Showing papers on "Electron published in 2009"

Physics of laser-driven plasma-based electron accelerators

Abstract: Laser-driven plasma-based accelerators, which are capable of supporting fields in excess of 100 GV/m, are reviewed. This includes the laser wakefield accelerator, the plasma beat wave accelerator, the self-modulated laser wakefield accelerator, plasma waves driven by multiple laser pulses, and highly nonlinear regimes. The properties of linear and nonlinear plasma waves are discussed, as well as electron acceleration in plasma waves. Methods for injecting and trapping plasma electrons in plasma waves are also discussed. Limits to the electron energy gain are summarized, including laser pulse diffraction, electron dephasing, laser pulse energy depletion, and beam loading limitations. The basic physics of laser pulse evolution in underdense plasmas is also reviewed. This includes the propagation, self-focusing, and guiding of laser pulses in uniform plasmas and with preformed density channels. Instabilities relevant to intense short-pulse laser-plasma interactions, such as Raman, self-modulation, and hose instabilities, are discussed. Experiments demonstrating key physics, such as the production of high-quality electron bunches at energies of 0.1-1 GeV, are summarized.

Optics and interferometry with atoms and molecules

Abstract: The development of wave optics for light brought many new insights into our understanding of physics, driven by fundamental experiments like the ones by Young, Fizeau, Michelson-Morley and others. Quantum mechanics, and especially the de Broglie’s postulate relating the momentum p of a particle to the wave vector k of an matter wave: k = 2 λ = p/ℏ, suggested that wave optical experiments should be also possible with massive particles (see table 1), and over the last 40 years electron and neutron interferometers have demonstrated many fundamental aspects of quantum mechanics [1].

Josephson current and noise at a superconductor/quantum-spin-Hall-insulator/superconductor junction

Abstract: We study junctions between superconductors mediated by the edge states of a quantum-spin-Hall insulator. We show that such junctions exhibit a fractional Josephson effect, in which the current phase relation has a $4\ensuremath{\pi}$ rather than a $2\ensuremath{\pi}$ periodicity. This effect is a consequence of the conservation of fermion parity---the number of electron $\text{mod}\text{ }2$---in a superconducting junction and is closely related to the ${Z}_{2}$ topological structure of the quantum-spin-Hall insulator. Inelastic processes, which violate the conservation of fermion parity, lead to telegraph noise in the equilibrium supercurrent. We predict that the low-frequency noise due these processes diverges exponentially with temperature $T$ as $T\ensuremath{\rightarrow}0$. Possible experiments on HgCdTe quantum wells will be discussed.

Photon-induced near-field electron microscopy

Abstract: In materials science and biology, optical near-field microscopies enable spatial resolutions beyond the diffraction limit, but they cannot provide the atomic-scale imaging capabilities of electron microscopy. Given the nature of interactions between electrons and photons, and considering their connections through nanostructures, it should be possible to achieve imaging of evanescent electromagnetic fields with electron pulses when such fields are resolved in both space (nanometre and below) and time (femtosecond). Here we report the development of photon-induced near-field electron microscopy (PINEM), and the associated phenomena. We show that the precise spatiotemporal overlap of femtosecond single-electron packets with intense optical pulses at a nanostructure (individual carbon nanotube or silver nanowire in this instance) results in the direct absorption of integer multiples of photon quanta (nhomega) by the relativistic electrons accelerated to 200 keV. By energy-filtering only those electrons resulting from this absorption, it is possible to image directly in space the near-field electric field distribution, obtain the temporal behaviour of the field on the femtosecond timescale, and map its spatial polarization dependence. We believe that the observation of the photon-induced near-field effect in ultrafast electron microscopy demonstrates the potential for many applications, including those of direct space-time imaging of localized fields at interfaces and visualization of phenomena related to photonics, plasmonics and nanostructures.

