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Showing papers on "Laser linewidth published in 2017"


Journal ArticleDOI
TL;DR: In this article, the authors show that encapsulation of monolayer MoS2 in hexagonal boron nitride can efficiently suppress the inhomogeneous contribution to the exciton linewidth, as they measure in photoluminescence and reflectivity a FWHM down to 2 meV at T=4
Abstract: The strong light-matter interaction and the valley selective optical selection rules make monolayer (ML) MoS2 an exciting 2D material for fundamental physics and optoelectronics applications. But, so far, optical transition linewidths even at low temperature are typically as large as a few tens of meV and contain homogeneous and inhomogeneous contributions. This prevented in-depth studies, in contrast to the better-characterized ML materials MoSe2 and WSe2. In this work, we show that encapsulation of ML MoS2 in hexagonal boron nitride can efficiently suppress the inhomogeneous contribution to the exciton linewidth, as we measure in photoluminescence and reflectivity a FWHM down to 2 meV at T=4 K. Narrow optical transition linewidths are also observed in encapsulated WS2, WSe2, and MoSe2 MLs. This indicates that surface protection and substrate flatness are key ingredients for obtaining stable, high-quality samples. Among the new possibilities offered by the well-defined optical transitions, we measure the homogeneous broadening induced by the interaction with phonons in temperature-dependent experiments. We uncover new information on spin and valley physics and present the rotation of valley coherence in applied magnetic fields perpendicular to the ML.

540 citations


Journal ArticleDOI
TL;DR: Two ultrastable lasers stabilized to single-crystal silicon Fabry-Pérot cavities at 124 K show unprecedented thermal noise-limited frequency instabilities of 4×10 and linewidths below 10 mHz.
Abstract: We report on two ultrastable lasers each stabilized to independent silicon Fabry-Perot cavities operated at 124 K. The fractional frequency instability of each laser is completely determined by the fundamental thermal Brownian noise of the mirror coatings with a flicker noise floor of 4×10^{-17} for integration times between 0.8 s and a few tens of seconds. We rigorously treat the notorious divergences encountered with the associated flicker frequency noise and derive methods to relate this noise to observable and practically relevant linewidths and coherence times. The individual laser linewidth obtained from the phase noise spectrum or the direct beat note between the two lasers can be as small as 5 mHz at 194 THz. From the measured phase evolution between the two laser fields we derive usable phase coherence times for different applications of 11 to 55 s.

340 citations


Journal ArticleDOI
26 May 2017-Science
TL;DR: A quantum sensing protocol is demonstrated in which the spectral precision goes beyond the sensor coherence time and is limited by the stability of a classical clock.
Abstract: Precise timekeeping is critical to metrology, forming the basis by which standards of time, length, and fundamental constants are determined Stable clocks are particularly valuable in spectroscopy because they define the ultimate frequency precision that can be reached In quantum metrology, the qubit coherence time defines the clock stability, from which the spectral linewidth and frequency precision are determined We demonstrate a quantum sensing protocol in which the spectral precision goes beyond the sensor coherence time and is limited by the stability of a classical clock Using this technique, we observed a precision in frequency estimation scaling in time T as T –3/2 for classical oscillating fields The narrow linewidth magnetometer based on single spins in diamond is used to sense nanoscale magnetic fields with an intrinsic frequency resolution of 607 microhertz, which is eight orders of magnitude narrower than the qubit coherence time

326 citations


Journal ArticleDOI
07 Jul 2017-Science
TL;DR: This work combines the use of a quantum memory and high magnetic fields with a dedicated quantum sensor based on nitrogen vacancy centers in diamond to achieve chemical shift resolution in 1H and 19F NMR spectroscopy of 20-zeptoliter sample volumes.
Abstract: Nuclear magnetic resonance (NMR) spectroscopy is a key analytical technique in chemistry, biology, and medicine However, conventional NMR spectroscopy requires an at least nanoliter-sized sample volume to achieve sufficient signal We combined the use of a quantum memory and high magnetic fields with a dedicated quantum sensor based on nitrogen vacancy centers in diamond to achieve chemical shift resolution in 1H and 19F NMR spectroscopy of 20-zeptoliter sample volumes We demonstrate the application of NMR pulse sequences to achieve homonuclear decoupling and spin diffusion measurements The best measured NMR linewidth of a liquid sample was ~1 part per million, mainly limited by molecular diffusion To mitigate the influence of diffusion, we performed high-resolution solid-state NMR by applying homonuclear decoupling and achieved a 20-fold narrowing of the NMR linewidth

