Journal ArticleDOI
Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review.
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TLDR
This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth, summarizing the theoretical and experimental achievements and endeavors to realize the practical applications of lithium metal batteries.Abstract:
The lithium metal battery is strongly considered to be one of the most promising candidates for high-energy-density energy storage devices in our modern and technology-based society. However, uncontrollable lithium dendrite growth induces poor cycling efficiency and severe safety concerns, dragging lithium metal batteries out of practical applications. This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth. First, the working principles and technical challenges of a lithium metal anode are underscored. Specific attention is paid to the mechanistic understandings and quantitative models for solid electrolyte interphase (SEI) formation, lithium dendrite nucleation, and growth. On the basis of previous theoretical understanding and analysis, recently proposed strategies to suppress dendrite growth of lithium metal anode and some other metal anodes are reviewed. A section dedicated to the potential of full-cell lithium metal batteries for practical applicatio...read more
Citations
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Performance and cost of materials for lithium-based rechargeable automotive batteries
TL;DR: In this article, the state-of-the-art advances in active materials, electrolytes and cell chemistries for automotive batteries are surveyed, along with an assessment of the potential to fulfil the ambitious targets of electric vehicle propulsion.
Journal ArticleDOI
Applications of 2D MXenes in energy conversion and storage systems
Jinbo Pang,Rafael G. Mendes,Rafael G. Mendes,Alicja Bachmatiuk,Alicja Bachmatiuk,Alicja Bachmatiuk,Liang Zhao,Huy Q. Ta,Thomas Gemming,Hong Liu,Hong Liu,Zhongfan Liu,Zhongfan Liu,Mark H. Rümmeli,Mark H. Rümmeli,Mark H. Rümmeli +15 more
TL;DR: The potential of MXenes for the photocatalytic degradation of organic pollutants in water, such as dye waste, is addressed, along with their promise as catalysts for ammonium synthesis from nitrogen.
Journal ArticleDOI
Advancing Lithium Metal Batteries
Bin Liu,Ji-Guang Zhang,Wu Xu +2 more
TL;DR: Li metal anodes are well known to be one of the most promising anodes due to their ultra-high capacity (3,860 mAh g −1 ) and the very low standard negative electrochemical potential (−3.040 V) as discussed by the authors.
Journal ArticleDOI
Recent Progress of the Solid-State Electrolytes for High-Energy Metal-Based Batteries
Journal ArticleDOI
Active Materials for Aqueous Zinc Ion Batteries: Synthesis, Crystal Structure, Morphology, and Electrochemistry
TL;DR: The current advances, existing limitations, along with the possible solutions in the pursuit of cathode materials with high voltage, fast kinetics, and long cycling stability are comprehensively covered and evaluated to guide the future design of aqueous ZIBs with a combination of high gravimetric energy density, good reversibility, and a long cycle life.
References
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Journal ArticleDOI
Microscopic properties of lithium, sodium, and magnesium battery anode materials related to possible dendrite growth
Markus Jäckle,Axel Groß +1 more
TL;DR: According to calculations, magnesium exhibits a tendency towards the growth of smooth surfaces as it exhibits lower diffusion barriers than lithium and sodium, and as an hcp metal it favors higher-coordinated configurations in contrast to the bcc metals Li and Na.
Journal ArticleDOI
Understanding undesirable anode lithium plating issues in lithium-ion batteries
TL;DR: In this paper, the adverse effects of anode lithium plating on the electrochemical performance of lithium-ion batteries are presented, and various in situ and ex situ techniques for characterizing and detecting anode-lithium plating are summarized.
Journal ArticleDOI
An Iodide-Based Li7P2S8I Superionic Conductor
Ezhiylmurugan Rangasamy,Zengcai Liu,Mallory Gobet,Kartik Pilar,Gayatri Sahu,Wei Zhou,Wei Zhou,Hui Wu,Hui Wu,Steve Greenbaum,Chengdu Liang +10 more
TL;DR: Low-temperature membrane processability enables facile fabrication of dense membranes, making this solid-state Li-ion conductor suitable for industrial adoption.
PatentDOI
Hybrid Electrolytes with Controlled Network Structures for Lithium Metal Batteries
Qiwei Pan,Christopher Y. Li +1 more
TL;DR: Solid polymer electrolytes with tunable network structures are prepared by a facile one-pot reaction of polyhedral oligomeric silsesquioxane and poly(ethylene glycol).
Journal ArticleDOI
Lithium Fluoride Additives for Stable Cycling of Lithium Batteries at High Current Densities
TL;DR: In this article, the effect of lithium fluoride salt additives on the electrodeposition of metals in batteries that use metallic lithium anodes was investigated through systematic electrochemical, spectroscopic, and microscopy studies.