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Showing papers by "ICFO – The Institute of Photonic Sciences published in 2015"


Journal ArticleDOI
21 Oct 2015-Nature
TL;DR: The data imply statistically significant rejection of the local-realist null hypothesis and could be used for testing less-conventional theories, and for implementing device-independent quantum-secure communication and randomness certification.
Abstract: More than 50 years ago, John Bell proved that no theory of nature that obeys locality and realism can reproduce all the predictions of quantum theory: in any local-realist theory, the correlations between outcomes of measurements on distant particles satisfy an inequality that can be violated if the particles are entangled. Numerous Bell inequality tests have been reported; however, all experiments reported so far required additional assumptions to obtain a contradiction with local realism, resulting in 'loopholes'. Here we report a Bell experiment that is free of any such additional assumption and thus directly tests the principles underlying Bell's inequality. We use an event-ready scheme that enables the generation of robust entanglement between distant electron spins (estimated state fidelity of 0.92 ± 0.03). Efficient spin read-out avoids the fair-sampling assumption (detection loophole), while the use of fast random-basis selection and spin read-out combined with a spatial separation of 1.3 kilometres ensure the required locality conditions. We performed 245 trials that tested the CHSH-Bell inequality S ≤ 2 and found S = 2.42 ± 0.20 (where S quantifies the correlation between measurement outcomes). A null-hypothesis test yields a probability of at most P = 0.039 that a local-realist model for space-like separated sites could produce data with a violation at least as large as we observe, even when allowing for memory in the devices. Our data hence imply statistically significant rejection of the local-realist null hypothesis. This conclusion may be further consolidated in future experiments; for instance, reaching a value of P = 0.001 would require approximately 700 trials for an observed S = 2.4. With improvements, our experiment could be used for testing less-conventional theories, and for implementing device-independent quantum-secure communication and randomness certification.

2,397 citations


Journal ArticleDOI
TL;DR: A Bell test is reported that closes the most significant of loopholes that provide loopholes for a local realist explanation of quantum mechanics, using a well-optimized source of entangled photons, rapid setting generation, and highly efficient superconducting detectors.
Abstract: Local realism is the worldview in which physical properties of objects exist independently of measurement and where physical influences cannot travel faster than the speed of light. Bell's theorem states that this worldview is incompatible with the predictions of quantum mechanics, as is expressed in Bell's inequalities. Previous experiments convincingly supported the quantum predictions. Yet, every experiment requires assumptions that provide loopholes for a local realist explanation. Here, we report a Bell test that closes the most significant of these loopholes simultaneously. Using a well-optimized source of entangled photons, rapid setting generation, and highly efficient superconducting detectors, we observe a violation of a Bell inequality with high statistical significance. The purely statistical probability of our results to occur under local realism does not exceed 3.74×10^{-31}, corresponding to an 11.5 standard deviation effect.

1,262 citations


Journal ArticleDOI
TL;DR: In this paper, the authors present a loophole-free violation of local realism using entangled photon pairs, ensuring that all relevant events in their Bell test are spacelike separated by placing the parties far enough apart and by using fast random number generators and high-speed polarization measurements.
Abstract: We present a loophole-free violation of local realism using entangled photon pairs. We ensure that all relevant events in our Bell test are spacelike separated by placing the parties far enough apart and by using fast random number generators and high-speed polarization measurements. A high-quality polarization-entangled source of photons, combined with high-efficiency, low-noise, single-photon detectors, allows us to make measurements without requiring any fair-sampling assumptions. Using a hypothesis test, we compute p values as small as 5.9×10^{-9} for our Bell violation while maintaining the spacelike separation of our events. We estimate the degree to which a local realistic system could predict our measurement choices. Accounting for this predictability, our smallest adjusted p value is 2.3×10^{-7}. We therefore reject the hypothesis that local realism governs our experiment.