292 citations


Journal ArticleDOI
20 Mar 2017-Nature
TL;DR: A way to decrease the band-edge degeneracy and single-dot photoluminescence linewidth in CQDs by means of uniform biaxial strain is demonstrated and continuous-wave lasing from CQD solids is demonstrated, expanding the library of solution-processed materials that may be capable of continuous- wave lasing.
Abstract: By switching shell growth on and off on the (0001) facet of wurtzite CdSe cores to produce a built-in biaxial strain that lowers the optical gain threshold, we achieve continuous-wave lasing in colloidal quantum dot films. The electronic structure of colloidal quantum dots lends them a host of desirable optical properties, but they typically perform poorly as laser materials. Fengjia Fan et al. have developed a scheme for tuning this electronic structure in such a way that the barriers to laser action might be overcome. Specifically, they developed a synthesis strategy in which the shell of material encompassing the core of the quantum dot is asymmetric and compressive. This effectively squeezes the particle, thereby modifying the electronic structure to favour laser-like emissions. Colloidal quantum dots (CQDs) feature a low degeneracy of electronic states at the band edges compared with the corresponding bulk material1, as well as a narrow emission linewidth2,3. Unfortunately for potential laser applications, this degeneracy is incompletely lifted in the valence band, spreading the hole population among several states at room temperature4,5,6. This leads to increased optical gain thresholds, demanding high photoexcitation levels to achieve population inversion (more electrons in excited states than in ground states—the condition for optical gain). This, in turn, increases Auger recombination losses7, limiting the gain lifetime to sub-nanoseconds and preventing steady laser action8,9. State degeneracy also broadens the photoluminescence linewidth at the single-particle level10. Here we demonstrate a way to decrease the band-edge degeneracy and single-dot photoluminescence linewidth in CQDs by means of uniform biaxial strain. We have developed a synthetic strategy that we term facet-selective epitaxy: we first switch off, and then switch on, shell growth on the (0001) facet of wurtzite CdSe cores, producing asymmetric compressive shells that create built-in biaxial strain, while still maintaining excellent surface passivation (preventing defect formation, which otherwise would cause non-radiative recombination losses). Our synthesis spreads the excitonic fine structure uniformly and sufficiently broadly that it prevents valence-band-edge states from being thermally depopulated. We thereby reduce the optical gain threshold and demonstrate continuous-wave lasing from CQD solids, expanding the library of solution-processed materials11,12 that may be capable of continuous-wave lasing. The individual CQDs exhibit an ultra-narrow single-dot linewidth, and we successfully propagate this into the ensemble of CQDs.

291 citations


Journal ArticleDOI
24 Jul 2017
TL;DR: In this article, the authors report methods for fabricating high quality TMDC monolayers with narrow photoluminescence (PL) linewidth approaching the intrinsic limit, using encapsulation in hexagonal boron nitride (h-BN) and passivation of the oxide substrate by an alkyl monolayer.
Abstract: Excitonic states in monolayer transition metal dichalcogenides (TMDCs) have been the subject of extensive recent interest. Their intrinsic properties can, however, be obscured due to the influence of inhomogeneity in the external environment. Here we report methods for fabricating high quality TMDC monolayers with narrow photoluminescence (PL) linewidth approaching the intrinsic limit. We find that encapsulation in hexagonal boron nitride (h-BN) sharply reduces the PL linewidth, and that passivation of the oxide substrate by an alkyl monolayer further decreases the linewidth and also minimizes the charged exciton (trion) peak. The combination of these sample preparation methods results in much reduced spatial variation in the PL emission, with a full-width-at-half-maximum as low as 1.7 meV. Analysis of the PL line shape yields a homogeneous width of 1.43 ± 0.08 meV and inhomogeneous broadening of 1.1 ± 0.3 meV.

