Journal ArticleDOI
Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review.
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TLDR
This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth, summarizing the theoretical and experimental achievements and endeavors to realize the practical applications of lithium metal batteries.Abstract:
The lithium metal battery is strongly considered to be one of the most promising candidates for high-energy-density energy storage devices in our modern and technology-based society. However, uncontrollable lithium dendrite growth induces poor cycling efficiency and severe safety concerns, dragging lithium metal batteries out of practical applications. This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth. First, the working principles and technical challenges of a lithium metal anode are underscored. Specific attention is paid to the mechanistic understandings and quantitative models for solid electrolyte interphase (SEI) formation, lithium dendrite nucleation, and growth. On the basis of previous theoretical understanding and analysis, recently proposed strategies to suppress dendrite growth of lithium metal anode and some other metal anodes are reviewed. A section dedicated to the potential of full-cell lithium metal batteries for practical applicatio...read more
Citations
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Journal ArticleDOI
The Regulating Role of Carbon Nanotubes and Graphene in Lithium‐Ion and Lithium–Sulfur Batteries
Ruopian Fang,Ke Chen,Ke Chen,Lichang Yin,Zhenhua Sun,Feng Li,Hui-Ming Cheng,Hui-Ming Cheng,Hui-Ming Cheng +8 more
TL;DR: Metrics for the evaluation of lithium batteries are discussed, based on which the regulating role of CNTs and graphene in Li-ion and Li-S batteries is comprehensively considered from fundamental electrochemical reactions to electrode structure and integral cell design.
Journal ArticleDOI
Dual-Layered Film Protected Lithium Metal Anode to Enable Dendrite-Free Lithium Deposition.
Chong Yan,Xin-Bing Cheng,Yang Tian,Xiang Chen,Xue-Qiang Zhang,Wen-Jun Li,Wen-Jun Li,Jia-Qi Huang,Qiang Zhang +8 more
TL;DR: This work demonstrates the concept of rational construction of dual-layered structured interfaces for safe rechargeable batteries through facile surface modification of Li metal anode through the immersion of lithium plates into the fluoroethylene carbonate solvent.
Journal ArticleDOI
Issues and Future Perspective on Zinc Metal Anode for Rechargeable Aqueous Zinc-ion Batteries
Journal ArticleDOI
Current Li-Ion Battery Technologies in Electric Vehicles and Opportunities for Advancements
TL;DR: In this paper, the authors present and compare key components of Li-ion batteries and describe associated battery management systems, as well as approaches to improve the overall battery efficiency, capacity, and lifespan.
Journal ArticleDOI
Towards practical lithium-metal anodes
TL;DR: This review summarizes the existing issues with regard to Li anodes and their underlying reasons and then highlights the recent progress made in the development of high-performance LiAnodes, and proposes the persisting challenges and opportunities toward the exploration of practical Li-metal anodes.
References
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Journal ArticleDOI
Issues and challenges facing rechargeable lithium batteries
TL;DR: A brief historical review of the development of lithium-based rechargeable batteries is presented, ongoing research strategies are highlighted, and the challenges that remain regarding the synthesis, characterization, electrochemical performance and safety of these systems are discussed.
Journal ArticleDOI
Electrical Energy Storage for the Grid: A Battery of Choices
TL;DR: The battery systems reviewed here include sodium-sulfur batteries that are commercially available for grid applications, redox-flow batteries that offer low cost, and lithium-ion batteries whose development for commercial electronics and electric vehicles is being applied to grid storage.
Journal ArticleDOI
Challenges for Rechargeable Li Batteries
John B. Goodenough,Youngsik Kim +1 more
TL;DR: In this paper, the authors reviewed the challenges for further development of Li rechargeable batteries for electric vehicles and proposed a nonflammable electrolyte with either a larger window between its lowest unoccupied molecular orbital and highest occupied molecular orbital (HOMO) or a constituent that can develop rapidly a solid/ electrolyte-interface (SEI) layer to prevent plating of Li on a carbon anode during a fast charge of the battery.
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Nonaqueous liquid electrolytes for lithium-based rechargeable batteries.
TL;DR: The phytochemical properties of Lithium Hexafluoroarsenate and its Derivatives are as follows: 2.2.1.
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Reviving the lithium metal anode for high-energy batteries
TL;DR: The current understanding on Li anodes is summarized, the recent key progress in materials design and advanced characterization techniques are highlighted, and the opportunities and possible directions for future development ofLi anodes in applications are discussed.