1,201 citations


Journal ArticleDOI
TL;DR: This work demonstrates the usefulness of the approach by proving that the fidelity-based geometric measure of coherence is a full convex coherence monotone, and deriving a closed formula for it on arbitrary single-qubit states.
Abstract: Quantum coherence is an essential ingredient in quantum information processing and plays a central role in emergent fields such as nanoscale thermodynamics and quantum biology. However, our understanding and quantitative characterization of coherence as an operational resource are still very limited. Here we show that any degree of coherence with respect to some reference basis can be converted to entanglement via incoherent operations. This finding allows us to define a novel general class of measures of coherence for a quantum system of arbitrary dimension, in terms of the maximum bipartite entanglement that can be generated via incoherent operations applied to the system and an incoherent ancilla. The resulting measures are proven to be valid coherence monotones satisfying all the requirements dictated by the resource theory of quantum coherence. We demonstrate the usefulness of our approach by proving that the fidelity-based geometric measure of coherence is a full convex coherence monotone, and deriving a closed formula for it on arbitrary single-qubit states. Our work provides a clear quantitative and operational connection between coherence and entanglement, two landmark manifestations of quantum theory and both key enablers for quantum technologies.

753 citations


Journal ArticleDOI
TL;DR: In this paper, an overview of the interplay between quantum information theory and thermodynamics of quantum systems is presented. But this is not a comprehensive review of the diverse field of quantum thermodynamics; rather, it is a convenient entry point for the thermo-curious information theorist.
Abstract: This topical review article gives an overview of the interplay between quantum information theory and thermodynamics of quantum systems. We focus on several trending topics including the foundations of statistical mechanics, resource theories, entanglement in thermodynamic settings, fluctuation theorems and thermal machines. This is not a comprehensive review of the diverse field of quantum thermodynamics; rather, it is a convenient entry point for the thermo-curious information theorist. Furthermore this review should facilitate the unification and understanding of different interdisciplinary approaches emerging in research groups around the world.

517 citations


Journal ArticleDOI
TL;DR: This work reports on highly stable and high-performance monolayer and bilayer MoS2 photodetectors encapsulated with atomic layer deposited hafnium oxide, showing enhanced electronic properties by isolating them from the ambience as strong n-type doping, vanishing hysteresis, and reduced device resistance.
Abstract: Semiconducting, two-dimensional molybdenum disulfide (MoS2) is considered a promising new material for highly sensitive photodetection, because of its atomically thin profile and favorable bandgap. However, reported photodetectors to date show strong variation in performance due to the detrimental and uncontrollable effects of environmental adsorbates on devices due to large surface to volume ratio. Here, we report on highly stable and high-performance monolayer and bilayer MoS2 photodetectors encapsulated with atomic layer deposited hafnium oxide. The protected devices show enhanced electronic properties by isolating them from the ambience as strong n-type doping, vanishing hysteresis, and reduced device resistance. By controlling the gate voltage the responsivity and temporal response can be tuned by several orders of magnitude with R ∼ 10-10(4) A/W and t ∼ 10 ms to 10 s. At strong negative gate voltage, the detector is operated at higher speed and simultaneously exhibits a low-bound, record sensitivity of D* ≥ 7.7 × 10(11) Jones. Our results lead the way for future application of ultrathin, flexible, and high-performance MoS2 detectors and prompt for further investigation in encapsulated transition metal dichalcogenide optoelectronics.

509 citations


Journal ArticleDOI
TL;DR: In this article, the authors presented a compact source that generates sub-two-cycle-duration pulses with an average power of 0.1μm and a spectral coverage of 6.8-16.4μm.
Abstract: A compact source that generates sub-two-cycle-duration pulses with an average power of 0.1 W spanning 6.8–16.4 μm combines the properties of power scalability, high repetition rate and phase coherence for the first time in this spectral region. Powerful coherent light with a spectrum spanning the mid-infrared (MIR) spectral range is crucial for a number of applications in natural as well as life sciences, but so far has only been available from large-scale synchrotron sources1. Here we present a compact apparatus that generates pulses with a sub-two-cycle duration and with an average power of 0.1 W and a spectral coverage of 6.8–16.4 μm (at −30 dB). The demonstrated source combines, for the first time in this spectral region, a high power, a high repetition rate and phase coherence. The MIR pulses emerge via difference-frequency generation (DFG) driven by the nonlinearly compressed pulses of a Kerr-lens mode-locked ytterbium-doped yttrium–aluminium–garnet (Yb:YAG) thin-disc oscillator. The resultant 100 MHz MIR pulse train is hundreds to thousands of times more powerful than state-of-the-art frequency combs that emit in this range2,3,4, and offers a high dynamic range for spectroscopy in the molecular fingerprint region4,5,6,7 and an ideal prerequisite for hyperspectral imaging8 as well as for the time-domain coherent control of vibrational dynamics9,10,11.

