Showing papers on "Spontaneous emission published in 2014"
TL;DR: It is shown, using photoluminescence studies, that radiative bimolecular recombination is dominant at higher excitation densities, Hence, the quantum efficiencies of the perovskite light-emitting diodes increase at higher current densities.
Abstract: Solid-state light-emitting devices based on direct-bandgap semiconductors have, over the past two decades, been utilized as energy-efficient sources of lighting. However, fabrication of these devices typically relies on expensive high-temperature and high-vacuum processes, rendering them uneconomical for use in large-area displays. Here, we report high-brightness light-emitting diodes based on solution-processed organometal halide perovskites. We demonstrate electroluminescence in the near-infrared, green and red by tuning the halide compositions in the perovskite. In our infrared device, a thin 15 nm layer of CH3NH3PbI(3-x)Cl(x) perovskite emitter is sandwiched between larger-bandgap titanium dioxide (TiO2) and poly(9,9'-dioctylfluorene) (F8) layers, effectively confining electrons and holes in the perovskite layer for radiative recombination. We report an infrared radiance of 13.2 W sr(-1) m(-2) at a current density of 363 mA cm(-2), with highest external and internal quantum efficiencies of 0.76% and 3.4%, respectively. In our green light-emitting device with an ITO/PEDOT:PSS/CH3NH3PbBr3/F8/Ca/Ag structure, we achieved a luminance of 364 cd m(-2) at a current density of 123 mA cm(-2), giving external and internal quantum efficiencies of 0.1% and 0.4%, respectively. We show, using photoluminescence studies, that radiative bimolecular recombination is dominant at higher excitation densities. Hence, the quantum efficiencies of the perovskite light-emitting diodes increase at higher current densities. This demonstration of effective perovskite electroluminescence offers scope for developing this unique class of materials into efficient and colour-tunable light emitters for low-cost display, lighting and optical communication applications.
3,466 citations
TL;DR: By nanopatterning ahyperbolic metamaterial made of Ag and Si multilayers, the spontaneous emission rate of rhodamine dye molecules is enhanced 76-fold at tunable frequencies and the emission intensity of the dye increases by ~80-fold compared with the same hyperbolic meetamaterial without nanostructuring.
Abstract: The spontaneous emission rate and emission intensity of dye molecules are significantly enhanced by using a nanopatterned multilayer hyperbolic metamaterial.
444 citations
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TL;DR: The observation of zero-dimensional anharmonic quantum emitters in monolayer tungsten diselenide with an energy that is 20-100 meV lower than that of two-dimensional excitons shows that the quantum dots have singlet ground states and an anisotropic confinement that is most probably induced by impurities or defects.
Abstract: Semiconductor quantum dots have emerged as promising candidates for implementation of quantum information processing since they allow for a quantum interface between stationary spin qubits and propagating single photons. In the meanwhile, transition metal dichalcogenide (TMD) monolayers have moved to the forefront of solid-state research due to their unique band structure featuring a large band gap with degenerate valleys and non-zero Berry curvature. Here we report the observation of quantum dots in monolayer tungsten-diselenide with an energy that is 20 to 100 meV lower than that of two dimensional excitons. Photon antibunching in second-order photon correlations unequivocally demonstrates the zero-dimensional anharmonic nature of these quantum emitters. The strong anisotropic magnetic response of the spatially localized emission peaks strongly indicates that radiative recombination stems from localized excitons that inherit their electronic properties from the host TMD. The large $\sim$ 1 meV zero-field splitting shows that the quantum dots have singlet ground states and an anisotropic confinement most likely induced by impurities or defects in the host TMD. Electrical control in van der Waals heterostructures and robust spin-valley degree of freedom render TMD quantum dots promising for quantum information processing.
423 citations
TL;DR: The directional spontaneous emission of photons by laser-trapped caesium atoms into an optical nanofibre is demonstrated and the spontaneous emission into the counter-propagating guided modes from symmetric to strongly asymmetric, where more than % of the optical power is launched into one or the other direction.
Abstract: Nanoscale confinement in an optical fibre induces coupling between a photon’s spin and orbital angular momentum. Here, the authors use this effect to control the direction of photons spontaneously emitted from trapped caesium atoms into a nanofibre.
