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Showing papers by "Geophysical Fluid Dynamics Laboratory published in 2009"


Journal ArticleDOI
TL;DR: A review of the state of scientific understanding in relation to global and regional air quality is outlined in this article, in terms of emissions, processing and transport of trace gases and aerosols.

760 citations


Journal ArticleDOI
TL;DR: Coordinated Ocean-ice Reference Experiments (COREs) as mentioned in this paper is a tool to explore the behaviour of global ocean-ice models under forcing from a common atmospheric dataset, which is suitable for our purposes, even though its evaluation originally focussed more on the ocean than on the sea ice.

654 citations


Journal ArticleDOI
TL;DR: In this article, a global atmospheric model with roughly 50-km horizontal grid spacing is used to simulate the interannual variability of tropical cyclones using observed sea surface temperatures (SSTs) as the lower boundary condition.
Abstract: A global atmospheric model with roughly 50-km horizontal grid spacing is used to simulate the interannual variability of tropical cyclones using observed sea surface temperatures (SSTs) as the lower boundary condition. The model’s convective parameterization is based on a closure for shallow convection, with much of the deep convection allowed to occur on resolved scales. Four realizations of the period 1981–2005 are generated. The correlation of yearly Atlantic hurricane counts with observations is greater than 0.8 when the model is averaged over the four realizations, supporting the view that the random part of this annual Atlantic hurricane frequency (the part not predictable given the SSTs) is relatively small (<2 hurricanes per year). Correlations with observations are lower in the east, west, and South Pacific (roughly 0.6, 0.5, and 0.3, respectively) and insignificant in the Indian Ocean. The model trends in Northern Hemisphere basin-wide frequency are consistent with the observed trends i...

604 citations


Journal ArticleDOI
TL;DR: In this paper, the authors evaluate black carbon (BC) model predictions from the AeroCom model intercomparison project by considering the diversity among year 2000 model simulations and comparing model predictions with available measurements.
Abstract: . We evaluate black carbon (BC) model predictions from the AeroCom model intercomparison project by considering the diversity among year 2000 model simulations and comparing model predictions with available measurements. These model-measurement intercomparisons include BC surface and aircraft concentrations, aerosol absorption optical depth (AAOD) retrievals from AERONET and Ozone Monitoring Instrument (OMI) and BC column estimations based on AERONET. In regions other than Asia, most models are biased high compared to surface concentration measurements. However compared with (column) AAOD or BC burden retreivals, the models are generally biased low. The average ratio of model to retrieved AAOD is less than 0.7 in South American and 0.6 in African biomass burning regions; both of these regions lack surface concentration measurements. In Asia the average model to observed ratio is 0.7 for AAOD and 0.5 for BC surface concentrations. Compared with aircraft measurements over the Americas at latitudes between 0 and 50N, the average model is a factor of 8 larger than observed, and most models exceed the measured BC standard deviation in the mid to upper troposphere. At higher latitudes the average model to aircraft BC ratio is 0.4 and models underestimate the observed BC loading in the lower and middle troposphere associated with springtime Arctic haze. Low model bias for AAOD but overestimation of surface and upper atmospheric BC concentrations at lower latitudes suggests that most models are underestimating BC absorption and should improve estimates for refractive index, particle size, and optical effects of BC coating. Retrieval uncertainties and/or differences with model diagnostic treatment may also contribute to the model-measurement disparity. Largest AeroCom model diversity occurred in northern Eurasia and the remote Arctic, regions influenced by anthropogenic sources. Changing emissions, aging, removal, or optical properties within a single model generated a smaller change in model predictions than the range represented by the full set of AeroCom models. Upper tropospheric concentrations of BC mass from the aircraft measurements are suggested to provide a unique new benchmark to test scavenging and vertical dispersion of BC in global models.

558 citations


Journal ArticleDOI
TL;DR: A review of the factors that contribute to this diversity, as well as potential means to improve the simulation of El Nino, is presented in this article, along with a review of several factors contributing to the diversity of model simulations.
Abstract: Determining how El Nino and its impacts may change over the next 10 to 100 years remains a difficult scientific challenge. Ocean-atmosphere coupled general circulation models (CGCMs) are routinely used both to analyze El Nino mechanisms and teleconnections and to predict its evolution on a broad range of time scales, from seasonal to centennial. The ability to simulate El Nino as an emergent property of these models has largely improved over the last few years. Nevertheless, the diversity of model simulations of present-day El Nino indicates current limitations in our ability to model this climate phenomenon and to anticipate changes in its characteristics. A review of the several factors that contribute to this diversity, as well as potential means to improve the simulation of El Nino, is presented.