267 citations


Journal ArticleDOI
TL;DR: In this article, the authors show that encapsulation of monolayer MoS2 in hexagonal boron nitride can efficiently suppress the inhomogeneous contribution to the exciton linewidth, as measured in photoluminescence and reflectivity a FWHM down to 2 meV at T = 4K.
Abstract: The strong light matter interaction and the valley selective optical selection rules make monolayer (ML) MoS2 an exciting 2D material for fundamental physics and optoelectronics applications. But so far optical transition linewidths even at low temperature are typically as large as a few tens of meV and contain homogenous and inhomogeneous contributions. This prevented in-depth studies, in contrast to the better-characterized ML materials MoSe2 and WSe2. In this work we show that encapsulation of ML MoS2 in hexagonal boron nitride can efficiently suppress the inhomogeneous contribution to the exciton linewidth, as we measure in photoluminescence and reflectivity a FWHM down to 2 meV at T = 4K. This indicates that surface protection and substrate flatness are key ingredients for obtaining stable, high quality samples. Among the new possibilities offered by the well-defined optical transitions we measure the homogeneous broadening induced by the interaction with phonons in temperature dependent experiments. We uncover new information on spin and valley physics and present the rotation of valley coherence in applied magnetic fields perpendicular to the ML.

263 citations


Journal ArticleDOI
TL;DR: TMDs are established as practical materials for integrated TMD-silicon nanolasers suitable for silicon-based nanophotonic applications in silicon-transparent wavelengths with the largest value reported for a TMD laser.
Abstract: Monolayer transition-metal dichalcogenides (TMDs) have the potential to become efficient optical-gain materials for low-energy-consumption nanolasers with the smallest gain media because of strong excitonic emission. However, until now TMD-based lasing has been realized only at low temperatures. Here we demonstrate for the first time a room-temperature laser operation in the infrared region from a monolayer of molybdenum ditelluride on a silicon photonic-crystal cavity. The observation is enabled by the unique combination of a TMD monolayer with an emission wavelength transparent to silicon, and a high-Q cavity of the silicon nanobeam. The laser is pumped by a continuous-wave excitation, with a threshold density of 6.6 W cm-2. Its linewidth is as narrow as 0.202 nm with a corresponding Q of 5,603, the largest value reported for a TMD laser. This demonstration establishes TMDs as practical materials for integrated TMD-silicon nanolasers suitable for silicon-based nanophotonic applications in silicon-transparent wavelengths.

249 citations


Journal ArticleDOI
TL;DR: Lim et al. as discussed by the authors show the noise characteristics of whispering gallery-mode resonators and demonstrate a resonator-stabilized laser at this limit by compensating the intrinsic thermal expansion, allowing a sub-25'Hz linewidth and a 32'Hz Allan deviation.
Abstract: Ultrastable high-spectral-purity lasers have served as the cornerstone behind optical atomic clocks, quantum measurements, precision optical microwave generation, high-resolution optical spectroscopy, and sensing. Hertz-level lasers stabilized to high-finesse Fabry-Perot cavities are typically used for these studies, which are large and fragile and remain laboratory instruments. There is a clear demand for rugged miniaturized lasers with stabilities comparable to those of bulk lasers. Over the past decade, ultrahigh-Q optical whispering-gallery-mode resonators have served as a platform for low-noise microlasers but have not yet reached the stabilities defined by their fundamental noise. Here, we show the noise characteristics of whispering-gallery-mode resonators and demonstrate a resonator-stabilized laser at this limit by compensating the intrinsic thermal expansion, allowing a sub-25 Hz linewidth and a 32 Hz Allan deviation. We also reveal the environmental sensitivities of the resonator at the thermodynamical noise limit and long-term frequency drifts governed by random-walk-noise statistics.High-quality optical resonators have the potential to provide a miniaturized frequency reference for metrology and sensing but they often lack stability. Here, Lim et al. experimentally characterize the stability of whispering-gallery resonators at their fundamental noise limits.

195 citations


Journal ArticleDOI
TL;DR: In this paper, a narrow linewidth magnetometer based on single spins in diamond is used to sense nanoscale magnetic fields with an intrinsic frequency resolution of 607 $\mu$Hz, 8 orders of magnitude narrower than the qubit coherence time.
Abstract: Precise timekeeping is critical to metrology, forming the basis by which standards of time, length and fundamental constants are determined. Stable clocks are particularly valuable in spectroscopy as they define the ultimate frequency precision that can be reached. In quantum metrology, where the phase of a qubit is used to detect external fields, the clock stability is defined by the qubit coherence time, which determines the spectral linewidth and frequency precision. Here we demonstrate a quantum sensing protocol where the spectral precision goes beyond the sensor coherence time and is limited by the stability of a classical clock. Using this technique, we observe a precision in frequency estimation scaling in time $T$, as $T^{-3/2}$ for classical oscillating fields. The narrow linewidth magnetometer based on single spins in diamond is used to sense nanoscale magnetic fields with an intrinsic frequency resolution of 607 $\mu$Hz, 8 orders of magnitude narrower than the qubit coherence time.