374 citations
TL;DR: In this paper, the density matrix renormalization group (DMRG) theory and its symmetrization scheme for quantum chemistry applied to calculate the excited states structure was used to understand the nature of the low-lying excited state structure.
211 citations
TL;DR: In this paper, it was shown that when the coupling between light and matter becomes strong enough, the Purcell effect decouples and the spontaneous emission rate decays with large enough couplings.
Abstract: Improvements in both the photonic confinement and the emitter design have led to a steady increase in the strength of the light-matter coupling in cavity quantum electrodynamics experiments. This has allowed us to access interaction-dominated regimes in which the state of the system can only be described in terms of mixed light-matter excitations. Here we show that, when the coupling between light and matter becomes strong enough, this picture breaks down, and light and matter degrees of freedom totally decouple. A striking consequence of such a counterintuitive phenomenon is that the Purcell effect is reversed and the spontaneous emission rate, usually thought to increase with the light-matter coupling strength, plummets instead for large enough couplings.
187 citations
TL;DR: In this article, a 10-fold PL lifetime shortening was achieved, as a consequence of Purcell enhancement of the spontaneous emission rate of photoluminescence (PL).
Abstract: Integration of quasi-two-dimensional (2D) films of metal–chalcogenides in optical microcavities permits new photonic applications of these materials. Here we present tunable microcavities with monolayer MoS2 or few monolayer GaSe films. We observe significant modification of spectral and temporal properties of photoluminescence (PL): PL is emitted in spectrally narrow and wavelength-tunable cavity modes with quality factors up to 7400; a 10-fold PL lifetime shortening is achieved, a consequence of Purcell enhancement of the spontaneous emission rate.
148 citations
TL;DR: In this paper, a quantum-optical (quantum-mechanical active medium and radiation field) theory is used to examine the emission properties of nanolasers under different experimental configurations.
Abstract: This review addresses ongoing discussions involving nanolaser experiments, particularly those related to thresholdless lasing or few-emitter devices. A quantum-optical (quantum-mechanical active medium and radiation field) theory is used to examine the emission properties of nanolasers under different experimental configurations. The active medium is treated as inhomogeneously broadened semiconductor quantum dots embedded in a quantum well, where carriers are introduced via current injection. Comparisons are made between a conventional laser and a nanolaser with a spontaneous emission factor of unity, as well as a laser with only a few quantum dots providing the gain. It is found that the combined exploration of intensity, coherence time, photon autocorrelation function and carrier spectral hole burning can provide a unique and consistent picture of nanolasers in the new regimes of laser operation during the transition from thermal to coherent emission. Furthermore, by reducing the number of quantum dots in the optical cavity, a clear indication of non-classical photon statistics is observed before the single-quantum-dot limit is reached. Nanolasers operate in a regime distinctly different to that of conventional lasers, and a consistent model of nanolasing physics is needed. Whereas conventional lasers are characterized by a marked intensity jump at the onset of lasing, micro- and nanocavity lasers with well-developed three-dimensional optical mode confinement can have a vanishing small intensity jump approaching thresholdless behavior. Weng Chow from Sandia National Laboratories in the United States, with colleagues Frank Jahnke and Christopher Gies from the University of Bremen in Germany, has reviewed recent nanolaser experiments and developed a model based on quantum-optical theory to examine photon statistics in the different operational regime of nanolasers compared with conventional lasers. The results dispute the notation of thresholdless lasing and suggests the emergence of non-classical photon statistics for few-atom or few-quantum-dot active regions.
146 citations
TL;DR: In this paper, a single-photon router using a single atom with an inversion center coupled to quantum multichannels made of coupled-resonator waveguides is proposed.
Abstract: We propose a single-photon router using a single atom with an inversion center coupled to quantum multichannels made of coupled-resonator waveguides. We show that the spontaneous emission of the atom can direct single photons from one quantum channel into another. The on-demand classical field perfectly switches off the single-photon routing due to the quantum interference in the atomic amplitudes of optical transitions. Total reflections in the incident channel are due to the photonic bound state in the continuum. Two virtual channels, named the scatter-free and controllable channels, are found, which are coherent superpositions of quantum channels. Any incident photon in the scatter-free channel is totally transmitted. The propagating states of the controllable channel are orthogonal to those of the scatter-free channel. Single photons in the controllable channel can be perfectly reflected or transmitted by the atom.