511 citations


Journal ArticleDOI
TL;DR: In this paper, the authors present new benthic foraminiferal d 18 O and d 13 C compilations for individual ocean basins that provide a robust estimate of benthicity foraminifera stable isotopic variations to � 80Ma andtentatively to � 110Ma.
Abstract: [1] Benthic foraminiferal oxygen isotopic (d 18 O) and carbon isotopic (d 13 C) trends, constructed from compilations of data series from multiple ocean sites, provide one of the primary means of reconstructing changes in the ocean interior. These records are also widely used as a general climate indicator for comparison with local and more specific marine and terrestrial climate proxy records. We present new benthic foraminiferal d 18 O and d 13 C compilations for individual ocean basins that provide a robust estimate of benthic foraminiferal stable isotopic variations to � 80Ma andtentatively to � 110Ma. First-order variations ininterbasinal isotopicgradients delineate transitions from interior ocean heterogeneity during the Late Cretaceous (>� 65 Ma) to early Paleogene (35– 65 Ma) homogeneity and a return to heterogeneity in the late Paleogene–early Neogene (35–0 Ma). We propose that these transitions reflect alterations in a first-order characteristic of ocean circulation: the ability of winds to make water in the deep ocean circulate. We document the initiation of large interbasinal d 18 O gradients in the early Oligocene and link the variations in interbasinal d 18 O gradients from the middle Eocene to Oligocene with the increasing influence of wind-driven mixing due to the gradual tectonic opening of Southern Ocean passages and initiation and strengthening of the Antarctic Circumpolar Current. The role of wind-driven upwelling, possibly associated with a Tethyan Circumequatorial Current, in controlling Late Cretaceous interior ocean heterogeneity should be the subject of further research.

495 citations


Journal ArticleDOI
TL;DR: In this paper, a control simulation of the GFDL CM2.1 global coupled GCM, run for 2000 years with its atmospheric composition, solar irradiance, and land cover held fixed at 1860 values, exhibits strong interdecadal and intercentennial modulation of its ENSO behavior.
Abstract: [1] A control simulation of the GFDL CM2.1 global coupled GCM, run for 2000 years with its atmospheric composition, solar irradiance, and land cover held fixed at 1860 values, exhibits strong interdecadal and intercentennial modulation of its ENSO behavior. To the extent that such modulation is realistic, it could attach large uncertainties to ENSO metrics diagnosed from centennial and shorter records ― with important implications for historical and paleo records, climate projections, and model assessment and intercomparison. Analysis of the wait times between ENSO warm events suggests that such slow modulation need not require multidecadal memory; it can arise simply from Poisson statistics applied to ENSO's interannual time scale and seasonal phase-locking.

471 citations


Journal ArticleDOI
TL;DR: In this article, an ensemble of 21 global and hemispheric chemical transport models is used to estimate the spatial average surface ozone (O-3) response over east Asia (EA), Europe (EU), North America (NA), and south Asia (SA) to 20% decreases in anthropogenic emissions of the O-3 precursors, NOx, NMVOC, and CO.
Abstract: Understanding the surface O-3 response over a "receptor" region to emission changes over a foreign "source" region is key to evaluating the potential gains from an international approach to abate ozone (O-3) pollution. We apply an ensemble of 21 global and hemispheric chemical transport models to estimate the spatial average surface O-3 response over east Asia (EA), Europe (EU), North America (NA), and south Asia (SA) to 20% decreases in anthropogenic emissions of the O-3 precursors, NOx, NMVOC, and CO (individually and combined), from each of these regions. We find that the ensemble mean surface O-3 concentrations in the base case (year 2001) simulation matches available observations throughout the year over EU but overestimates them by > 10 ppb during summer and early fall over the eastern United States and Japan. The sum of the O-3 responses to NOx, CO, and NMVOC decreases separately is approximately equal to that from a simultaneous reduction of all precursors. We define a continental-scale "import sensitivity" as the ratio of the O-3 response to the 20% reductions in foreign versus "domestic" (i.e., over the source region itself) emissions. For example, the combined reduction of emissions from the three foreign regions produces an ensemble spatial mean decrease of 0.6 ppb over EU (0.4 ppb from NA), less than the 0.8 ppb from the reduction of EU emissions, leading to an import sensitivity ratio of 0.7. The ensemble mean surface O-3 response to foreign emissions is largest in spring and late fall (0.7-0.9 ppb decrease in all regions from the combined precursor reductions in the three foreign regions), with import sensitivities ranging from 0.5 to 1.1 (responses to domestic emission reductions are 0.8-1.6 ppb). High O-3 values are much more sensitive to domestic emissions than to foreign emissions, as indicated by lower import sensitivities of 0.2 to 0.3 during July in EA, EU, and NA when O-3 levels are typically highest and by the weaker relative response of annual incidences of daily maximum 8-h average O-3 above 60 ppb to emission reductions in a foreign region(< 10-20% of that to domestic) as compared to the annual mean response (up to 50% of that to domestic). Applying the ensemble annual mean results to changes in anthropogenic emissions from 1996 to 2002, we estimate a Northern Hemispheric increase in background surface O-3 of about 0.1 ppb a(-1), at the low end of the 0.1-0.5 ppb a(-1) derived from observations. From an additional simulation in which global atmospheric methane was reduced, we infer that 20% reductions in anthropogenic methane emissions from a foreign source region would yield an O-3 response in a receptor region that roughly equals that produced by combined 20% reductions of anthropogenic NOx, NMVOC, and CO emissions from the foreign source