187 citations


Posted Content
TL;DR: In this paper, the authors report methods for fabricating high quality TMDC monolayers with narrow photoluminescence (PL) linewidth approaching the intrinsic limit, using encapsulation in hexagonal boron nitride (h-BN) and passivation of the oxide substrate by an alkyl monolayer.
Abstract: Excitonic states in monolayer transition metal dichalcogenides (TMDCs) have been the subject of extensive recent interest. Their intrinsic properties can, however, be obscured due to the influence of inhomogeneity in the external environment. Here we report methods for fabricating high quality TMDC monolayers with narrow photoluminescence (PL) linewidth approaching the intrinsic limit. We find that encapsulation in hexagonal boron nitride (h-BN) sharply reduces the PL linewidth, and that passivation of the oxide substrate by an alkyl monolayer further decreases the linewidth and also minimizes the charged exciton (trion) peak. The combination of these sample preparation methods results in much reduced spatial variation in the PL emission, with a full-width-at-half-maximum as low as 1.7 meV. Analysis of the PL line shape yields a homogeneous width of 1.43$\pm$0.08 meV and inhomogeneous broadening of 1.1$\pm$0.3 meV.

Journal ArticleDOI
TL;DR: In this paper, a silicon-based Brillouin laser oscillator was demonstrated to produce phonon linewidth narrowing in the presence of optical self-oscillation, and the results provided a platform to develop a range of applications for monolithic integration within silicon photonic circuits.
Abstract: Brillouin laser oscillators offer powerful and flexible dynamics as the basis for mode-locked lasers, microwave oscillators, and optical gyroscopes in a variety of optical systems. However, Brillouin interactions are exceedingly weak in conventional silicon photonic waveguides, stifling progress towards silicon-based Brillouin lasers. The recent advent of hybrid photonic-phononic waveguides has revealed Brillouin interactions to be one of the strongest and most tailorable nonlinearities in silicon. Here, we harness these engineered nonlinearities to demonstrate Brillouin lasing in silicon. Moreover, we show that this silicon-based Brillouin laser enters an intriguing regime of dynamics, in which optical self-oscillation produces phonon linewidth narrowing. Our results provide a platform to develop a range of applications for monolithic integration within silicon photonic circuits.

Journal ArticleDOI
TL;DR: In this paper, the analysis of the self-injection locking of a single-frequency laser diode to a high-Q whispering gallery mode (WGM) microresonator with Rayleigh backscattering is presented.
Abstract: We present the analysis of the self-injection locking of a single-frequency laser diode to a high-Q whispering gallery mode (WGM) microresonator with Rayleigh backscattering. Simple analytical formulas for the width of the locking band and resulting laser linewidth are derived.

Journal ArticleDOI
TL;DR: The noise characteristics of whispering-gallery-mode resonators are shown and a resonator-stabilized laser at this limit is demonstrated by compensating the intrinsic thermal expansion, allowing a sub-25 Hz linewidth and a 32 Hz Allan deviation.
Abstract: Ultrastable high-spectral-purity lasers have served as the cornerstone behind optical atomic clocks, quantum measurements, precision optical-microwave generation, high resolution optical spectroscopy and sensing. Hertz-level lasers stabilized to high finesse Fabry-Perot mirror cavities are typically used for these studies but are large and fragile such that they have remained laboratory instruments. There is a clear demand in rugged miniaturized lasers operating potentially at comparable stabilities to those bulk lasers. Over the past decade, ultrahigh-Q optical whispering-gallery-mode (WGM) resonators have served as a platform for low-noise microlasers but have not yet reached the ultimate stabilities defined by their fundamental noise. Here, we show the noise characteristics of WGM resonators and demonstrate a resonator-stabilized laser at the fundamental limit by compensating the intrinsic thermal expansion of a WGM resonator, allowing a sub-25 Hz linewidth and a 32 Hz Allan deviation on the 191 THz carrier in 100 ms integration. We also reveal the environmental sensitivities of the resonator at the thermodynamical noise limit and long-term frequency drifts governed by random-walk-noise statistics.