Evidence of a Cascade and Dissipation of Solar-Wind Turbulence at the Electron Gyroscale

Abstract: We report the first direct determination of the dissipation range of magnetofluid turbulence in the solar wind at the electron scales. Combining high resolution magnetic and electric field data of the Cluster spacecraft, we computed the spectrum of turbulence and found two distinct breakpoints in the magnetic spectrum at 0.4 and 35 Hz, which correspond, respectively, to the Doppler-shifted proton and electron gyroscales, ${f}_{{\ensuremath{\rho}}_{p}}$ and ${f}_{{\ensuremath{\rho}}_{e}}$. Below ${f}_{{\ensuremath{\rho}}_{p}}$, the spectrum follows a Kolmogorov scaling ${f}^{\ensuremath{-}1.62}$, typical of spectra observed at 1 AU. Above ${f}_{{\ensuremath{\rho}}_{p}}$, a second inertial range is formed with a scaling ${f}^{\ensuremath{-}2.3}$ down to ${f}_{{\ensuremath{\rho}}_{e}}$. Above ${f}_{{\ensuremath{\rho}}_{e}}$, the spectrum has a steeper power law $\ensuremath{\sim}{f}^{\ensuremath{-}4.1}$ down to the noise level of the instrument. We interpret this as the dissipation range and show a remarkable agreement with theoretical predictions of a quasi-two-dimensional cascade into Kinetic Alfv\'en Waves (KAW).

Quantum dot sensitized solar cells. A tale of two semiconductor nanocrystals: CdSe and CdTe.

Abstract: CdSe and CdTe nanocrystals are linked to nanostructured TiO2 films using 3-mercaptopropionic acid as a linker molecule for establishing the mechanistic aspects of interfacial charge transfer processes. Both these quantum dots are energetically capable of sensitizing TiO2 films and generating photocurrents in quantum dot solar cells. These two semiconductor nanocrystals exhibit markedly different external quantum efficiencies (∼70% for CdSe and ∼0.1% for CdTe at 555 nm). Although CdTe with a more favorable conduction band energy (ECB = −1.0 V vs NHE) is capable of injecting electrons into TiO2 faster than CdSe (ECB = −0.6 V vs NHE), hole scavenging by a sulfide redox couple remains a major bottleneck. The sulfide ions dissolved in aqueous solutions are capable of scavenging photogenerated holes in photoirradiated CdSe system but not in CdTe. The anodic corrosion and exchange of Te with S dominate the charge transfer at the CdTe interface. Factors that dictate the efficiency and photostability of CdSe and C...

Impact of donor-acceptor geometry and metal chelation on photophysical properties and applications of triarylboranes.

Abstract: Three-coordinate organoboron compounds have recently found a wide range of applications in materials chemistry as nonlinear optical materials, chemical sensors, and emitters for organic light-emitting diodes (OLEDs). These compounds are excellent electron acceptors due to the empty pπ orbital on the boron center. When accompanied by electron donors such as amines, these molecules possess large electronic dipoles, which promote donor−acceptor charge-transfer upon excitation with light. Because of this, donor−acceptor triarylboranes are often highly luminescent both in the solid state and in solution. In this Account, we describe our research to develop donor−acceptor triarylboranes as efficient blue emitters for OLEDs. Through the use of hole-transporting donor groups such as 1-napthylphenylamines, we have prepared multifunctional triarylboranes that can act as the emissive, electron transport, or hole transport layers in OLEDs. We have also examined donor−acceptor compounds based on 2,2′-dipyridylamine or...

Indium tin oxide nanoparticles with compositionally tunable surface plasmon resonance frequencies in the near-IR region.