430 citations


Journal ArticleDOI
TL;DR: In this article, the authors developed a dynamic land model (LM3V) able to simulate ecosystem dynamics and exchanges of water, energy, and CO2 between land and atmosphere, which is specifically designed to address the consequences of land use and land management changes including cropland and pasture dynamics, shifting cultivation, logging, fire, and resulting patterns of secondary regrowth.
Abstract: [1] We have developed a dynamic land model (LM3V) able to simulate ecosystem dynamics and exchanges of water, energy, and CO2 between land and atmosphere. LM3V is specifically designed to address the consequences of land use and land management changes including cropland and pasture dynamics, shifting cultivation, logging, fire, and resulting patterns of secondary regrowth. Here we analyze the behavior of LM3V, forced with the output from the Geophysical Fluid Dynamics Laboratory (GFDL) atmospheric model AM2, observed precipitation data, and four historic scenarios of land use change for 1700–2000. Our analysis suggests a net terrestrial carbon source due to land use activities from 1.1 to 1.3 GtC/a during the 1990s, where the range is due to the difference in the historic cropland distribution. This magnitude is substantially smaller than previous estimates from other models, largely due to our estimates of a secondary vegetation sink of 0.35 to 0.6 GtC/a in the 1990s and decelerating agricultural land clearing since the 1960s. For the 1990s, our estimates for the pastures' carbon flux vary from a source of 0.37 to a sink of 0.15 GtC/a, and for the croplands our model shows a carbon source of 0.6 to 0.9 GtC/a. Our process-based model suggests a smaller net deforestation source than earlier bookkeeping models because it accounts for decelerated net conversion of primary forest to agriculture and for stronger secondary vegetation regrowth in tropical regions. The overall uncertainty is likely to be higher than the range reported here because of uncertainty in the biomass recovery under changing ambient conditions, including atmospheric CO2 concentration, nutrients availability, and climate.

354 citations


Journal ArticleDOI
TL;DR: The ability of eight climate models to simulate the Madden-Julian oscillation (MJO) is examined using diagnostics developed by the U.S. Climate Variability and Predictability (CLIVAR) Working Group as mentioned in this paper.
Abstract: The ability of eight climate models to simulate the Madden‐Julian oscillation (MJO) is examined using diagnostics developed by the U.S. Climate Variability and Predictability (CLIVAR) MJO Working Group. Although the MJO signal has been extracted throughout the annual cycle, this study focuses on the boreal winter (November‐April) behavior. Initially, maps of the mean state and variance and equatorial space‐time spectra of 850-hPa zonal wind and precipitation are compared with observations. Models best represent the intraseasonal space‐time spectral peak in the zonal wind compared to that of precipitation. Using the phase‐ space representation of the multivariate principal components (PCs), the life cycle properties of the simulated MJOs are extracted, including the ability to represent how the MJO evolves from a given subphase and the associated decay time scales. On average, the MJO decay (e-folding) time scale for all models is shorter (;20‐ 29 days) than observations (;31 days). All models are able to produce a leading pair of multivariate principal components that represents eastward propagation of intraseasonal wind and precipitation anomalies, although the fraction of the variance is smaller than observed for all models. In some cases, the dominant time scale of these PCs is outside of the 30‐80-day band. Several key variables associated with the model’s MJO are investigated, including the surface latent heat flux, boundary layer (925 hPa) moisture convergence, and the vertical structure of moisture. Low-level moisture convergence ahead (east) of convection is associated with eastward propagation in most of the models. A few models are also able to simulate the gradual moistening of the lower troposphere that precedes observed MJO convection, as well as the observed geographical difference in the vertical structure of moisture associated with the MJO. The dependence of rainfall on lower tropospheric relative humidity and the fraction of rainfall that is stratiform are also discussed, including implications these diagnostics have for MJO simulation. Based on having the most realistic intraseasonal multivariate empirical orthogonal functions, principal component power spectra, equatorial eastward propagating outgoing longwave radiation (OLR), latent heat flux, low-level moisture convergence signals, and vertical structure of moisture over the Eastern Hemisphere, the superparameterized Community Atmosphere Model (SPCAM) and the ECHAM4/ Ocean Isopycnal Model (OPYC) show the best skill at representing the MJO.