238 citations


Journal ArticleDOI
TL;DR: An on-chip ultrafast photodetector based on a two-dimensional heterostructure consisting of high-quality graphene encapsulated in hexagonal boron nitride that enables optical on- chip autocorrelation measurements with picosecond-scale timing resolution and exceptionally low peak powers.
Abstract: Graphene and other two-dimensional (2D) materials have emerged as promising materials for broadband and ultrafast photodetection and optical modulation These optoelectronic capabilities can augment complementary metal–oxide–semiconductor (CMOS) devices for high-speed and low-power optical interconnects Here, we demonstrate an on-chip ultrafast photodetector based on a two-dimensional heterostructure consisting of high-quality graphene encapsulated in hexagonal boron nitride Coupled to the optical mode of a silicon waveguide, this 2D heterostructure-based photodetector exhibits a maximum responsivity of 036 A/W and high-speed operation with a 3 dB cutoff at 42 GHz From photocurrent measurements as a function of the top-gate and source-drain voltages, we conclude that the photoresponse is consistent with hot electron mediated effects At moderate peak powers above 50 mW, we observe a saturating photocurrent consistent with the mechanisms of electron–phonon supercollision cooling This nonlinear photore

193 citations


Journal ArticleDOI
TL;DR: It is observed that when an Al nanocrystal is coupled to an underlying Al film, its dipolar plasmon resonance linewidth narrows remarkably and shows an enhanced scattering efficiency, which provides a new mechanism for narrowing plAsmon resonances in aluminum-based systems.
Abstract: Aluminum nanocrystals and fabricated nanostructures are emerging as highly promising building blocks for plasmonics in the visible region of the spectrum. Even at the individual nanocrystal level, however, the localized plasmons supported by Al nanostructures possess a surprisingly broad spectral response. We have observed that when an Al nanocrystal is coupled to an underlying Al film, its dipolar plasmon resonance linewidth narrows remarkably and shows an enhanced scattering efficiency. This behavior is observable in other plasmonic metals, such as gold; however, it is far more dramatic in the aluminum nanoparticle-film system, reducing the dipolar plasmon linewidth by more than half. A substrate-mediated hybridization of the dipolar and quadrupolar plasmons of the nanoparticle reduces the radiative losses of the dipolar plasmon. While this is a general effect that applies to all metallic nanoparticle-film systems, this finding specifically provides a new mechanism for narrowing plasmon resonances in aluminum-based systems, quite possibly expanding the potential of Al-based plasmonics in real-world applications.

148 citations


Journal ArticleDOI
TL;DR: In this paper, a generalized "input-output" formalism is proposed for quantum information processing with photons or quantum many-body states of light, but treating such systems generally remains a difficult task theoretically.
Abstract: There has been rapid development of systems that yield strong interactions between freely propagating photons in one-dimension via controlled coupling to quantum emitters. This raises interesting possibilities such as quantum information processing with photons or quantum many-body states of light, but treating such systems generally remains a difficult task theoretically. Here, we describe a novel technique in which the dynamics and correlations of a few photons can be exactly calculated, based upon knowledge of the initial photonic state and the solution of the reduced effective dynamics of the quantum emitters alone. We show that this generalized 'input–output' formalism allows for a straightforward numerical implementation regardless of system details, such as emitter positions, external driving, and level structure. As a specific example, we apply our technique to show how atomic systems with infinite-range interactions and under conditions of electromagnetically induced transparency enable the selective transmission of correlated multi-photon states.