141 citations
TL;DR: In this article, the state-of-the-art in the field of crystal laser devices is reviewed and an outlook and personal view is provided on the further developments of laser crystals and their applications.
Abstract: Because of long-range order and high chemical purity, organic crystals have exhibit unique properties and attracted a lot of interest for application in solid-state lasers. As optical gain materials, they exhibit high stimulated emission cross section and broad tunable wavelength emission as similar to their amorphous counterpart; moreover, high purity and high order give them superior properties such as low scattering trap densities, high thermal stability, as well as highly polarized emission. As electronic materials, they are potentially able to support high current densities, thus making it possible to realize current driven lasers. This paper mainly describes recent research progress in organic semiconductor laser crystals. The building molecules, crystal growth methods, as well as their stimulated emission characteristics related with crystal structures are introduced; in addition, the current state-of-the-art in the field of crystal laser devices is reviewed. Furthermore, recent advances of crystal lasers at the nanoscale and single crystal light-emitting transistors (LETs) are presented. Finally, an outlook and personal view is provided on the further developments of laser crystals and their applications.
141 citations
TL;DR: In this article, a unified model for the direct gap absorption coefficient (band-edge and sub-bandgap) is developed that encompasses the functional forms of the Urbach, Thomas-Fermi, screened Thomas Fermi and Franz-Keldysh models of subbandgap absorption as specific cases.
Abstract: A unified model for the direct gap absorption coefficient (band-edge and sub-bandgap) is developed that encompasses the functional forms of the Urbach, Thomas-Fermi, screened Thomas-Fermi, and Franz-Keldysh models of sub-bandgap absorption as specific cases. We combine this model of absorption with an occupation-corrected non-equilibrium Planck law for the spontaneous emission of photons to yield a model of photoluminescence (PL) with broad applicability to band-band photoluminescence from intrinsic, heavily doped, and strongly compensated semiconductors. The utility of the model is that it is amenable to full-spectrum fitting of absolute intensity PL data and yields: (1) the quasi-Fermi level splitting, (2) the local lattice temperature, (3) the direct bandgap, (4) the functional form of the sub-bandgap absorption, and (5) the energy broadening parameter (Urbach energy, magnitude of potential fluctuations, etc.). The accuracy of the model is demonstrated by fitting the room temperature PL spectrum of GaAs. It is then applied to Cu(In,Ga)(S,Se)2 (CIGSSe) and Cu2ZnSn(S,Se)4 (CZTSSe) to reveal the nature of their tail states. For GaAs, the model fit is excellent, and fitted parameters match literature values for the bandgap (1.42 eV), functional form of the sub-bandgap states (purely Urbach in nature), and energy broadening parameter (Urbach energy of 9.4 meV). For CIGSSe and CZTSSe, the model fits yield quasi-Fermi leveling splittings that match well with the open circuit voltages measured on devices made from the same materials and bandgaps that match well with those extracted from EQE measurements on the devices. The power of the exponential decay of the absorption coefficient into the bandgap is found to be in the range of 1.2 to 1.6, suggesting that tunneling in the presence of local electrostatic potential fluctuations is a dominant factor contributing to the sub-bandgap absorption by either purely electrostatic (screened Thomas-Fermi) or a photon-assisted tunneling mechanism (Franz-Keldysh). A Gaussian distribution of bandgaps (local Eg fluctuation) is found to be inconsistent with the data. The sub-bandgap absorption of the CZTSSe absorber is found to be larger than that for CIGSSe for materials that yield roughly equivalent photovoltaic devices (8% efficient). Further, it is shown that fitting only portions of the PL spectrum (e.g., low energy for energy broadening parameter and high energy for quasi-Fermi level splitting) may lead to significant errors for materials with substantial sub-bandgap absorption and emission.
TL;DR: A novel photonic structure and a technology allowing the deterministic implementation of electrical control for a quantum dot in a microcavity are presented and a deterministic and electrically tunable single-photon source with an extraction efficiency is demonstrated.