353 citations


Journal ArticleDOI
TL;DR: In this paper, the authors compute statistical relationships between aerosol optical depth (τa) and various cloud and radiation quantities in a manner that is consistent between the models and the satellite data.
Abstract: . Aerosol indirect effects continue to constitute one of the most important uncertainties for anthropogenic climate perturbations. Within the international AEROCOM initiative, the representation of aerosol-cloud-radiation interactions in ten different general circulation models (GCMs) is evaluated using three satellite datasets. The focus is on stratiform liquid water clouds since most GCMs do not include ice nucleation effects, and none of the model explicitly parameterises aerosol effects on convective clouds. We compute statistical relationships between aerosol optical depth (τa) and various cloud and radiation quantities in a manner that is consistent between the models and the satellite data. It is found that the model-simulated influence of aerosols on cloud droplet number concentration (Nd) compares relatively well to the satellite data at least over the ocean. The relationship between τa and liquid water path is simulated much too strongly by the models. This suggests that the implementation of the second aerosol indirect effect mainly in terms of an autoconversion parameterisation has to be revisited in the GCMs. A positive relationship between total cloud fraction (fcld) and τa as found in the satellite data is simulated by the majority of the models, albeit less strongly than that in the satellite data in most of them. In a discussion of the hypotheses proposed in the literature to explain the satellite-derived strong fcld–τa relationship, our results indicate that none can be identified as a unique explanation. Relationships similar to the ones found in satellite data between τa and cloud top temperature or outgoing long-wave radiation (OLR) are simulated by only a few GCMs. The GCMs that simulate a negative OLR–τa relationship show a strong positive correlation between τa and fcld. The short-wave total aerosol radiative forcing as simulated by the GCMs is strongly influenced by the simulated anthropogenic fraction of τa, and parameterisation assumptions such as a lower bound on Nd. Nevertheless, the strengths of the statistical relationships are good predictors for the aerosol forcings in the models. An estimate of the total short-wave aerosol forcing inferred from the combination of these predictors for the modelled forcings with the satellite-derived statistical relationships yields a global annual mean value of −1.5±0.5 Wm−2. In an alternative approach, the radiative flux perturbation due to anthropogenic aerosols can be broken down into a component over the cloud-free portion of the globe (approximately the aerosol direct effect) and a component over the cloudy portion of the globe (approximately the aerosol indirect effect). An estimate obtained by scaling these simulated clear- and cloudy-sky forcings with estimates of anthropogenic τa and satellite-retrieved Nd–τa regression slopes, respectively, yields a global, annual-mean aerosol direct effect estimate of −0.4±0.2 Wm−2 and a cloudy-sky (aerosol indirect effect) estimate of −0.7±0.5 Wm−2, with a total estimate of −1.2±0.4 Wm−2.

Journal ArticleDOI
TL;DR: In this paper, the response of tropical precipitation to extratropical thermal forcing is reexamined using an idealized moist atmospheric GCM that has no water vapor or cloud feedbacks.
Abstract: The response of tropical precipitation to extratropical thermal forcing is reexamined using an idealized moist atmospheric GCM that has no water vapor or cloud feedbacks, simplifying the analysis while retaining the aquaplanet configuration coupled to a slab ocean from the authors’ previous study. As in earlier studies, tropical precipitation in response to high-latitude forcing is skewed toward the warmed hemisphere. Comparisons with a comprehensive GCM in an identical aquaplanet, mixed-layer framework reveal that the tropical responses tend to be much larger in the comprehensive GCM as a result of positive cloud and water vapor feedbacks that amplify the imposed extratropical thermal forcing. The magnitude of the tropical precipitation response in the idealized model is sensitive to convection scheme parameters. This sensitivity as well as the tropical precipitation response can be understood from a simple theory with two ingredients: the changes in poleward energy fluxes are predicted using a ...

Journal ArticleDOI
TL;DR: In this article, an intercomparison of single-column and cloud-resolving model simulations of a cold-air outbreak mixed-phase stratocumulus cloud observed during the Atmospheric Radiation Measurement (ARM) programme's Mixed-Phase Arctic Cloud Experiment is presented.
Abstract: Results are presented from an intercomparison of single-column and cloud-resolving model simulations of a cold-air outbreak mixed-phase stratocumulus cloud observed during the Atmospheric Radiation Measurement (ARM) programme's Mixed-Phase Arctic Cloud Experiment. The observed cloud occurred in a well-mixed boundary layer with a cloud-top temperature of −15 ◦ C. The average liquid water path of around 160 g m −2 was about two-thirds of the adiabatic value and far greater than the average mass of ice which when integrated from the surface to cloud top was around 15 gm −2 . Simulations of 17 single-column models (SCMs) and 9 cloud-resolving models (CRMs) are compared. While the simulated ice water path is generally consistent with observed values, the median SCM and CRM liquid water path is a factor-of-three smaller than observed. Results from a sensitivity study in which models removed ice microphysics suggest that in many models the interaction between liquid and ice-phase microphysics is responsible for the large model underestimate of liquid water path. Despite this underestimate, the simulated liquid and ice water paths of several models are consistent with observed values. Furthermore, models with more sophisticated microphysics simulate liquid and ice water paths that are in better agreement with the observed values, although considerable scatter exists. Although no single factor guarantees a good simulation, these results emphasize the need for improvement in the model representation of mixed-phase microphysics. Copyright c � 2009 Royal Meteorological Society

Journal ArticleDOI
TL;DR: In this article, the authors investigated the climate response of the equatorial Pacific to increased greenhouse gases using numerical experiments from 11 climate models participating in the Intergovernmental Panel on Climate Change's Fourth Assessment Report.
Abstract: The climate response of the equatorial Pacific to increased greenhouse gases is investigated using numerical experiments from 11 climate models participating in the Intergovernmental Panel on Climate Change’s Fourth Assessment Report. Multimodel mean climate responses to CO2 doubling are identified and related to changes in the heat budget of the surface layer. Weaker ocean surface currents driven by a slowing down of the Walker circulation reduce ocean dynamical cooling throughout the equatorial Pacific. The combined anomalous ocean dynamical plus radiative heating from CO2 is balanced by different processes in the western and eastern basins: Cloud cover feedbacks and evaporation balance the heating over the warm pool, while increased cooling by ocean vertical heat transport balances the warming over the cold tongue. This increased cooling by vertical ocean heat transport arises from increased near-surface thermal stratification, despite a reduction in vertical velocity. The stratification respo...

