstract: The Center for Synchrotron Biosciences (CSB) operates five beamlines at the National Synchrotron Light Source (NSLS). Infrared (IR) micro-spectroscopy, X-ray absorption spectroscopy, structural proteomics and macromolecular footprinting are among the major technologies available through the Center. IR micro-spectroscopy is used to examine protein-folding in the microsecond time regime, image bone, neurons, seeds and other biological tissues, as well as image samples of interest in the chemical and environmental sciences. Structural proteomics research of New York Structural Genomics Research Consortium (NYSGRC) is steadily increasing the number of solved protein structures, with a goal to solve 100–200 structures per year. To speed up the research, a high-throughput method called ‘metallomics’ was implemented for NYSGRC crystallographers to detect intrinsic anomalous scatterers using X-ray absorption spectroscopy. Hydroxyl radical mediated X-ray footprinting is capable of resolving folding events of RNA, at single base resolution on millisecond timescales using a synchrotron white beam. The high brightness of synchrotron source is essential for CSB projects as it permits the use of smaller sample sizes and/or concentration, and allows studies of more complicated biological systems than with conventional sources.

Synchrotron Radiation Based Aerosol Time-of-Flight Mass Spectrometry for Organic Constituents

Abstract: A synchrotron radiation based aerosol time-of-flight mass spectrometer using tunable vacuum−ultraviolet (VUV) light is described for real-time analysis of organic compounds in ultrafine and large aerosol particles. Particles are sampled from atmospheric pressure and are focused through an aerodynamic lens assembly into the mass spectrometer. As the particles enter the source region, they impinge on a cartridge heater and are vaporized. The particle vapor expands back into the source region and is softly ionized with tunable, quasicontinuous VUV light generated with synchrotron radiation. The radiation can be tuned to an energy close to the ionization energy of the sample molecules, thus minimizing the complications resulting from ion fragmentation. Photoionization efficiency scans (photon scans) can be readily collected, which permit measurement of the molecule's ionization energy and fragmentation onsets. Four high molecular weight, low vapor pressure organic compounds of importance in atmospheric aeroso...

A refocusing modified velocity map imaging electron/ion spectrometer adapted to synchrotron radiation studies

Abstract: We present a modified velocity map imaging (VMI) spectrometer to be used in angle-resolved molecular photoionization studies in the gas phase with synchrotron radiation (SR) in the VUV/soft x-ray range The main modifications as compared to the original design of Eppink and Parker [A T J B Eppink and D H Parker, Rev Sci Instrum 68, 3477 (1997)] are an open repeller which allows the VMI spectrometer to be coupled to an independent dispersive electrostatic analyzer for combined operation in coincidence mode experiments, and the introduction of a coupled double Einzel lens in the flight tube in order to collect the full 4π solid angle for higher kinetic energy particles The length and position of the lenses have been optimized by a genetic algorithm to obtain the maximum kinetic energy possible without compromising the energy resolution Ray-tracing simulations and SR experiments show that the lenses can increase the kinetic energy bandwidth by a factor of up to 25 Furthermore, a remarkable impro

Synchrotron radiation from radiatively inefficient accretion flow simulations: applications to sagittarius a^*

Abstract: We calculate synchrotron radiation in three-dimensional pseudo-Newtonian magnetohydrodynamic simulations of radiatively inefficient accretion flows. We show that the emission is highly variable at optically thin frequencies, with order-of-magnitude variability on timescales as short as the orbital period near the last stable orbit; this emission is linearly polarized at the ~20%-50% level because of the coherent toroidal magnetic field in the flow. At optically thick frequencies, both the variability amplitude and polarization fraction decrease significantly with decreasing photon frequency. We argue that these results are broadly consistent with the observed properties of Sgr A* at the Galactic center, including the rapid infrared flaring.

Nanoelectron spectroscopy for chemical analysis: a novel energy filter for imaging x-ray photoemission spectroscopy

Abstract: An ovel instrument for imaging ESCA is described. It is based on a tandem arrangement of two hemispherical energy analysers used as an imaging energy filter. The main spherical aberration (α 2 -term) of the analyser is corrected by the antisymmetry of the tandem configuration. The kinetic energy range useable for imaging extends up to 1.6 keV; this is compatible with Mg and Al Kα laboratory x-ray sources. First experiments on the chemical surface composition of a Cu0.98Bi0.02 polycrystal, a GaAs/AlGaAs heterostructure and Ag crystallites on Si(111) have been performed using synchrotron radiation. The results reveal an energy resolutio no f190 meV and a lateral resolution (edge resolution) of 120 nm. Besides elimination of the analyser’s spherical aberration, the tandem arrangement largely retains the time structure of the electron signal, unlike a singl eh emispherical analyser.