Journal ArticleDOI
Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review.
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TLDR
This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth, summarizing the theoretical and experimental achievements and endeavors to realize the practical applications of lithium metal batteries.Abstract:
The lithium metal battery is strongly considered to be one of the most promising candidates for high-energy-density energy storage devices in our modern and technology-based society. However, uncontrollable lithium dendrite growth induces poor cycling efficiency and severe safety concerns, dragging lithium metal batteries out of practical applications. This review presents a comprehensive overview of the lithium metal anode and its dendritic lithium growth. First, the working principles and technical challenges of a lithium metal anode are underscored. Specific attention is paid to the mechanistic understandings and quantitative models for solid electrolyte interphase (SEI) formation, lithium dendrite nucleation, and growth. On the basis of previous theoretical understanding and analysis, recently proposed strategies to suppress dendrite growth of lithium metal anode and some other metal anodes are reviewed. A section dedicated to the potential of full-cell lithium metal batteries for practical applicatio...read more
Citations
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Sn layer decorated copper mesh with superior lithiophilicity for stable lithium metal anode
TL;DR: In this article, the authors proposed to decorate copper mesh by electrodeposition as current collector, which could induce the lithium nucleation uniformly and stabilize the process of lithium plating and stripping, leading to dendrite free lithium deposition behavior and excellent stable cycling performance.
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Status and prospects of porous graphene networks for lithium–sulfur batteries
Chongbo Sun,Yingqi Liu,Jinzhi Sheng,Qikai Huang,Wei Lv,Guangmin Zhou,Hui-Ming Cheng,Hui-Ming Cheng +7 more
TL;DR: In this article, the authors provide an overview of the roles and functions of PGNs in Li-S batteries, including increasing sulfur utilization, confining sulfur species, accommodating the volume change of sulfur, improving the conversion kinetics of polysulfides, reducing the consumption of lithium, preventing the dendrite growth, and acting as flexible hosts.
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From Lithium-Metal toward Anode-Free Solid-State Batteries: Current Developments, Issues, and Challenges
Christian Heubner,Sebastian Maletti,Henry Auer,Juliane Hüttl,Karsten Voigt,Oliver Lohrberg,Kristian Nikolowski,Mareike Partsch,Alexander Michaelis,Alexander Michaelis +9 more
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Dendrites in Solid-State Batteries: Ion Transport Behavior, Advanced Characterization, and Interface Regulation
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Failure modes and mechanisms for rechargeable Lithium-based batteries: a state-of-the-art review
Dandan Lyu,Bo Ren,Shaofan Li +2 more
TL;DR: It has been a general consensus that Li-ion batteries will continue to dominate the battery market in the foreseen future as a convenient electric power source and authors’ perspectives on future directions and challenges on experimental and computational modeling aspects of Li-based battery researches are provided.
References
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Journal ArticleDOI
Issues and challenges facing rechargeable lithium batteries
TL;DR: A brief historical review of the development of lithium-based rechargeable batteries is presented, ongoing research strategies are highlighted, and the challenges that remain regarding the synthesis, characterization, electrochemical performance and safety of these systems are discussed.
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Electrical Energy Storage for the Grid: A Battery of Choices
TL;DR: The battery systems reviewed here include sodium-sulfur batteries that are commercially available for grid applications, redox-flow batteries that offer low cost, and lithium-ion batteries whose development for commercial electronics and electric vehicles is being applied to grid storage.
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Challenges for Rechargeable Li Batteries
John B. Goodenough,Youngsik Kim +1 more
TL;DR: In this paper, the authors reviewed the challenges for further development of Li rechargeable batteries for electric vehicles and proposed a nonflammable electrolyte with either a larger window between its lowest unoccupied molecular orbital and highest occupied molecular orbital (HOMO) or a constituent that can develop rapidly a solid/ electrolyte-interface (SEI) layer to prevent plating of Li on a carbon anode during a fast charge of the battery.
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Nonaqueous liquid electrolytes for lithium-based rechargeable batteries.
TL;DR: The phytochemical properties of Lithium Hexafluoroarsenate and its Derivatives are as follows: 2.2.1.
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Reviving the lithium metal anode for high-energy batteries
TL;DR: The current understanding on Li anodes is summarized, the recent key progress in materials design and advanced characterization techniques are highlighted, and the opportunities and possible directions for future development ofLi anodes in applications are discussed.