135 citations


Journal ArticleDOI
TL;DR: In this paper, a generalized "input-output" formalism is proposed to calculate the dynamics and correlations of a few photons, based upon knowledge of the initial photonic state and the solution of the reduced effective dynamics of the quantum emitters alone.
Abstract: There has been rapid development of systems that yield strong interactions between freely propagating photons in one dimension via controlled coupling to quantum emitters. This raises interesting possibilities such as quantum information processing with photons or quantum many-body states of light, but treating such systems generally remains a difficult task theoretically. Here, we describe a novel technique in which the dynamics and correlations of a few photons can be exactly calculated, based upon knowledge of the initial photonic state and the solution of the reduced effective dynamics of the quantum emitters alone. We show that this generalized "input-output" formalism allows for a straightforward numerical implementation regardless of system details, such as emitter positions, external driving, and level structure. As a specific example, we apply our technique to show how atomic systems with infinite-range interactions and under conditions of electromagnetically induced transparency enable the selective transmission of correlated multi-photon states.

Journal ArticleDOI
TL;DR: This work provides a hierarchy of sufficient conditions for the steerability of bipartite quantum states of any dimension, including continuous variable states, and provides a systematic framework to analytically derive nonlinear steering criteria.
Abstract: Einstein-Podolsky-Rosen steering is a manifestation of quantum correlations exhibited by quantum systems that allows for entanglement certification when one of the subsystems is not characterized. Detecting the steerability of quantum states is essential to assess their suitability for quantum information protocols with partially trusted devices. We provide a hierarchy of sufficient conditions for the steerability of bipartite quantum states of any dimension, including continuous variable states. Previously known steering criteria are recovered as special cases of our approach. The proposed method allows us to derive optimal steering witnesses for arbitrary families of quantum states and provides a systematic framework to analytically derive nonlinear steering criteria. We discuss relevant examples and, in particular, provide an optimal steering witness for a lossy single-photon Bell state; the witness can be implemented just by linear optics and homodyne detection and detects steering with a higher loss tolerance than any other known method. Our approach is readily applicable to multipartite steering detection and to the characterization of joint measurability.

Journal ArticleDOI
TL;DR: In this article, the authors exploit the high contrast in the optical properties of the phase change material Ge2Sb2Te5 to control the propagation of surface plasmon polaritons at a Au/SiO2 interface.
Abstract: The ability to manipulate light propagation at the nanoscale is of vital importance for future integrated photonic circuits. In this work we exploit the high contrast in the optical properties of the phase change material Ge2Sb2Te5 to control the propagation of surface plasmon polaritons at a Au/SiO2 interface. Using grating couplers, normally incident light at λ = 1.55 μm is converted into propagating surface plasmons on a Au waveguide. Single laser pulses (λ = 975 nm) are applied to a thin film of Ge2Sb2Te5 placed on top of the device, which, upon transition from its amorphous to crystalline structural phase, dramatically increases both its refractive index and absorption coefficient, thus inhibiting propagation of the plasmonic mode. This effect is investigated for different interaction lengths between the phase change material and the Au waveguide, and contrast values in the transmitted intensity up to several tens of percents are demonstrated.

Journal ArticleDOI
TL;DR: The electron-fed optical antennas described here are critical devices for interfacing electrons and photons, enabling thus the development of optical transceivers for on-chip wireless broadcasting of information at the nanoscale.
Abstract: Nanoscale electronics and photonics are among the most promising research areas providing functional nanocomponents for data transfer and signal processing. By adopting metal-based optical antennas...

Journal ArticleDOI
TL;DR: This work proposes a powerful ansatz for the one-dimensional Fermi gas in a harmonic potential near the limit of infinite short-range repulsion, and shows that the classical Pascal’s triangle emerges in the expression for the ground-state wave function.
Abstract: A major challenge in modern physics is to accurately describe strongly interacting quantum many-body systems. One-dimensional systems provide fundamental insights because they are often amenable to exact methods. However, no exact solution is known for the experimentally relevant case of external confinement. We propose a powerful ansatz for the one-dimensional Fermi gas in a harmonic potential near the limit of infinite short-range repulsion. For the case of a single impurity in a Fermi sea, we show that our ansatz is indistinguishable from numerically exact results in both the few- and many-body limits. We furthermore derive an effective Heisenberg spin-chain model corresponding to our ansatz, valid for any spin-mixture, within which we obtain the impurity eigenstates analytically. In particular, the classical Pascal’s triangle emerges in the expression for the ground-state wave function. As well as providing an important benchmark for strongly correlated physics, our results are relevant for emerging quantum technologies, where a precise knowledge of one-dimensional quantum states is paramount.

