Journal ArticleDOI
Size Matters More Than Chemistry for Cloud-Nucleating Ability of Aerosol Particles
Ulrike Dusek,Göran Frank,Lea Hildebrandt,Lea Hildebrandt,Joachim Curtius,Johannes Schneider,S. Walter,Duli Chand,Frank Drewnick,Silke S. Hings,D Jung,Stephan Borrmann,Meinrat O. Andreae +12 more
TLDR
Size-resolved cloud condensation nuclei spectra measured for various aerosol types at a non-urban site in Germany showed that CCN concentrations are mainly determined by the aerosol number size distribution.Abstract:
Size-resolved cloud condensation nuclei (CCN) spectra measured for various aerosol types at a non-urban site in Germany showed that CCN concentrations are mainly determined by the aerosol number size distribution. Distinct variations of CCN activation with particle chemical composition were observed but played a secondary role. When the temporal variation of chemical effects on CCN activation is neglected, variation in the size distribution alone explains 84 to 96% of the variation in CCN concentrations. Understanding that particles' ability to act as CCN is largely controlled by aerosol size rather than composition greatly facilitates the treatment of aerosol effects on cloud physics in regional and global models.read more
Citations
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Book Chapter
Changes in Atmospheric Constituents and in Radiative Forcing
Piers M. Forster,Venkatachalam Ramaswamy,Paulo Artaxo,Terje Koren Berntsen,Richard Betts,David W. Fahey,Jim Haywood,Judith Lean,David C. Lowe,Gunnar Myhre,John Nganga,Ronald G. Prinn,Graciela B. Raga,Michael Schulz,Rob van Dorland,Greg Bodeker,Oliver Boucher,William D. Collins,T.J. Conway,Edward J. Dlugokencky,James W. Elkins,David Etheridge,P. Foukal,Paul J. Fraser,Marvyn Geller,Fortunat Joos,Charles D. Keeling,Stefan Kinne,K. Lassey,Ulrike Lohmann,Andrew C. Manning,S. A. Montzka,David E. Oram,K. O'Shaughnessy,S. Piper,Gian-Kasper Plattner,Michael Ponater,Navin Ramankutty,G. Reid,David Rind,Karen H. Rosenlof,Robert Sausen,D. Schwarzkopf,S.K. Solanki,Garry Stenchikov,N. Stuber,Toshihiko Takemura,Christiane Textor,R. Wang,Ray F. Weiss,T. Whorf +50 more
Journal ArticleDOI
Bounding the role of black carbon in the climate system: A scientific assessment
Tami C. Bond,Sarah J. Doherty,David W. Fahey,Piers M. Forster,Terje Koren Berntsen,Benjamin DeAngelo,Mark Flanner,Steven J. Ghan,Bernd Kärcher,Dorothy Koch,Stefan Kinne,Yutaka Kondo,Patricia K. Quinn,Marcus C. Sarofim,Martin G. Schultz,Michael Schulz,Chandra Venkataraman,Hua Zhang,Shiqiu Zhang,Nicolas Bellouin,Sarath K. Guttikunda,Philip K. Hopke,Mark Z. Jacobson,Johannes W. Kaiser,Zbigniew Klimont,Ulrike Lohmann,Joshua P. Schwarz,Drew Shindell,Trude Storelvmo,Stephen G. Warren,Charles S. Zender +30 more
TL;DR: In this paper, the authors provided an assessment of black-carbon climate forcing that is comprehensive in its inclusion of all known and relevant processes and that is quantitative in providing best estimates and uncertainties of the main forcing terms: direct solar absorption; influence on liquid, mixed phase, and ice clouds; and deposition on snow and ice.
Journal ArticleDOI
Ubiquity and dominance of oxygenated species in organic aerosols in anthropogenically-influenced Northern Hemisphere midlatitudes
Qi Zhang,Jose L. Jimenez,Manjula R. Canagaratna,James Allan,Hugh Coe,Ingrid M. Ulbrich,M. R. Alfarra,Akinori Takami,Ann M. Middlebrook,Yele Sun,Katja Dzepina,Edward J. Dunlea,Kenneth S. Docherty,Peter F. DeCarlo,D. Salcedo,Timothy B. Onasch,J. T. Jayne,Takao Miyoshi,A. Shimono,Shiro Hatakeyama,Nobuyuki Takegawa,Yutaka Kondo,Johannes Schneider,Frank Drewnick,Stephan Borrmann,Silke Weimer,Kenneth L. Demerjian,Paul I. Williams,Keith Bower,Roya Bahreini,Roya Bahreini,L. Cottrell,Robert J. Griffin,J. Rautiainen,J. Y. Sun,Yaping Zhang,D. R. Worsnop +36 more
TL;DR: In this article, organic aerosol data acquired by the AMS in 37 field campaigns were deconvolved into hydrocarbon-like OA (HOA) and several types of oxygenated OA components.
Journal ArticleDOI
A single parameter representation of hygroscopic growth and cloud condensation nucleus activity
TL;DR: In this paper, a method to describe the relationship between particle dry diameter and cloud condensation activity using a single hygroscopicity parameter is presented. But this method is limited to single and multi-component particles with varying amounts of inorganic, organic and surface active compounds.
Journal ArticleDOI
Flood or drought: How do aerosols affect precipitation?
Daniel Rosenfeld,Ulrike Lohmann,Graciela B. Raga,Colin D. O'Dowd,Markku Kulmala,Sandro Fuzzi,Anni Reissell,Meinrat O. Andreae +7 more
TL;DR: A conceptual model is proposed that explains this apparent dichotomy of pristine tropical clouds with low CCN concentrations rain out too quickly to mature into long-lived clouds and heavily polluted clouds evaporate much of their water before precipitation can occur.
References
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Journal ArticleDOI
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Development of an Aerosol Mass Spectrometer for Size and Composition Analysis of Submicron Particles
John T. Jayne,Danna C. Leard,Xuefeng Zhang,P. Davidovits,Kenneth A. Smith,Charles E. Kolb,Douglas R. Worsnop +6 more
TL;DR: In this article, the authors describe an aerosol mass spectrometer (AMS) which has been developed in response to these aerosol sampling needs and demonstrate quantitative mea surement capability for a laboratory-generated pure component NH4 NO3 aerosol.
Journal ArticleDOI
Cloud albedo enhancement by surface-active organic solutes in growing droplets
TL;DR: In this paper, the authors report measurements on vacuum-evaporated samples of cloud water from the Po Valley, Italy, that show a large decrease in surface tension, by up to about one-third relative to pure water, for realistic concentrations of organic solutes expected to exist in growing droplets.
Journal ArticleDOI
Strong present-day aerosol cooling implies a hot future
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