Abstract: The scalability of a quantum network based on semiconductor quantum dots lies in the possibility of having an electrical control of the quantum dot state as well as controlling its spontaneous emission. The technological challenge is then to define electrical contacts on photonic microstructures optimally coupled to a single quantum emitter. Here we present a novel photonic structure and a technology allowing the deterministic implementation of electrical control for a quantum dot in a microcavity. The device consists of a micropillar connected to a planar cavity through one-dimensional wires; confined optical modes are evidenced with quality factors as high as 33,000. We develop an advanced in-situ lithography technique and demonstrate the deterministic spatial and spectral coupling of a single quantum dot to the connected pillar cavity. Combining this cavity design and technology with a diode structure, we demonstrate a deterministic and electrically tunable single-photon source with an extraction efficiency of around 53±9%. Bright and tunable single-photon sources are essential for future quantum technologies. Here, the authors deterministically couple a quantum dot to a pillar structure that enables application of electric fields to provide a tunable single-photon source with a demonstrated extraction efficiency of 53%.
TL;DR: C cavity QED conditions in the Purcell regime for single quantum emitters on the surface of an optical nanofiber are demonstrated, paving the way for enhanced on-fiber light-matter interfaces with clear applications to quantum networks.
Abstract: Spontaneous emission from a cavity made of an optical nanofiber and a nanostructured grating is demonstrated, which would allow single quantum emitters to be easily integrated into an optical network.
TL;DR: A distinct dependence of the backward UV spectrum on pump laser polarization and intensity is observed, pointing to the occurrence of backward amplified spontaneous emission inside filaments.
Abstract: We report on strong backward stimulated emission at 337 nm in nitrogen gas pumped by circularly polarized femtosecond laser pulses at 800 nm. A distinct dependence of the backward UV spectrum on pump laser polarization and intensity is observed, pointing to the occurrence of backward amplified spontaneous emission inside filaments. We attribute the population inversion to inelastic collision between the free electrons produced by the pump laser and neutral N2 molecules. The addition of oxygen molecules is detrimental for the gain, reducing it to near threshold at atmospheric concentration.
TL;DR: In this paper, the effects of nonlocal response by metallic nanospheres in three distinct settings were investigated: atomic spontaneous emission, electron energy loss spectroscopy, and light scattering.
Abstract: Inspired by recent measurements on individual metallic nanospheres that cannot be explained with traditional classical electrodynamics, we theoretically investigate the effects of nonlocal response by metallic nanospheres in three distinct settings: atomic spontaneous emission, electron energy loss spectroscopy, and light scattering. These constitute two near-field and one far-field measurements, with zero-, one-, and two-dimensional excitation sources, respectively. We search for the clearest signatures of hydrodynamic pressure waves in nanospheres. We employ a linearized hydrodynamic model, and Mie–Lorenz theory is applied for each case. Nonlocal response shows its mark in all three configurations, but for the two near-field measurements, we predict especially pronounced nonlocal effects that are not exhibited in far-field measurements. Associated with every multipole order is not only a single blueshifted surface plasmon but also an infinite series of bulk plasmons that have no counterpart in a local-r...
TL;DR: This work shows that superabsorption can be achieved and sustained in certain simple nanostructures, by trapping the system in a highly excited state through transition rate engineering, which opens the prospect of a new class of quantum nanotechnology with potential applications including photon detection and light-based power transmission.
Abstract: Almost 60 years ago Dicke introduced the term superradiance to describe a signature quantum effect: N atoms can collectively emit light at a rate proportional to N(2). Structures that superradiate must also have enhanced absorption, but the former always dominates in natural systems. Here we show that this restriction can be overcome by combining several well-established quantum control techniques. Our analytical and numerical calculations show that superabsorption can then be achieved and sustained in certain simple nanostructures, by trapping the system in a highly excited state through transition rate engineering. This opens the prospect of a new class of quantum nanotechnology with potential applications including photon detection and light-based power transmission. An array of quantum dots or a molecular ring structure could provide a suitable platform for an experimental demonstration.
TL;DR: A simple new scheme for the efficient coupling of single molecules and photons is presented and strategies for exploring a range of quantum-optical phenomena are discussed, including polaritonic interactions in a mesoscopic ensemble of molecules mediated by a single mode of propagating photons.
Abstract: Many of the currently pursued experiments in quantum optics would greatly benefit from a strong interaction between light and matter. Here, we present a simple new scheme for the efficient coupling of single molecules and photons. A glass capillary with a diameter of 600 nm filled with an organic crystal tightly guides the excitation light and provides a maximum spontaneous emission coupling factor (β) of 18% for the dye molecules doped in the organic crystal. A combination of extinction, fluorescence excitation, and resonance fluorescence spectroscopy with microscopy provides high-resolution spatiospectral access to a very large number of single molecules in a linear geometry. We discuss strategies for exploring a range of quantum-optical phenomena, including polaritonic interactions in a mesoscopic ensemble of molecules mediated by a single mode of propagating photons.