Journal ArticleDOI
TL;DR: It is demonstrated extraction of randomness from spontaneous-emission events less than 36 ns in the past, giving output bits with excess predictability below 10-5 and strong metrological randomness assurances.
Abstract: We demonstrate extraction of randomness from spontaneous-emission events less than 36 ns in the past, giving output bits with excess predictability below 10^{-5} and strong metrological randomness assurances. This randomness generation strategy satisfies the stringent requirements for unpredictable basis choices in current "loophole-free Bell tests" of local realism [Hensen et al., Nature (London) 526, 682 (2015); Giustina et al., this issue, Phys. Rev. Lett. 115, 250401 (2015); Shalm et al., preceding Letter, Phys. Rev. Lett. 115, 250402 (2015)].

Journal ArticleDOI
TL;DR: In this paper, the authors introduce the concept of total correlations, a concept from quantum information theory capturing multipartite correlations, to the study of many-body localization (MBL) and demonstrate that the total correlations of the diagonal ensemble provides a meaningful diagnostic tool to pin-down, probe, and better understand the MBL transition and ergodicity breaking in quantum systems.
Abstract: The intriguing phenomenon of many-body localization (MBL) has attracted significant interest recently, but a complete characterization is still lacking. In this work we introduce the total correlations, a concept from quantum information theory capturing multipartite correlations, to the study of this phenomenon. We demonstrate that the total correlations of the diagonal ensemble provides a meaningful diagnostic tool to pin-down, probe, and better understand the MBL transition and ergodicity breaking in quantum systems. In particular, we show that the total correlations has sublinear dependence on the system size in delocalized, ergodic phases, whereas we find that it scales extensively in the localized phase developing a pronounced peak at the transition. We exemplify the power of our approach by means of an exact diagonalization study of a Heisenberg spin chain in a disordered field. By a finite size scaling analysis of the peak position and crossover point from log to linear scaling we collect evidence that ergodicity is broken before the MBL transition in this model.

Journal ArticleDOI
TL;DR: In this paper, a TiO2-Ag-ITO (TAI)-based TE is introduced and its use is demonstrated in an inverted polymer solar cell (I-PSCs).
Abstract: Transparent electrodes (TEs) having electrooptical trade-offs better than state-of-the-art indium tin oxide (ITO) are continuously sought as they are essential to enable flexible electronic and optoelectronic devices. In this work, a TiO2-Ag-ITO (TAI)-based TE is introduced and its use is demonstrated in an inverted polymer solar cell (I-PSCs). Thanks to the favorable nucleation and wetting conditions provided by the TiO2, the ultrathin silver film percolates and becomes continuous with high smoothness at very low thicknesses (3–4 nm), much lower than those required when it is directly deposited on a plastic or glass substrate. Compared to conventional ITO-TE, the proposed TAI-TE exhibits exceptionally lower electrical sheet resistance (6.2 Ω sq−1), higher optical transmittance, a figure-of-merit two times larger, and mechanical flexibility, the latter confirmed by the fact that the resistance increases only 6.6% after 103 tensile bending cycles. The I-PSCs incorporating the TAI-TE show record power conversion efficiency (8.34%), maintained at 96% even after 400 bending cycles.

