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Open AccessJournal ArticleDOI

Emerging Device Applications for Semiconducting Two-Dimensional Transition Metal Dichalcogenides

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TLDR
By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.
Abstract
With advances in exfoliation and synthetic techniques, atomically thin films of semiconducting transition metal dichalcogenides have recently been isolated and characterized. Their two-dimensional structure, coupled with a direct band gap in the visible portion of the electromagnetic spectrum, suggests suitability for digital electronics and optoelectronics. Toward that end, several classes of high-performance devices have been reported along with significant progress in understanding their physical properties. Here, we present a review of the architecture, operating principles, and physics of electronic and optoelectronic devices based on ultrathin transition metal dichalcogenide semiconductors. By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.

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Citations
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Journal ArticleDOI

A theoretical study of the electrical contact between metallic and semiconducting phases in monolayer MoS 2

TL;DR: In this article, a theoretical study of the electrical contact between the two most common crystallographic phases of MoS2 monolayer crystals is presented, where the stable semiconducting 2H phase and the metastable metallic 1T phase are compared.
Book ChapterDOI

Electronic structure calculations: the many-body perturbation theory (MBPT)

TL;DR: In this article, a detailed description of the electronic structure calculation techniques based on the so-called density functional theory (DFT) was presented, and some empirical solutions exist to overcome the problem of DFT band gap underestimation, such as the scissor technique, which consists in correcting the LDA/GGA gap error by shifting the conduction band up so as to match the gap relative to the experiment.
Journal ArticleDOI

Ping‐Pong Energy Transfer in Covalently Linked Porphyrin‐MoS2 Architectures

TL;DR: In this paper, the potential of transition-metal dichalcogenides in photosensitization processes was revealed, showing that a complex ping-pong energy-transfer mechanism, namely from the porphyrin to MoS2 and back to porphrin, operated.
Journal ArticleDOI

Intrinsic Limit for Contact Resistance in Exfoliated Multilayered MoS 2 FET

TL;DR: In this article, a new method for the separation of contact resistance into Schottky barrier resistance and interlayer resistance was proposed for multilayered MoS2 FETs.
Journal ArticleDOI

Engineering the optoelectronic properties of MoS2 photodetectors through reversible noncovalent functionalization

TL;DR: In this article, an easy drop-casting based functionalization of MoS2-based photodetectors was presented, which results in an enhancement of the photoresponse of about four orders of magnitude, reaching responsivities up to 100 A/W.
References
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Journal ArticleDOI

Electric Field Effect in Atomically Thin Carbon Films

TL;DR: Monocrystalline graphitic films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands and they exhibit a strong ambipolar electric field effect.
Journal ArticleDOI

The electronic properties of graphene

TL;DR: In this paper, the basic theoretical aspects of graphene, a one-atom-thick allotrope of carbon, with unusual two-dimensional Dirac-like electronic excitations, are discussed.
Proceedings Article

Physics of semiconductor devices

S. M. Sze
Journal ArticleDOI

Electronics and optoelectronics of two-dimensional transition metal dichalcogenides.

TL;DR: This work reviews the historical development of Transition metal dichalcogenides, methods for preparing atomically thin layers, their electronic and optical properties, and prospects for future advances in electronics and optoelectronics.
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