Journal ArticleDOI
TL;DR: In this article, an updated analysis of observed stratospheric temperature variability and trends is presented on the basis of satellite, radiosonde, and lidar observations, with some differences in detail among the different radiosonde and satellite data sets.
Abstract: An updated analysis of observed stratospheric temperature variability and trends is presented on the basis of satellite, radiosonde, and lidar observations. Satellite data include measurements from the series of NOAA operational instruments, including the Microwave Sounding Unit covering 1979–2007 and the Stratospheric Sounding Unit (SSU) covering 1979–2005. Radiosonde results are compared for six different data sets, incorporating a variety of homogeneity adjustments to account for changes in instrumentation and observational practices. Temperature changes in the lower stratosphere show cooling of ∼0.5 K/decade over much of the globe for 1979–2007, with some differences in detail among the different radiosonde and satellite data sets. Substantially larger cooling trends are observed in the Antarctic lower stratosphere during spring and summer, in association with development of the Antarctic ozone hole. Trends in the lower stratosphere derived from radiosonde data are also analyzed for a longer record (back to 1958); trends for the presatellite era (1958–1978) have a large range among the different homogenized data sets, implying large trend uncertainties. Trends in the middle and upper stratosphere have been derived from updated SSU data, taking into account changes in the SSU weighting functions due to observed atmospheric CO2 increases. The results show mean cooling of 0.5–1.5 K/decade during 1979–2005, with the greatest cooling in the upper stratosphere near 40–50 km. Temperature anomalies throughout the stratosphere were relatively constant during the decade 1995–2005. Long records of lidar temperature measurements at a few locations show reasonable agreement with SSU trends, although sampling uncertainties are large in the localized lidar measurements. Updated estimates of the solar cycle influence on stratospheric temperatures show a statistically significant signal in the tropics (∼30°N–S), with an amplitude (solar maximum minus solar minimum) of ∼0.5 K (lower stratosphere) to ∼1.0 K (upper stratosphere).

Journal ArticleDOI
TL;DR: In this paper, the authors examined the interannual variability in the timing and magnitude of the North Atlantic phytoplankton bloom using a combination of satellite data and output from an ocean biogeochemistry general circulation model.
Abstract: [1] The interannual to decadal variability in the timing and magnitude of the North Atlantic phytoplankton bloom is examined using a combination of satellite data and output from an ocean biogeochemistry general circulation model. The timing of the bloom as estimated from satellite chlorophyll data is used as a novel metric for validating the model's skill. Maps of bloom timing reveal that the subtropical bloom begins in winter and progresses northward starting in May in subpolar regions. A transition zone, which experiences substantial interannual variability in bloom timing, separates the two regions. Time series of the modeled decadal (1959-2004) variability in bloom timing show no long-term trend toward earlier or delayed blooms in any of the three regions considered here. However, the timing of the subpolar bloom does show distinct decadal-scale periodicity, which is found to be correlated with the North Atlantic Oscillation (NAO) index. The mechanism underpinning the relationship is identified as anomalous wind-driven mixing conditions associated with the NAO. In positive NAO phases, stronger westerly winds result in deeper mixed layers, delaying the start of the subpolar spring bloom by 2-3 weeks. The subpolar region also expands during positive phases, pushing the transition zone further south in the central North Atlantic. The magnitude of the bloom is found to be only weakly dependent on bloom timing, but is more strongly correlated with mixed layer depth. The extensive interannual variability in the timing of the bloom, particularly in the transition region, is expected to strongly impact the availability of food to higher trophic levels.

Journal ArticleDOI
TL;DR: The authors compare satellite ocean color-based models (SatPPMs) and those generated from biogeochemical ocean general circulation models (BOGCMs) to a tropical Pacific primary productivity (PP) database consisting of ∼ 1000 14C measurements spanning more than a decade (1983-1996).

Journal ArticleDOI
TL;DR: In this paper, a case study of nocturnal stratocumulus under a dry inversion, with embedded pockets of heavily drizzling open cellular convection is presented.
Abstract: Cloud water sedimentation and drizzle in a stratocumulus-topped boundary layer are the focus of an intercomparison of large-eddy simulations. The context is an idealized case study of nocturnal stratocumulus under a dry inversion, with embedded pockets of heavily drizzling open cellular convection. Results from 11 groups are used. Two models resolve the size distributions of cloud particles, and the others parameterize cloud water sedimentation and drizzle. For the ensemble of simulations with drizzle and cloud water sedimentation, the mean liquid water path (LWP) is remarkably steady and consistent with the measurements, the mean entrainment rate is at the low end of the measured range, and the ensemble-average maximum vertical wind variance is roughly half that measured. On average, precipitation at the surface and at cloud base is smaller, and the rate of precipitation evaporation greater, than measured. Including drizzle in the simulations reduces convective intensity, increases boundary layer stratification, and decreases LWP for nearly all models. Including cloud water sedimentation substantially decreases entrainment, decreases convective intensity, and increases LWP for most models. In nearly all cases, LWP responds more strongly to cloud water sedimentation than to drizzle. The omission of cloud water sedimentation in simulations is strongly discouraged, regardless of whether or not precipitation is present below cloud base.