Journal ArticleDOI
TL;DR: In this article, the recent advances of single-frequency fiber oscillators and amplifiers are briefly reviewed in the broad wavelength region of 1-3 μm. And the solution to achieving higher power/energy is also discussed, accompanied by the start-of-the-art results achieved to date.
Abstract: Single-frequency fiber lasers have drawn intense attention for their extensive applications from high-resolution spectroscopy and gravitational wave detection to materials processing due to the outstanding properties of low noise, narrow linewidth, and the resulting long coherence length. In this paper, the recent advances of single-frequency fiber oscillators and amplifiers are briefly reviewed in the broad wavelength region of 1–3 μm. Performance improvements in laser noise and linewidth are addressed with the newly developed physical mechanisms. The solution to achieving higher power/energy is also discussed, accompanied by the start-of-the-art results achieved to date.

Journal ArticleDOI
TL;DR: In this article, the authors studied the lattice modes supported by gold and aluminum nanoparticle arrays in the visible and UV, both experimentally and theoretically, and provided design rules for high quality factor resonances.
Abstract: Metallic nanoparticles arranged in arrays have been shown to support both localized surface plasmons (LSPs) and diffractive grating behavior, related to the inter-particle period. By selecting both the period and particle size, it is possible to generate lattice modes that are caused by interference of the LSP and the grating Rayleigh anomaly. These hybrid modes show a Fano-like lineshape with reduced linewidth relative to the LSP mode. In this paper, we study the lattice modes supported by gold and aluminum nanoparticle arrays in the visible and UV, both experimentally and theoretically. The measured and simulated dispersion curves allow us to comprehensively analyze the details of the LSP coupling in the array. We show that when the spectral position of the Rayleigh anomaly, dependent on the period of the array, is slightly blue-shifted with respect to the LSP resonance, the quality factor of the lattice mode is significantly increased. We also provide evidence that the formation of the lattice modes critically depends on the incident light polarization, with maximum coupling efficiency between LSPs and the in-plane scattered light when the polarization direction is perpendicular to the propagation direction of the grazing wave. The results obtained provide design rules for high quality factor resonances throughout the visible and ultraviolet spectral ranges.

Proceedings ArticleDOI
14 May 2017
TL;DR: In this paper, two ultrastable lasers were stabilized to single-crystal silicon Fabry-Perot cavities at 124 K. The lasers show unprecedented thermal noise-limited frequency instabilities of 4×10−17 and linewidths below 10 mHz.
Abstract: We report on two ultrastable lasers stabilized to single-crystal silicon Fabry-Perot cavities at 124 K. The lasers show unprecedented thermal noise-limited frequency instabilities of 4×10−17 and linewidths below 10 mHz.

Journal ArticleDOI
TL;DR: A high slope efficiency of 90% with diffraction-limited beam quality and without any sign of TMI or stimulated Raman scattering for a spectral dynamic range of higher than -80 dB was obtained.
Abstract: We investigate the average power scaling of two diode-pumped Yb-doped fiber amplifiers emitting a diffraction-limited beam. The first fiber under investigation with a core diameter of 30 µm was able to amplify a 10 W narrow linewidth seed laser up to 2.8 kW average output power before the onset of transverse mode instabilities (TMI). A further power scaling was achieved using a second fiber with a smaller core size (23µm), which allowed for a narrow linewidth output power of 3.5 kW limited by stimulated Brillouin scattering (SBS). We mitigated SBS using a spectral broadening mechanism, which allowed us to further increase the output power to 4.3 kW only limited by the available pump power. Up to this power level, a high slope efficiency of 90% with diffraction-limited beam quality and without any sign of TMI or stimulated Raman scattering for a spectral dynamic range of higher than -80 dB was obtained.

