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Open AccessJournal ArticleDOI

Energy Transfer with Semiconductor Quantum Dot Bioconjugates: A Versatile Platform for Biosensing, Energy Harvesting, and Other Developing Applications.

TLDR
This work discusses how QDs are steadily revolutionizing the development of new biosensors along with a myriad of other photonically active nanomaterial-based bioconjugates, and how this field has grown over a relatively short time span.
Abstract
Luminescent semiconductor quantum dots (QDs) are one of the more popular nanomaterials currently utilized within biological applications. However, what is not widely appreciated is their growing role as versatile energy transfer (ET) donors and acceptors within a similar biological context. The progress made on integrating QDs and ET in biological configurations and applications is reviewed in detail here. The goal is to provide the reader with (1) an appreciation for what QDs are capable of in this context, (2) how this field has grown over a relatively short time span, and, in particular, (3) how QDs are steadily revolutionizing the development of new biosensors along with a myriad of other photonically active nanomaterial-based bioconjugates. An initial discussion of QD materials along with key concepts surrounding their preparation and bioconjugation is provided given the defining role these aspects play in the QDs ability to succeed in subsequent ET applications. The discussion is then divided around...

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Citations
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Journal ArticleDOI

Evolution and Synthesis of Carbon Dots: From Carbon Dots to Carbonized Polymer Dots

TL;DR: CPDs are revealed as an emerging class of CDs with distinctive polymer/carbon hybrid structures and properties, and critical insights into facilitating their potential in various application fields are proposed.
Journal ArticleDOI

Long-Lived Emissive Probes for Time-Resolved Photoluminescence Bioimaging and Biosensing

TL;DR: The design and applications of various kinds of long-lived emissive probes for bioimaging and biosensing via time-resolved photoluminescence techniques are summarized and the imaging contrast and sensing sensitivity are remarkably improved.
Journal ArticleDOI

Recent advances in dual-emission ratiometric fluorescence probes for chemo/biosensing and bioimaging of biomarkers

TL;DR: This review systematically summarizes the recent progress on dual-emission ratiometric FL probes and covers a wide range of scientific disciplines and benefits further development of functionalized optical materials, luminescent devices and bioimaging technique.
Journal Article

Resonant Energy Transfer from Individual Semiconductor Nanocrystals to Graphene

TL;DR: This study quantifies energy transfer to and fluorescence quenching by graphene, critical properties for novel applications in photovoltaic devices and as a molecular ruler.
References
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Journal ArticleDOI

Electrochemical Photolysis of Water at a Semiconductor Electrode

TL;DR: Water photolysis is investigated by exploiting the fact that water is transparent to visible light and cannot be decomposed directly, but only by radiation with wavelengths shorter than 190 nm.
Journal ArticleDOI

Semiconductor Nanocrystals as Fluorescent Biological Labels

TL;DR: Semiconductor nanocrystals prepared for use as fluorescent probes in biological staining and diagnostics have a narrow, tunable, symmetric emission spectrum and are photochemically stable.
Journal ArticleDOI

Synthesis and characterization of nearly monodisperse CdE (E = sulfur, selenium, tellurium) semiconductor nanocrystallites

TL;DR: In this paper, a simple route to the production of high-quality CdE (E=S, Se, Te) semiconductor nanocrystallites is presented, based on pyrolysis of organometallic reagents by injection into a hot coordinating solvent.
Journal ArticleDOI

The origins and the future of microfluidics

TL;DR: The manipulation of fluids in channels with dimensions of tens of micrometres — microfluidics — has emerged as a distinct new field that has the potential to influence subject areas from chemical synthesis and biological analysis to optics and information technology.
Journal ArticleDOI

A Theory of Sensitized Luminescence in Solids

TL;DR: In this article, the resonance theory of Forster, which involves only allowed transitions, is extended to include transfer by means of forbidden transitions which, it is concluded, are responsible for the transfer in all inorganic systems yet investigated.
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