Biomimetic mineralization of metal-organic frameworks as protective coatings for biomacromolecules.
Kang Liang,Raffaele Ricco,Cara M. Doherty,Mark J. Styles,Stephen Bell,Nigel Kirby,Stephen T. Mudie,David N. Haylock,Anita J. Hill,Christian J. Doonan,Paolo Falcaro +10 more
TLDR
It is shown that proteins, enzymes and DNA rapidly induce the formation of protective metal-organic framework coatings under physiological conditions by concentrating the framework building blocks and facilitating crystallization around the biomacromolecules.Abstract:
Robust biomacromolecules could be used for a wide range of biotechnological applications. Here the authors report a biomimetic mineralization process, in which biomolecules are encapsulated within metal-organic frameworks, and their stability is subsequently increased without significant bioactivity loss.read more
Citations
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Insight into Bioactivity of In-situ Trapped Enzyme-Covalent-organic Frameworks.
Jieying Liang,Juanfang Ruan,Bosiljka Njegic,Aditya Rawal,Jason Scott,Jiangtao Jason Xu,Cyrille Boyer,Kang Liang +7 more
TL;DR: In this article , three kinds of covalent-organic frameworks (COFs) were constructed via a biofriendly and one-pot synthetic strategy at room temperature in aqueous solution.
Journal ArticleDOI
Biomimetic Mineralization of Iron-Fumarate Nanoparticles for Protective Encapsulation and Intracellular Delivery of Proteins
Negar Mirzazadeh Dizaji,Yi Hung Lin,Thomas Bein,Ernst Wagner,Stefan Wuttke,Ulrich Lächelt,Hanna Engelke +6 more
TL;DR: This work presents a green room-temperature synthesis of amorphous iron-fumarate nanoparticles under mildly acidic conditions in water to encapsulate bovine serum albumin (BSA), horseradish peroxidase (HRP), green fluorescent protein (GFP), and Cas9/sgRNA ribonucleoproteins (RNPs).
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Lipase-based MIL-100(Fe) biocomposites as chiral stationary phase for high-efficiency capillary electrochromatographic enantioseparation
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Biomineralized Nano-Assemblies of Poly(Ethylene Glycol) Derivative with Lanthanide Ions as Ratiometric Fluorescence Sensors for Detection of Water and Fe3+ Ions
Tong Chen,San-Ping Zhao +1 more
TL;DR: In this paper , an effective strategy was developed to fabricate novel lanthanide ions-pyromellitic acid-methoxy poly(ethylene glycol) (Ln-PMA-MPEG) nanoassemblies.
Journal ArticleDOI
When enzyme meet MOFs: Emerging opportunities toward water treatment
Junning Wang,Yanhong Zhao,Rongfu Peng,Yiming Wang,Jinhui Zhang,Xin Yuan Zhu,Ha-Na Kang,C Guo,Yanli Mao,Chaohai Wang +9 more
TL;DR: In this article , the authors provide a new perspective on the emerging enzyme-MOFs-based platform for innovative employment in water treatment and to accelerate the development of this field for early industrial application.
References
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Hiroyasu Furukawa,Hiroyasu Furukawa,Kyle E. Cordova,Kyle E. Cordova,Michael O'Keeffe,Michael O'Keeffe,Omar M. Yaghi,Omar M. Yaghi,Omar M. Yaghi +8 more
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Reticular synthesis and the design of new materials
Omar M. Yaghi,Michael O'Keeffe,Nathan W. Ockwig,Hee K. Chae,Hee K. Chae,Mohamed Eddaoudi,Jaheon Kim +6 more
TL;DR: This work has shown that highly porous frameworks held together by strong metal–oxygen–carbon bonds and with exceptionally large surface area and capacity for gas storage have been prepared and their pore metrics systematically varied and functionalized.
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Exceptional chemical and thermal stability of zeolitic imidazolate frameworks
Kyo Sung Park,Zheng Ni,Adrien P. Côté,Jae Yong Choi,Rudan Huang,Fernando J. Uribe-Romo,Hee K. Chae,Michael O'Keeffe,Omar M. Yaghi +8 more
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Book ChapterDOI
The assay of catalases and peroxidases.
Britton Chance,A.C. Maehly +1 more
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Metal-organic frameworks in biomedicine.
Patricia Horcajada,Ruxandra Gref,Tarek Baati,Phoebe K. Allan,Guillaume Maurin,Patrick Couvreur,Gérard Férey,Russell E. Morris,Christian Serre +8 more
TL;DR: Metal Organic Frameworks in Biomedicine Patricia Horcajada, Ruxandra Gref, Tarek Baati, Phoebe K. Allan, Guillaume Maurin, Patrick Couvreur, G erard F erey, Russell E. Morris, and Christian Serre.