Abstract: Here we report the synthesis of conducting indium tin oxide (ITO) nanoparticles (NPs) and their surface plasmon resonance (SPR) properties. The SPR peaks of the ITO NPs can be easily tuned by changing the concentration of Sn doping from 3 to 30 mol %. The shortest SPR wavelength of 1618 nm in 10% Sn-doped ITO NPs may reflect the highest electron carrier density in the ITO NPs. The controllable SPR frequencies of metal oxides may offer a novel approach for noble-metal-free SPR applications. Unlike noble-metal nanostructures, ITO has no inter- and intraband transitions in the vis−near-IR region and represents a free-electron conduction, allowing us to systematically study the origin of optical effects arising from the SPRs of conduction electrons.

Density-functional calculations of the structure of near-surface oxygen vacancies and electron localization on CeO2(111).

Abstract: One of the most topical issues surrounding oxygen vacancies on CeO2(111) is the relative stability of surface and subsurface defects. Using density-functional theory (DFT) with the HSE06 (Heyd-Scuseria-Ernzerhof) hybrid functional as well as the DFT+U approach (where U is a Hubbard-like term describing the on-site Coulomb interactions), we find subsurface vacancies with (2x2) periodicity to be energetically more favorable by 0.45 (HSE06), 0.47 [PBE+U (Perdew-Burke-Ernzerhof functional)], and 0.22 eV [LDA+U (local density approximation)]. The excess electrons localize not on Ce ions which are the nearest neighbor to the defect as priorly suggested, but instead on those that are next-nearest neighbors. The excess-electron distribution and the preference for subsurface vacancies are explained in terms of defect-induced lattice relaxation effects.

Ultrafast Carrier Dynamics in Graphite

Abstract: Optical pump-probe spectroscopy with 7-fs pump pulses and a probe spectrum wider than 0.7 eV reveals the ultrafast carrier dynamics in freestanding thin graphite films. We discern for the first time a rapid intraband carrier equilibration within 30 fs, leaving the system with separated electron and hole chemical potentials. Phonon-mediated intraband cooling of electrons and holes occurs on a 100 fs time scale. The kinetics are in agreement with simulations based on Boltzmann equations.

Polarization Control of Electron Tunneling into Ferroelectric Surfaces

Abstract: We demonstrate a highly reproducible control of local electron transport through a ferroelectric oxide via its spontaneous polarization. Electrons are injected from the tip of an atomic force microscope into a thin film of lead-zirconate titanate, Pb(Zr0.2Ti0.8)O3, in the regime of electron tunneling assisted by a high electric field (Fowler-Nordheim tunneling). The tunneling current exhibits a pronounced hysteresis with abrupt switching events that coincide, within experimental resolution, with the local switching of ferroelectric polarization. The large spontaneous polarization of the PZT film results in up to 500-fold amplification of the tunneling current upon ferroelectric switching. The magnitude of the effect is subject to electrostatic control via ferroelectric switching, suggesting possible applications in ultrahigh-density data storage and spintronics.

Electron-electron interactions and doping dependence of the two-phonon Raman intensity in graphene

Abstract: Raman spectroscopy is a fast and nondestructive means to characterize graphene samples. In particular, the Raman spectra are strongly affected by doping. While the resulting change in position and width of the $G$ peak can be explained by the nonadiabatic Kohn anomaly at $\ensuremath{\Gamma}$, the significant doping dependence of the $2D$ peak intensity has not been understood yet. Here we show that this is due to a combination of electron-phonon and electron-electron scattering. Under full resonance, the photogenerated electron-hole pairs can scatter not just with phonons but also with doping-induced electrons or holes, and this changes the intensity. We explain the doping dependence and show how it can be used to determine the corresponding electron-phonon coupling. This is higher than predicted by density-functional theory, as a consequence of renormalization by Coulomb interactions.

