Journal ArticleDOI
Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review.
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TLDR
This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth, summarizing the theoretical and experimental achievements and endeavors to realize the practical applications of lithium metal batteries.Abstract:
The lithium metal battery is strongly considered to be one of the most promising candidates for high-energy-density energy storage devices in our modern and technology-based society. However, uncontrollable lithium dendrite growth induces poor cycling efficiency and severe safety concerns, dragging lithium metal batteries out of practical applications. This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth. First, the working principles and technical challenges of a lithium metal anode are underscored. Specific attention is paid to the mechanistic understandings and quantitative models for solid electrolyte interphase (SEI) formation, lithium dendrite nucleation, and growth. On the basis of previous theoretical understanding and analysis, recently proposed strategies to suppress dendrite growth of lithium metal anode and some other metal anodes are reviewed. A section dedicated to the potential of full-cell lithium metal batteries for practical applicatio...read more
Citations
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Performance and cost of materials for lithium-based rechargeable automotive batteries
TL;DR: In this article, the state-of-the-art advances in active materials, electrolytes and cell chemistries for automotive batteries are surveyed, along with an assessment of the potential to fulfil the ambitious targets of electric vehicle propulsion.
Journal ArticleDOI
Applications of 2D MXenes in energy conversion and storage systems
Jinbo Pang,Rafael G. Mendes,Rafael G. Mendes,Alicja Bachmatiuk,Alicja Bachmatiuk,Alicja Bachmatiuk,Liang Zhao,Huy Q. Ta,Thomas Gemming,Hong Liu,Hong Liu,Zhongfan Liu,Zhongfan Liu,Mark H. Rümmeli,Mark H. Rümmeli,Mark H. Rümmeli +15 more
TL;DR: The potential of MXenes for the photocatalytic degradation of organic pollutants in water, such as dye waste, is addressed, along with their promise as catalysts for ammonium synthesis from nitrogen.
Journal ArticleDOI
Advancing Lithium Metal Batteries
Bin Liu,Ji-Guang Zhang,Wu Xu +2 more
TL;DR: Li metal anodes are well known to be one of the most promising anodes due to their ultra-high capacity (3,860 mAh g −1 ) and the very low standard negative electrochemical potential (−3.040 V) as discussed by the authors.
Journal ArticleDOI
Recent Progress of the Solid-State Electrolytes for High-Energy Metal-Based Batteries
Journal ArticleDOI
Active Materials for Aqueous Zinc Ion Batteries: Synthesis, Crystal Structure, Morphology, and Electrochemistry
TL;DR: The current advances, existing limitations, along with the possible solutions in the pursuit of cathode materials with high voltage, fast kinetics, and long cycling stability are comprehensively covered and evaluated to guide the future design of aqueous ZIBs with a combination of high gravimetric energy density, good reversibility, and a long cycle life.
References
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Journal ArticleDOI
The effects of current density and amount of discharge on dendrite formation in the lithium powder anode electrode
TL;DR: In this article, the amount of discharge and current density which suppress dendrite formation at the surface of a lithium powder electrode were investigated on an experimental basis, and the relationship between current density and total amount of discharging was deduced as a simple mathematical model.
Journal ArticleDOI
Lithium Metal Stability in Batteries with Block Copolymer Electrolytes
Daniel T. Hallinan,Scott Mullin,Scott Mullin,Gregory M. Stone,Gregory M. Stone,Nitash P. Balsara,Nitash P. Balsara +6 more
Journal ArticleDOI
In Situ Chemical Imaging of Solid-Electrolyte Interphase Layer Evolution in Li–S Batteries
Manjula I. Nandasiri,Luis E. Camacho-Forero,Ashleigh M. Schwarz,Vaithiyalingam Shutthanandan,Suntharampillai Thevuthasan,Perla B. Balbuena,Karl T. Mueller,Vijayakumar Murugesan +7 more
TL;DR: In this paper, an in situ X-ray photoelectron spectroscopy (XPS) and chemical imaging analysis combined with ab initio molecular dynamics (AIMD) computational modeling is presented to gain fundamental understanding regarding the evolution of SEI layers on Li-anodes within Li-S batteries.
Journal ArticleDOI
Ta-Doped Li7La3Zr2O12 for Water-Stable Lithium Electrode of Lithium-Air Batteries
K. Ishiguro,H. Nemori,S. Sunahiro,Y. Nakata,R. Sudo,Masaki Matsui,Masaki Matsui,Y. Takeda,Osamu Yamamoto,Nobuyuki Imanishi +9 more
TL;DR: In this paper, the Li6.75La3Zr1.75Ta 0.25O12 (LLZ-0.25Ta) composition sintered at 1,180°C for 36 h showed the highest relative density of 96.7% and resistance to water permeation.
Journal ArticleDOI
Excellent rate capability and cycle life of Li metal batteries with ZrO2/POSS multilayer-assembled PE separators
Mingming Chi,Liyi Shi,Zhuyi Wang,Jiefang Zhu,Xufeng Mao,Yin Zhao,Meihong Zhang,Lining Sun,Shuai Yuan +8 more
TL;DR: Li et al. as mentioned in this paper reported a distinctive ZrO 2 /POSS multilayer deposited on PE separators by a simple layer-by-layer self-assembly process to enable excellent rate capability and cycle life of lithium metal batteries.