TL;DR: In this article, the authors investigated the optical properties of phosphate glasses codoped with Er3+−Yb3+ as a function of Yb3−concentration in order to evaluate their potential as both glass laser systems and amplifier materials.
TL;DR: To extract the plasmonic modes of the structure into the far field, two types of 1D grating with triangular and rectangular profile are implemented, obtaining a 10-fold radiative enhancement at visible frequencies.
Abstract: Hyperbolic metamaterials can enhance spontaneous emission, but the radiation-matter coupling is not optimized if the light source is placed outside such media. We demonstrate a 3-fold improvement of the Purcell factor over its outer value and a significant enlargement in bandwidth by including the emitter within a Si/Ag periodic multilayer metamaterial. To extract the plasmonic modes of the structure into the far field we implement two types of 1D grating with triangular and rectangular profile, obtaining a 10-fold radiative enhancement at visible frequencies.
TL;DR: An ultrafast non-local moulding of the vacuum field in a coupled-cavity system is proposed and the dynamic control of the spontaneous emission (SE) of quantum dots (QDs) in a photonic crystal (PhC) cavity on a ∼ 200 ps timescale, much faster than their natural SE lifetimes.
Abstract: Non-local moulding of the vacuum field in a photonic cavity structure enables control of the spontaneous emission of quantum dots. The radiative interaction of solid-state emitters with cavity fields is the basis of semiconductor microcavity lasers and cavity quantum electrodynamics (CQED) systems1. Its control in real time would open new avenues for the generation of non-classical light states, the control of entanglement and the modulation of lasers. However, unlike atomic CQED or circuit quantum electrodynamics2,3,4,5,6, the real-time control of radiative processes has not yet been achieved in semiconductors because of the ultrafast timescales involved. Here we propose an ultrafast non-local moulding of the vacuum field in a coupled-cavity system as an approach to the control of radiative processes and demonstrate the dynamic control of the spontaneous emission (SE) of quantum dots (QDs) in a photonic crystal (PhC) cavity on a ∼200 ps timescale, much faster than their natural SE lifetimes.
TL;DR: In this article, a quasi-type-II band alignment in graded alloy CdSxSe1-x nanocrystals revealed by femtosecond fluorescence upconversion spectroscopy was reported.
Abstract: Interaction of charge carriers with the surface of semiconductor nanocrystals plays an integral role in determining the ultimate fate of the excited state. The surface contains a dynamic ensemble of trap states that can localize excited charges, preventing radiative recombination and reducing fluorescence quantum yields. Here we report quasi-type-II band alignment in graded alloy CdSxSe1–x nanocrystals revealed by femtosecond fluorescence upconversion spectroscopy. Graded alloy CdSxSe1–x quantum dots are a compositionally inhomogeneous nano-heterostructure designed to decouple the exciton from the nanocrystal surface. The large valence band offset between the CdSe-rich core and CdS-rich shell separates the excited hole from the surface by confining it to the core of the nanocrystal. The small conduction band offset, however, allows the electron to delocalize throughout the entire nanocrystal and maintain overlap with the surface. Indeed, the ultrafast charge carrier dynamics reveal that the fast 1–3 ps ho...
TL;DR: In this paper, a photon Green's function method was used to control the quantum optical properties of a quantum dot coupled to a metallic nanoparticle, which is based on the exact quantization of the electromagnetic fields in a dissipative medium.
Abstract: We investigate the coherent control of the quantum optical properties of a quantum dot coupled to a metallic nanoparticle using a photon Green's function method, which is based on the exact quantization of the electromagnetic fields in a dissipative medium. The properties of the spontaneous emission spectra of such a system are studied in detail with and without involving the coherent field. The Rabi splitting effect in the spectrum emitted by the quantum dot under particular conditions is predicted for different sizes of the metal nanoparticles. We show that the spontaneous emission spectra of the transition coupled to surface plasmons may be further modified by adjusting the external coherent control on the adjacent transitions. Furthermore, the pronounced oscillatory behavior for the quantum-dot dynamics is demonstrated with the presence of the metal nanoparticle by the non-Markovian treatment. Our results may have potential applications in plasmonic-based quantum manipulation.