Journal ArticleDOI
TL;DR: In this article, the authors focus on quantification of the seasonal to multidecadal time scale response of the ocean to explosive volcanism and simulate the response to the 1991 Pinatubo and the 1815 Tambora eruptions.
Abstract: [1] Sulfate aerosols resulting from strong volcanic explosions last for 2–3 years in the lower stratosphere. Therefore it was traditionally believed that volcanic impacts produce mainly short-term, transient climate perturbations. However, the ocean integrates volcanic radiative cooling and responds over a wide range of time scales. The associated processes, especially ocean heat uptake, play a key role in ongoing climate change. However, they are not well constrained by observations, and attempts to simulate them in current climate models used for climate predictions yield a range of uncertainty. Volcanic impacts on the ocean provide an independent means of assessing these processes. This study focuses on quantification of the seasonal to multidecadal time scale response of the ocean to explosive volcanism. Itemploysthecoupledclimate modelCM2.1,developedrecently attheNational Oceanic and Atmospheric Administration’s Geophysical Fluid Dynamics Laboratory, to simulate the response to the 1991 Pinatubo and the 1815 Tambora eruptions, which were the largest in the 20th and 19th centuries, respectively. The simulated climate perturbations compare well with available observations for the Pinatubo period. The stronger Tambora forcing produces responses with higher signal-to-noise ratio. Volcanic cooling tends to strengthen the Atlantic meridional overturning circulation. Sea ice extent appears to be sensitive to volcanic forcing, especially during the warm season. Because of the extremely long relaxation time of ocean subsurface temperature and sea level, the perturbations caused by the Tambora eruption could have lasted well into the 20th century.

Journal ArticleDOI
TL;DR: In this paper, a modified version of the Geophysical Fluid Dynamics Laboratory atmosphere general circulation model (AM2.1) coupled with a mixed layer ocean model is used to study the equilibrium temperature and hydrological responses to the total aerosol effects.
Abstract: The equilibrium temperature and hydrological responses to the total aerosol effects (i.e., direct, semidirect, and indirect effects) are studied using a modified version of the Geophysical Fluid Dynamics Laboratory atmosphere general circulation model (AM2.1) coupled to a mixed layer ocean model. The treatment of aerosol‐liquid cloud interactions and associated indirect effects is based upon a prognostic scheme of cloud droplet number concentration, with an explicit representation of cloud condensation nuclei activation involving sulfate, organic carbon, and sea salt aerosols. Increasing aerosols from preindustrial (1860) to presentday (1990) levels leads to a decrease of 1.9 K in the global annual mean surface temperature. The cooling is relatively strong over the Northern Hemisphere midlatitude land owing to the high aerosol burden there, while being amplified at high latitudes. When being subject to aerosols and radiatively active gases (i.e., wellmixed greenhouse gases and ozone) simultaneously, the model climate behaves nonlinearly; the simulated increase in surface temperature (0.55 K) is considerably less than the arithmetic sum of separate aerosol and gas effects (0.86 K). The thermal responses are accompanied by the nonlinear changes in cloud fields, which are amplified owing to the surface albedo feedback at high latitudes. The two effects completely offset each other in the Northern Hemisphere, while gas effect is dominant in the Southern Hemisphere. Both factors are crucial in shaping the regional responses. Interhemispheric asymmetry in aerosol-induced cooling yields a southward shift of the intertropical convergence zone, thus giving rise to a significant reduction in precipitation north of the equator, and an increase to the south. The simulations show that the change of precipitation in response to the simultaneous increases in aerosols and gases not only largely follows the same pattern as that for aerosols alone, but that it is also substantially strengthened in terms of magnitude south of 108N. This is quite different from the damping expected from adding up individual responses, and further indicates the nonlinearity in the model’s hydrological response.

