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Emerging Device Applications for Semiconducting Two-Dimensional Transition Metal Dichalcogenides

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TLDR
By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.
Abstract
With advances in exfoliation and synthetic techniques, atomically thin films of semiconducting transition metal dichalcogenides have recently been isolated and characterized. Their two-dimensional structure, coupled with a direct band gap in the visible portion of the electromagnetic spectrum, suggests suitability for digital electronics and optoelectronics. Toward that end, several classes of high-performance devices have been reported along with significant progress in understanding their physical properties. Here, we present a review of the architecture, operating principles, and physics of electronic and optoelectronic devices based on ultrathin transition metal dichalcogenide semiconductors. By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.

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Citations
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Journal ArticleDOI

Collective Dipole‐Dominated Doping of Monolayer MoS2: Orientation and Magnitude Control via the Supramolecular Approach

TL;DR: In this paper, a method for the molecular functionalization of monolayer transition metal dichalcogenides (TMDCs) relying on the molecular self-assembly of metal phthalocyanine and the orientation-controlled coordination chemistry of axial ligands is reported.
Journal ArticleDOI

Doping of Two-Dimensional Semiconductors: A Rapid Review and Outlook

TL;DR: In this article, a rapid review on the recent achievements and challenges in the metastable and substitutional doping of 2D materials is presented, followed by an outlook on integrating two-dimensional materials into more advanced electronic architectures.
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Ab Initio Investigation of Atomistic Insights into the Nanoflake Formation of Transition-Metal Dichalcogenides: The Examples of MoS2, MoSe2, and MoTe2

TL;DR: In this article, a density functional theory (DFT) study of the evolution of the structural, energetic, and electronic properties of (MoQ2)n nanoflakes, where Q = S, Se, and Te and n = 1.
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Two-Dimensional Magnetic Nanostructures

TL;DR: In this article, the authors highlight recent progress on the synthesis and magnetic properties of intrinsic 2D magnetic van der Waals nanostructures, such as VS2, CrI3, and 2D metal-organic frameworks.
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Enhancing the ambient stability of few-layer black phosphorus by surface modification

TL;DR: In this article, the authors investigated the adsorption characteristics of various elements across the Periodic Table on few-layer black phosphorus (BP) and selected fifteen elements based on high-throughput density functional theory calculations.
References
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Journal ArticleDOI

Electric Field Effect in Atomically Thin Carbon Films

TL;DR: Monocrystalline graphitic films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands and they exhibit a strong ambipolar electric field effect.
Journal ArticleDOI

The electronic properties of graphene

TL;DR: In this paper, the basic theoretical aspects of graphene, a one-atom-thick allotrope of carbon, with unusual two-dimensional Dirac-like electronic excitations, are discussed.
Proceedings Article

Physics of semiconductor devices

S. M. Sze
Journal ArticleDOI

Electronics and optoelectronics of two-dimensional transition metal dichalcogenides.

TL;DR: This work reviews the historical development of Transition metal dichalcogenides, methods for preparing atomically thin layers, their electronic and optical properties, and prospects for future advances in electronics and optoelectronics.
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