TL;DR: It is shown that enhanced directional emission of spontaneous radiation can be produced also with statistically independent incoherent sources, via the measurement of higher-order correlation functions of the emitted radiation.
Abstract: Superradiance has been an outstanding problem in quantum optics since Dicke introduced the concept of enhanced directional spontaneous emission by an ensemble of identical two-level atoms. The effect is based on the correlated collective Dicke states which turn out to be highly entangled. Here we show that enhanced directional emission of spontaneous radiation can be produced also with statistically independent incoherent sources, via the measurement of higher-order correlation functions of the emitted radiation. Our analysis is applicable to a wide variety of quantum emitters, like trapped atoms, ions, quantum dots, or nitrogen-vacancy centers, and is also valid for incoherent classical emitters. This is experimentally confirmed with up to eight statistically independent thermal light sources. The arrangement to measure the higher-order correlation functions corresponds to a generalized Hanbury Brown--Twiss setup, demonstrating that the two phenomena, superradiance and the Hanbury Brown--Twiss effect, stem from the same interference phenomenon.
TL;DR: It is reported that a seed pulse injected in the backward direction can be amplified by ~200 times inside this plasma amplifier, indicating that the amplification is largely in the unsaturated regime and that further improvement of laser energy is possible.
Abstract: Recently, S. Mitryukovskiy et al. presented experimental evidence showing that backward Amplified Spontaneous Emission (ASE) at 337 nm can be obtained from plasma filaments in nitrogen gas pumped by circularly polarized 800 nm femtosecond pulses (Opt. Express, 22, 12750 (2014)). Here, we report that a seed pulse injected in the backward direction can be amplified by ~200 times inside this plasma amplifier. The amplified 337 nm radiation can be either linearly or circularly polarized, dictated by the seeding pulse, which is distinct from the non-polarized nature of the ASE. We performed comprehensive measurements of the spatial profile, optical gain dynamics, and seed pulse energy dependence of this amplification process. These measurements allow us to deduce the pulse duration of the ASE and the amplified 337 nm radiation as well as the corresponding laser intensity inside the plasma amplifier. It indicates that the amplification is largely in the unsaturated regime and that further improvement of laser energy is possible. Moreover, we observed optical gain in plasma created in ambient air. This represents an important step towards future applications exploiting backward lasing for remote atmospheric sensing.
TL;DR: A new technique for Brillouin scattering-based, distributed fiber-optic measurements of temperature and strain is proposed, analyzed, simulated, and demonstrated, and the expected spatial resolution and the measurement signal-to-noise ratio is provided.
Abstract: A new technique for Brillouin scattering-based, distributed fiber-optic measurements of temperature and strain is proposed, analyzed, simulated, and demonstrated. Broadband Brillouin pump and signal waves are drawn from the filtered amplified spontaneous emission of an erbium-doped fiber amplifier, providing high spatial resolution. The reconstruction of the position-dependent Brillouin gain spectra along 5 cm of a silica single-mode fiber under test, with a spatial resolution of 4 mm, is experimentally demonstrated using a 25 GHz-wide amplified spontaneous emission source. A 4 mm-long localized hot spot is identified by the measurements. The uncertainty in the reconstruction of the local Brillouin frequency shift is ± 1.5 MHz. The single correlation peak between the pump and signal is scanned along a fiber under test using a mechanical variable delay line. The analysis of the expected spatial resolution and the measurement signal-to-noise ratio is provided. The measurement principle is supported by numerical simulations of the stimulated acoustic field as a function of position and time. Unlike most other Brillouin optical correlation domain analysis configurations, the proposed scheme is not restricted by the bandwidth of available electro-optic modulators, microwave synthesizers, or pattern generators. Resolution is scalable to less than one millimeter in highly nonlinear media.
TL;DR: In this article, the authors studied the scattering of guided light from a multilevel cesium atom with the transitions between the hyperfine levels $6{S}_{1/2}F=4$ and$6{P}_{3/2}{F^{\ensuremath{'}}=5$ of the guided modes of a nanofiber.