Journal ArticleDOI
TL;DR: The authors analyzed results from 15 global and 1 hemispheric chemical transport models and compared these to Clean Air Status and Trends Network (CASTNet) observations in the United States (US) for 2001.
Abstract: . As part of the Hemispheric Transport of Air Pollution (HTAP; http:// www.htap.org ) project, we analyze results from 15 global and 1 hemispheric chemical transport models and compare these to Clean Air Status and Trends Network (CASTNet) observations in the United States (US) for 2001. Using the policy-relevant maximum daily 8-h average ozone (MDA8 O3) statistic, the multi-model ensemble represents the observations well (mean r2=0.57, ensemble bias = +4.1 ppbv for all US regions and all seasons) despite a wide range in the individual model results. Correlations are strongest in the northeastern US during spring and fall (r2=0.68); and weakest in the midwestern US in summer (r2=0.46). However, large positive mean biases exist during summer for all eastern US regions, ranging from 10–20 ppbv, and a smaller negative bias is present in the western US during spring (~3 ppbv). In nearly all other regions and seasons, the biases of the model ensemble simulations are ≤5 ppbv. Sensitivity simulations in which anthropogenic O3-precursor emissions (NOx + NMVOC + CO + aerosols) were decreased by 20% in four source regions: East Asia (EA), South Asia (SA), Europe (EU) and North America (NA) show that the greatest response of MDA8 O3 to the summed foreign emissions reductions occurs during spring in the West (0.9 ppbv reduction due to 20% emissions reductions from EA + SA + EU). East Asia is the largest contributor to MDA8 O3 at all ranges of the O3 distribution for most regions (typically ~0.45 ppbv) followed closely by Europe. The exception is in the northeastern US where emissions reductions in EU had a slightly greater influence than EA emissions, particularly in the middle of the MDA8 O3 distribution (response of ~0.35 ppbv between 35–55 ppbv). EA and EU influences are both far greater (about 4x) than that from SA in all regions and seasons. In all regions and seasons O3-precursor emissions reductions of 20% in the NA source region decrease MDA8 O3 the most – by a factor of 2 to nearly 10 relative to foreign emissions reductions. The O3 response to anthropogenic NA emissions is greatest in the eastern US during summer at the high end of the O3 distribution (5–6 ppbv for 20% reductions). While the impact of foreign emissions on surface O3 in the US is not negligible – and is of increasing concern given the recent growth in Asian emissions – domestic emissions reductions remain a far more effective means of decreasing MDA8 O3 values, particularly those above 75 ppb (the current US standard).

Journal ArticleDOI
TL;DR: Cyclone Nargis (Figure 1a) made landfall in Myanmar (formerly Burma) on 2 May 2008 with sustained winds of approximately 210 kilometers per hour, equivalent to a category 3-4 hurricane as discussed by the authors.
Abstract: Cyclone Nargis (Figure 1a) made landfall in Myanmar (formerly Burma) on 2 May 2008 with sustained winds of approximately 210 kilometers per hour, equivalent to a category 3–4 hurricane. In addition, Nargis brought approximately 600 millimeters of rain and a storm surge of 3–4 meters to the low-lying and densely populated Irrawaddy River delta. In its wake, the storm left an estimated 130,000 dead or missing and more than $10 billion in economic losses. It was the worst natural disaster to strike the Indian Ocean region since the 26 December 2004 tsunami and the worst recorded natural disaster ever to affect Myanmar.

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TL;DR: In this article, a multi-model set of atmospheric simulations forced by historical sea surface temperature (SST) or SSTs plus Greenhouse gases and aerosol forcing agents for the period of 1950-1999 is studied to identify and understand which components of the Asian-Australian monsoon (A-AM) variability are forced and reproducible.
Abstract: A multi-model set of atmospheric simulations forced by historical sea surface temperature (SST) or SSTs plus Greenhouse gases and aerosol forcing agents for the period of 1950–1999 is studied to identify and understand which components of the Asian–Australian monsoon (A–AM) variability are forced and reproducible. The analysis focuses on the summertime monsoon circulations, comparing model results against the observations. The priority of different components of the A–AM circulations in terms of reproducibility is evaluated. Among the subsystems of the wide A–AM, the South Asian monsoon and the Australian monsoon circulations are better reproduced than the others, indicating they are forced and well modeled. The primary driving mechanism comes from the tropical Pacific. The western North Pacific monsoon circulation is also forced and well modeled except with a slightly lower reproducibility due to its delayed response to the eastern tropical Pacific forcing. The simultaneous driving comes from the western Pacific surrounding the maritime continent region. The Indian monsoon circulation has a moderate reproducibility, partly due to its weakened connection to June–July–August SSTs in the equatorial eastern Pacific in recent decades. Among the A–AM subsystems, the East Asian summer monsoon has the lowest reproducibility and is poorly modeled. This is mainly due to the failure of specifying historical SST in capturing the zonal land-sea thermal contrast change across the East Asia. The prescribed tropical Indian Ocean SST changes partly reproduce the meridional wind change over East Asia in several models. For all the A–AM subsystem circulation indices, generally the MME is always the best except for the Indian monsoon and East Asian monsoon circulation indices.

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TL;DR: This paper used a simple methodology to test whether a set of atmospheric climate models with prescribed radiative forcings and ocean surface conditions can reproduce twentieth century climate variability, finding a strong relationship between the Southern Oscillation in global temperature and the rate of global warming.
Abstract: We use a simple methodology to test whether a set of atmospheric climate models with prescribed radiative forcings and ocean surface conditions can reproduce twentieth century climate variability. Globally, rapid land surface warming since the 1970s is reproduced by some models but others warm too slowly. In the tropics, air-sea coupling allows models to reproduce the Southern Oscillation but its strength varies between models. We find a strong relationship between the Southern Oscillation in global temperature and the rate of global warming, which could in principle be used to identify models with realistic climate sensitivity. This relationship and a weak response to ENSO suggests weak sensitivity to changes in sea surface temperature in some of the models used here. In the tropics, most models reproduce part of the observed Sahel drought. In the extratropics, models do not reproduce the observed increase in the North Atlantic Oscillation in response to forcings, through internal variability, or as a combination of both.