Journal ArticleDOI
TL;DR: This work establishes a rigorous connection between fundamental resource theories at the quantum scale, and considers the generation of genuine quantum correlations, focusing on the fundamental constituents of the authors' universe: fermions and bosons, and finds the optimal entangling protocol.
Abstract: We establish a rigorous connection between fundamental resource theories at the quantum scale Correlations and entanglement constitute indispensable resources for numerous quantum information tasks However, their establishment comes at the cost of energy, the resource of thermodynamics, and is limited by the initial entropy Here, the optimal conversion of energy into correlations is investigated Assuming the presence of a thermal bath, we establish general bounds for arbitrary systems and construct a protocol saturating them The amount of correlations, quantified by the mutual information, can increase at most linearly with the available energy, and we determine where the linear regime breaks down We further consider the generation of genuine quantum correlations, focusing on the fundamental constituents of our universe: fermions and bosons For fermionic modes, we find the optimal entangling protocol For bosonic modes, we show that while Gaussian operations can be outperformed in creating entanglement, their performance is optimal for high energies

Journal ArticleDOI
TL;DR: In this paper, the authors propose a related approach for the resource theory of quantum coherence, where two distant parties can only perform measurements which do not create coherence and can communicate their outcomes via a classical channel.
Abstract: The search for a simple description of fundamental physical processes is an important part of quantum theory. One example for such an abstraction can be found in the distance lab paradigm: if two separated parties are connected via a classical channel, it is notoriously difficult to characterize all possible operations these parties can perform. This class of operations is widely known as local operations and classical communication (LOCC). Surprisingly, the situation becomes comparably simple if the more general class of separable operations is considered, a finding which has been extensively used in quantum information theory for many years. Here, we propose a related approach for the resource theory of quantum coherence, where two distant parties can only perform measurements which do not create coherence and can communicate their outcomes via a classical channel. We call this class local incoherent operations and classical communication (LICC). While the characterization of this class is also difficult in general, we show that the larger class of separable incoherent operations (SI) has a simple mathematical form, yet still preserving the main features of LICC. We demonstrate the relevance of our approach by applying it to three different tasks: assisted coherence distillation, quantum teleportation, and single-shot quantum state merging. We expect that the results obtained in this work also transfer to other concepts of coherence which are discussed in recent literature. The approach presented here opens new ways to study the resource theory of coherence in distributed scenarios.

Journal ArticleDOI
TL;DR: In this paper, the authors predict unity-order changes in the transmission and absorption of vis-NIR light produced upon electrical doping of graphene sheets coupled to realistically engineered optical cavities.
Abstract: Fast modulation and switching of light at visible and near-infrared (vis-NIR) frequencies is of utmost importance for optical signal processing and sensing technologies. No fundamental limit appears to prevent us from designing wavelength-sized devices capable of controlling the light phase and intensity at gigaherts (and even terahertz) speeds in those spectral ranges. However, this problem remains largely unsolved, despite recent advances in the use of quantum wells and phase-change materials for that purpose. Here, we explore an alternative solution based upon the remarkable electro-optical properties of graphene. In particular, we predict unity-order changes in the transmission and absorption of vis-NIR light produced upon electrical doping of graphene sheets coupled to realistically engineered optical cavities. The light intensity is enhanced at the graphene plane, and so is its absorption, which can be switched and modulated via Pauli blocking through varying the level of doping. Specifically, we explore dielectric planar cavities operating under either tunneling or Fabry-Perot resonant transmission conditions, as well as Mie modes in silicon nanospheres and lattice resonances in metal particle arrays. Our simulations reveal absolute variations in transmission exceeding 90% as well as an extinction ratio >15 dB with small insertion losses using feasible material parameters, thus supporting the application of graphene in fast electro-optics at vis-NIR frequencies.

Journal ArticleDOI
TL;DR: In this paper, a partially-parity-time (pPT)-symmetric azimuthal potentials composed from individual PT-sparse cells located on a ring were introduced, and the vortex solitons in these potential excitations were shown to exhibit qualitatively different internal current distributions.
Abstract: We introduce partially-parity-time (pPT)-symmetric azimuthal potentials composed from individual PT-symmetric cells located on a ring, where two azimuthal directions are nonequivalent in a sense that in such potential excitations carrying topological dislocations exhibit different dynamics for different directions of energy circulation in the initial field distribution. Such nonconservative ratchetlike structures support rich families of stable vortex solitons in cubic nonlinear media, whose properties depend on the sign of the topological charge due to the nonequivalence of azimuthal directions. In contrast, oppositely charged vortex solitons remain equivalent in similar fully-PT-symmetric potentials. The vortex solitons in the pPT- and PT-symmetric potentials are shown to feature qualitatively different internal current distributions, which are described by different discrete rotation symmetries of the intensity profiles.

