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Emerging Device Applications for Semiconducting Two-Dimensional Transition Metal Dichalcogenides

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TLDR
By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.
Abstract
With advances in exfoliation and synthetic techniques, atomically thin films of semiconducting transition metal dichalcogenides have recently been isolated and characterized. Their two-dimensional structure, coupled with a direct band gap in the visible portion of the electromagnetic spectrum, suggests suitability for digital electronics and optoelectronics. Toward that end, several classes of high-performance devices have been reported along with significant progress in understanding their physical properties. Here, we present a review of the architecture, operating principles, and physics of electronic and optoelectronic devices based on ultrathin transition metal dichalcogenide semiconductors. By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.

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Citations
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Contact engineering for 2D materials and devices

TL;DR: The phenomenon of Fermi level pinning at the metal/2D contact interface, the Schottky versus Ohmic nature of the contacts and various contact engineering approaches including interlayer contacts, phase engineered contacts, and basal versus edge plane contacts are elucidated.
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Charge-transfer-based gas sensing using atomic-layer MoS2.

TL;DR: A high-performance gas sensor constructed using atomic-layered MoS2 synthesised by chemical vapour deposition (CVD) was developed and the in situ PL characterisation of the changes in the peaks corresponding to charged trions and neutral excitons via gas adsorption processes was used to elucidate the mechanisms of charge transfer between theMoS2 and the gas molecules.
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Nanostructured Photodetectors: From Ultraviolet to Terahertz.

TL;DR: Recent advances in nanoscale photodetectors constructed by diverse low-dimensional nanostructured materials are discussed here; meanwhile, challenges and promising future directions in this research field are proposed.
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High performance pseudocapacitor based on 2D layered metal chalcogenide nanocrystals

TL;DR: The structural and electrochemical properties of few-layer TiS2 nanocrystals are described, showing two-dimensional morphology leads to very different behavior, compared to corresponding bulk materials, leading to materials that exhibit both high energy and power density.
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Strain and structure heterogeneity in MoS2 atomic layers grown by chemical vapour deposition.

TL;DR: This work systematically characterize chemical vapour deposition-grown Monolayer molybdenum disulfide by photoluminescence spectroscopy and mapping and demonstrates non-uniform strain in single-crystalline monolayer MoS2 and strain-induced bandgap engineering.
References
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Journal ArticleDOI

Electric Field Effect in Atomically Thin Carbon Films

TL;DR: Monocrystalline graphitic films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands and they exhibit a strong ambipolar electric field effect.
Journal ArticleDOI

The electronic properties of graphene

TL;DR: In this paper, the basic theoretical aspects of graphene, a one-atom-thick allotrope of carbon, with unusual two-dimensional Dirac-like electronic excitations, are discussed.
Proceedings Article

Physics of semiconductor devices

S. M. Sze
Journal ArticleDOI

Electronics and optoelectronics of two-dimensional transition metal dichalcogenides.

TL;DR: This work reviews the historical development of Transition metal dichalcogenides, methods for preparing atomically thin layers, their electronic and optical properties, and prospects for future advances in electronics and optoelectronics.
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