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TL;DR: In this article, the authors analyzed the effect of China's emissions of SO2,S O 4�, OC and BC in 2000 and for three emission scenarios in 2030 on global surface aerosol concentrations, premature mortality, and radiative forcing (RF).

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TL;DR: In this paper, an aerosol-cloud modeling framework is described to simulate the activation of ice particles and droplets by biological aerosol particles, such as airborne ice-nucleation active (INA) bacteria.
Abstract: . An aerosol-cloud modeling framework is described to simulate the activation of ice particles and droplets by biological aerosol particles, such as airborne ice-nucleation active (INA) bacteria. It includes the empirical parameterisation of heterogeneous ice nucleation and a semi-prognostic aerosol component, which have been incorporated into a cloud-system resolving model (CSRM) with double-moment bulk microphysics. The formation of cloud liquid by soluble material coated on these partially insoluble organic aerosols is represented. It determines their partial removal from deep convective clouds by accretion onto precipitation in the cloud model. This "aerosol-cloud model" is validated for diverse cases of deep convection with contrasting aerosol conditions, against satellite, ground-based and aircraft observations. Simulations are performed with the aerosol-cloud model for a month-long period of summertime convective activity over Oklahoma. It includes three cases of continental deep convection simulated previously by Phillips and Donner (2006). Elevated concentrations of insoluble organic aerosol, boosted by a factor of 100 beyond their usual values for this continental region, are found to influence significantly the following quantities: (1) the average numbers and sizes of ice crystals and droplets in the clouds; (2) the horizontal cloud coverage in the free troposphere; (3) precipitation at the ground; and (4) incident solar insolation at the surface. This factor of 100 is plausible for natural fluctuations of the concentration of insoluble organic aerosol, in view of variability of cell concentrations for airborne bacteria seen by Lindemann et al. (1982). In nature, such boosting of the insoluble organic aerosol loading could arise from enhanced emissions of biological aerosol particles from a land surface. Surface wetness and solar insolation at the ground are meteorological quantities known to influence rates of growth of certain biological particles (e.g. bacteria). Their rates of emission into the atmosphere must depend on these same quantities, in addition to surface wind speed, turbulence and convection. Finally, the present study is the first attempt at evaluating the impacts from biological aerosols on mesoscale cloud ensembles in the literature.

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TL;DR: In this paper, Liu et al. quantified the global impact on premature mortality of inter-continental transport of fine aerosols (including sulfate, black carbon, organic carbon, and mineral dust) using the global modeling results.

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TL;DR: In this paper, the authors used the Infrared Atmospheric Sounding Interferometer (IASI) and Advanced Microwave Sounding Unit (AMSU) to retrieve a mid-to-upper tropospheric content of methane (CH4) in clear-sky conditions, in the tropics, over sea, for the first 16 months of operation of MetOp (July 2007-October 2008).
Abstract: . Simultaneous observations from the Infrared Atmospheric Sounding Interferometer (IASI) and from the Advanced Microwave Sounding Unit (AMSU), launched together onboard the European MetOp platform in October 2006, are used to retrieve a mid-to-upper tropospheric content of methane (CH4) in clear-sky conditions, in the tropics, over sea, for the first 16 months of operation of MetOp (July 2007–October 2008). With its high spectral resolution, IASI provides nine channels in the 7.7 μm band highly sensitive to CH4 with reduced sensitivities to other atmospheric variables. These channels, sensitive to both CH4 and temperature, are used in conjunction with AMSU channels, only sensitive to temperature, to decorrelate both signals through a non-linear inference scheme based on neural networks. A key point of this approach is that no use is made of prior information in terms of methane seasonality, trend, or geographical patterns. The precision of the retrieval is estimated to be about 16 ppbv (~0.9%). Features of the retrieved methane space-time distribution include: (1) a strong seasonal cycle of 30 ppbv in the northern tropics with a maximum in January–March and a minimum in July–September, and a flat seasonal cycle in the southern tropics, in agreement with in-situ measurements; (2) a latitudinal decrease of 30 ppbv from 20° N to 20° S, in boreal spring and summer, lower than what is observed at the surface but in excellent agreement with tropospheric aircraft measurements; (3) geographical patterns in good agreement with simulations from the atmospheric transport and chemistry model MOZART-2, but with a higher variability and a higher concentration in boreal winter; (4) signatures of CH4 emissions transported to the middle troposphere such as a large plume of elevated tropospheric methane south of the Asian continent, which might be due to Asian emissions from rice paddies uplifted by deep convection during the monsoon period and then transported towards Indonesia. In addition to bringing a greatly improved view of methane distribution, these results from IASI should provide a means to observe and understand atmospheric transport pathways of methane from the surface to the upper troposphere.


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TL;DR: In this paper, the authors evaluate inter-continental source-receptor relationships for fine aerosols and identify the regions whose emissions have dominant influence on receptor continents using a global coupled chemistry-aerosol model driven with NCEP/NCAR reanalysis meteorology.