Emergence of the persistent spin helix in semiconductor quantum wells

Abstract: According to Noether's theorem, for every symmetry in nature there is a corresponding conservation law. For example, invariance with respect to spatial translation corresponds to conservation of momentum. In another well-known example, invariance with respect to rotation of the electron's spin, or SU(2) symmetry, leads to conservation of spin polarization. For electrons in a solid, this symmetry is ordinarily broken by spin-orbit coupling, allowing spin angular momentum to flow to orbital angular momentum. However, it has recently been predicted that SU(2) can be achieved in a two-dimensional electron gas, despite the presence of spin-orbit coupling. The corresponding conserved quantities include the amplitude and phase of a helical spin density wave termed the 'persistent spin helix'. SU(2) is realized, in principle, when the strengths of two dominant spin-orbit interactions, the Rashba (strength parameterized by alpha) and linear Dresselhaus (beta(1)) interactions, are equal. This symmetry is predicted to be robust against all forms of spin-independent scattering, including electron-electron interactions, but is broken by the cubic Dresselhaus term (beta(3)) and spin-dependent scattering. When these terms are negligible, the distance over which spin information can propagate is predicted to diverge as alpha approaches beta(1). Here we report experimental observation of the emergence of the persistent spin helix in GaAs quantum wells by independently tuning alpha and beta(1). Using transient spin-grating spectroscopy, we find a spin-lifetime enhancement of two orders of magnitude near the symmetry point. Excellent quantitative agreement with theory across a wide range of sample parameters allows us to obtain an absolute measure of all relevant spin-orbit terms, identifying beta(3) as the main SU(2)-violating term in our samples. The tunable suppression of spin relaxation demonstrated in this work is well suited for application to spintronics.

Observing the Quantization of Zero Mass Carriers in Graphene

Abstract: Application of a magnetic field to conductors causes the charge carriers to circulate in cyclotron orbits with quantized energies called Landau levels (LLs). These are equally spaced in normal metals and two-dimensional electron gases. In graphene, however, the charge carrier velocity is independent of their energy (like massless photons). Consequently, the LL energies are not equally spaced and include a characteristic zero-energy state (the n = 0 LL). With the use of scanning tunneling spectroscopy of graphene grown on silicon carbide, we directly observed the discrete, non-equally–spaced energy-level spectrum of LLs, including the hallmark zero-energy state of graphene. We also detected characteristic magneto-oscillations in the tunneling conductance and mapped the electrostatic potential of graphene by measuring spatial variations in the energy of the n = 0 LL.

Diameter-dependent electron mobility of InAs nanowires.

Abstract: Temperature-dependent I−V and C−V spectroscopy of single InAs nanowire field-effect transistors were utilized to directly shed light on the intrinsic electron transport properties as a function of nanowire radius. From C−V characterizations, the densities of thermally activated fixed charges and trap states on the surface of untreated (i.e., without any surface functionalization) nanowires are investigated while enabling the accurate measurement of the gate oxide capacitance, therefore leading to the direct assessment of the field-effect mobility for electrons. The field-effect mobility is found to monotonically decrease as the radius is reduced to <10 nm, with the low temperature transport data clearly highlighting the drastic impact of the surface roughness scattering on the mobility degradation for miniaturized nanowires. More generally, the approach presented here may serve as a versatile and powerful platform for in-depth characterization of nanoscale, electronic materials.

Injection and Trapping of Tunnel Ionized Electrons into Laser Produced Wakes

Abstract: A method, which utilizes the large difference in ionization potentials between successive ionization states of trace atoms, for injecting electrons into a laser-driven wakefield is presented. Here a mixture of helium and trace amounts of nitrogen gas was used. Electrons from the K shell of nitrogen were tunnel ionized near the peak of the laser pulse and were injected into and trapped by the wake created by electrons from majority helium atoms and the L shell of nitrogen. The spectrum of the accelerated electrons, the threshold intensity at which trapping occurs, the forward transmitted laser spectrum, and the beam divergence are all consistent with this injection process. The experimental measurements are supported by theory and 3D OSIRIS simulations.