Abstract: We study the scattering of guided light from a multilevel cesium atom with the transitions between the hyperfine levels $6{S}_{1/2}F=4$ and $6{P}_{3/2}{F}^{\ensuremath{'}}=5$ of the ${D}_{2}$ line into the guided modes of a nanofiber. We show that the rate of scattering of guided light from the atom in the steady-state regime into the guided modes is asymmetric with respect to the forward and backward directions and depends on the polarization of the probe field. The asymmetry between the forward and backward scattering is a result of the complex transition structure of the atom and the existence of a longitudinal component of the guided-mode profile function. In the case of a two-level atom, the rates of spontaneous emission (and consequently the rates of scattering) into the forward and backward guided modes differ from each other when the atomic dipole matrix-element vector is a complex vector in the plane that contains the fiber axis and the atomic position.
TL;DR: In this article, the authors report on progress in the development of GaAsBi/(Al)GaAs based laser grown using metal-organic vapour phase epitaxy and focus on the underlying processes governing their efficiency and temperature dependence.
Abstract: This paper reports on progress in the development of GaAsBi/(Al)GaAs based lasers grown using metal-organic vapour phase epitaxy and focuses on the underlying processes governing their efficiency and temperature dependence. Room temperature lasing has been achieved in devices with 2.2% Bi and lasing in devices with 4.4% Bi was observed up to 180 K. We show that the device performance can be improved by optimizing both electrical and optical confinement in the laser structures. Analysis of the temperature dependence of the threshold current together with pure spontaneous emission and high hydrostatic pressure measurements indicate that device performance is currently dominated by non-radiative recombination through defects (>80% of the threshold current at room temperature in 2.2% Bi samples) and that to further improve the device performance and move towards longer wavelengths for optical telecommunications (1.3–1.5 µm) further effort is required to improve and optimize material quality.
TL;DR: In this article, the authors demonstrate the ability to control spontaneous emission from a superconducting qubit coupled to a cavity, where the time domain profile of the emitted photon is shaped into a symmetric truncated exponential.
Abstract: We demonstrate the ability to control spontaneous emission from a superconducting qubit coupled to a cavity. The time domain profile of the emitted photon is shaped into a symmetric truncated exponential. The experiment is enabled by a qubit coupled to a cavity, with a coupling strength that can be tuned in tens of nanoseconds while maintaining a constant dressed state emission frequency. Symmetrization of the photonic wave packet will enable use of photons as flying qubits for transferring the quantum state between atoms in distant cavities.
TL;DR: In this article, the authors report on the lasing action of atmospheric air pumped by an 800-nm femtosecond laser pulse with peak power up to 4 TW, which shows a doughnut profile, reflecting the spatial distribution of the pump-generated white-light continuum that acts as a seed for lasing.
Abstract: We report on the lasing action of atmospheric air pumped by an 800 nm femtosecond laser pulse with peak power up to 4 TW. Lasing emission at 428 nm increases rapidly over a small range of pump laser power, followed by saturation above ∼1.5 TW. The maximum lasing pulse energy is measured at 2.6 μJ corresponding to an emission power in the MW range, while a maximum conversion efficiency of 3.5×10−5 is measured at moderate pump pulse energy. The optical gain inside the filament plasma is estimated to be in excess of 0.7/cm. Lasing emission shows a doughnut profile, reflecting the spatial distribution of the pump-generated white-light continuum that acts as a seed for the lasing. We attribute the pronounced saturation to the defocusing of the seed in the plasma amplifying region and to the saturation of the seed intensity.
TL;DR: In this paper, spontaneous emission properties and control of the zero phonon line (ZPL) from a diamond nitrogen-vacancy (NV) center coherently driven by a single elliptically polarized control field were investigated.
Abstract: We investigate spontaneous emission properties and control of the zero phonon line (ZPL) from a diamond nitrogen–vacancy (NV) center coherently driven by a single elliptically polarized control field. We use the Schrodinger equation to calculate the probability amplitudes of the wave function of the coupled system and derive analytical expressions of the spontaneous emission spectra. The numerical results show that a few interesting phenomena such as enhancement, narrowing, suppression, and quenching of the ZPL spontaneous emission can be realized by modulating the polarization-dependent phase, the Zeeman shift, and the intensity of the control field in our system. In the dressed-state picture of the control field, we find that multiple spontaneously generated coherence arises due to three close-lying states decaying to the same state. These results are useful in real experiments.