Journal ArticleDOI
TL;DR: A demonstration of a III-V-on-Si comb laser that can function as a compact, low-cost frequency comb generator after frequency stabilization and the use of low-loss passive silicon waveguides enables the integration of a long laser cavity, which enables the laser to be locked in the passive mode at a record-low 1 GHz repetition rate.
Abstract: Optical frequency combs emerge as a promising technology that enables highly sensitive, near-real-time spectroscopy with a high resolution The currently available comb generators are mostly based on bulky and high-cost femtosecond lasers for dense comb generation (line spacing in the range of 100 MHz to 1 GHz) However, their integrated and low-cost counterparts, which are integrated semiconductor mode-locked lasers, are limited by their large comb spacing, small number of lines and broad optical linewidth In this study, we report a demonstration of a III-V-on-Si comb laser that can function as a compact, low-cost frequency comb generator after frequency stabilization The use of low-loss passive silicon waveguides enables the integration of a long laser cavity, which enables the laser to be locked in the passive mode at a record-low 1 GHz repetition rate The 12-nm 10-dB output optical spectrum and the notably small optical mode spacing results in a dense optical comb that consists of over 1400 equally spaced optical lines The sub-kHz 10-dB radio frequency linewidth and the narrow longitudinal mode linewidth (<400 kHz) indicate notably stable mode-locking Such integrated dense comb lasers are very promising, for example, for high-resolution and real-time spectroscopy applications

Journal ArticleDOI
TL;DR: An integrated silicon nitride/III-V laser leveraging the narrowband backreflection of a high-Q microring resonator for output coupling and feedback is demonstrated.
Abstract: We design and demonstrate a compact, narrow-linewidth integrated laser based on low-loss silicon nitride waveguides coupled to a III-V gain chip. By using a highly confined optical mode, we simultaneously achieve compact bends and ultra-low loss. We leverage the narrowband backreflection of a high-Q microring resonator to act as a cavity output mirror, a single-mode filter, and a propagation delay all in one. This configuration allows the ring to provide feedback and obtain a laser linewidth of 13 kHz with 1.7 mW output power around 1550 nm. This demonstration realizes a compact sub-millimeter silicon nitride laser cavity with a narrow linewidth.

Proceedings ArticleDOI
TL;DR: In this paper, the authors investigated the microscopic origin of the homogeneous linewidth and coherence lifetime of excitonic resonances in monolayer molybdenum disulfide, taking exciton phonon scattering and radiative recombination into account.
Abstract: Monolayers of transition metal dichalcogenides are direct gap semiconductors, which have attracted much attention in the recent past. Due to a strong Coulomb interaction, they possess strongly bound electron-hole pairs, with binding energies of hundreds of meV which is an order of magnitude larger than in conventional materials. Here, we investigate the microscopic origin of the homogeneous linewidth and coherence lifetime of excitonic resonances in monolayer molybdenum disulfide, taking exciton phonon scattering and radiative recombination into account. We find a superlinear increasing homogeneous linewidth from 2 meV at 5K to 14 meV at room temperature corresponding to a coherence lifetime of 160 fs and 25 fs.

Journal ArticleDOI
TL;DR: This work uses a fibre-coupled integrating sphere to generate wavelength-dependent speckle patterns, in combination with algorithms based on the transmission matrix method and principal component analysis, to realize a broadband and sensitive wavemeter that compares favourably to the performance of conventional wavemeters.
Abstract: The accurate determination and control of the wavelength of light is fundamental to many fields of science. Speckle patterns resulting from the interference of multiple reflections in disordered media are well-known to scramble the information content of light by complex but linear processes. However, these patterns are, in fact, exceptionally rich in information about the illuminating source. We use a fibre-coupled integrating sphere to generate wavelength-dependent speckle patterns, in combination with algorithms based on the transmission matrix method and principal component analysis, to realize a broadband and sensitive wavemeter. We demonstrate sub-femtometre wavelength resolution at a centre wavelength of 780 nm, and a broad calibrated measurement range from 488 to 1,064 nm. This compares favourably to the performance of conventional wavemeters. Using this speckle wavemeter as part of a feedback loop, we stabilize a 780 nm diode laser to achieve a linewidth better than 1 MHz.

Journal ArticleDOI
TL;DR: In this article, the authors demonstrate strong coupling between the charge degree of freedom in a gate-detuned GaAs double quantum dot (DQD) and a frequency-tunable high impedance resonator realized using an array of superconducting quantum interference devices (SQUIDs).
Abstract: The strong coupling limit of cavity quantum electrodynamics (QED) implies the capability of a matter-like quantum system to coherently transform an individual excitation into a single photon within a resonant structure. This not only enables essential processes required for quantum information processing but also allows for fundamental studies of matter-light interaction. In this work we demonstrate strong coupling between the charge degree of freedom in a gate-detuned GaAs double quantum dot (DQD) and a frequency-tunable high impedance resonator realized using an array of superconducting quantum interference devices (SQUIDs). In the resonant regime, we resolve the vacuum Rabi mode splitting of size $2g/2\pi = 238$ MHz at a resonator linewidth $\kappa/2\pi = 12$ MHz and a DQD charge qubit dephasing rate of $\gamma_2/2\pi = 80$ MHz extracted independently from microwave spectroscopy in the dispersive regime. Our measurements indicate a viable path towards using circuit based cavity QED for quantum information processing in semiconductor nano-structures.