Pd(II)-Catalyzed Amination of C−H Bonds Using Single-Electron or Two-electron Oxidants

Abstract: Pd(II)-catalyzed intramolecular amination of arenes is developed using either a one- or two-electron oxidant. The reaction protocol tolerates a wide range of deactivating groups including acetyl, cyano, and nitro groups. This catalytic reaction allows expedient syntheses of broadly useful substituted indolines or indoles.

Laser-driven soft-X-ray undulator source

Abstract: High-intensity X-ray sources such as synchrotrons and free-electron lasers need large particle accelerators to drive them. The demonstration of a synchrotron X-ray source that uses a laser-driven particle accelerator could widen the availability of intense X-rays for research in physics, materials science and biology. Synchrotrons and free-electron lasers are the most powerful sources of X-ray radiation. They constitute invaluable tools for a broad range of research1; however, their dependence on large-scale radiofrequency electron accelerators means that only a few of these sources exist worldwide. Laser-driven plasma-wave accelerators2,3,4,5,6,7,8,9,10 provide markedly increased accelerating fields and hence offer the potential to shrink the size and cost of these X-ray sources to the university-laboratory scale. Here, we demonstrate the generation of soft-X-ray undulator radiation with laser-plasma-accelerated electron beams. The well-collimated beams deliver soft-X-ray pulses with an expected pulse duration of ∼10 fs (inferred from plasma-accelerator physics). Our source draws on a 30-cm-long undulator11 and a 1.5-cm-long accelerator delivering stable electron beams10 with energies of ∼210 MeV. The spectrum of the generated undulator radiation typically consists of a main peak centred at a wavelength of ∼18 nm (fundamental), a second peak near ∼9 nm (second harmonic) and a high-energy cutoff at ∼7 nm. Magnetic quadrupole lenses11 ensure efficient electron-beam transport and demonstrate an enabling technology for reproducible generation of tunable undulator radiation. The source is scalable to shorter wavelengths by increasing the electron energy. Our results open the prospect of tunable, brilliant, ultrashort-pulsed X-ray sources for small-scale laboratories.

Wave–particle duality of single surface plasmon polaritons

Abstract: When light interacts with metal surfaces, it excites electrons, which can form propagating excitation waves called surface plasmon polaritons. These collective electronic excitations can produce strong electric fields localized to subwavelength distance scales 1 , which makes surface plasmon polaritons interesting for several applications. Many of these potential uses, and in particular those related to quantum networks 2 , r equire a deep understanding of the fundamental quantum properties of surface plasmon polaritons. Remarkably, these collective electron states preserve many key quantum mechanical properties of the photons used to excite them, including entanglement 3,4 and sub-Poissonian statistics 5 . Here, we show that a single-photon source coupled to a silver nanowire excites single surface plasmon polaritons that exhibit both wave and particle properties, similar to those of single photons. Furthermore, the detailed analysis of the spectral interference pattern provides a new method to characterize the dimensions of metallic waveguides with nanometre accuracy.

Strong coupling between single-electron tunneling and nanomechanical motion.

Abstract: Nanoscale resonators that oscillate at high frequencies are useful in many measurement applications. We studied a high-quality mechanical resonator made from a suspended carbon nanotube driven into motion by applying a periodic radio frequency potential using a nearby antenna. Single-electron charge fluctuations created periodic modulations of the mechanical resonance frequency. A quality factor exceeding 10 5 allows the detection of a shift in resonance frequency caused by the addition of a single-electron charge on the nanotube. Additional evidence for the strong coupling of mechanical motion and electron tunneling is provided by an energy transfer to the electrons causing mechanical damping and unusual nonlinear behavior. We also discovered that a direct current through the nanotube spontaneously drives the mechanical resonator, exerting a force that is coherent with the high-frequency resonant mechanical motion.