Journal ArticleDOI
TL;DR: In this article, a mobile optical trap operated under feedback control enables cooling and long range 3D manipulation of a silica nanoparticle in high vacuum by loading a single particle into a high-finesse optical cavity through a load-lock vacuum system.
Abstract: Accurate delivery of small targets in high vacuum is a pivotal task in many branches of science and technology Beyond the different strategies developed for atoms, proteins, macroscopic clusters, and pellets, the manipulation of neutral particles over macroscopic distances still poses a formidable challenge Here, we report an approach based on a mobile optical trap operated under feedback control that enables cooling and long range 3D manipulation of a silica nanoparticle in high vacuum We apply this technique to load a single nanoparticle into a high-finesse optical cavity through a load-lock vacuum system We foresee our scheme to benefit the field of optomechanics with levitating nano-objects as well as ultrasensitive detection and monitoring

Journal ArticleDOI
TL;DR: It is demonstrated that systems containing only a few bosons are an ideal setting in which to realize the highly sought-after itinerant ferromagnetic phase.
Abstract: We consider two species of bosons in one dimension near the Tonks-Girardeau limit of infinite interactions. For the case of equal masses and equal intraspecies interactions, the system can be mapped to a $S=1/2$ $XXZ$ Heisenberg spin chain, thus allowing one to access different magnetic phases. Using a powerful ansatz developed for the two-component Fermi system, we elucidate the evolution from few to many particles for the experimentally relevant case of an external harmonic confinement. In the few-body limit, we already find clear evidence of both ferromagnetic and antiferromagnetic spin correlations as the ratio of intraspecies and interspecies interactions is varied. Furthermore, we observe the rapid emergence of symmetry-broken magnetic ground states as the particle number is increased. We therefore demonstrate that systems containing only a few bosons are an ideal setting in which to realize the highly sought-after itinerant ferromagnetic phase.

Journal ArticleDOI
TL;DR: It is shown that a single quantum emitter can efficiently couple to the tunable plasmons of a highly doped single-wall carbon nanotube (SWCNT) and the coupling efficiency close to 100% over a very broad spectral range.
Abstract: We show that a single quantum emitter can efficiently couple to the tunable plasmons of a highly doped single-wall carbon nanotube (SWCNT). Plasmons in these quasi-one-dimensional carbon structures exhibit deep subwavelength confinement that pushes the coupling efficiency close to 100% over a very broad spectral range. This phenomenon takes place for distances and tube diameters comprising the nanometer and micrometer scales. In particular, we find a β factor ≈1 for QEs placed 1-100 nm away from SWCNTs that are just a few nanometers in diameter, while the corresponding Purcell factor exceeds 10(6).

Journal ArticleDOI
TL;DR: In this paper, the authors exploit the strong per-photon fields associated with tightly confined graphene plasmons in combination with spatially nonlocal nonlinear optical interactions to achieve strong second-order nonlinearities.
Abstract: Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other quantum emitters, while the possibility of achieving strong second-order nonlinearities remains unexplored. Here, we describe a novel technique to realize such nonlinearities using graphene, exploiting the strong per-photon fields associated with tightly confined graphene plasmons in combination with spatially nonlocal nonlinear optical interactions. We show that in properly designed graphene nanostructures, these conditions enable extremely strong internal down-conversion between a single quantized plasmon and an entangled plasmon pair, or the reverse process of second harmonic generation. A separate issue is how such strong internal nonlinearities can be observed, given the nominally weak coupling between these plasmon resonances and free-space radiative fields. On one hand, by using the collective coupling to radiation of nanostructure arrays, we show that the internal nonlinearities can manifest themselves as efficient frequency conversion of radiative fields at extremely low input powers. On the other hand, the development of techniques to efficiently couple to single nanostructures would allow these nonlinear processes to occur at the level of single input photons.