Journal ArticleDOI
TL;DR: In this paper, a new method of spectrally resolved photon-induced near-field electron microscopy (SRPINEM) was proposed to obtain nm-fs-resolved maps of nanoparticle plasmons with an energy resolution determined by the laser linewidth.
Abstract: The electronic, optical, and magnetic properties of quantum solids are determined by their low-energy (< 100 meV) many-body excitations. Dynamical characterization and manipulation of such excitations relies on tools that combine nm-spatial, fs-temporal, and meV-spectral resolution. Currently, phonons and collective plasmon resonances can be imaged in nanostructures with sub-nm and 10s meV space/energy resolution using state-of-the-art energy-filtered transmission electron microscopy (TEM), but only under static conditions, while fs-resolved measurements are common but lack spatial or energy resolution. Here, we demonstrate a new method of spectrally resolved photon-induced near-field electron microscopy (SRPINEM) that allows us to obtain nm-fs-resolved maps of nanoparticle plasmons with an energy resolution determined by the laser linewidth (20 meV in this work), and not limited by electron beam and spectrometer energy spreading. This technique can be extended to any optically-accessible low-energy mode, thus pushing TEM to a previously inaccessible spectral domain with an unprecedented combination of space, energy and temporal resolution.

Journal ArticleDOI
TL;DR: This work achieves narrow-linewidth visible-frequency lasing at room temperature by leveraging surface plasmons propagating in an open Fabry-Perot cavity formed by a flat metal surface coated with a subwavelength-thick layer of optically pumped gain medium and orthogonally bound by a pair of flat metal sidewalls.
Abstract: Recent years have witnessed a growing interest in the development of small-footprint lasers for potential applications in small-volume sensing and on-chip optical communications. Surface plasmons—electromagnetic modes evanescently confined to metal-dielectric interfaces—offer an effective route to achieving lasing at nanometer-scale dimensions when resonantly amplified in contact with a gain medium. We achieve narrow-linewidth visible-frequency lasing at room temperature by leveraging surface plasmons propagating in an open Fabry-Perot cavity formed by a flat metal surface coated with a subwavelength-thick layer of optically pumped gain medium and orthogonally bound by a pair of flat metal sidewalls. We show how the lasing threshold and linewidth can be lowered by incorporating a low-profile tapered grating on the cavity floor to couple the excitation beam into a pump surface plasmon polariton providing a strong modal overlap with the gain medium. Low-perturbation transmission-configuration sampling of the lasing plasmon mode is achieved via an evanescently coupled recessed nanoslit, opening the way to high–figure of merit refractive index sensing of analytes interacting with the open metallic trench.

Journal ArticleDOI
TL;DR: In this paper, the authors demonstrate an experimental study on scaling mode instability (MI) threshold in fiber amplifiers based on fiber coiling and show that coiling the active fiber in the cylindrical spiral shape is superior to the coiling in the plane spiral shape.
Abstract: We demonstrate an experimental study on scaling mode instability (MI) threshold in fiber amplifiers based on fiber coiling. The experimental results show that coiling the active fiber in the cylindrical spiral shape is superior to the coiling in the plane spiral shape. When the polarization maintained Yb-doped fiber (PM YDF: with a core/inner-cladding diameter of 20/400 ?m) is coiled on an aluminous plate with a bend diameter of 9?16?cm, the MI threshold is ~1.55 kW. When such a PM YDF is coiled on an aluminous cylinder with diameter of 9?cm, no MI is observed at the output power of 2.43 kW, which is limited by the available pump power. The spectral width and polarization extinction ratio is 0.255?nm and 18.3 dB, respectively, at 2.43 kW. To the best of our knowledge, this is the highest output power from a linear polarized narrow linewidth all-fiberized amplifier. By using a theoretical model, the potential MI-free scaling capability in such an amplifier is estimated to be 3.5 kW.

