Institution
Yanshan University
Education•Qinhuangdao, China•
About: Yanshan University is a education organization based out in Qinhuangdao, China. It is known for research contribution in the topics: Microstructure & Control theory. The organization has 19544 authors who have published 16904 publications receiving 184378 citations. The organization is also known as: Yānshān dàxué.
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TL;DR: The existence of the network equilibrium point is proved, and the expression of solution is given, and an inequality for the Caputo fractional derivative is improved, which plays central roles in the investigation of the global Mittag-Leffler stability.
80 citations
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TL;DR: The fabricated flexible all-solid-state supercapacitor (ASSP) device at the mass proportion of BP/CNTs 1:4 was found to deliver the highest volumetric capacitance, superior to the ASSP based on the bare graphene or BP.
Abstract: We proposed a simple route for fabrication of the flexible BP nanoflake/carbon nanotube (CNT) composite paper as flexible electrodes in all-solid-state supercapacitors. The highly conductive CNTs not only play a role as active materials but also increase conductivity of the hybrid electrode, enhance electrolyte shuttling and prevent the restacking between BP nanoflakes. The fabricated flexible all-solid-state supercapacitor (ASSP) device at the mass proportion of BP/CNTs 1:4 was found to deliver the highest volumetric capacitance of up to 41.1 F/cm3 at 0.005 V/s, superior to the ASSP based on the bare graphene or BP. The BP/CNTs (1:4) device delivers a rapid charging/discharging up to 500 V/s, which exhibits the characteristic of a high power density of 821.62 W/cm3, while having outstanding mechanical flexibility and high cycling stability over 10 000 cycles (91.5% capacitance retained). Moreover the BP/CNTs (1:4) ASSP device still retains large volumetric capacitance (35.7 F/cm3 at the scan rate of 0.00...
80 citations
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TL;DR: A complex system, which show intense circularly polarized ultraviolet luminescence (CPUVL) with large glum value, enabling a chiral UV light triggered enantioselective polymerization and paves the way for the further development of functional application of CPL active materials.
Abstract: Chiral optical materials based on circularly polarized luminescence (CPL) have emerged rapidly due to their feasible applications in diverse fields of research. However, limited to the small luminescence dissymmetry factor (glum), real application examples have rarely been reported. Here, we present a complex system, which show intense circularly polarized ultraviolet luminescence (CPUVL) with large glum value, enabling a chiral UV light triggered enantioselective polymerization. By integrating sensitized triplet-triplet annihilation upconversion and CPL, both visible-to-UV upconversion emission and upconverted circularly polarized ultraviolet luminescence (UC-CPUVL) were obtained in the systems, built of chiral annihilator R(S)-4,12-biphenyl[2,2]paracyclophane (R-/S-TP), and a thermally activated delayed fluorescence (TADF) sensitizer. After dispersing this upconversion system into room-temperature nematic liquid crystal, induced chiral nematic liquid crystal could significantly amplify the glum value (0.19) of UC-CPUVL. Further, the UC-CPUVL emission has been used to trigger the enantioselective photopolymerization of diacetylene. This work paves the way for the further development of functional application of CPL active materials. Chiral functional materials with circularly polarized luminescence can be used in various applications but rarely reported. Here the authors show, a complex system, which show intense circularly polarized ultraviolet luminescence with large glum value, enabling a chiral UV light triggered enantioselective polymerization.
80 citations
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TL;DR: In this paper, a rational design of cobalt-embedded nitrogen-doped hollow carbon microspheres (Co@N-HCMSs) as a multifunctional sulfur host for Li-S batteries was reported.
80 citations
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TL;DR: In this article, a high entropy concept is utilized to design an NiFeCoMnAl oxide with amorphous structure as an oxygen evolution reaction (OER) catalyst.
Abstract: The exploration of an efficient electrocatalyst for the oxygen evolution reaction (OER) is urgently required for sustainable renewable-energy conversion and storage. Due to the increased chemical complexity, multimetallic catalysts provide flexibility to alter their electronic and crystal structure to attain a superior intrinsic catalytic activity via synergistic effects, which is seldom accomplished using single metal catalysts. However, the high chemical complexity increases the difficulty to prepare elemental homogenous catalysts and reveal their synergistic effect during OER process, which further hinder the design of multimetallic catalysts. Here, high entropy concept is utilized to design an NiFeCoMnAl oxide with amorphous structure as OER catalyst. The direct evidence of active Ni sites is provided by the operando Raman measurements and Fe can modify oxygen intermediates binding energy on Ni sites. The X-ray photoelectron spectroscopy (XPS) and X-ray absorption spectroscopy (XAS) reveal that the incorporation of Mn can construct the electron-rich environment of active Ni center, and the relatively lower oxidation state of Ni facilitates the self-construction of β-NiOOH intermediates, which shows promoted OER activity as confirmed by density functional theory calculations. Doping Co can enhance the conductivity and doping Al leads to the formation of nanoporous structure through dealloying process, thus each component is essential for improving OER performance. The optimized NiFeCoMnAl catalyst exhibits an overpotential of 190 mV at 10 mA cm−2 in 1 M KOH solution, much superior to the ternary and quaternary counterparts. This work sheds light on understanding the origin of high entropy catalysts’ OER activity and thereby enables the rational design of multinary transition metallic catalysts.
80 citations
Authors
Showing all 19693 results
Name | H-index | Papers | Citations |
---|---|---|---|
Jian Yang | 142 | 1818 | 111166 |
Peng Shi | 137 | 1371 | 65195 |
Tao Zhang | 123 | 2772 | 83866 |
David Zhang | 111 | 1027 | 55118 |
Lei Liu | 98 | 2041 | 51163 |
Guoliang Li | 84 | 795 | 31122 |
Hao Yu | 81 | 981 | 27765 |
Jian Yu Huang | 81 | 339 | 26599 |
Chen Chen | 76 | 665 | 24846 |
Wei Jin | 71 | 929 | 21569 |
Xiaoli Li | 69 | 877 | 20690 |
K. L. Ngai | 64 | 412 | 15505 |
Zhiqiang Zhang | 60 | 595 | 16675 |
Hak-Keung Lam | 59 | 414 | 12890 |
Wei Wang | 58 | 229 | 14230 |