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Recycling of Spent Lithium-Ion Battery: A Critical Review

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TLDR
In this article, the authors review the current status of the recycling processes of spent lithium ion batteries, introduce the structure and components of the batteries, and summarize all available single contacts in batch mode operation, including pretreatment, secondary treatment, and deep recovery.
Abstract
Lithium-ion battery (LIB) applications in consumer electronics and electric vehicles are rapidly growing, resulting in boosting resources demand, including cobalt and lithium. So recycling of batteries will be a necessity, not only to decline the consumption of energy, but also to relieve the shortage of rare resources and eliminate the pollution of hazardous components, toward sustainable industries related to consumer electronics and electric vehicles. The authors review the current status of the recycling processes of spent LIBs, introduce the structure and components of the batteries, and summarize all available single contacts in batch mode operation, including pretreatment, secondary treatment, and deep recovery. Additionally, many problems and prospect of the current recycling processes will be presented and analyzed. It is hoped that this effort would stimulate further interest in spent LIBs recycling and in the appreciation of its benefits.

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Citations
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Journal ArticleDOI

Recovery of Li(Ni0.33Mn0.33Co0.33)O2 from Lithium-Ion Battery Cathodes: Aspects of Degradation

TL;DR: This work presented an approach to recover NMC particles from spent lithium-ion battery cathodes while preserving their chemical and morphological properties, with a minimal use of chemicals.
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Understanding the effect of nonmetallic impurities in regenerated cathode materials for lithium-ion battery recycling by tracking down impurity elements

TL;DR: In this article, Li[NixMnyCoz]O2 (NMC) is regenerated from actual industrial scale leachates and purified leachate to investigate the precipitation behavior of impurities, which include potentially toxic elements, such as F, Cl, and S. This categorization of impurity elements will certainly provide the LIB recycling industry with a valuable quality control guide.
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Maleic, glycolic and acetoacetic acids-leaching for recovery of valuable metals from spent lithium-ion batteries: leaching parameters, thermodynamics and kinetics.

TL;DR: The kinetic study showed that the leaching processes fit well with the shrinking-core model, and the efficacy and availability of the three acids is as follows: maleic acid > acetoacetic acid > glycolic acid.
References
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Journal ArticleDOI

Issues and challenges facing rechargeable lithium batteries

TL;DR: A brief historical review of the development of lithium-based rechargeable batteries is presented, ongoing research strategies are highlighted, and the challenges that remain regarding the synthesis, characterization, electrochemical performance and safety of these systems are discussed.
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Building better batteries

TL;DR: Researchers must find a sustainable way of providing the power their modern lifestyles demand to ensure the continued existence of clean energy sources.
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Electrical Energy Storage for the Grid: A Battery of Choices

TL;DR: The battery systems reviewed here include sodium-sulfur batteries that are commercially available for grid applications, redox-flow batteries that offer low cost, and lithium-ion batteries whose development for commercial electronics and electric vehicles is being applied to grid storage.
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Nonaqueous liquid electrolytes for lithium-based rechargeable batteries.

TL;DR: The phytochemical properties of Lithium Hexafluoroarsenate and its Derivatives are as follows: 2.2.1.
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Electrodes with high power and high capacity for rechargeable lithium batteries.

TL;DR: By modifying its crystal structure, lithium nickel manganese oxide is obtained unexpectedly high rate-capability, considerably better than lithium cobalt oxide (LiCoO2), the current battery electrode material of choice.
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