Journal ArticleDOI
TL;DR: The theoretical investigation indicates that 300 W-level linearly-polarized single-mode 1st order Stokes light can be obtained from incoherently pumped RFL with 100 m PM passive fiber, and to the best of the knowledge, this is the first demonstration of linearly -polarization high-order R FL with hundred-watt output power.
Abstract: We present a hundred-watt-level linearly-polarized random fiber laser (RFL) pumped by incoherent broadband amplified spontaneous emission (ASE) source and prospect the power scaling potential theoretically. The RFL employs half-opened cavity structure which is composed by a section of 330 m polarization maintained (PM) passive fiber and two PM high reflectivity fiber Bragg gratings. The 2nd order Stokes light centered at 1178 nm reaches the pump limited maximal power of 100.7 W with a full width at half-maximum linewidth of 2.58 nm and polarization extinction ratio of 23.5 dB. The corresponding ultimate quantum efficiency of pump to 2nd order Stokes light is 86.43%. To the best of our knowledge, this is the first demonstration of linearly-polarized high-order RFL with hundred-watt output power. Furthermore, the theoretical investigation indicates that 300 W-level linearly-polarized single-mode 1st order Stokes light can be obtained from incoherently pumped RFL with 100 m PM passive fiber.

Journal ArticleDOI
TL;DR: It is shown that the precision and accuracy of the sensing system are affected by the frequency and amplitude of perturbation as well as the pulse width and linewidth of the probe pulse.
Abstract: A distributed optical fibre acoustic sensor is numerically modelled. To increase the flexibility of the model, the building blocks of the sensing system are modelled separately and later combined to form the numerical model. This approach is adopted to facilitate the evaluation of each of the individual building blocks and their effects on the output of the sensor. The numerical model is used to assess the effect of parameters such as the linewidth of the laser source, the width of the probe pulse, and the frequency and amplitude of perturbation on the response of the sensing system. It is shown that the precision and accuracy of the sensing system are affected by the frequency and amplitude of perturbation as well as the pulse width and linewidth of the probe pulse.

Journal ArticleDOI
TL;DR: In this article, the positions of single self-assembled InAs/GaAs quantum dots with respect to alignment marks with < 5 nm uncertainty were measured, allowing them to measure their behavior before and after fabrication.
Abstract: Single self-assembled InAs/GaAs quantum dots are a promising solid-state quantum technology, with which vacuum Rabi splitting, single-photon-level nonlinearities, and bright, pure, and indistinguishable single-photon generation having been demonstrated. For such achievements, nanofabrication is used to create structures in which the quantum dot preferentially interacts with strongly-confined optical modes. An open question is the extent to which such nanofabrication may also have an adverse influence, through the creation of traps and surface states that could induce blinking, spectral diffusion, and dephasing. Here, we use photoluminescence imaging to locate the positions of single InAs/GaAs quantum dots with respect to alignment marks with < 5 nm uncertainty, allowing us to measure their behavior before and after fabrication. We track the quantum dot emission linewidth and photon statistics as a function of distance from an etched surface, and find that the linewidth is significantly broadened (up to several GHz) for etched surfaces within a couple hundred nanometers of the quantum dot. However, we do not observe appreciable reduction of the quantum dot radiative efficiency due to blinking. We also show that atomic layer deposition can stabilize spectral diffusion of the quantum dot emission, and partially recover its linewidth.

Journal ArticleDOI
TL;DR: An experimental study on the spectral dependence of depolarized guided acoustic-wave Brillouin scattering in a silica single-mode fiber on acoustic impedance of external materials and the characteristics are potentially applicable to acoustic impedance sensing.
Abstract: We report an experimental study on the spectral dependence of depolarized guided acoustic-wave Brillouin scattering (GAWBS) in a silica single-mode fiber (SMF) on acoustic impedance of external materials. The GAWBS spectrum was measured when the acoustic impedance was changed from 1.51 to 2.00 kg/s·mm2. With increasing acoustic impedance, the linewidth increased; the dependence was almost linear with an acoustic impedance dependence coefficient of 0.16 MHz/kg/s·mm2. Meanwhile, with increasing acoustic impedance, the central frequency linearly decreased with an acoustic impedance dependence coefficient of −0.07 MHz/kg/s·mm2. These characteristics are potentially applicable to acoustic impedance sensing.