Cosmic-ray ionization of molecular clouds

Abstract: Context Low-energy cosmic rays are a fundamental source of ionization for molecular clouds, influencing their chemical, thermal, and dynamical evolution Aims The purpose of this work is to explore the possibility that a low-energy component of cosmic rays, not directly measurable from the Earth, can account for the discrepancy between the ionization rate measured in diffuse and dense interstellar clouds Methods We collected the most recent experimental and theoretical data on the cross sections for the production of H + and He + by electron and proton impact and discuss the available constraints on the cosmic-ray fluxes in the local interstellar medium Starting from different extrapolations at low energies of the demodulated cosmic-ray proton and electron spectra, we computed the propagated spectra in molecular clouds in the continuous slowing-down approximation taking all the relevant energy loss processes into account Results The theoretical value of the cosmic-ray ionization rate as a function of the column density of traversed matter agrees with the observational data only if the flux of either cosmic-ray electrons or of protons increases at low energies The most successful models are characterized by a significant (or even dominant) contribution of the electron component to the ionization rate, in agreement with previous suggestions However, the large spread of cosmic-ray ionization rates inferred from chemical models of molecular cloud cores remains to be explained Conclusions Available data combined with simple propagation models support the existence of a low-energy component (below ∼100 MeV) of cosmic-ray electrons or protons responsible for the ionization of molecular cloud cores and dense protostellar envelopes

Spectroscopic Analysis of DA White Dwarfs: Stark Broadening of Hydrogen Lines Including Non-Ideal Effects

Abstract: We present improved calculations for the Stark broadening of hydrogen lines in dense plasmas typical of white dwarf atmospheres. Our new model is based on the unified theory of Stark broadening from Vidal, Cooper, & Smith. For the first time, we account for the non-ideal effects in a consistent way directly inside the line profile calculations. The Hummer & Mihalas theory is used to describe the non-ideal effects due to perturbations on the absorber from protons and electrons. We use a truncation of the electric microfield distribution in the quasi-static proton broadening to take into account the fact that high electric microfields dissociate the upper state of a transition. This approach represents a significant improvement over previous calculations that relied on the use of an ad hoc parameter to mimic these non-ideal effects. We obtain the first model spectra with line profiles that are consistent with the equation of state. We revisit the properties of DA stars in the range 40,000 K > Teff > 13,000 K by analyzing the optical spectra with our improved models. The updated atmospheric parameters are shown to differ substantially from those published in previous studies, with a mean mass shifted by +0.034 Msun. We also show that these revised atmospheric parameters yield absolute visual magnitudes that remain in excellent agreement with trigonometric parallax measurements.

Laser-driven plasma-wave electron accelerators

Abstract: Surfing a plasma wave, a bunch of electrons or positrons can experience much higher accelerating gradients than a conventional RF linac could provide.

Coronal Holes

Abstract: Coronal holes are the darkest and least active regions of the Sun, as observed both on the solar disk and above the solar limb. Coronal holes are associated with rapidly expanding open magnetic fields and the acceleration of the high-speed solar wind. This paper reviews measurements of the plasma properties in coronal holes and how these measurements are used to reveal details about the physical processes that heat the solar corona and accelerate the solar wind. It is still unknown to what extent the solar wind is fed by flux tubes that remain open (and are energized by footpoint-driven wave-like fluctuations), and to what extent much of the mass and energy is input intermittently from closed loops into the open-field regions. Evidence for both paradigms is summarized in this paper. Special emphasis is also given to spectroscopic and coronagraphic measurements that allow the highly dynamic non-equilibrium evolution of the plasma to be followed as the asymptotic conditions in interplanetary space are established in the extended corona. For example, the importance of kinetic plasma physics and turbulence in coronal holes has been affirmed by surprising measurements from UVCS that heavy ions are heated to hundreds of times the temperatures of protons and electrons. These observations point to specific kinds of collisionless Alfven wave damping (i.e., ion cyclotron resonance), but complete models do not yet exist. Despite our incomplete knowledge of the complex multi-scale plasma physics, however, much progress has been made toward the goal of understanding the mechanisms responsible for producing the observed properties of coronal holes.