Journal ArticleDOI
TL;DR: In this paper, the authors generalize the previous results by demonstrating that one can construct self-testing protocols based on the chained Bell inequalities, defined for two devices implementing an arbitrary number of two-output measurements.
Abstract: Self testing is a device-independent technique based on non-local correlations whose aim is to certify the effective uniqueness of the quantum state and measurements needed to produce these correlations. It is known that the maximal violation of some Bell inequalities suffices for this purpose. However, most of the existing self-testing protocols for two devices exploit the well-known Clauser-Horne-Shimony-Holt Bell inequality or modifications of it, and always with two measurements per party. Here, we generalize the previous results by demonstrating that one can construct self-testing protocols based on the chained Bell inequalities, defined for two devices implementing an arbitrary number of two-output measurements. On the one hand, this proves that the quantum state and measurements leading to the maximal violation of the chained Bell inequality are unique. On the other hand, in the limit of a large number of measurements, our approach allows one to self-test the entire plane of measurements spanned by the Pauli matrices X and Z. Our results also imply that the chained Bell inequalities can be used to certify two bits of perfect randomness.

Journal ArticleDOI
TL;DR: This work considers quantum nondemolition measurements applied to atomic ensembles undergoing magnetically driven coherent oscillation and identifies measurement schemes requiring only Gaussian states as inputs and giving a significant LGI violation with realistic experimental parameters and imperfections.
Abstract: We show how a test of macroscopic realism based on Leggett-Garg inequalities (LGIs) can be performed in a macroscopic system. Using a continuous-variable approach, we consider quantum nondemolition (QND) measurements applied to atomic ensembles undergoing magnetically driven coherent oscillation. We identify measurement schemes requiring only Gaussian states as inputs and giving a significant LGI violation with realistic experimental parameters and imperfections. The predicted violation is shown to be due to true quantum effects rather than to a classical invasivity of the measurement. Using QND measurements to tighten the "clumsiness loophole" forces the stubborn macrorealist to recreate quantum backaction in his or her account of measurement.

Journal ArticleDOI
TL;DR: In this article, the authors employed ab initio methods of quantum chemistry to investigate spin-1/2 fermions interacting via a two-body contact potential in a one-dimensional harmonic trap.
Abstract: We employ ab initio methods of quantum chemistry to investigate spin-1/2 fermions interacting via a two-body contact potential in a one-dimensional harmonic trap. The convergence of the total energy with the size of the one-particle basis set is analytically investigated for the two-body problem and the same form of the convergence formula is numerically confirmed to be valid for the many-body case. Benchmark calculations for two to six fermions with the full configuration interaction method equivalent to the exact diagonalization approach, and the coupled cluster (CC) method including single, double, triple, and quadruple excitations are presented. The convergence of the correlation energy with the level of excitations included in the CC model is analyzed. The range of the interaction strength for which single-reference CC methods work is examined. Next, the CC method restricted to single, double, and noniterative triple excitations, CCSD(T), is employed to study a two-component Fermi gas composed of 6–80 atoms in a one-dimensional harmonic trap. The density profiles of trapped atomic clouds are also reported. Finally, a comparison with experimental results for few-fermion systems is presented. Upcoming possible applications and extensions of the presented approach are discussed.

Journal ArticleDOI
TL;DR: In this article, the authors investigate an alternative approach, in which atomic interactions arise via their common coupling to photonic crystal waveguides, taking advantage of the ability to separately tailor the strength and range of interactions via the dispersion engineering of the structure itself.
Abstract: Realizing systems that support robust, controlled interactions between individual photons is an exciting frontier of nonlinear optics. To this end, one approach that has emerged recently is to leverage atomic interactions to create strong and spatially non-local interactions between photons. In particular, effective interactions have been successfully created via interactions between atoms excited to Rydberg levels. Here, we investigate an alternative approach, in which atomic interactions arise via their common coupling to photonic crystal waveguides. This technique takes advantage of the ability to separately tailor the strength and range of interactions via the dispersion engineering of the structure itself, which can lead to qualitatively new types of phenomena. As an example, we discuss the formation of correlated transparency windows, in which photonic states of a certain number and shape selectively propagate through the system. Through this technique, we show in particular that one can create molecular-like potentials that lead to molecular bound states of photon pairs.