Superconductivity at the Two-Dimensional Limit

Abstract: Superconductivity in the extreme two-dimensional limit is studied on ultrathin lead films down to two atomic layers, where only a single channel of quantum well states exists. Scanning tunneling spectroscopy reveals that local superconducting order remains robust until two atomic layers, where the transition temperature abruptly plunges to a lower value, depending sensitively on the exact atomic structure of the film. Our result shows that Cooper pairs can still form in the last two-dimensional channel of electron states, although their binding is strongly affected by the substrate.

Calculation of One-Electron Redox Potentials Revisited. Is It Possible to Calculate Accurate Potentials with Density Functional Methods?

Abstract: Density Functional calculations have been performed to calculate the one-electron oxidation potential for ferrocene and the redox couples for a series of small transition metal compounds of the first-, second-, and third-row elements. The solvation effects are incorporated via a self-consistent reaction field (SCRF), using the polarized continuum model (PCM). From our study of seven different density functionals combined with three different basis sets for ferrocene, we find that no density functional method can reproduce the redox trends from experiment when referencing our results to the experimental absolute standard hydrogen electrode (SHE) potential. In addition, including additional necessary assumptions such as solvation effects does not lead to any conclusion regarding the appropriate functional. However, we propose that if one references their transition metal compounds results to the calculated absolute half-cell potential of ferrocene, they can circumvent the additional assumptions necessary to...

Near-GeV Acceleration of Electrons by a Nonlinear Plasma Wave Driven by a Self-Guided Laser Pulse

Abstract: The acceleration of electrons to approximately 0.8 GeV has been observed in a self-injecting laser wakefield accelerator driven at a plasma density of 5.5x10(18) cm(-3) by a 10 J, 55 fs, 800 nm laser pulse in the blowout regime. The laser pulse is found to be self-guided for 1 cm (>10zR), by measurement of a single filament containing >30% of the initial laser energy at this distance. Three-dimensional particle in cell simulations show that the intensity within the guided filament is amplified beyond its initial focused value to a normalized vector potential of a0>6, thus driving a highly nonlinear plasma wave.

Study of runaway electron behaviour during electron cyclotron resonance heating in the HL-2A Tokamak

Abstract: During the current flat-top phase of electron cyclotron resonance heating discharges in the HL-2A Tokamak, the behaviour of runaway electrons has been studied by means of hard x-ray detectors and neutron diagnostics. During electron cyclotron resonance heating, it can be found that both hard x-ray radiation intensity and neutron emission flux fall rapidly to a very low level, which suggests that runaway electrons have been suppressed by electron cyclotron resonance heating. From the set of discharges studied in the present experiments, it has also been observed that the efficiency of runaway suppression by electron cyclotron resonance heating was apparently affected by two factors: electron cyclotron resonance heating power and duration. These results have been analysed by using a test particle model. The decrease of the toroidal electric field due to electron cyclotron resonance heating results in a rapid fall in the runaway electron energy that may lead to a suppression of runaway electrons. During electron cyclotron resonance heating with different powers and durations, the runaway electrons will experience different slowing down processes. These different decay processes are the major cause for influencing the efficiency of runaway suppression. This result is related to the safe operation of the Tokamak and may bring an effective control of runaway electrons.

Reconstruction of molecular orbital densities from photoemission data.

Abstract: Photoemission spectroscopy is commonly applied to study the band structure of solids by measuring the kinetic energy versus angular distribution of the photoemitted electrons. Here, we apply this experimental technique to characterize discrete orbitals of large π-conjugated molecules. By measuring the photoemission intensity from a constant initial-state energy over a hemispherical region, we generate reciprocal space maps of the emitting orbital density. We demonstrate that the real-space electron distribution of molecular orbitals in both a crystalline pentacene film and a chemisorbed p-sexiphenyl monolayer can be obtained from a simple Fourier transform of the measurement data. The results are in good agreement with density functional calculations.